Pub Date : 2024-09-01DOI: 10.1016/j.photonics.2024.101299
This is an introduction to the special issue “Micro and nano structured mid-IR to Terahertz materials and devices” which aims to cover recent developments in terms of photonics devices operating from the mid-infrared to terahertz wavelength ranges, with possible applications in spectroscopy, sensing, or communications.
{"title":"Preface to the special issue in micro and nano structured mid-IR to terahertz materials and devices","authors":"","doi":"10.1016/j.photonics.2024.101299","DOIUrl":"10.1016/j.photonics.2024.101299","url":null,"abstract":"<div><p>This is an introduction to the special issue “Micro and nano structured mid-IR to Terahertz materials and devices” which aims to cover recent developments in terms of photonics devices operating from the mid-infrared to terahertz wavelength ranges, with possible applications in spectroscopy, sensing, or communications.</p></div>","PeriodicalId":49699,"journal":{"name":"Photonics and Nanostructures-Fundamentals and Applications","volume":null,"pages":null},"PeriodicalIF":2.5,"publicationDate":"2024-09-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141838838","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2024-09-01DOI: 10.1016/j.photonics.2024.101287
{"title":"Corrigendum to “High sensitivity plasmonic refractive index sensor for early anaemia detection” [Photonics Nanostruct. - Fundam. Appl. 58(01) (2024) 101235]","authors":"","doi":"10.1016/j.photonics.2024.101287","DOIUrl":"10.1016/j.photonics.2024.101287","url":null,"abstract":"","PeriodicalId":49699,"journal":{"name":"Photonics and Nanostructures-Fundamentals and Applications","volume":null,"pages":null},"PeriodicalIF":2.5,"publicationDate":"2024-09-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.sciencedirect.com/science/article/pii/S1569441024000622/pdfft?md5=50e50fd1804dc4ed78b7192971f5cf54&pid=1-s2.0-S1569441024000622-main.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142147839","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2024-08-14DOI: 10.1016/j.photonics.2024.101301
Humidity monitoring is paramount in diverse applications, industrial, and medical applications. Surface Plasmon Resonance (SPR) is an optical detection technique capable of sensing various environmental parameters through changes in reflected optical spectra and has garnered significant attention. Typically, SPR sensing employs a single-point detection strategy with the sample at a fixed concentration to achieve optimal sensitivity, limiting its application in dynamic environmental testing. This study proposes an image-based SPR humidity monitoring method, integrating SPR with image processing, enabling dynamic parameter reconstruction, and achieving high responsiveness. Au-PVA is used as a sensing film. To attain the best sensing film thickness, sensing film thicknesses ranging from 94.0 to 243.3 were tested. Through optimizing film thickness and image data processing, high precision and dynamic responsiveness were achieved. Experimental results demonstrate a response time of 84 and an average relative prediction error of 1.57 % for the sensor. Our research holds significant promise for dynamic and accurate humidity detection.
{"title":"SPR humidity dynamic monitoring method via PVA sensing membrane thickness variation and image processing techniques","authors":"","doi":"10.1016/j.photonics.2024.101301","DOIUrl":"10.1016/j.photonics.2024.101301","url":null,"abstract":"<div><p>Humidity monitoring is paramount in diverse applications, industrial, and medical applications. Surface Plasmon Resonance (SPR) is an optical detection technique capable of sensing various environmental parameters through changes in reflected optical spectra and has garnered significant attention. Typically, SPR sensing employs a single-point detection strategy with the sample at a fixed concentration to achieve optimal sensitivity, limiting its application in dynamic environmental testing. This study proposes an image-based SPR humidity monitoring method, integrating SPR with image processing, enabling dynamic parameter reconstruction, and achieving high responsiveness. Au-PVA is used as a sensing film. To attain the best sensing film thickness, sensing film thicknesses ranging from 94.0 <span><math><mrow><mi>n</mi><mi>m</mi></mrow></math></span> to 243.3 <span><math><mrow><mi>n</mi><mi>m</mi></mrow></math></span> were tested. Through optimizing film thickness and image data processing, high precision and dynamic responsiveness were achieved. Experimental results demonstrate a response time of 84 <span><math><mrow><mi>m</mi><mi>s</mi></mrow></math></span> and an average relative prediction error of 1.57 % for the sensor. Our research holds significant promise for dynamic and accurate humidity detection.</p></div>","PeriodicalId":49699,"journal":{"name":"Photonics and Nanostructures-Fundamentals and Applications","volume":null,"pages":null},"PeriodicalIF":2.5,"publicationDate":"2024-08-14","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142047993","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2024-07-23DOI: 10.1016/j.photonics.2024.101300
As a typical two-dimensional (2D) ferromagnetic insulator (FI), the Cr2Si2Te6 (CST) has performance ferromagnetic properties. The previous investigation has shown that quantum mechanical simulation can get structure and electronic properties of CST, and the indirect gap value of CST is 0.6 eV by establishing its layered calculation. It implies that the CST is an excellent optical modulator due to larger infrared radiation absorption interval. Based on that, some groups conducted the research of fiber laser based on CST saturable absorber (SA). However, the exploration and application of 2D CST in optics is still in the early stage. In this investigation, the CST was utilized as a SA in an Er-doped fiber laser. The dual-wavelength mode-locked pulse could be observed when the pump power was adjusted from 25 to 140 mW. The CST was applied in Er-doped fiber as SA for generating dual-wavelength mode-locked pulse for the first time. It exhibits performance optical properties that provide a significant reference for exploring the application of 2D materials in ultrafast laser.
{"title":"Application of Cr2Si2Te6 saturable absorber in Er-doped fiber laser for generating dual-wavelength mode-locked pulse","authors":"","doi":"10.1016/j.photonics.2024.101300","DOIUrl":"10.1016/j.photonics.2024.101300","url":null,"abstract":"<div><p>As a typical two-dimensional (2D) ferromagnetic insulator (FI), the Cr<sub>2</sub>Si<sub>2</sub>Te<sub>6</sub> (CST) has performance ferromagnetic properties. The previous investigation has shown that quantum mechanical simulation can get structure and electronic properties of CST, and the indirect gap value of CST is 0.6 eV by establishing its layered calculation. It implies that the CST is an excellent optical modulator due to larger infrared radiation absorption interval. Based on that, some groups conducted the research of fiber laser based on CST saturable absorber (SA). However, the exploration and application of 2D CST in optics is still in the early stage. In this investigation, the CST was utilized as a SA in an Er-doped fiber laser. The dual-wavelength mode-locked pulse could be observed when the pump power was adjusted from 25 to 140 mW. The CST was applied in Er-doped fiber as SA for generating dual-wavelength mode-locked pulse for the first time. It exhibits performance optical properties that provide a significant reference for exploring the application of 2D materials in ultrafast laser.</p></div>","PeriodicalId":49699,"journal":{"name":"Photonics and Nanostructures-Fundamentals and Applications","volume":null,"pages":null},"PeriodicalIF":2.5,"publicationDate":"2024-07-23","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141852454","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2024-07-23DOI: 10.1016/j.photonics.2024.101298
Optical technology has seen a revival from the previous decade, in terms of innovations and research, especially relating to optical integrated circuits. Similarly, Photonic Crystals (PCs) are one of the main contenders for the purpose. Therefore, this research work implicates different arrangements of the 3-Dimensional PC units based on the employment of a varying radius PC-cavity and its position i.e., at the beginning and within the middle of the PC-lattice. The effects of these PC-cavities are studied, investigating higher shifting in resonant wavelength, a narrower linewidth around 0.0061 µm and a quality factor of 99.59, comprising of a PC-cavity of radius 0.300 µm using input signal only i.e., coupled into the optical structure using the phenomenon of the Guided-mode-resonances (GMR). The structures are computed using an open-source FDTD platform, employing a stripe-model-based structure utilizing the Periodic Boundary Condition to save time and computational resources and later the PML for the realization of the Finite models. Moreover, the concluded structures based on the position of the PC-cavity, are demonstrated for the design of the all-optical-amplification device, executing a control signal reporting an 8 % of the amplification in the output of the input signal.
与前十年相比,光学技术在创新和研究方面出现了复苏,尤其是在光集成电路方面。同样,光子晶体(PC)也是这一目的的主要竞争者之一。因此,这项研究工作基于不同半径的 PC 腔及其位置(即 PC 晶格的起始位置和中间位置),对三维 PC 单元进行了不同的排列。我们研究了这些 PC 腔的影响,调查了共振波长的更高偏移、0.0061 微米左右的更窄线宽和 99.59 的品质因数,包括半径为 0.300 微米的 PC 腔,仅使用输入信号,即使用导模共振现象耦合到光学结构中。这些结构是利用开源 FDTD 平台计算得出的,采用了基于条纹模型的结构,利用周期边界条件来节省时间和计算资源,随后利用 PML 来实现有限模型。此外,根据 PC 腔的位置总结出的结构还用于全光放大设备的设计,执行一个控制信号,报告输入信号输出中 8% 的放大率。
{"title":"A comparative study of the photonic crystals-based cavities and usage in all-optical-amplification phenomenon","authors":"","doi":"10.1016/j.photonics.2024.101298","DOIUrl":"10.1016/j.photonics.2024.101298","url":null,"abstract":"<div><p>Optical technology has seen a revival from the previous decade, in terms of innovations and research, especially relating to optical integrated circuits. Similarly, Photonic Crystals (PCs) are one of the main contenders for the purpose. Therefore, this research work implicates different arrangements of the 3-Dimensional PC units based on the employment of a varying radius PC-cavity and its position i.e., at the beginning and within the middle of the PC-lattice. The effects of these PC-cavities are studied, investigating higher shifting in resonant wavelength, a narrower linewidth around 0.0061 µm and a quality factor of 99.59, comprising of a PC-cavity of radius 0.300 µm using input signal only i.e., coupled into the optical structure using the phenomenon of the Guided-mode-resonances (GMR). The structures are computed using an open-source FDTD platform, employing a stripe-model-based structure utilizing the Periodic Boundary Condition to save time and computational resources and later the PML for the realization of the Finite models. Moreover, the concluded structures based on the position of the PC-cavity, are demonstrated for the design of the all-optical-amplification device, executing a control signal reporting an 8 % of the amplification in the output of the input signal.</p></div>","PeriodicalId":49699,"journal":{"name":"Photonics and Nanostructures-Fundamentals and Applications","volume":null,"pages":null},"PeriodicalIF":2.5,"publicationDate":"2024-07-23","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.sciencedirect.com/science/article/pii/S1569441024000737/pdfft?md5=782a7f7b90168d7b428f874e925401d4&pid=1-s2.0-S1569441024000737-main.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141951255","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2024-07-14DOI: 10.1016/j.photonics.2024.101297
We find that the spontaneous and collective emissions have a strong influence on the excitation of two-level absorbers (atoms, molecules) interacting in resonance with the plasmonic mode near the metal nanoparticle. The spontaneous and collective emissions limit the absorption enhancement by the plasmonic mode and make the enhancement possible only with a fast, picosecond population relaxation of the upper absorbing states. Conditions for the maximum of plasmon-enhanced absorption in the presence of spontaneous and collective emissions are found. The nonlinearity in the nanoparticle-absorber interaction and in collective emission causes the bistability in the plasmon-enhanced absorption at high external field intensities and the plasmonic mode excitation.
{"title":"Spontaneous emission, collective phenomena and the efficiency of plasmon-stimulated photoexcitation","authors":"","doi":"10.1016/j.photonics.2024.101297","DOIUrl":"10.1016/j.photonics.2024.101297","url":null,"abstract":"<div><p>We find that the spontaneous and collective emissions have a strong influence on the excitation of two-level absorbers (atoms, molecules) interacting in resonance with the plasmonic mode near the metal nanoparticle. The spontaneous and collective emissions limit the absorption enhancement by the plasmonic mode and make the enhancement possible only with a fast, picosecond population relaxation of the upper absorbing states. Conditions for the maximum of plasmon-enhanced absorption in the presence of spontaneous and collective emissions are found. The nonlinearity in the nanoparticle-absorber interaction and in collective emission causes the bistability in the plasmon-enhanced absorption at high external field intensities and the plasmonic mode excitation.</p></div>","PeriodicalId":49699,"journal":{"name":"Photonics and Nanostructures-Fundamentals and Applications","volume":null,"pages":null},"PeriodicalIF":2.5,"publicationDate":"2024-07-14","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141951254","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2024-07-09DOI: 10.1016/j.photonics.2024.101296
We simulated the light extraction efficiency (LEE) of porous GaN-based InGaN/GaN micrometer-sized light-emitting diodes (μLEDs) emitting within the visible wavelength range using the finite-difference time-domain (FDTD) method. The simulations show that the embedding of a porous GaN layer with 40 % porosity reduces the bottom LEE, while the top side LEE of the μLEDs is increased. In addition, it also exhibits complex scattering properties that affect the microcavity structure of these devices. The LEE and the degree of microcavity structure disruption are related to nanopore size and location. This association weakens with increasing wavelength. Also, a decrease in nanopore size corresponds to a diminished impact on μLED optical properties. Since the porous GaN layer contributes to the deposition of high-quality InGaN, controlling pore size of the porous GaN layer will aid the development of GaN-based red μLEDs and full-color displays.
我们利用有限差分时域(FDTD)方法模拟了多孔氮化镓基 InGaN/GaN 微米级发光二极管(μLEDs)在可见光波长范围内的光萃取效率(LEE)。模拟结果表明,嵌入孔隙率为 40% 的多孔 GaN 层后,μLED 的底部 LEE 降低,而顶部 LEE 增加。此外,它还表现出复杂的散射特性,影响了这些器件的微腔结构。LEE和微腔结构的破坏程度与纳米孔的大小和位置有关。这种关联随着波长的增加而减弱。此外,纳米孔径的减小也会降低对 μLED 光学特性的影响。由于多孔 GaN 层有助于高质量 InGaN 的沉积,因此控制多孔 GaN 层的孔径将有助于开发基于 GaN 的红色 μLED 和全彩显示屏。
{"title":"Impact of nanopores in porous GaN on LED emission based on FDTD simulations","authors":"","doi":"10.1016/j.photonics.2024.101296","DOIUrl":"10.1016/j.photonics.2024.101296","url":null,"abstract":"<div><p>We simulated the light extraction efficiency (LEE) of porous GaN-based InGaN/GaN micrometer-sized light-emitting diodes (μLEDs) emitting within the visible wavelength range using the finite-difference time-domain (FDTD) method. The simulations show that the embedding of a porous GaN layer with 40 % porosity reduces the bottom LEE, while the top side LEE of the μLEDs is increased. In addition, it also exhibits complex scattering properties that affect the microcavity structure of these devices. The LEE and the degree of microcavity structure disruption are related to nanopore size and location. This association weakens with increasing wavelength. Also, a decrease in nanopore size corresponds to a diminished impact on μLED optical properties. Since the porous GaN layer contributes to the deposition of high-quality InGaN, controlling pore size of the porous GaN layer will aid the development of GaN-based red μLEDs and full-color displays.</p></div>","PeriodicalId":49699,"journal":{"name":"Photonics and Nanostructures-Fundamentals and Applications","volume":null,"pages":null},"PeriodicalIF":2.5,"publicationDate":"2024-07-09","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141698476","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2024-07-05DOI: 10.1016/j.photonics.2024.101295
Laurent Boulley, Paul Goulain, Pierre Laffaille, Thomas Maroutian, Raffaele Colombelli, Adel Bousseksou
Meta-surfaces arrays are 2D meta-materials with a periodicity below the diffraction limit that permits to obtain homogeneous layers of resonant effective refractive index. In this work we present an analytical model that describes the electromagnetic behavior of meta-surfaces constituted by split-ring resonators (SRR). SRR resonance frequency can be adjusted by choosing their geometric parameters and the materials they are made of. Their deposition on a phase change material enables an optical modulation of resonance peak during the phase transition. We demonstrate a mid-infrared tunable SRR meta-surface using Vanadium dioxide (VO2) as phase change material deposited on III-V semiconductors by low temperature pulsed laser ablation technique. The presented measurements exhibit a maximum of 100 cm−1 resonance shift. This result is very promising for the conception of monolithic, robust, compact, frequency tunable III-V based devices in the mid-infrared.
{"title":"Frequency tunable mid-infrared split ring resonators on a phase change material","authors":"Laurent Boulley, Paul Goulain, Pierre Laffaille, Thomas Maroutian, Raffaele Colombelli, Adel Bousseksou","doi":"10.1016/j.photonics.2024.101295","DOIUrl":"https://doi.org/10.1016/j.photonics.2024.101295","url":null,"abstract":"<div><p>Meta-surfaces arrays are 2D meta-materials with a periodicity below the diffraction limit that permits to obtain homogeneous layers of resonant effective refractive index. In this work we present an analytical model that describes the electromagnetic behavior of meta-surfaces constituted by split-ring resonators (SRR). SRR resonance frequency can be adjusted by choosing their geometric parameters and the materials they are made of. Their deposition on a phase change material enables an optical modulation of resonance peak during the phase transition. We demonstrate a mid-infrared tunable SRR meta-surface using Vanadium dioxide (VO<sub>2</sub>) as phase change material deposited on III-V semiconductors by low temperature pulsed laser ablation technique. The presented measurements exhibit a maximum of 100 cm<sup>−1</sup> resonance shift. This result is very promising for the conception of monolithic, robust, compact, frequency tunable III-V based devices in the mid-infrared.</p></div>","PeriodicalId":49699,"journal":{"name":"Photonics and Nanostructures-Fundamentals and Applications","volume":null,"pages":null},"PeriodicalIF":2.5,"publicationDate":"2024-07-05","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141583321","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2024-07-02DOI: 10.1016/j.photonics.2024.101293
Georges Humbert
The development of terahertz (THz) waveguides is limited by the high-conductivity losses of metals, the surface roughness, and the high-absorption of the dielectric materials. Consequently, dry air is certainly the most favorable medium to propagate THz radiations. A novel hollow-core THz waveguide enabling efficient THz wave propagation over 72 cm long length, is presented in this study. THz waves guiding in a hollow-core is achieved by an out-of-plane Photonic Band Gap (PBG) crystal cladding with a design inspired from the technology of hollow core PBG-crystal fibers. These fibers developed in the optical domains have demonstrated exceptional performances such as single mode propagation of light with low attenuation on kilometer length scales. The properties of the PBG guiding mechanism to forbid THz waves extension in the crystal cladding is exploited for enabling low-loss propagation in a waveguide fabricated with a highly absorptive material (ex. silica). PBG guidance into this new class of hollow-core THz waveguide were demonstrated theoretically and experimentally.
{"title":"Demonstration of THz waves propagation within a hollow-core THz waveguide based on an out-of-plane photonic bandgap crystal cladding","authors":"Georges Humbert","doi":"10.1016/j.photonics.2024.101293","DOIUrl":"https://doi.org/10.1016/j.photonics.2024.101293","url":null,"abstract":"<div><p>The development of terahertz (THz) waveguides is limited by the high-conductivity losses of metals, the surface roughness, and the high-absorption of the dielectric materials. Consequently, dry air is certainly the most favorable medium to propagate THz radiations. A novel hollow-core THz waveguide enabling efficient THz wave propagation over 72 cm long length, is presented in this study. THz waves guiding in a hollow-core is achieved by an out-of-plane Photonic Band Gap (PBG) crystal cladding with a design inspired from the technology of hollow core PBG-crystal fibers. These fibers developed in the optical domains have demonstrated exceptional performances such as single mode propagation of light with low attenuation on kilometer length scales. The properties of the PBG guiding mechanism to forbid THz waves extension in the crystal cladding is exploited for enabling low-loss propagation in a waveguide fabricated with a highly absorptive material (ex. silica). PBG guidance into this new class of hollow-core THz waveguide were demonstrated theoretically and experimentally.</p></div>","PeriodicalId":49699,"journal":{"name":"Photonics and Nanostructures-Fundamentals and Applications","volume":null,"pages":null},"PeriodicalIF":2.5,"publicationDate":"2024-07-02","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.sciencedirect.com/science/article/pii/S1569441024000683/pdfft?md5=b0272fae620ebfed818b9cde2cb77267&pid=1-s2.0-S1569441024000683-main.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141596778","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2024-07-01DOI: 10.1016/j.photonics.2024.101294
Mario Malerba , Mathieu Jeannin, Paul Goulain, Adel Bousseksou, Raffaele Colombelli, Jean-Michel Manceau
We present an experimental technique to accurately predict the formation of vibro-polaritons from a molecular polymeric film embedded in a resonant mid-infrared cavity. Using simple Fourier-transform reflectance measurement, we extract the complex dielectric function of a polyethylene film using Kramers-Kronig relations. The fitted dielectric function can be plugged into a numerical code to predict the strength and dispersion of the strong light-matter coupling regime between the quantized electromagnetic modes of a microcavity and the vibrational bands of the molecules. As a demonstration, we experimentally resolve the simultaneous formation of multiple vibro-polariton modes issued from the strong coupling of some vibrational bands of the methylene group (CH2) in a 2.5-μm-thick polyethylene film embedded in a microcavity. We measure a Rabi splitting of 6.3 THz for the stretching doublet around 87.5 THz and a Rabi splitting of 1.1 THz for the scissoring doublet around 43.7 THz, in excellent agreement with numerical predictions.
{"title":"Multiple micro-cavity vibro-polaritons formation with different vibrational bands of the methylene group","authors":"Mario Malerba , Mathieu Jeannin, Paul Goulain, Adel Bousseksou, Raffaele Colombelli, Jean-Michel Manceau","doi":"10.1016/j.photonics.2024.101294","DOIUrl":"https://doi.org/10.1016/j.photonics.2024.101294","url":null,"abstract":"<div><p>We present an experimental technique to accurately predict the formation of vibro-polaritons from a molecular polymeric film embedded in a resonant mid-infrared cavity. Using simple Fourier-transform reflectance measurement, we extract the complex dielectric function of a polyethylene film using Kramers-Kronig relations. The fitted dielectric function can be plugged into a numerical code to predict the strength and dispersion of the strong light-matter coupling regime between the quantized electromagnetic modes of a microcavity and the vibrational bands of the molecules. As a demonstration, we experimentally resolve the simultaneous formation of multiple vibro-polariton modes issued from the strong coupling of some vibrational bands of the methylene group (CH<sub>2</sub>) in a 2.5-μm-thick polyethylene film embedded in a microcavity. We measure a Rabi splitting of 6.3 THz for the stretching doublet around 87.5 THz and a Rabi splitting of 1.1 THz for the scissoring doublet around 43.7 THz, in excellent agreement with numerical predictions.</p></div>","PeriodicalId":49699,"journal":{"name":"Photonics and Nanostructures-Fundamentals and Applications","volume":null,"pages":null},"PeriodicalIF":2.5,"publicationDate":"2024-07-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141539842","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}