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Effects of particle size, storage conditions, and chemical pretreatments on carbon and oxygen isotopic measurements of modern tooth enamel 粒度、储存条件和化学预处理对现代牙釉质碳和氧同位素测量的影响
IF 1.9 4区 医学 Q2 Medicine Pub Date : 2024-02-02 DOI: 10.1016/j.scijus.2024.01.004
Francesca Spencer , Kirsten Verostick , Alejandro Serna , Chris Stantis , Gabriel J. Bowen

Isotopic analysis of human tooth enamel can provide life history information useful in forensic identification. These applications depend on the availability of reference data documenting isotopic values for individuals with known life history and on the comparability of data from reference and case work samples. Here we build on previous methodological research, which has largely focused on paleontological and archaeological samples, and conduct experiments using enamel from modern human teeth targeting three sample preparation variables (sample particle size, storage conditions, and chemical pretreatments). Our results suggest that differences in particle size affect the efficiency of sample reactions during pretreatment and analysis, with coarse particles giving reduced loss of enamel carbonate during acid pretreatments but producing slightly higher oxygen isotope values than fine particles during analysis. Data for samples stored in dry and ambient environments following pretreatment were indistinguishable, suggesting no exchange of oxygen between samples and ambient water vapor. Finally, chemical pretreatments with a range of commonly used reactants and conditions showed a pervasive, moderate oxygen isotope shift associated with acetic acid treatment, which may be caused by exchange of enamel hydroxyl groups with reagents or rinse waters. Collectively, the results emphasize the importance of methodological standardization to improve comparability and reduce potential for bias in the forensic application of tooth enamel isotope data.

人类牙釉质的同位素分析可以提供有助于法医鉴定的生活史信息。这些应用取决于是否有参考数据记录已知生活史个体的同位素值,以及参考样本和案例样本数据的可比性。以前的方法学研究主要集中在古生物学和考古学样本上,我们在此基础上利用现代人牙齿的珐琅质进行实验,针对三个样本制备变量(样本粒度、储存条件和化学预处理)进行研究。我们的结果表明,颗粒大小的不同会影响样品在预处理和分析过程中的反应效率,粗颗粒在酸预处理过程中会减少珐琅质碳酸盐的损失,但在分析过程中产生的氧同位素值却略高于细颗粒。预处理后保存在干燥环境和环境中的样本数据没有区别,表明样本与环境水蒸气之间没有氧气交换。最后,在一系列常用反应物和条件下进行的化学预处理显示,与醋酸处理相关的氧同位素偏移普遍、适度,这可能是珐琅质羟基与试剂或冲洗水发生交换造成的。总之,这些结果强调了方法标准化的重要性,以提高可比性并减少牙釉质同位素数据在法医应用中可能出现的偏差。
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引用次数: 0
Cross-border forensic profiling of fraudulent identity and travel documents: A pilot project between France and Switzerland 伪造身份证件和旅行证件的跨境法证特征分析:法国和瑞士之间的试点项目
IF 1.9 4区 医学 Q2 Medicine Pub Date : 2024-02-01 DOI: 10.1016/j.scijus.2024.01.003
Solène Lugon Moulin , Emre Ertan , Didier Martin , Simon Baechler

The serial character of document fraud and its connection to organised crime groups who produce, sell and/or use fraudulent documents is a challenge for security and crime fighting. As a response, the added value of forensic intelligence is increasingly recognised. Using a forensic profiling method and a dedicated system deployed in Switzerland, document examiners can detect series (i.e., documents that share a common source) of fraudulent documents conveniently and efficiently. This detection can trigger or orientate investigations, supports crime intelligence efforts, and facilitates cross-jurisdictional cooperation. This study aims to assess the suitability of the forensic profiling system for international purpose and the efficiency of the method to detect cross-border series. The forensic profiling system has been deployed in France in the framework of a cross-border pilot project conducted by the School of Criminal Justice from the University of Lausanne and the French National Police (Division Nationale de Lutte contre la Fraude Documentaire et à l'Identité) over the period July 2019–May 2020. Data from the Swiss and French forensic profiling systems were compared to each other to detect cross-border series. The study sought to create operating conditions as close as possible to the real-life conditions of the profiling systems. The results are extremely positive both quantitatively and qualitatively. They demonstrate the benefit of setting up a systematic exchange of forensic data issued from profiling systems for fraudulent identity documents between France and Switzerland, let alone between any other countries. The results open up a very promising prospect for a sustained operational implementation by the police services of both countries and the extension of the exchanges internationally.

证件欺诈的连续性及其与制作、销售和/或使用欺诈性证件的有组织犯罪团伙的联系是安全和打击犯罪方面的一项挑战。作为应对措施,法证情报的附加值日益得到认可。利用在瑞士部署的法证剖析方法和专用系统,文件检验人员可以方便、高效地检测出欺诈性文件的系列(即具有共同来源的文件)。这种检测可以触发或引导调查,支持犯罪情报工作,并促进跨司法管辖区的合作。本研究旨在评估法证特征分析系统是否适用于国际目的,以及该方法检测跨境系列的效率。法证特征分析系统已在法国的一个跨境试点项目框架内部署,该项目由 XXX(为匿名审查而节录)和 XXX(为匿名审查而节录)在 2019 年 7 月至 2020 年 5 月期间进行。瑞士和法国法医特征分析系统的数据相互比较,以发现跨境系列。该研究试图创造尽可能接近特征分析系统实际情况的操作条件。研究结果在定量和定性方面都非常积极。这些结果表明,在法国和瑞士之间,更不用说在任何其他国家之间,系统地交换从伪造身份证件特征分析系统中获得的法证数据是有益的。这些结果为两国警察部门持续开展业务活动和在国际上扩大交流开辟了非常广阔的前景。
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引用次数: 0
Horizontal fire spread by foam-backed, polypropylene carpet 泡沫衬垫聚丙烯地毯的水平火势蔓延
IF 1.9 4区 医学 Q2 Medicine Pub Date : 2024-01-19 DOI: 10.1016/j.scijus.2024.01.002
M Jones

An eight year old boy was badly injured by a fire in his bedroom in May 2005. He spent his ninth birthday in intensive care and died a month later. This case study discusses a missing link into the pattern of fire development which made it difficult to identify the point of ignition. An absence of burning to the floor and isolated areas of burning seemed incongruous with the general pattern of fire development. Several fire investigation texts suggest that carpet cannot spread fire by itself; those texts that do mention the possibility, do not describe the mechanism in detail, nor what evidence an investigator might expect to see after the fire.

Experimentation with samples of carpet gave good insight into the mechanism and its effects, thereby providing the missing link by which to connect the areas of burning and identify the point of origin. If elements of the mechanism described in this paper are known, a reader could discern enough from the many papers available to support a working hypothesis but as yet, there is no single paper that describes the phenomenon mechanistically from start to finish, especially to those who have not encountered elements of it before; hence, this paper presents some novel findings.

The test involved polypropylene fibre carpets with integral polyurethane foam underlay, a very common type of carpet owing to its low cost and high durability. This is, therefore, an important mechanism of fire spread for fire investigators to be aware of and to understand. As this is a case study, rather than a research paper, the matters are dealt with empirically so the author cautions that when considering this mechanism in a new matter, the investigator should make their own tests of its validity.

2005 年 5 月,一名八岁男孩因卧室失火而严重受伤。他在重症监护室度过了九岁生日,一个月后死亡。本案例研究讨论了火灾发展模式中的一个缺失环节,该环节导致难以确定起火点。地板上没有燃烧痕迹和孤立的燃烧区域似乎与火灾的总体发展模式不符。一些火灾调查文章指出,地毯本身不能传播火势;那些提到这种可能性的文章并没有详细描述其机理,也没有说明调查人员在火灾发生后可能会看到哪些证据。如果读者知道本文所描述的机理要素,就可以从现有的许多论文中发现足够的信息来支持一个可行的假设,但到目前为止,还没有一篇论文从头到尾对这一现象进行机理描述,尤其是对那些以前没有接触过这一要素的人来说;因此,本文提出了一些新的发现。因此,这是火灾调查人员需要注意和了解的一种重要的火灾蔓延机制。由于这是一项案例研究,而不是一篇研究论文,因此,作者以经验为基础来处理问题,并告诫调查人员在考虑新问题中的这一机制时,应自行测试其有效性。
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引用次数: 0
Considerations on the application of a mutation model for Y-STR interpretation 将突变模型应用于 Y-STR 解释的考虑因素
IF 1.9 4区 医学 Q2 Medicine Pub Date : 2024-01-17 DOI: 10.1016/j.scijus.2024.01.001
Roberto Puch-Solis , Susan Pope , Gillian Tully

If Y-STR profiling is to be more effective in criminal casework, the methods used to evaluate evidential weight require improvement. Many forensic scientists assign an evidential weight by estimating the number of times a Y-STR profile obtained from a questioned sample has been observed in YHRD datasets. More sophisticated models have been suggested but not yet implemented into routine casework, e.g. Andersen & Balding [1]. Mutation is inherent to STR meiosis (or inheritance) and is encountered in practice. We evaluated a mutation model that can be incorporated into a method for assigning evidential weight to Y-STR profiles, an essential part of bringing any method into practice. Since an important part of implementation to casework is communication, the article is written in an accessible format for practitioners as well as statisticians.

The mutation component within the MUTEA model by Willems et al. [2] incorporates the potential for multistep mutations and a tendency for alleles to revert towards a central length, reflecting observed mutation data, e.g. [3]. We have estimated the parameters in this model and in a simplified symmetric version of this model, using sequence data from father/son pairs [4] and deep-rooted pedigrees [5]. Both datasets contain multistep mutations, which may have an effect on models based on simulations [1].

We introduce Beta-Binomial and Beta-Geometric conjugate analyses for estimating rate and step parameters for the mutation models presented here, which require only summations and multiplications. We proved mathematically that the parameters can be estimated independently. We show the importance of reporting the variability of the parameters and not only a point estimate. The parameters can be easily incorporated into statistical models, and updated sequentially as more data becomes available. We recommend fuller publication of data to enable the development and evaluation of a wider range of mutation models.

要想使 Y-STR 图谱分析在刑事案件工作中更加有效,就必须改进用于评估证据权重的方法。许多法证科学家通过估算从可疑样本中获得的 Y-STR 图谱在 YHRD 数据集中出现的次数来确定证据权重。有人提出了更复杂的模型,但尚未在常规案件工作中实施,例如 Andersen & Balding [1]。变异是 STR 减数分裂(或遗传)的固有特性,在实际工作中也会遇到。我们对突变模型进行了评估,该模型可纳入为 Y-STR 图谱分配证据权重的方法中,这是将任何方法付诸实践的重要部分。Willems 等人[2]的 MUTEA 模型中的突变部分包含了多步突变的可能性和等位基因向中心长度回归的趋势,反映了观察到的突变数据,如[3]。我们利用父子配对[4]和深根血统[5]的序列数据估算了该模型和该模型简化对称版的参数。这两个数据集都包含多步突变,这可能会对基于模拟的模型产生影响[1]。我们引入了贝塔-二项式分析和贝塔-几何共轭分析来估算本文介绍的突变模型的速率和步长参数,这两种方法只需要求和和乘法。我们用数学方法证明了参数可以独立估算。我们证明了报告参数的可变性而不仅仅是点估计的重要性。这些参数可以很容易地纳入统计模型,并随着更多数据的获得而不断更新。我们建议更全面地公布数据,以便开发和评估更广泛的突变模型。
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引用次数: 0
BM1: Events Guide BM1:活动指南
IF 1.9 4区 医学 Q2 Medicine Pub Date : 2024-01-01 DOI: 10.1016/S1355-0306(23)00141-7
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引用次数: 0
Estimate of the random match frequency of acquired characteristics in footwear: Part I — Impressions in blood 鞋类后天特征随机匹配频率的估计:第一部分 - 血液印迹
IF 1.9 4区 医学 Q2 Medicine Pub Date : 2024-01-01 DOI: 10.1016/j.scijus.2023.10.005
Alyssa N. Smale, Jacqueline A. Speir

The aim of this study was to estimate random match frequency of randomly acquired characteristics (RAC-RMF) for laboratory-simulated crime scene impressions. Part I of this investigation reports this metric using a dataset of more than 160 questioned impressions created in blood and deposited on tile. A total of 759 RACs were identified in the blood impressions and compared to RACs with positional similarity in test impressions from 1,299 unrelated outsoles. Geometric similarity was quantified using a combination of visual comparisons and mathematical modeling based on percent area overlap. Results indicated that RACs in blood impressions were typically smaller, and therefore exhibited a two-thirds increase in the number of indistinguishable pairs compared to their mated test impressions. For shoes contributing at least one RAC, relative RAC-RMF values 0.0008 were encountered at a rate between 3.4% and 34% for the blood impressions examined in this study. Part II of this investigation provides analogous results based on dust impressions deposited on paper and tile. Although the results in Part I and Part II are specific to randomly acquired characteristics and do not translate into an impression-wide RMF estimate, this research shows that RACs in questioned impressions of the type expected in casework co-occur in position and geometry with RACs in non-mated test impressions. Since theoretical models have traditionally been the basis for estimating RAC-RMF in footwear, the overall contribution of this research to the forensic footwear community is a calibration of this estimate based on empirical data.

本研究旨在估算实验室模拟的犯罪现场印痕的随机匹配频率(RAC-RMF)。本次调查的第一部分使用了一个数据集,该数据集包含 160 多个经质疑的血印,这些血印沉积在瓷砖上。在血印中总共识别出 759 个 RAC,并将其与 1299 个无关外底测试印迹中位置相似的 RAC 进行比较。通过视觉比较和基于重叠面积百分比的数学建模相结合的方法,对几何相似性进行了量化。结果表明,血印中的 RAC 通常较小,因此与配对的测试鞋印相比,无法区分的鞋对数量增加了三分之二。对于至少有一个 RAC 的鞋来说,在本研究中检测的血印中,RAC-RMF 相对值⩾ 0.0008 的比率介于 3.4% 和 34% 之间。本调查的第二部分根据沉积在纸张和瓷砖上的灰尘印迹提供了类似的结果。虽然第一部分和第二部分的结果是针对随机获得的特征,并不能转化为整个印模的 RMF 估计值,但这项研究表明,在个案工作中预期会出现的受质疑印模中的 RAC 与非配对测试印模中的 RAC 在位置和几何形状上是共存的。由于理论模型历来是估算鞋类 RAC-RMF 的基础,本研究对法医鞋类界的总体贡献在于根据经验数据校准了这一估算值。
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引用次数: 0
BM2: Council Information BM2:理事会信息
IF 1.9 4区 医学 Q2 Medicine Pub Date : 2024-01-01 DOI: 10.1016/S1355-0306(23)00142-9
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引用次数: 0
Prelim 3: Contents 预赛 3:内容
IF 1.9 4区 医学 Q2 Medicine Pub Date : 2024-01-01 DOI: 10.1016/S1355-0306(23)00140-5
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引用次数: 0
Estimate of the random match frequency of acquired characteristics in footwear: Part II — Impressions in dust 鞋类后天特征随机匹配频率的估算:第二部分 - 灰尘印迹
IF 1.9 4区 医学 Q2 Medicine Pub Date : 2024-01-01 DOI: 10.1016/j.scijus.2023.10.006
Alyssa N. Smale, Jacqueline A. Speir

This study serves as Part II of an investigation into the random match frequency of randomly acquired characteristics (RAC-RMF) in footwear evidence. In Part I, RAC-RMF was estimated in a dataset of laboratory-simulated crime scene impressions deposited in blood. For Part II, a second dataset was created composed of impressions deposited in dust on paper or tile, with the latter lifted using gelatin or Mylar film. A total of 1,513 RACs were identified from more than 160 dust impressions and compared to RACs with positional similarity in test impressions from 1,299 non-mated outsoles. RACs of any size deposited in dust exhibited a 31% decrease in shoes with non-zero RAC-RMFs as compared to their mated test impressions, while those deposited in blood exhibited a 45% increase. When only considering shoes with at least one RAC deemed forensically-reliable (length 2.8 mm), 3.1% of shoes contributing dust impressions and 3.4% of shoes contributing blood impressions exhibited relative RAC-RMFs at a value 0.0008. Although each dataset resulted in a comparable rate for encountering non-zero RAC-RMFs, the estimate for dust was based on twice the number of RAC comparisons (154,477) than those performed when assessing blood (77,566). While these results are considered specific to the non-mated impressions and methods of analysis described herein, and continued work is required before rates can be fully understood and reported in forensic casework, this study encountered non-zero RAC-RMFs for shoes exhibiting at least one forensically-reliable RAC at a more frequent rate than any estimates previously reported.

本研究是鞋类证据中随机获得特征的随机匹配频率(RAC-RMF)调查的第二部分。在第一部分中,对实验室模拟的犯罪现场血印数据集进行了 RAC-RMF 估算。在第二部分中,创建了第二个数据集,由沉积在纸张或瓷砖上灰尘中的印痕组成,后者使用明胶或聚酯薄膜提取。从 160 多个灰尘印迹中识别出 1513 个 RAC,并与 1299 个非配对外底测试印迹中位置相似的 RAC 进行比较。与配对的测试印模相比,沉积在灰尘中的任何大小的 RAC(RAC-RMFs 不为零)都减少了 31%,而沉积在血液中的 RAC 则增加了 45%。如果只考虑至少有一个 RAC 被认为是取证可靠的(长度 ⩾ 2.8 毫米),3.1% 的灰尘印迹鞋和 3.4% 的血液印迹鞋的相对 RAC-RMF 值 ⩾ 0.0008。虽然每个数据集都导致出现非零 RAC-RMF 的比率相当,但灰尘的估计值是基于两倍的 RAC 比较次数(154,477 次)得出的,而血液的估计值是基于 77,566 次的 RAC 比较次数得出的。虽然这些结果被认为是本文所述的非配对印模和分析方法所特有的,在充分了解和报告法医案件工作中的比率之前,还需要继续开展工作,但本研究发现,至少有一个法医上可靠的 RAC 的鞋子出现非零 RAC-RMF 的频率高于之前报告的任何估计值。
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引用次数: 0
A proof-of-concept study: Determining the geographical origin of Brazilwood, (Paubrasilia echinata) with the use of strontium isotopic fingerprinting 概念验证研究:利用锶同位素指纹图谱确定巴西木(Paubrasilia echinata)的地理来源
IF 1.9 4区 医学 Q2 Medicine Pub Date : 2023-12-30 DOI: 10.1016/j.scijus.2023.12.006
Camilla Vasconcelos Kafino , Isabela Moreno Cordeiro de Sousa , Cristina Barazetti Barbieri , Artur Moraes de Amorim , Roberto Ventura Santos

The illicit exploitation of Brazilwood (Paubrasilia echinata) presents a significant challenge in Brazil, given its substantial value in the global production of bows for musical instruments. To address timber provenance, the use of strontium (Sr) isotope ratios as indicators of bedrock signatures has emerged as a robust tool in forensic investigations. In this study, we critically evaluate the efficacy of this approach using Sr isotope data derived from bulk soils and trees collected at two distinct sites in Brazil. Despite the statistically indistinguishable 87Sr/86Sr ratios observed in the investigated tree species, the compiled 87Sr/86Sr isotope ratios of Brazilwood from Brazilwood National Park (PNPB) and the ES Group provide valuable insights into the potential application of this method for tracing forensic timber seizures. This pilot study also addresses crucial sampling considerations.

While the regional signatures exhibit clear distinctions, the limited sample sizes underscore the necessity for supplementary methods to confidently attribute timber to a specific source forest. In isolation, this method proves most effective in refuting presumed timber provenances rather than definitively confirming them. The discussion delves into the nuances of the Sr isotope data, emphasizing the importance of increasing the number of samples and exploring complementary techniques for a more comprehensive and reliable assessment of timber origin.

鉴于巴西木(Paubrasilia echinata)在全球乐器弓生产中的巨大价值,对巴西木的非法开采是一项重大挑战。为了解决木材来源问题,使用锶(Sr)同位素比值作为基岩特征的指标已成为法医调查的有力工具。在本研究中,我们利用从巴西两个不同地点采集的大块土壤和树木中获得的锶同位素数据,对这种方法的有效性进行了严格评估。尽管在所调查的树种中观察到的 87Sr/86Sr 比率在统计上没有区别,但巴西国家公园 (PNPB) 和 ES 集团的巴西木的 87Sr/86Sr 同位素比率汇编为应用这种方法追踪法证木材扣押情况提供了宝贵的见解。这项试点研究还解决了取样方面的关键问题。虽然区域特征显示出明显的区别,但有限的样本量突出表明,有必要采用补充方法,以确定木材的具体来源森林。孤立地看,这种方法在反驳推测的木材产地方面最有效,而不是最终确认。讨论深入探讨了锶同位素数据的细微差别,强调了增加样本数量和探索补充技术对于更全面、更可靠地评估木材来源的重要性。
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引用次数: 0
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