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Improved electrical conductivity of graphene film using thermal expansion-assisted hot pressing method 利用热膨胀辅助热压法提高石墨烯薄膜的导电性
IF 0.8 4区 物理与天体物理 Q3 PHYSICS, MULTIDISCIPLINARY Pub Date : 2024-10-17 DOI: 10.1007/s40042-024-01184-7
Dongpyo Hong, Gun-Sik Park

Achieving highly conductive graphene films requires the elimination of pores formed during the thermal reduction of graphene oxide (GO). Conventional methods such as hydraulic pressing often struggle to remove these pores effectively, especially in sub-micron large area films for uniform high pressure. In this study, we introduce a thermal expansion-assisted hot pressing (TEHP) technique that leverages the differential thermal expansion between graphite and tungsten to achieve pore-free, highly conductive graphene films. Here we heat the GO film sandwiched between graphite (high thermal expansion coefficient) and tungsten (low thermal expansion coefficient) to 1800 °C where pressures of 13–48 MPa are estimated. The TEHP resulted in graphene films with a smooth, metallic surface, free of macropores. Raman spectroscopy and electron microscopy analyses confirmed the enhanced crystallinity and compactness of the films. The electrical conductivity of the hot-pressed graphene films shows a threefold improvement over normally annealed films. This scalable method offers a viable pathway for producing high-performance graphene films for advanced applications.

要获得高导电性石墨烯薄膜,就必须消除氧化石墨烯(GO)热还原过程中形成的孔隙。液压压制等传统方法往往难以有效消除这些孔隙,尤其是在亚微米级大面积薄膜的均匀高压下。在本研究中,我们介绍了一种热膨胀辅助热压(TEHP)技术,该技术利用石墨和钨之间的热膨胀差来实现无孔隙、高导电性的石墨烯薄膜。在这里,我们将夹在石墨(热膨胀系数高)和钨(热膨胀系数低)之间的 GO 薄膜加热到 1800 °C,估计压力为 13-48 兆帕。TEHP 使石墨烯薄膜具有光滑的金属表面,没有大孔。拉曼光谱和电子显微镜分析证实,薄膜的结晶度和致密性得到了增强。热压石墨烯薄膜的导电性比正常退火的薄膜提高了三倍。这种可扩展的方法为生产用于先进应用的高性能石墨烯薄膜提供了一条可行的途径。
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引用次数: 0
A study on the effect of correlated data on predictive capabilities 相关数据对预测能力影响的研究
IF 0.8 4区 物理与天体物理 Q3 PHYSICS, MULTIDISCIPLINARY Pub Date : 2024-10-17 DOI: 10.1007/s40042-024-01197-2
Ui-Jung Hwang, Jeong-Eun Rah

The purpose of this study is to design a predictive model for a daily quality assurance (QA) system that remains unaffected by specific patterns in correlated time series data. All data were sampled from the measured output factor at specific times over a 5-year period during the daily QA process for a 6 MV photon beam of the Varian linear accelerator (LINAC) system. Before constructing predictive structures, an autocorrelation function (ACF) analysis was conducted to verify the correlation of the given time series data. This study determined the optimal configuration for the autoregressive integrated moving average (ARIMA) and nonlinear autoregressive (NAR) neural network models for prediction. Additionally, it utilized correlated time series data to evaluate its impact on the predictive capability. We then compared the actual QA values to those predicted by the selected ARIMA and NAR models for the sampled daily output. Our findings suggest that while the ARIMA model offers a quick and relatively easy approach without requiring complex computational methods, the NAR model outperforms ARIMA, especially in the context of correlated time series data, demonstrating its real clinical utility as a prediction model. This result reveals that correlations are frequently observed in daily QA data. We concluded that these correlations can substantially influence the accuracy of machine behavior predicted based on historical observations. Consequently, analyzing specific patterns and correlated data is imperative for designing predictive structures.

本研究的目的是为日常质量保证(QA)系统设计一个不受相关时间序列数据特定模式影响的预测模型。在瓦里安直线加速器(LINAC)系统的 6 MV 光子束的日常质量保证过程中,所有数据都是在 5 年的特定时间从测量的输出因子中采样的。在构建预测结构之前,进行了自相关函数 (ACF) 分析,以验证给定时间序列数据的相关性。这项研究确定了用于预测的自回归综合移动平均(ARIMA)和非线性自回归(NAR)神经网络模型的最佳配置。此外,研究还利用相关时间序列数据来评估其对预测能力的影响。然后,我们将实际质量保证值与所选的 ARIMA 和 NAR 模型对每日采样输出的预测值进行了比较。我们的研究结果表明,ARIMA 模型提供了一种快速且相对简单的方法,无需复杂的计算方法,而 NAR 模型则优于 ARIMA 模型,尤其是在相关时间序列数据的情况下,这证明了它作为预测模型的真正临床实用性。这一结果揭示了日常质量保证数据中经常出现的相关性。我们得出结论,这些相关性会严重影响根据历史观察结果预测机器行为的准确性。因此,分析特定模式和相关数据对于设计预测结构至关重要。
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引用次数: 0
A customized template matching classification system 定制模板匹配分类系统
IF 0.8 4区 物理与天体物理 Q3 PHYSICS, MULTIDISCIPLINARY Pub Date : 2024-10-08 DOI: 10.1007/s40042-024-01182-9
Jie Xu, Changmao Yang, Jianping Chen

This paper presents two novel classification techniques, the customized template matching classifier (CTMC) and the dynamic template matching classifier (DTMC), which aim to significantly enhance the performance of the minimum distance classifier (MDC). CTMC tailors a feature subspace specifically for MDC, leveraging a set of effective templates that capture the distinguishing characteristics of each class. This customized feature space ensures accurate representation and enhanced distinguishability between classes, thereby improving MDC’s classification accuracy. DTMC, on the other hand, builds upon the CTMC approach by introducing a dynamic template optimization process. Inspired by semi-supervised learning techniques, DTMC utilizes unlabeled data to enrich class information and iteratively update the templates in the feature space. This dynamic optimization process allows DTMC to adapt to variations in the data, further enhancing the classification performance of MDC. Our key contributions include: (1) introducing the concept of a customized feature space tailored for MDC, demonstrating its effectiveness in improving classifier performance; (2) presenting CTMC and DTMC as comprehensive classification systems that seamlessly integrate feature extraction and classification, outperforming traditional loosely coupled approaches; and (3) incorporating a reliability mechanism to assess the classification of test samples, enabling the selection of high-reliability samples to update class templates, effectively addressing the issue of limited labeled data and further boosting the overall performance of the classification system.

本文介绍了两种新颖的分类技术--定制模板匹配分类器(CTMC)和动态模板匹配分类器(DTMC),旨在显著提高最小距离分类器(MDC)的性能。CTMC 专门为 MDC 定制了一个特征子空间,利用一组有效模板捕捉每个类别的显著特征。这种定制的特征空间可确保类别之间的准确表征和更强的可区分性,从而提高 MDC 的分类准确性。另一方面,DTMC 在 CTMC 方法的基础上引入了动态模板优化过程。受半监督学习技术的启发,DTMC 利用未标记数据来丰富类别信息,并迭代更新特征空间中的模板。这种动态优化过程使 DTMC 能够适应数据的变化,从而进一步提高 MDC 的分类性能。我们的主要贡献包括(1) 引入了为 MDC 量身定制的特征空间概念,证明了其在提高分类器性能方面的有效性;(2) 将 CTMC 和 DTMC 作为综合分类系统,无缝集成了特征提取和分类,优于传统的松散耦合方法;以及 (3) 采用可靠性机制来评估测试样本的分类,从而能够选择高可靠性样本来更新类模板,有效解决了标记数据有限的问题,进一步提高了分类系统的整体性能。
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引用次数: 0
Characterization of SERS–fluorescence bimodal nanocomposites from Au-decorated CaTiO3:Eu3+ 金装饰 CaTiO3:Eu3+ SERS 荧光双模纳米复合材料的表征
IF 0.8 4区 物理与天体物理 Q3 PHYSICS, MULTIDISCIPLINARY Pub Date : 2024-10-03 DOI: 10.1007/s40042-024-01181-w
Da Young Kim, Gyeong Bok Jung

Surface-enhanced Raman scattering (SERS)–fluorescence bimodal composites have attracted great interest for biomedical applications. Herein, we report the characterization of Au-decorated CaTiO3:Eu3+ nanocomposites (CaTiO3:Eu3+@Au NCs) using SERS and fluorescence properties. X-ray diffraction (XRD) of the CaTiO3:Eu3+@Au NCs shows orthorhombic phases, which are in good agreement with the standard CaTiO3 XRD peaks. The photoluminescence (PL) spectra show a strong visible red emission at 614 nm (5D0 → 7F2) with an excitation wavelength of 380 nm. The PL-emission intensity of the CaTiO3:Eu3+@Au NCs increased more than that of the CaTiO3:Eu3+ powder. The maximum PL-emission intensity of the CaTiO3:Eu3+@Au NCs was obtained at an Au doping concentration of 0.8 mol/L; however, the intensity at higher Au doping concentrations (> 0.8 mol/L) was lower. This behavior is consistent with the SERS results. These results suggest that varying the Au nanoparticle concentration can control the PL-emission intensity and SERS of the CaTiO3:Eu3+@Au NCs. Therefore, CaTiO3:Eu3+@Au NCs may be useful for multiplex detection and bioimaging.

表面增强拉曼散射(SERS)-荧光双模复合材料在生物医学应用中引起了极大的兴趣。在此,我们利用 SERS 和荧光特性对金装饰的 CaTiO3:Eu3+ 纳米复合材料(CaTiO3:Eu3+@Au NCs)进行了表征。CaTiO3:Eu3+@Au NCs 的 X 射线衍射 (XRD) 显示出正菱形相,与标准 CaTiO3 XRD 峰值非常吻合。光致发光(PL)光谱显示,在波长为 380 nm 的激发波长下,在 614 nm 处有强烈的可见红色发射(5D0 → 7F2)。与 CaTiO3:Eu3+ 粉末相比,CaTiO3:Eu3+@Au NCs 的 PL 发射强度增加得更多。在金掺杂浓度为 0.8 摩尔/升时,CaTiO3:Eu3+@Au NCs 的 PL 发射强度达到最大值;然而,在较高的金掺杂浓度(> 0.8 摩尔/升)下,其强度较低。这一行为与 SERS 结果一致。这些结果表明,改变金纳米粒子的浓度可以控制 CaTiO3:Eu3+@Au NCs 的 PL 发射强度和 SERS。因此,CaTiO3:Eu3+@Au NCs 可用于多重检测和生物成像。
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引用次数: 0
Resistivity characteristics near the metal–insulator transition in the half-filled Anderson–Hubbard model 半填充安德森-哈伯德模型中金属-绝缘体转变附近的电阻特性
IF 0.8 4区 物理与天体物理 Q3 PHYSICS, MULTIDISCIPLINARY Pub Date : 2024-10-03 DOI: 10.1007/s40042-024-01186-5
Thi-Hai-Yen Nguyen, Anh-Tuan Hoang, Duc-Anh Le

In this study, we calculate the dc resistivity of the half-filled disordered Hubbard model near the Mott and Anderson metal–insulator transitions. We employ the standard Kubo formula with typical medium dynamical mean field theory to perform our calculations. Our investigation explores the effects of random potential, on-site Coulomb interaction, and temperature on the dc resistivity within the model. In addition, we highlight and discuss the distinct resistivity behaviors observed near the Mott and Anderson transitions.

在本研究中,我们计算了莫特和安德森金属绝缘体转变附近半填充无序哈伯德模型的直流电阻率。我们采用标准久保公式和典型的介质动力学均场理论进行计算。我们的研究探讨了随机电势、现场库仑相互作用和温度对模型内直流电阻率的影响。此外,我们还强调并讨论了在莫特和安德森转变附近观察到的不同电阻率行为。
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引用次数: 0
Erratum: Comparative analysis of single and triple material 10 nm Tri-gate FinFET 勘误:单材料和三材料 10 纳米三栅极 FinFET 的比较分析
IF 0.8 4区 物理与天体物理 Q3 PHYSICS, MULTIDISCIPLINARY Pub Date : 2024-10-03 DOI: 10.1007/s40042-024-01191-8
Shankhamitra Sunani, Satya Sopan Mahato, Kanjalochan Jena, Raghunandan Swain
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引用次数: 0
Revisit to the fluid Love numbers and the permanent tide of the Earth 重温流动的爱的数字和地球永久的潮汐
IF 0.8 4区 物理与天体物理 Q3 PHYSICS, MULTIDISCIPLINARY Pub Date : 2024-10-03 DOI: 10.1007/s40042-024-01174-9
Sung-Ho Na, Yu Yi, Young-Hong Shin

Love numbers h, k, and l are convenient parameters to assess the deformation of the Earth or other planet due to external perturbing forces. While the elastic Love numbers are used for tidal deformation, the correct amount of permanent tidal deformation can be assessed using the fluid Love numbers. Accurate values of the elastic Love numbers of Earth have been repeatedly attained for several Earth models, and also the fluid Love numbers hf and kf of the Earth were recently reported. In this short note, new evaluation of the Earth’s fluid Love number as well as secular Love number, both originally defined by Munk and MacDonald, is presented using updated values of the Earth’s physical property model and with minute enhancement in the formulation; ({(h}_{s}, {k}_{s}) =(1.9437, 0.9437)) by their 1st approach and ({(h}_{f}, {k}_{f}) =(1.9337, 0.9337)) by their 2nd approach. Through numerical calculations with gradual stepwise reduction in rigidity, the three fluid Love numbers of the Earth were determined as: (hf, kf, lf) = (1.935, 0.935, 1.07) for PREM and (hf, kf, lf) = (1.937, 0.937, 1.07) for ak135-F Earth models. In addition, the fluid Love numbers of other spherical harmonic degrees 0, 3, 4, and 5 were estimated. The permanent tide of the Earth ellipsoid due to the Moon and the Sun has been re-calculated: the vertical displacement of the permanent tide is 0.1924 m at the equator and (- 0.3801) m at the pole, while the horizontal displacement of the permanent tide is found to be 0.317 m at mid-latitude.

爱数 h、k 和 l 是评估地球或其他行星在外部扰动力作用下发生形变的便捷参数。弹性爱数用于潮汐形变,而永久潮汐形变的正确量则可以用流体爱数来评估。在几个地球模型中,地球弹性爱数的精确值已被反复求得,最近还报告了地球流体爱数 hf 和 kf。在这篇短文中,使用地球物理性质模型的更新值和微小的改进公式,对最初由 Munk 和 MacDonald 定义的地球流体爱数和世俗爱数进行了新的评估;({(h}_{s}, {k}_{s}) =(1.9437,0.9437);第二种方法是 ({(h}_{f}, {k}_{f})=(1.9337,0.9337))。通过逐步降低刚度的数值计算,确定了地球的三个流体洛夫数:(hf, kf, lf) = (1.935, 0.935, 1.07);ak135-F 地球模型的 (hf, kf, lf) = (1.937, 0.937, 1.07)。此外,还估算了其他球谐波度 0、3、4 和 5 的流体爱数。重新计算了月球和太阳引起的地球椭球体永久潮汐:永久潮汐的垂直位移在赤道为 0.1924 米,在极点为(- 0.3801)米,而永久潮汐的水平位移在中纬度为 0.317 米。
{"title":"Revisit to the fluid Love numbers and the permanent tide of the Earth","authors":"Sung-Ho Na,&nbsp;Yu Yi,&nbsp;Young-Hong Shin","doi":"10.1007/s40042-024-01174-9","DOIUrl":"10.1007/s40042-024-01174-9","url":null,"abstract":"<div><p>Love numbers <i>h</i>, <i>k</i>, and <i>l</i> are convenient parameters to assess the deformation of the Earth or other planet due to external perturbing forces. While the elastic Love numbers are used for tidal deformation, the correct amount of permanent tidal deformation can be assessed using the fluid Love numbers. Accurate values of the elastic Love numbers of Earth have been repeatedly attained for several Earth models, and also the fluid Love numbers <i>h</i><sub><i>f</i></sub> and <i>k</i><sub><i>f</i></sub> of the Earth were recently reported. In this short note, new evaluation of the Earth’s fluid Love number as well as secular Love number, both originally defined by Munk and MacDonald, is presented using updated values of the Earth’s physical property model and with minute enhancement in the formulation; <span>({(h}_{s}, {k}_{s}) =(1.9437, 0.9437))</span> by their 1st approach and <span>({(h}_{f}, {k}_{f}) =(1.9337, 0.9337))</span> by their 2nd approach. Through numerical calculations with gradual stepwise reduction in rigidity, the three fluid Love numbers of the Earth were determined as: (<i>h</i><sub><i>f</i></sub>, <i>k</i><sub><i>f</i></sub>, <i>l</i><sub><i>f</i></sub>) = (1.935, 0.935, 1.07) for PREM and (<i>h</i><sub><i>f</i></sub>, <i>k</i><sub><i>f</i></sub>, <i>l</i><sub><i>f</i></sub>) = (1.937, 0.937, 1.07) for ak135-F Earth models. In addition, the fluid Love numbers of other spherical harmonic degrees 0, 3, 4, and 5 were estimated. The permanent tide of the Earth ellipsoid due to the Moon and the Sun has been re-calculated: the vertical displacement of the permanent tide is 0.1924 m at the equator and <span>(- 0.3801)</span> m at the pole, while the horizontal displacement of the permanent tide is found to be 0.317 m at mid-latitude.</p></div>","PeriodicalId":677,"journal":{"name":"Journal of the Korean Physical Society","volume":"85 9","pages":"783 - 790"},"PeriodicalIF":0.8,"publicationDate":"2024-10-03","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142540563","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Dictionary learning-based denoising algorithm with expected patch log likelihood in diffusion-weighted magnetic resonance image 基于字典学习的去噪算法与扩散加权磁共振图像中的预期补丁对数似然法
IF 0.8 4区 物理与天体物理 Q3 PHYSICS, MULTIDISCIPLINARY Pub Date : 2024-09-25 DOI: 10.1007/s40042-024-01167-8
Kyuseok Kim, Hyun-Woo Jeong, Youngjin Lee

Diffusion-weighted imaging (DWI) is one of the most sensitive techniques to noise among magnetic resonance imaging (MRI) techniques. As the b-value used to acquire the DWI image increases, an image in which the difference in diffusion is emphasized can be obtained. However, DWI images with increased b-values inevitably have a major drawback in that noise is amplified. Thus, in this study, a dictionary learning (DL)-based denoising algorithm was modeled and applied to DWI images. The designed algorithm was modeled as a DL-based algorithm using the expected patch log likelihood. The DWI images were obtained by adjusting the b-value from 400 to 400 intervals. When the proposed DL-based denoising algorithm was applied to DWI, we confirmed that the contrast-to-noise ratio and coefficient of variation were improved by approximately 4.26 and 5.22 times, respectively, compared with noisy images. In conclusion, we expect that the proposed DL-based denoising algorithm will be highly efficient in acquiring DWI images using a high b-value, which is useful for observing acute cerebral infarction and microvascular disease.

扩散加权成像(DWI)是磁共振成像(MRI)技术中对噪音最敏感的技术之一。随着获取 DWI 图像所用 b 值的增加,可获得弥散差异突出的图像。然而,增加 b 值的 DWI 图像不可避免地存在一个主要缺点,即噪声会被放大。因此,本研究建立了一种基于字典学习(DL)的去噪算法模型,并将其应用于 DWI 图像。所设计的算法是利用期望补丁对数似然建立的基于词典学习的算法模型。DWI 图像是通过将 b 值从 400 调整到 400 间隔来获得的。当将所提出的基于 DL 的去噪算法应用于 DWI 时,我们证实对比度-噪声比和变异系数与噪声图像相比分别提高了约 4.26 倍和 5.22 倍。总之,我们希望所提出的基于 DL 的去噪算法能高效获取高 b 值的 DWI 图像,这对观察急性脑梗塞和微血管疾病非常有用。
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引用次数: 0
Microscopic property of Li impurity in biphasic calcium phosphate 双相磷酸钙中李杂质的显微特性
IF 0.8 4区 物理与天体物理 Q3 PHYSICS, MULTIDISCIPLINARY Pub Date : 2024-09-25 DOI: 10.1007/s40042-024-01180-x
Maengsuk Kim, Chul Hong Park

Recently Li doping is employed to control the properties of bioceramic biphasic calcium phosphate (BCP), which consists of (beta -hbox {Ca}_{3}(hbox {PO}_4)_2) ((beta)-TCP) and hydroxyapatite(HAp). We investigated the microscopic properties of Li in BCP through first-principles electronic structure calculations. The stable microscopic structure of Li-driven state is identified by comparing the formation enthalpies of Li-driven structures: interstitial ((hbox {Li}_{int})) and substitutional ((hbox {Li}_{Ca})). It is found that the (hbox {Li}_{int}) is more stable than the substitutional state (hbox {Li}_{Ca}). The (hbox {Li}_{int}) atom is strongly coupled to three or four O atoms, which stabilizes the interstitial state. The (hbox {Li}_{int}) is calculated to be relatively more stable in (beta)-TCP than in HAp, because the electronic level of (hbox {Li}_{int}) is much lower in (beta)-TCP than in HAp.

最近,掺杂锂被用来控制生物陶瓷双相磷酸钙(BCP)的性质,它由((betahbox {Ca}_{3}(hbox {PO}_4)_2) ((beta)-TCP)和羟基磷灰石(HAp)组成。我们通过第一原理电子结构计算研究了锂在 BCP 中的微观性质。通过比较锂驱动结构:间隙结构((hbox {Li}_{int})和取代结构((hbox {Li}_{Ca})的形成焓,确定了锂驱动态的稳定微观结构。)研究发现,(hbox {Li}_{int}/)比置换态(hbox {Li}_{Ca}/)更稳定。(/hbox{Li}_{int}/)原子与三个或四个 O 原子强耦合,从而稳定了间隙态。根据计算,(hbox {Li}_{int})在(beta)-TCP中比在HAp中相对更稳定,因为(hbox {Li}_{int})的电子水平在(beta)-TCP中比在HAp中低得多。
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引用次数: 0
Experimental comparative study between simple and multi-tube DBD ozone generator with same volume discharge for wastewater treatment 用于废水处理的简易和多管 DBD 臭氧发生器在相同排出量下的实验对比研究
IF 0.8 4区 物理与天体物理 Q3 PHYSICS, MULTIDISCIPLINARY Pub Date : 2024-09-25 DOI: 10.1007/s40042-024-01179-4
Essama Ahmed Ghaitaoui, Kamel Nassour, Said Nemmich, Brahim El Khalil Oulad Naoui, Touhami Ghaitaoui, Amar Tilmatine, Nadia Ramdani

Numerous studies have focused on analyzing and enhancing the performance of ozone generation systems to achieve higher ozone concentrations with lower energy consumption. This paper presents an experimental comparative study between a multi-tube DBD ozone generator with a parallel tube configuration and a simple DBD ozone generator with the same discharge volume, where the energy efficiency and produced ozone concentration were analyzed. Subsequently, the multi-tube ozone generator was employed for the wastewater treatment of the Moulay Slissen sewage-treatment plant in Sidi Bel Abbes. The results demonstrated that the new multi-tube ozone generator exhibited significantly improved performance in terms of energy efficiency and produced ozone concentration levels compared to the simple DBD generator. Furthermore, through the analyses conducted on the wastewater samples before and after treatment, the advanced generator proved its efficacy in improving the physicochemical and bacteriological quality of wastewater.

许多研究都侧重于分析和提高臭氧发生系统的性能,以便在降低能耗的同时获得更高的臭氧浓度。本文介绍了平行管配置的多管 DBD 臭氧发生器与相同排出量的简单 DBD 臭氧发生器之间的实验对比研究,分析了能量效率和产生的臭氧浓度。随后,多管臭氧发生器被用于 Sidi Bel Abbes 的 Moulay Slissen 污水处理厂的废水处理。结果表明,与简单的 DBD 臭氧发生器相比,新型多管臭氧发生器在能效和产生的臭氧浓度水平方面都有显著提高。此外,通过对处理前后的废水样本进行分析,先进的发生器证明了其在改善废水物理化学和细菌学质量方面的功效。
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引用次数: 0
期刊
Journal of the Korean Physical Society
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