Progress in Materials Science最新文献_第10页

Corrigendum to “Progress in recent sustainable materials for greenhouse gas (NOx and SOx) emission mitigation”. [Prog. Mater. Sci. 132 (2023) 101033] “减少温室气体（氮氧化物和硫氧化物）排放的近期可持续材料的进展”的勘误。[掠夺。板牙。科学通报，132 (2023)101033]

IF 4 1区材料科学 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY

Progress in Materials Science

Pub Date : 2026-02-01 Epub Date: 2025-09-21 DOI: 10.1016/j.pmatsci.2025.101566

Aminul Islam , Siow Hwa Teo , Chi Huey Ng , Yun Hin Taufiq-Yap , Shean Yaw Thomas Choong , Md. Rabiul Awual

引用次数: 0

Towards preferential lithium recovery from spent lithium-ion batteries: phase transition mechanisms, technical innovation and future perspectives 从废锂离子电池中优先回收锂：相变机制、技术创新和未来展望

IF 4 1区材料科学 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY

Progress in Materials Science

Pub Date : 2026-02-01 Epub Date: 2025-08-22 DOI: 10.1016/j.pmatsci.2025.101557

Mengyu Lin , Yongqiang Chen , Chengyan Wang , Shengming Xu , Jialiang Zhang

Lithium is an indispensable element for the sustainable development of the new energy industry. However, the strong market demand for LIBs has led to a shortage of lithium resources. Recycling lithium from spent LIBs is an effective approach to alleviate the lithium shortage. However, LIBs are all artificially synthesized complex materials, and phase transition is an indispensable pathway to extract lithium selectively and efficiently. The phase transition methods can be divided into two types: lithium selective leaching in the liquid phase and lithium preferential extraction in the solid phase. This review systematically summarizes the available methods for selective lithium recovery and analyzes the phase transition mechanism from a thermodynamic perspective. The environmental impact and economic benefits analysis were presented for selective lithium extraction methods in liquid phase systems. Innovatively, the “reactivity-selectivity principle” was first employed to evaluate the main solid phase transition methods, indicating the importance of phase transition control for higher lithium recovery efficiency and selectivity. Finally, the prospects of lithium recycling development were outlined from four dimensions of technological innovation, entire-process optimization, economical efficiency and environmental friendliness. This review aims to provide references and enlightenment for the efficient recycling of spent LIBs from the perspective of phase transition and assist in the healthy and long-term development of new energy industry.

锂是新能源产业可持续发展不可缺少的元素。然而，市场对锂电池的强劲需求导致锂资源短缺。从废锂中回收锂是缓解锂短缺的有效途径。然而，锂离子化合物都是人工合成的复杂材料，相变是选择性高效提取锂不可或缺的途径。相变方法可分为液相锂选择性浸出法和固相锂优先萃取法两种。本文系统总结了现有的选择性回收锂的方法，并从热力学角度分析了锂的相变机理。分析了液相法选择性提取锂的环境影响和经济效益。创新性地采用“反应选择性原理”对主要固相转变方法进行了评价，表明相变控制对提高锂回收率和选择性的重要性。最后，从技术创新、全过程优化、经济效益和环境友好四个维度对锂回收的发展前景进行了展望。本文旨在从相变的角度为废旧lib的高效回收利用提供参考和启示，助力新能源产业的健康、长远发展。

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引用次数: 0

Advanced fast-charging anode designs for sodium-ion batteries 用于钠离子电池的先进快速充电阳极设计

IF 4 1区材料科学 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY

Progress in Materials Science

Pub Date : 2026-02-01 Epub Date: 2025-08-29 DOI: 10.1016/j.pmatsci.2025.101564

Jiaxin Wang , Yanling Yang , Jingeng Chen , Xiao-Lei Shi , Yu Sun , Xuefeng Tian , Hao Che , Yuefeng Chen , Zhi-Gang Chen

Sodium-ion batteries (SIBs) are emerging as a promising next-generation fast-charging technology due to their abundant raw resources, low cost, and low desolvation energy advantages that are especially beneficial under low-temperature conditions. However, achieving ultra-fast charging (i.e., charging times under 15 min) remains challenging. The kinetics of Na⁺ ions are primarily hindered by Na⁺ desolvation sluggish, restricted ion transport within the solid electrolyte interphase (SEI), and slow solid-state diffusion in the anode. Moreover, several fundamental challenges, such as significant volume changes during sodiation/desodiation and interfacial chemistry-induced side reactions, are further exacerbated. This review provides a comprehensive analysis of the key factors limiting the fast-charging capability of SIB anodes and outlines targeted optimization strategies, including bulk structure engineering, synergistic electrolyte design, and the controlled formation of favorable SEI layers. Representative case studies are presented to illustrate both the challenges and recent advances. Finally, this review presents future perspectives and potential pathways to guide the rational design of advanced fast-charging anode materials for SIBs.

钠离子电池（sib）因其原料资源丰富、成本低、低溶解能量的优势，特别是在低温条件下的优势，正在成为有前景的下一代快速充电技术。然而，实现超快速充电（即充电时间低于15 min）仍然具有挑战性。Na+离子的动力学主要受到Na+溶解缓慢、在固体电解质界面（SEI）内离子传输受限以及在阳极中缓慢的固态扩散等因素的阻碍。此外，一些基本的挑战，如在钠化/脱钠过程中显著的体积变化和界面化学诱导的副反应，将进一步加剧。本文全面分析了限制SIB阳极快速充电能力的关键因素，并概述了有针对性的优化策略，包括体结构工程、协同电解质设计和有利SEI层的可控形成。提出了具有代表性的案例研究，以说明挑战和最近的进展。最后，综述了未来的发展趋势和可能的途径，以指导sib先进快速充电阳极材料的合理设计。

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引用次数: 0

Regenerated cellulose fibres and their composites: From fundamental properties to advanced applications 再生纤维素纤维及其复合材料：从基本特性到高级应用

IF 4 1区材料科学 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY

Progress in Materials Science

Pub Date : 2026-02-01 Epub Date: 2025-08-07 DOI: 10.1016/j.pmatsci.2025.101547

Tim Huber , Nina Graupner , Jörg Müssig

Despite their good mechanical properties, especially their toughness, there are hardly any industrial applications for regenerated cellulose fibre-reinforced composites (RCFCs) apart from the classic elastomer applications in the automotive sector (tyres and hoses). The present review demonstrates that although there is some research work dealing with RCFCs, the amount of data is considered to be rather low compared to, e.g., natural fibre-reinforced composites. This review paper provides an overview of different regenerated cellulose fibres (RCFs) and their areas of application, as well as the processing of RCFs into RCFCs. It shows a comprehensive comparison of the mechanical properties of different fibre types and semi-finished products in various polymer matrices, an assessment of biodegradation and durability, and an overview of applications. RCFCs demonstrate significant potential for lightweight construction of composite materials, particularly in applications involving surface loads under bending and high toughness, due to their low density and environmental benefits compared to, e.g., glass fibres. However, further optimisation of stiffness and tensile strength is required to enhance their competitiveness for highly stressed composite materials, while increased attention to material perception is essential for successful product development and market adoption. Further research should be focused on standardising processing methods and achievable properties to transfer the technology to advanced industrial applications.

尽管再生纤维素纤维增强复合材料（rcfc）具有良好的机械性能，特别是韧性，但除了汽车领域（轮胎和软管）的经典弹性体应用外，几乎没有任何工业应用。目前的审查表明，虽然有一些关于RCFCs的研究工作，但与天然纤维增强复合材料等相比，数据量被认为相当少。本文综述了再生纤维素纤维（rcf）的不同种类及其应用领域，以及将rcf加工成RCFCs的方法。它全面比较了不同纤维类型和半成品在各种聚合物基质中的机械性能，评估了生物降解和耐久性，并概述了应用。与玻璃纤维相比，RCFCs具有低密度和环境效益，因此在复合材料轻量化结构方面具有巨大潜力，特别是在涉及弯曲和高韧性表面载荷的应用中。然而，需要进一步优化刚度和抗拉强度，以提高他们在高应力复合材料方面的竞争力，同时增加对材料感知的关注，对于成功的产品开发和市场采用至关重要。进一步的研究应集中在标准化加工方法和可实现的特性，以便将该技术转移到先进的工业应用。

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引用次数: 0

Corrigendum to “Roadmap for integrating deep eutectic solvents into adsorption processes: A critical review & design blueprint” [Progress Mater. Sci. 154 (2025) 101501] “将深共晶溶剂整合到吸附过程的路线图：一个关键的审查和设计蓝图”的勘误表[进展材料]。科学通报。154 (2025)101501]

IF 4 1区材料科学 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY

Progress in Materials Science

Pub Date : 2026-02-01 Epub Date: 2025-10-29 DOI: 10.1016/j.pmatsci.2025.101598

Ghaiath Almustafa , Rawan Abu Alwan , Ho Kyong Shon , Jorge Rodriguez , Inas AlNashef

引用次数: 0

Advancing ionic thermoelectric materials for heat recovery 热回收离子热电材料的研究进展

IF 4 1区材料科学 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY

Progress in Materials Science

Pub Date : 2026-02-01 Epub Date: 2025-09-06 DOI: 10.1016/j.pmatsci.2025.101575

Yifan Wang , Ibrahim Mwamburi Mwakitawa , Hao Yang , Mingyu Song , Qian Huang , Xinzhe Li , Pengchi Zhang , Wei Fang , Lijun Hu , Yongli Zhou , Chen Li , Jianyong Ouyang , Kuan Sun

Ionic thermoelectrics (i-TEs) are emerging as a promising, sustainable technology for low-grade heat recovery, notable for their absence of moving mechanical parts. In recent years, significant advancements in i-TE materials and devices have been propelled by their advantages in thermal power generation, compatibility with room-temperature operation, and potential for integration into flexible, wearable devices. However, challenges remain to be addressed for practical future applications, primarily due to insufficient evaluations of innovative operational modes and materials. This review aims to bridge this gap by summarizing key existing theories and providing an in-depth analysis of ion migration mechanisms within i-TE capacitors. We also highlight significant contributions from leading studies, focusing on material selection, operational modes, performance characteristics, and pivotal discoveries. Ultimately, this review seeks to identify transformative approaches in i-TEs to foster innovative designs for practical applications.

离子热电（i-TEs）正成为一种有前途的、可持续的低等级热回收技术，值得注意的是它们没有移动的机械部件。近年来，i-TE材料和器件在热发电、与室温操作的兼容性以及集成到灵活可穿戴设备中的潜力方面的优势推动了它们的重大进步。然而，由于对创新操作模式和材料的评估不足，未来的实际应用仍然面临挑战。本文旨在通过总结现有的关键理论和深入分析i-TE电容器中的离子迁移机制来弥补这一空白。我们还强调了主要研究的重要贡献，重点是材料选择，操作模式，性能特征和关键发现。最后，这篇综述试图找出i-TEs的变革方法，以促进实际应用的创新设计

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引用次数: 0

Progress in cathode materials for rechargeable Zinc-Ion batteries: from inorganic and organic systems to hybrid frameworks and biomass-derived innovations 可充电锌离子电池正极材料的进展：从无机和有机系统到混合框架和生物质衍生的创新

IF 4 1区材料科学 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY

Progress in Materials Science

Pub Date : 2026-02-01 Epub Date: 2025-07-31 DOI: 10.1016/j.pmatsci.2025.101543

Amjad Ali , Jamile Mohammadi Moradian , Ahmad Naveed , Shu Zhang , Mudassir Hussain Tahir , Khurram Shehzad , Mika Sillanpää

Zinc-ion batteries (ZIBs) have gained significant attention as promising candidates for large-scale energy storage systems owing to their low cost, environmental friendliness, and inherent safety, and have become a key focus of both academic research and industrial development strategies. However, significant challenges must be resolved, such as suboptimal charge kinetics, inadequate electrode structural stability, and complicated and costly manufacturing methods, prior to achieving meaningful advancements. Building on this foundation, this review offers a comprehensive overview of electrode materials, beginning with the fundamental factors that influence their electrochemical performance, such as electronic conductivity, ion diffusion pathways, structural stability, redox activity, and surface/interface characteristics. A clear understanding of these parameters is essential for guiding the rational design and optimization of high-performance electrodes for ZIBs. Secondly, we critically assess the current progress, identify persistent limitations, and explore potential strategies to overcome the challenges in achieving long-term cycling stability and fast reaction kinetics. Detailed analyses of structural engineering approaches, electrochemical behavior, and zinc-ion storage mechanisms across diverse material systems are presented to provide deep insights into the design principles driving next-generation AZB development. Finally, we also included a comprehensive outlook on the future development of ZIBs by identifying critical challenges and promising opportunities to drive their rapid progress and extensive practical deployment in the field.

锌离子电池（zib）由于其低成本、环境友好和固有的安全性而成为大规模储能系统的有前途的候选材料，并已成为学术研究和产业发展战略的重点。然而，在取得有意义的进展之前，必须解决重大挑战，例如次优电荷动力学，电极结构稳定性不足以及复杂且昂贵的制造方法。在此基础上，本文从影响电极材料电化学性能的基本因素（如电导率、离子扩散途径、结构稳定性、氧化还原活性和表面/界面特性）开始，对电极材料进行了全面的综述。清楚地了解这些参数对于指导zib高性能电极的合理设计和优化至关重要。其次，我们批判性地评估当前的进展，确定持续的局限性，并探索潜在的策略来克服实现长期循环稳定性和快速反应动力学的挑战。详细分析了不同材料系统的结构工程方法、电化学行为和锌离子储存机制，为推动下一代AZB开发的设计原则提供了深入的见解。最后，我们还通过确定关键挑战和有希望的机会，对ZIBs的未来发展进行了全面展望，以推动它们在该领域的快速进展和广泛的实际部署。

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引用次数: 0

Rational design of mechanical bio-metamaterials for biomedical applications 用于生物医学应用的机械生物超材料的合理设计

IF 4 1区材料科学 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY

Progress in Materials Science

Pub Date : 2026-02-01 Epub Date: 2025-08-03 DOI: 10.1016/j.pmatsci.2025.101545

Haoyu Wang , Yanshen Yang , Xiaqing Zhou , Jin Tian , Xinci Duan , Ang Li , Tian Jian Lu , Xiaokang Li , Dandan Pei , Feng Xu

Mechanical bio-metamaterials are an emerging class of engineered structures tailored to meet complex mechanical and biological demands in biomedical engineering. This review adopts a new perspective, moving beyond traditional formula-based approaches to explore design inspirations shaped by bioinspired, stimuli-responsive, and function-driven factors. We introduce a novel classification framework that organizes these metastructures from simple to complex and from static to dynamic, encompassing a broad range of structural designs. This structural-based classification emphasizes that it is the structure, rather than the material composition, that primarily defines the unique mechanical and biological properties of these materials. Furthermore, we discuss the transformative role of Artificial Intelligence in advancing the design of mechanical bio-metamaterials, facilitating forward and inverse design approaches, additive manufacturing, and predictive modeling. By establishing the term “mechanical bio-metamaterials,” this review connects structural design to biomedical applications in four key areas: engineered microenvironments, tissue implants, external devices, and invasive devices. This holistic approach aims to create accessible insights for a diverse audience, bridging engineering and clinical perspectives and illustrating how these metastructures influence cellular, tissue and organ behaviors. Finally, a roadmap outlines future directions, proposing evolutionary pathways for mechanical bio-metamaterials in healthcare. These innovations hold the potential to drive next-generation biomedical applications, offering improved patient outcomes and fostering creative advancements.

机械生物超材料是一种新兴的工程结构，用于满足生物医学工程中复杂的机械和生物需求。这篇综述采用了一个新的视角，超越了传统的基于公式的方法，探索由生物启发、刺激响应和功能驱动因素塑造的设计灵感。我们引入了一个新的分类框架来组织这些元结构，从简单到复杂，从静态到动态，涵盖了广泛的结构设计。这种基于结构的分类强调，主要是结构而不是材料成分决定了这些材料独特的机械和生物性能。此外，我们还讨论了人工智能在推进机械生物超材料设计、促进正向和逆设计方法、增材制造和预测建模方面的变革作用。通过建立术语“机械生物超材料”，本综述将结构设计与生物医学应用在四个关键领域联系起来：工程微环境、组织植入物、外部设备和侵入性设备。这种整体方法旨在为不同的受众创造可访问的见解，连接工程和临床观点，并说明这些元结构如何影响细胞，组织和器官行为。最后，路线图概述了未来的发展方向，提出了医疗保健领域机械生物超材料的进化途径。这些创新具有推动下一代生物医学应用的潜力，为患者提供更好的治疗效果，并促进创造性的进步。

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引用次数: 0

In vitro assays and development strategies for magnesium-based biodegradable cardiovascular stent: A decade of review 镁基可生物降解心血管支架的体外检测和发展策略：十年回顾

IF 4 1区材料科学 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY

Progress in Materials Science

Pub Date : 2026-02-01 Epub Date: 2025-07-25 DOI: 10.1016/j.pmatsci.2025.101541

Jiaqi Xu , Jiawei Zou , Dianyi Zhang , Kaili Zhang , Yining Qi , Changwen Yan , Eui-Seok Lee , Qi Jia , Chen Ma , Heng Bo Jiang

Cardiovascular disease (CVD) remains a leading global cause of mortality, underscoring the urgent need for innovative therapeutic solutions. Biodegradable magnesium-based stents (BMgS) have emerged as groundbreaking alternatives for coronary artery disease, offering temporary vascular support with safe biodegradation to minimize complications associated with permanent implants. Over the past decade, significant strides have been made in BMgS research, particularly in material science, advanced manufacturing techniques, and surface modifications. However, challenges such as uncontrolled degradation rates, insufficient mechanical strength, and limited biocompatibility continue to hinder their clinical adoption. This review provides a comprehensive and critical analysis of BMgS development advancements, with a particular focus on in vitro testing methodologies. Core areas include corrosion performance evaluation, mechanical property testing, and biocompatibility assessments, highlighting innovative approaches such as novel corrosion reactors, finite element analysis (FEA), and advanced biological assays. Development strategies center on alloy optimization (Mg-Zn and Mg-RE systems), cutting-edge manufacturing processes, and sophisticated surface modifications, including polymer, inorganic, and composite coatings, all tailored to enhance stent functionality. By synthesizing recent progress, this review not only identifies persistent challenges but also provides actionable insights for overcoming them. These findings serve as a valuable resource for researchers and industry stakeholders, paving the way for next-generation BMgS that strive to revolutionize cardiovascular care and improve patient outcomes.

心血管疾病（CVD）仍然是全球主要的死亡原因，强调迫切需要创新的治疗解决方案。可生物降解镁基支架（bmg）已成为冠状动脉疾病的突破性替代方案，提供安全的生物降解临时血管支持，以减少永久性植入物相关的并发症。在过去的十年中，bmg的研究取得了重大进展，特别是在材料科学、先进制造技术和表面改性方面。然而，诸如不受控制的降解率、机械强度不足和有限的生物相容性等挑战继续阻碍着它们的临床应用。这篇综述对bmg的发展进展进行了全面和批判性的分析，特别关注体外测试方法。核心领域包括腐蚀性能评估、机械性能测试和生物相容性评估，突出创新方法，如新型腐蚀反应器、有限元分析（FEA）和先进的生物分析。开发战略的核心是合金优化（Mg-Zn和Mg-RE系统）、尖端制造工艺和复杂的表面改性，包括聚合物、无机和复合涂层，所有这些都是为了增强支架功能而量身定制的。通过综合最近的进展，本综述不仅确定了持续存在的挑战，而且为克服这些挑战提供了可行的见解。这些发现为研究人员和行业利益相关者提供了宝贵的资源，为下一代bmg铺平了道路，努力改变心血管护理和改善患者预后。

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引用次数: 0

Recent progress in metal chalcogenide-MXene and MOF-derived composites for supercapacitors: synthesis, challenges, and future solutions 金属硫族化合物- mxene和mof衍生超级电容器复合材料的最新进展：合成、挑战和未来解决方案

IF 4 1区材料科学 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY

Progress in Materials Science

Pub Date : 2026-02-01 Epub Date: 2025-08-15 DOI: 10.1016/j.pmatsci.2025.101558

Avinash C. Mendhe , Swathi Lekshmi , Neha S. Barse , Iftikhar Hussain , Minjae Kim , Satish B. Jadhav , Haigun Lee

Metal chalcogenide-based electrode materials have gained a substantial attention as high-performance electrode alternative for supercapacitors owing to their tunable redox characteristics, high electrical conductivity, and enrich electrochemical activity. Recent advancements in composite materials, especially the integration of metal chalcogenides with MXenes and metal organic framework (MOF)-derived structures have unlocked innovative paths for surpassing inherent challenges such as poor cycling stability, accumulation, and low surface area. This review article delivers an inclusive summary of the synthesis strategies employed for evolving these hybrid composites electrodes, including hydrothermal, chemical bath deposition, and in situ growth techniques. The synergistic integration of MXenes, recognized for their excellent electrical conductivity and mechanical strength, with metal chalcogenides improves electron transport and structural stability. Correspondingly, the MOF-derived porous frameworks begin with a high surface area and controlled structure, further enhancing capacitance and ion diffusion. Despite these developments some key challenges remain, such as structural degradation, complex synthesis processes, and meager long-term electrochemical stability. This review also focusses on emerging approaches to resolve these challenges, such as defect engineering, heteroatom doping, and surface functionalization. Conclusively, the future perspectives are anticipated for scalable fabrication, flexible device integration, and performance optimization, pointing toward the next generation of high-energy–density supercapacitor systems.

金属硫族化合物电极材料因其可调的氧化还原特性、高导电性和丰富的电化学活性而成为超级电容器的高性能电极替代品。复合材料的最新进展，特别是金属硫族化合物与MXenes和金属有机框架（MOF）衍生结构的集成，为克服循环稳定性差、积累和低表面积等固有挑战开辟了创新途径。这篇综述文章提供了一个全面的总结，用于发展这些杂化复合材料电极的合成策略，包括水热、化学浴沉积和原位生长技术。MXenes具有优异的导电性和机械强度，与金属硫族化合物协同集成，提高了电子传递和结构稳定性。相应地，mof衍生的多孔框架具有高表面积和可控结构，进一步增强了电容和离子扩散。尽管取得了这些进展，但仍存在一些关键挑战，如结构降解、复杂的合成过程和长期电化学稳定性差。本文还重点介绍了解决这些挑战的新方法，如缺陷工程、杂原子掺杂和表面功能化。最后，展望了可扩展制造、灵活器件集成和性能优化的未来前景，并指出了下一代高能量密度超级电容器系统。

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引用次数: 0