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Critical current density in advanced superconductors 先进超导体中的临界电流密度
IF 33.6 1区 材料科学 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2025-05-26 DOI: 10.1016/j.pmatsci.2025.101492
H.S. Ruiz , J. Hänisch , M. Polichetti , A. Galluzzi , L. Gozzelino , D. Torsello , S. Milošević-Govedarović , J. Grbović-Novaković , O.V. Dobrovolskiy , W. Lang , G. Grimaldi , A. Crisan , P. Badica , A.M. Ionescu , P. Cayado , R. Willa , B. Barbiellini , S. Eley , A. Badía–Majós
This review paper delves into the concept of critical current density (Jc) in high-temperature superconductors (HTS) across macroscopic, mesoscopic, and microscopic perspectives. Through this exploration, a comprehensive range of connections is unveiled aiming to foster advancements in the physics, materials science, and the engineering of applied superconductors. Beginning with the macroscopic interpretation of Jc as a central material law, the review traces its development from C.P. Bean’s foundational work to modern extensions. Mesoscopic challenges in understanding vortex dynamics and their coherence with thermodynamic anisotropy regimes are addressed, underscoring the importance of understanding the limitations and corrections implicit in the macroscopic measurement of Jc, linked with mesoscopic phenomena such as irradiation effects, defect manipulation, and vortex interactions. The transition to supercritical current densities is also discussed, detailing the superconductor behavior beyond critical thresholds with a focus on flux-flow instability regimes relevant to fault current limiters and fusion energy magnets. Enhancing Jc through tailored material microstructures, engineered pinning centers, grain boundary manipulation, and controlled doping is explored, along with radiation techniques and their impact on large-scale energy systems. Emphasizing the critical role of Jc, this review focuses on its physical optimization and engineering manipulation, highlighting its significance across diverse sectors.
本文从宏观、介观和微观三个角度对高温超导体中的临界电流密度(Jc)的概念进行了探讨。通过这种探索,揭示了一系列全面的联系,旨在促进物理学、材料科学和应用超导体工程的进步。本文从宏观解读作为核心物质法则的JcJc开始,追溯其从C.P. Bean的基础性工作到现代扩展的发展历程。在理解涡旋动力学及其与热力学各向异性机制的一致性方面的介观挑战得到了解决,强调了理解JcJc宏观测量中隐含的局限性和修正的重要性,这些限制和修正与介观现象如辐射效应、缺陷操纵和涡旋相互作用有关。还讨论了向超临界电流密度的过渡,详细介绍了超过临界阈值的超导体行为,重点介绍了与故障电流限制器和聚变能磁体相关的通量不稳定机制。通过定制材料微观结构、工程钉钉中心、晶界操纵和控制掺杂,以及辐射技术及其对大规模能量系统的影响,探索了JcJc的增强。本文强调了JcJc的关键作用,重点介绍了JcJc的物理优化和工程操作,强调了JcJc在不同领域的重要性。
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引用次数: 0
Mechanical behavior of microstructurally stable nanocrystalline alloys: Processing, properties, performance, and prospects 微观结构稳定的纳米晶合金的力学行为:加工、性质、性能和前景
IF 33.6 1区 材料科学 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2025-05-25 DOI: 10.1016/j.pmatsci.2025.101519
K.A. Darling , Y. Mishin , N.N. Thadhani , Q. Wei , K. Solanki
This review presents a comprehensive overview of the scientific revolution enabled by recent emergence of structurally stabilized NC materials. It captures major breakthroughs in achieving nanoscale stability through thermodynamic and kinetic pathways, and critically examines the fundamental mechanisms underpinning the stabilization, including GB segregation, solute drag, Zener pinning, and nanocluster formation. It describes how stabilization of NC materials can enable unprecedented access to their intrinsic mechanical and physical behaviors, revealing phenomena previously inaccessible due to the microstructural evolution during testing. Examples include superlative strength-ductility synergy, infinite fatigue endurance limits, creep resistance rivaling single crystals, radiation damage tolerance, and evidence of defect-mediated self-healing. The review also explores how stabilized NC materials challenge long-held assumptions about the mechanisms of deformation, recrystallization, and phase transformations. It further examines how stabilized NC alloys have revolutionized our theoretical understanding of these mechanisms and created new avenues for their fabrication as well as industrial applications. While significant challenges remain with scalable fabrication processes and standardization, we outline new design principles, manufacturing pathways, and strategic directions for future exploration and application frontiers that are poised to overcome long-standing limitations making structurally stabilized NC materials as a transformative class of structural materials for extreme environments and advanced technologies.
本文综述了最近结构稳定的数控材料的出现所带来的科学革命的全面概述。它抓住了通过热力学和动力学途径实现纳米级稳定性的重大突破,并批判性地研究了支持稳定的基本机制,包括GB偏析,溶质阻力,齐纳钉钉和纳米团簇形成。它描述了NC材料的稳定性如何能够前所未有地获得其内在的机械和物理行为,揭示了以前由于测试过程中的微观结构演变而无法获得的现象。例子包括最高级的强度-延性协同作用,无限疲劳耐力极限,与单晶相媲美的蠕变抗力,辐射损伤耐受性,以及缺陷介导的自我修复的证据。本文还探讨了稳定的数控材料如何挑战长期以来关于变形、再结晶和相变机制的假设。它进一步研究了稳定的NC合金如何彻底改变了我们对这些机制的理论理解,并为它们的制造和工业应用创造了新的途径。虽然可扩展的制造工艺和标准化仍然存在重大挑战,但我们概述了未来探索和应用前沿的新设计原则,制造途径和战略方向,这些原则和战略方向有望克服长期存在的限制,使结构稳定的NC材料成为极端环境和先进技术的结构材料变革类。
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引用次数: 0
Additively manufactured function-tailored bone implants made of graphene-containing biodegradable metal matrix composites 增材制造的功能定制骨植入物由含石墨烯的可生物降解金属基复合材料制成
IF 33.6 1区 材料科学 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2025-05-24 DOI: 10.1016/j.pmatsci.2025.101517
Keyu Chen, Jiahui Dong, Niko Eka Putra, Lidy Elena Fratila-Apachitei, Jie Zhou, Amir A. Zadpoor
While conventionally manufactured metallic biomaterials can hardly meet all the requirements for bone implants including complex geometry, exact dimensions, adequate biodegradability, bone-matching mechanical properties, and biological function, two additional tools have recently appeared in the arsenal of biomaterials scientists which promise to deliver the desired combination of properties. First, the unique mechanical, electrical, and biological properties of graphene (Gr) and its derivatives (GDs), e.g., a Young’s modulus up to 1 TPa, can be utilized to create metal matrix composites in which GDs of varied contents (typically not more than 2 wt%), sizes (lateral sizes from a few nanometers to several micrometers), surface areas (up to the theoretical value of 2630 m2/g), and layer numbers (typically up to 10) are embedded in the biodegradable metal matrix, thereby endowing the composite implants with extraordinary properties. Second, the distinct advantages of additive manufacturing (AM) make it possible for GD-containing composite materials to precisely mimic the complex shapes and structures of bones at multiple length scales. Here, a comprehensive review of the recent advances in the development of GD-containing biodegradable metal matrix composites (GBMMCs), ranging from composite fabrication, including composite powder preparation, and AM processes, to the evaluation of AM composites in terms of their mechanical and biological properties, is presented. Furthermore, the constraints in processing composite powders, the advantages and disadvantages of applicable AM techniques, and the mechanisms of mechanical reinforcement, biodegradation modulation, osteogenesis improvement, and cytotoxicity/antibacterial balance are critically analyzed. Thereafter, the foreseeable challenges faced in the development of the next-generation of bone implants based on GBMMCs are presented and some future directions of research are identified.
虽然传统制造的金属生物材料很难满足骨植入物的所有要求,包括复杂的几何形状、精确的尺寸、足够的生物降解性、骨匹配的机械性能和生物功能,但最近在生物材料科学家的武器库中出现了两种额外的工具,它们承诺提供所需的性能组合。首先,石墨烯(Gr)及其衍生物(GDs)独特的机械、电气和生物特性,例如高达1 TPa的杨氏模量,可用于制造金属基复合材料,其中不同含量的GDs(通常不超过2 wt%)、尺寸(横向尺寸从几纳米到几微米)、表面积(高达理论值2630 m2/g)和层数(通常高达10层)嵌入在可生物降解的金属基体中。从而赋予复合植入物非凡的性能。其次,增材制造(AM)的独特优势使含gd的复合材料能够在多个长度尺度上精确模拟骨骼的复杂形状和结构。本文综述了含gd的可生物降解金属基复合材料(GBMMCs)的最新进展,从复合材料的制备,包括复合粉末的制备,AM工艺,到AM复合材料的力学和生物性能的评价。此外,本文还分析了复合粉末的加工限制,适用AM技术的优缺点,以及机械增强,生物降解调节,骨生成改善和细胞毒性/抗菌平衡的机制。在此基础上,提出了基于gbmmc的下一代骨种植体发展中可预见的挑战,并指出了未来的研究方向
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引用次数: 0
Developing safe and high-performance lithium-ion batteries: Strategies and approaches 开发安全和高性能锂离子电池:策略和方法
IF 33.6 1区 材料科学 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2025-05-23 DOI: 10.1016/j.pmatsci.2025.101516
Guanjun Chen , Rui Tan , Chunlin Zeng , Yan Li , Zexin Zou , Hansen Wang , Chuying Ouyang , Jiayu Wan , Jinlong Yang
Lithium-ion batteries (LIBs) as an effective low carbon technology provide a solution for achieving NetZero emissions, in line with the Sustainable Development Goals set by the United Nations. Research efforts have been devoted to increasing the energy density and efficiency of LIBs. However, large-scale deployment of LIBs is challenged by thermal runaway and safety problems, particularly under abusive conditions. To tackle this challenge, we must gain insight into the safety features of batteries and design durable strategies by fundamentally analyzing battery thermal runaway processes. In this review, we systematically summarize the abusive indicators that may trigger the thermal issues at the macroscopic level from thermal, chemical, and mechanical perspectives, and point out failure mechanisms that correlate with each component, e.g., cathode, anode, separator, electrolyte and current collector. Beyond material innovations, we emphasize the importance of optimizing industrial-scale manufacturing, integrating regulatory frameworks through advanced battery management systems, and enhancing safety engineering from an battery external perspective. Moreover, we systematically evaluate the contributions of theoretical and computational approaches to battery safety, critically comparing physics-based, machine learning, and hybrid models, and proposing targeted improvements. The broader implications of these safety strategies are considered in the context of environmental sustainability and recycling. Finally, we present design principles for safer, high-performance batteries and outline emerging research and industrial directions through a critical synthesis of thermal runaway mechanisms and mitigation strategies.
锂离子电池(lib)作为一种有效的低碳技术,为实现零净排放提供了解决方案,符合联合国制定的可持续发展目标。研究人员一直致力于提高lib的能量密度和效率。然而,lib的大规模部署受到热失控和安全问题的挑战,特别是在恶劣条件下。为了应对这一挑战,我们必须深入了解电池的安全特性,并从根本上分析电池热失控过程,设计出耐用的策略。本文从热学、化学和力学的角度系统地总结了可能在宏观层面引发热问题的滥用指标,并指出了与阴极、阳极、分离器、电解质和集流器等各部件相关的失效机制。除了材料创新,我们还强调优化工业规模制造、通过先进的电池管理系统整合监管框架以及从电池外部角度加强安全工程的重要性。此外,我们系统地评估了理论和计算方法对电池安全的贡献,批判性地比较了基于物理、机器学习和混合模型,并提出了有针对性的改进。在环境可持续性和循环利用的背景下考虑这些安全战略的更广泛影响。最后,我们提出了更安全、高性能电池的设计原则,并通过对热失控机制和缓解策略的关键综合,概述了新兴研究和工业方向
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引用次数: 0
Surface biofunctionalised porous materials: advances, challenges, and future prospects 表面生物功能化多孔材料:进展、挑战和未来前景
IF 33.6 1区 材料科学 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2025-05-23 DOI: 10.1016/j.pmatsci.2025.101518
Anyu Zhang , Johnny Kuan Un Wong , Yiyun Xia , Marcela Bilek , Giselle Yeo , Behnam Akhavan
This review highlights the transformative potential of three-dimensional (3D) porous materials in tissue engineering and regenerative medicine, focusing on the critical role of surface biofunctionalisation in modulating cell-material interactions. Surface biofunctionalisation, through biomolecule and hydrogel incorporation, enhances cellular adhesion, growth, and differentiation by providing essential biochemical and mechanical cues. However, achieving effective biofunctionalisation within the intricate, tissue-mimicking architectures of porous materials remains a significant challenge. The complex architectures often hinder uniform exposure to reaction media, i.e. liquids, gases, or plasma, thereby limiting the scalability and efficiency of existing methods. This review uncovers state-of-the-art strategies, elucidates the underlying mechanisms of surface biofunctionalisation, and identifies key challenges, including achieving uniform coverage, maintaining bioactivity, and enabling spatial control of biomolecule distribution. We identify that solvent-free approaches will drive the advancement of scalable surface biofunctionalisation for industrial and clinical applications, while novel surface treatment methods using biorthogonal click/cleavage chemistry or stimuli-responsive materials enable selective, efficient, and precise functionalisation processes. By synthesising recent advancements, we provide a forward-looking perspective on the future of surface biofunctionalisation, proposing directions to advance scalable, sustainable, and precision biomolecule immobilisation on porous materials. These insights aim to facilitate the development of biofunctional interfaces for next-generation tissue engineering and regenerative medicine applications.
这篇综述强调了三维(3D)多孔材料在组织工程和再生医学中的变革潜力,重点是表面生物功能化在调节细胞-材料相互作用中的关键作用。表面生物功能化,通过生物分子和水凝胶的掺入,通过提供必要的生化和机械线索,增强细胞粘附、生长和分化。然而,在多孔材料复杂的组织模拟结构中实现有效的生物功能化仍然是一个重大挑战。复杂的结构常常阻碍反应介质的均匀暴露,如液体、气体或等离子体,从而限制了现有方法的可扩展性和效率。这篇综述揭示了最先进的策略,阐明了表面生物功能化的潜在机制,并确定了关键挑战,包括实现均匀覆盖,保持生物活性,以及实现生物分子分布的空间控制。我们发现无溶剂方法将推动工业和临床应用中可扩展表面生物功能化的进步,而使用双正交点击/切割化学或刺激响应材料的新型表面处理方法可以实现选择性,高效和精确的功能化过程。通过综合最近的进展,我们对表面生物功能化的未来提供了前瞻性的观点,提出了在多孔材料上推进可扩展、可持续和精确的生物分子固定化的方向。这些见解旨在促进下一代组织工程和再生医学应用的生物功能接口的发展。
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引用次数: 0
Metal-Organic frameworks for optical sensor arrays 光学传感器阵列的金属-有机框架
IF 33.6 1区 材料科学 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2025-05-16 DOI: 10.1016/j.pmatsci.2025.101507
Xin Zhang, Yuanjing Cui, Guodong Qian
Precisely identifying subtle structural distinctions among various analytes remains a crucial yet difficult endeavor, primarily due to their extensive diversity, structural resemblance, and the potential for mutual interference. Traditional sensors, which operate on the “lock-and-key” principle, offer high selectivity and specificity for detecting particular analytes. However, this design makes them unsuitable for the simultaneous detection of multiple analytes. Metal-organic frameworks (MOFs) have attracted considerable interest in the realm of optical sensor arrays due to their diverse metal nodes and ligands, as well as the guest species that can be encapsulated within their channels or pores. This versatility makes MOFs highly advantageous for developing multi-channel single-sensing-element sensor arrays. The primary emphasis of this comprehensive review is on the intrinsic structure-performance relationship and development status of MOF-based optical sensor arrays. First, this review offers a concise explanation of the underlying theory and operational steps involved in optical sensor arrays. Second, the construction strategies for cross-reactive sensing elements are thoroughly presented. Third, the applications of MOF-based optical sensor arrays in identifying and detecting target analytes are explored comprehensively. This includes their use in environmental monitoring, disease diagnosis, food quality assessment, and the analysis of complex systems. Finally, the existing limitations and future research opportunities concerning MOF-based optical sensor arrays are thoroughly examined.
精确地识别各种分析物之间细微的结构差异仍然是一项至关重要但又困难的努力,主要是因为它们的广泛多样性、结构相似性和相互干扰的可能性。传统的传感器,其操作的“锁和钥匙”原则,提供高选择性和特异性检测特定的分析物。然而,这种设计使它们不适合同时检测多种分析物。金属有机框架(mof)由于其不同的金属节点和配体,以及可以封装在其通道或孔内的客体物质,在光学传感器阵列领域引起了相当大的兴趣。这种通用性使得mof在开发多通道单传感元件传感器阵列方面非常有利。本文主要综述了基于mof的光学传感器阵列的内在结构-性能关系及其发展现状。首先,本文简要介绍了光学传感器阵列的基本理论和操作步骤。其次,详细介绍了交叉反应传感元件的构建策略。第三,全面探讨了基于mof的光学传感器阵列在目标分析物识别和检测中的应用。这包括它们在环境监测、疾病诊断、食品质量评估和复杂系统分析中的应用。最后,对基于mof的光学传感器阵列的现有局限性和未来的研究机会进行了深入的分析。
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引用次数: 0
The wide range of battery systems: From micro- to structural batteries, from biodegradable to high performance batteries 广泛的电池系统:从微型电池到结构电池,从可生物降解电池到高性能电池
IF 33.6 1区 材料科学 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2025-05-14 DOI: 10.1016/j.pmatsci.2025.101506
Carlos M. Costa , Manuel Salado , Chiara Ferrara , Riccardo Ruffo , Piercarlo Mustarelli , Rui Mao , Sheng Feng , Yuxiang Shang , Xiaochen Wang , Zhenkun Lei , Ruixiang Bai , Cheng Yan , Kwon-Hyung Lee , Sang-Woo Kim , Tae-Hee Kim , Sang-Young Lee , Long Kong , Qiang Zhang , Harsha Devnani , Shikha Gupta , S. Lanceros-Mendez
Battery systems are essential components of the on-going energy transition and digitalization of society. With the need to power an increasing variety of portable and stationary systems, ranging from disposable point-of-care devices or smart packaging systems to applications in portable computers and electric cars, an increasing variety of batteries and battery systems are being developed, each aiming to specific sets of required performance parameters, including energy and power density, cycling stability, flexibility, degradability, environmental impact or improved integration into the specific application context.
This work analyzed the state of the art of the different materials and geometries, performance parameters and applications of the different battery systems.
We discuss the rationale behind each material selection, the processing technologies and the integration into the specific application, taking into account the whole life-cycle of the battery. Further, the main challenges posed for each battery type will provide a roadmap for their successful development and application.
电池系统是正在进行的能源转型和社会数字化的重要组成部分。从一次性护理设备或智能包装系统到便携式电脑和电动汽车的应用,越来越多的便携式和固定系统需要供电,越来越多的电池和电池系统正在开发中,每种电池和电池系统都针对所需的特定性能参数集,包括能量和功率密度、循环稳定性、灵活性、可降解性、环境影响或改进集成到特定应用程序上下文。这项工作分析了不同材料和几何形状的最新技术,不同电池系统的性能参数和应用。考虑到电池的整个生命周期,我们讨论了每种材料选择背后的基本原理,加工技术以及与特定应用的集成。此外,每种电池类型所面临的主要挑战将为它们的成功开发和应用提供路线图。
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引用次数: 0
Extreme wetting metallic devices: Structures, fabrication, applications and prospects 极端润湿金属装置:结构、制造、应用和前景
IF 33.6 1区 材料科学 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2025-05-09 DOI: 10.1016/j.pmatsci.2025.101505
Guiwei Li , Zeling Yang , Wenzheng Wu , Lei Ren , Ji Zhao , Luquan Ren
Extreme wetting metallic devices hold promising prospects in numerous fields, including aerospace, marine engineering and civil equipment, owing to their distinctive surface properties. The structures and fabrication of these surfaces have significant impacts on their functionality and applications. Herein, an overview of extreme wetting metallic devices are presented, focusing on their structures, fabrication, applications and prospects. Initially, the definitions and theoretical foundations of superhydrophilic and superhydrophobic surfaces, along with recent research advancements are discussed. Next, the additive and subtractive manufacturing employed for the precise construction of these surfaces is analyzed, with an emphasis on evaluating the performance of various metallic materials. Then, surface modification techniques are reviewed, highlighting their mechanisms, benefits and limitations. Additionally, potential application scenarios for extreme wetting metallic devices are summarized, including their roles in corrosion protection, anti-icing, self-cleaning functionalities and so on. Finally, the trend of extreme wetting metallic devices and the perspectives for this exciting new field are highlighted.
极端润湿金属器件由于其独特的表面特性,在航空航天、海洋工程和民用设备等众多领域具有广阔的应用前景。这些表面的结构和制造对其功能和应用有重大影响。本文综述了极端润湿金属器件的结构、制造、应用和前景。首先讨论了超亲水表面和超疏水表面的定义、理论基础以及近年来的研究进展。接下来,分析了用于精确构建这些表面的增材制造和减法制造,重点是评估各种金属材料的性能。然后,对表面改性技术进行了综述,重点介绍了其机理、优点和局限性。此外,总结了极湿金属器件的潜在应用前景,包括其在防腐蚀、防冰、自清洁等方面的作用。最后,对极端润湿金属器件的发展趋势和发展前景进行了展望。
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引用次数: 0
Engineering ion transport in all-solid-state sodium-ion batteries: fundamentals, strategies, and perspectives 全固态钠离子电池中的工程离子传输:基本原理、策略和前景
IF 33.6 1区 材料科学 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2025-05-06 DOI: 10.1016/j.pmatsci.2025.101503
Pan Yang , Zhenzhen Wu , Yuhao Liang , Hao Chen , Chaoliang Lin , Jingxia Qiu , Junxia Meng , Yanbing He , Shanqing Zhang
Rechargeable sodium-ion batteries (SIBs) offer a promising solution for large-scale energy storage systems due to their abundant availability and cost-effectiveness. Recently, all-solid-state sodium-ion batteries (ASSSIBs) with solid electrolytes have garnered significant attention for their superior energy density and safety compared to traditional SIBs with organic liquid electrolytes (OLEs). Despite notable progress, the sluggish ion transport remains a substantial barrier to the practical application of ASSSIBs. This review comprehensively examines the ion transport mechanisms and challenges in solid electrolytes, electrode/solid electrolyte interfaces, and electrodes of ASSSIBs. Additionally, it systematically explores representative strategies to enhance ion transport through engineering solid electrolytes, interfaces, and electrodes. Furthermore, it addresses the remaining challenges and future directions for advancing high-performance practical ASSSIBs. By providing development history, fundamental insights, effective strategies, and perspectives on designing ASSSIBs for rapid ion transport, this review could serve as a comprehensive guide for scientific research and practical development in the field.
可充电钠离子电池(sib)由于其丰富的可用性和成本效益,为大规模储能系统提供了一个很有前途的解决方案。近年来,采用固体电解质的全固态钠离子电池(ASSSIBs)因其比传统的采用有机液体电解质的全固态钠离子电池(ASSSIBs)具有更高的能量密度和安全性而备受关注。尽管取得了显著进展,但缓慢的离子传输仍然是ASSSIBs实际应用的重大障碍。本文综述了离子在固体电解质、电极/固体电解质界面和asssib电极中的传输机制和面临的挑战。此外,它系统地探讨了通过工程固体电解质、界面和电极增强离子传输的代表性策略。此外,它还解决了推进高性能实用assib的剩余挑战和未来方向。本文综述了快速离子输运assib的发展历史、基本见解、有效策略和观点,为该领域的科学研究和实践发展提供了全面的指导。
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引用次数: 0
Advanced evaporative cooling materials: From designs to applications 先进的蒸发冷却材料:从设计到应用
IF 33.6 1区 材料科学 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2025-05-06 DOI: 10.1016/j.pmatsci.2025.101504
Kaisong Huang, Hanyue Lan, Shuangqing Li, Renjie Tan, Yifan Si, Leqi Lei, Kaiwen Wang, Xiaoyun Xu, Wenjie Fang, Xinshuo Liang, Wen Jung Li, Jinlian Hu
Passive evaporative cooling materials harness perspiration or ambient humidity to dissipate surface heat through vaporization. This review systematically examines advanced evaporative cooling materials for applications in textiles, food preservation, buildings, photovoltaic (PV) panels, batteries, flexible electronics, thermoelectric generators (TEGs), etc. It discusses fundamental mechanisms, structural designs, cooling power calculations, and wettability/hygroscopicity modulation strategies. Furthermore, the integration of extended functionalities, including humidity/thermal responsiveness, radiative cooling, heat conduction, and thermal insulation for performance optimization, is analyzed. While progress has been achieved, industrial applications face challenges in scalability, durability, and cost efficiency. Practical solutions involve optimizing material formulations, improving durability through protective strategies, developing scalable manufacturing methods, and long-term standardized testing. Addressing these challenges could accelerate technology widespread adoption, advancing thermal comfort, energy conservation, sustainable development, and transformation in thermal management systems.
被动蒸发冷却材料利用汗液或环境湿度通过蒸发消散表面热量。本文系统地综述了先进的蒸发冷却材料在纺织、食品保鲜、建筑、光伏(PV)板、电池、柔性电子产品、热电发电机等领域的应用。它讨论了基本机制、结构设计、冷却功率计算和润湿性/吸湿性调制策略。此外,还分析了扩展功能的集成,包括湿度/热响应性、辐射冷却、热传导和隔热性能优化。虽然取得了进展,但工业应用仍面临着可扩展性、持久性和成本效率方面的挑战。实际的解决方案包括优化材料配方,通过保护策略提高耐久性,开发可扩展的制造方法,以及长期的标准化测试。解决这些挑战可以加速技术的广泛采用,促进热舒适、节能、可持续发展和热管理系统的转型。
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Progress in Materials Science
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