The combination of vacuum preloading and electroosmosis (VPE) enables simultaneous consolidation and remediation of dredged sediments, supporting the sustainable development of global dredging industry. However, the lack of a coupled model for dredged sediments improvement under VPE has become an obstacle to the optimisation of VPE. Therefore, a coupled model integrating electrical, hydraulic, mechanical, and chemical fields was established in this study. The numerical simulations using different consolidation equations were compared with the experimental results, including electric field intensity, excess pore water pressure, settlement, and Cu concentrations. The results indicated that the adoption of Biot’s consolidation equation in the coupled model enabled a more accurate prediction of dredged sediments consolidation and remediation performance. The numerical simulations further revealed that a lower electric potential combined with a longer treatment time resulted in a more uniform treatment effect, whereas a higher electric potential combined with a shorter treatment time accelerated Cu removal. The removal of pollutants in the deeper dredged sediment layers was markedly enhanced as the applied vacuum pressure increased. An early intervention of vacuum pressure enhanced the consolidation of dredged sediments; however, this effect gradually diminished as the treatment progressed.
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