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Electromagnetic Functions Modulation of Recycled By-Products by Heterodimensional Structure
IF 26.6 1区 材料科学 Q1 Engineering Pub Date : 2025-02-06 DOI: 10.1007/s40820-025-01659-7
Ze Nan, Wei Wei, Zhenhua Lin, Ruimei Yuan, Miao Zhang, Jincheng Zhang, Jianyong Ouyang, Jingjing Chang, Hejun Li, Yue Hao

Highlights

  • Turning trash into treasure: The outstanding tunable aerogels were fabricated via heterodimensional by-products of silver nanowires. The first tunable form, aerogel film, shields electromagnetic interference (EMI SE > 89 dB), while the second tunable form, aerogel foam, performs dual EM functions (EMI SE > 30 dB and RL < -35 dB, EAB > 6.7 GHz).

  • Recycle again: The secondary recycled aerogels retain nearly all of their EM protection qualities, making this closed-loop cycle desirable.

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引用次数: 0
Light Management in 2D Perovskite Toward High-Performance Optoelectronic Applications
IF 26.6 1区 材料科学 Q1 Engineering Pub Date : 2025-02-06 DOI: 10.1007/s40820-024-01643-7
Kailian Dong, Tao Jiang, Guoyi Chen, Hongsen Cui, Shuxin Wang, Shun Zhou, Chen Wang, Yi Yang, Fang Yao, Chen Tao, Weijun Ke, Guojia Fang

Highlights

  • The light management strategy is introduced into two-dimensional Dion-Jacobson (2D DJ) perovskite and subsequently elucidated both experimentally and theoretically.

  • The synthesis of surface-patterned BDAPbBr4 microplates with high crystalline quality demonstrates the first reported instance of growing such 2D DJ-type perovskite microplates.

  • The optimized device exhibits excellent photodetection performance under UV region. Moreover, this work represents the successful demonstration of BDAPbBr4 perovskite for UV weak-light communication, imaging, and polarized light detection.

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引用次数: 0
Multifunctional Carbon Foam with Nanoscale Chiral Magnetic Heterostructures for Broadband Microwave Absorption in Low Frequency
IF 26.6 1区 材料科学 Q1 Engineering Pub Date : 2025-02-06 DOI: 10.1007/s40820-025-01658-8
Hao Zhang, Kaili Kuang, Yifeng Zhang, Chen Sun, Tingkang Yuan, Ruilin Yin, Zeng Fan, Renchao Che, Lujun Pan

The construction of carbon nanocoil (CNC)-based chiral-dielectric-magnetic trinity composites is considered as a promising approach to achieve excellent low-frequency microwave absorption. However, it is still challenging to further enhance the low frequency microwave absorption and elucidate the related loss mechanisms. Herein, the chiral CNCs are first synthesized on a three-dimensional (3D) carbon foam and then combined with the FeNi/NiFe2O4 nanoparticles to form a novel chiral-dielectric-magnetic trinity foam. The 3D porous CNC-carbon foam network provides excellent impedance matching and strong conduction loss. The formation of the FeNi-carbon interfaces induces interfacial polarization loss, which is confirmed by the density functional theory calculations. Further permeability analysis and the micromagnetic simulation indicate that the nanoscale chiral magnetic heterostructures achieve magnetic pinning and coupling effects, which enhance the magnetic anisotropy and magnetic loss capability. Owing to the synergistic effect between dielectricity, chirality, and magnetism, the trinity composite foam exhibits excellent microwave absorption performance with an ultrabroad effective absorption bandwidth (EAB) of 14 GHz and a minimum reflection of loss less than − 50 dB. More importantly, the C-band EAB of the foam is extended to 4 GHz, achieving the full C-band coverage. This study provides further guidelines for the microstructure design of the chiral-dielectric-magnetic trinity composites to achieve broadband microwave absorption.

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引用次数: 0
Artificial Intelligence-Powered Materials Science
IF 26.6 1区 材料科学 Q1 Engineering Pub Date : 2025-02-06 DOI: 10.1007/s40820-024-01634-8
Xiaopeng Bai, Xingcai Zhang

The advancement of materials has played a pivotal role in the advancement of human civilization, and the emergence of artificial intelligence (AI)-empowered materials science heralds a new era with substantial potential to tackle the escalating challenges related to energy, environment, and biomedical concerns in a sustainable manner. The exploration and development of sustainable materials are poised to assume a critical role in attaining technologically advanced solutions that are environmentally friendly, energy-efficient, and conducive to human well-being. This review provides a comprehensive overview of the current scholarly progress in artificial intelligence-powered materials science and its cutting-edge applications. We anticipate that AI technology will be extensively utilized in material research and development, thereby expediting the growth and implementation of novel materials. AI will serve as a catalyst for materials innovation, and in turn, advancements in materials innovation will further enhance the capabilities of AI and AI-powered materials science. Through the synergistic collaboration between AI and materials science, we stand to realize a future propelled by advanced AI-powered materials.

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引用次数: 0
Multifunctional Janus-Structured Polytetrafluoroethylene-Carbon Nanotube-Fe3O4/MXene Membranes for Enhanced EMI Shielding and Thermal Management
IF 26.6 1区 材料科学 Q1 Engineering Pub Date : 2025-02-06 DOI: 10.1007/s40820-025-01647-x
Runze Shao, Guilong Wang, Jialong Chai, Jun Lin, Guoqun Zhao, Zhihui Zeng, Guizhen Wang

Highlights

  • The Janus-type multifunctional ultra-flexible polytetrafluoroethylene-carbon nanotube-Fe3O4/MXene (FCFe/M) membranes were fabricated via a shear-induced in situ fibrillation technique followed by vacuum-assisted filtration.

  • Thanks to the strategic distribution of the MXene conductive reflection layer and the silk-like FCFe electromagnetic wave’s absorption layer, the membranes achieve robust electromagnetic interference shielding and effective antireflection through the absorption-reflection-reabsorption mechanism.

  • The membranes exhibit exceptional thermal management performance, including efficient heat dissipation and electrothermal/photothermal conversion capabilities, further enhancing their promising potential for applications in flexible wearable technologies.

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引用次数: 0
Functionalized Separators Boosting Electrochemical Performances for Lithium Batteries
IF 26.6 1区 材料科学 Q1 Engineering Pub Date : 2025-02-05 DOI: 10.1007/s40820-024-01596-x
Zixin Fan, Xiaoyu Chen, Jingjing Shi, Hui Nie, Xiaoming Zhang, Xingping Zhou, Xiaolin Xie, Zhigang Xue

Highlights

  • The commonly used modification methods for separator of lithium batteries are summarized, which include surface coating, in situ modification and grafting modification.

  • The adhesion of coating materials with the separators and wettability of the modified separators prepared from the three methods are compared.

  • The challenges and future directions of separator modification are provided.

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引用次数: 0
Multiscale Biomimetic Evaporators Based on Liquid Metal/Polyacrylonitrile Composite Fibers for Highly Efficient Solar Steam Generation
IF 26.6 1区 材料科学 Q1 Engineering Pub Date : 2025-02-05 DOI: 10.1007/s40820-025-01661-z
Yuxuan Sun, Dan Liu, Fei Zhang, Xiaobo Gao, Jie Xue, Qingbin Zheng

Highlights

  • A three-dimensional multiscale liquid metal/polyacrylonitrile evaporator is fabricated through wet spinning and assembly.

  • The evaporator exhibits an outstanding water evaporation rate of 2.66 kg m−2 h−1 with a solar energy efficiency of 96.5% under one sun irradiation.

  • The evaporator demonstrates a superior purification performance for seawater and sewage under light irradiation.

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引用次数: 0
Enhanced Conductivity of Multilayer Copper–Carbon Nanofilms via Plasma Immersion Deposition
IF 26.6 1区 材料科学 Q1 Engineering Pub Date : 2025-02-05 DOI: 10.1007/s40820-024-01628-6
Haotian Weng, Xiwu Zhang, Xuan Liu, Yunhui Tang, Hewei Yuan, Yang Xu, Kun Li, Xiaolu Huang

Although room-temperature superconductivity is still difficult to achieve, researching materials with electrical conductivity significantly higher than that of copper will be of great importance in improving energy efficiency, reducing costs, lightening equipment weight, and enhancing overall performance. Herein, this study presents a novel copper–carbon nanofilm composite with enhanced conductivity which has great applications in the electronic devices and electrical equipment. Multilayer copper–carbon nanofilms and interfaces with superior electronic structures are formed based on copper materials using plasma immersion nanocarbon layer deposition technology, effectively enhancing conductivity. Experimental results show that for a five-layer copper–carbon nanofilm composite, the conductivity improves significantly when the thickness of the carbon nanofilm increases. When the carbon nanofilm accounts for 16% of the total thickness, the overall conductivity increases up to 30.20% compared to pure copper. The mechanism of the enhanced conductivity is analyzed including roles of copper atom adsorption sites and electron migration pathways by applying effective medium theory, first-principles calculations and density of states analysis. Under an applied electric field, the high-density electrons in the copper film can migrate into the nanocarbon film, forming highly efficient electron transport channels, which significantly enhance the material’s conductivity. Finally, large-area electrode coating equipment is developed based on this study, providing the novel and robust strategy to enhance the conductivity of copper materials, which enables industrial application of copper–carbon nanocomposite films in the field of high conductivity materials.

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引用次数: 0
Advanced Bismuth-Based Anode Materials for Efficient Potassium Storage: Structural Features, Storage Mechanisms and Modification Strategies
IF 26.6 1区 材料科学 Q1 Engineering Pub Date : 2025-01-31 DOI: 10.1007/s40820-024-01641-9
Yiye Tan, Fanglan Mo, Hongyan Li

Highlights

  • Various bismuth-based materials used in potassium-ion batteries (PIBs) anode are classified and overviewed, and the structure and potassium storage mechanism of various materials are discussed.

  • The advantages and challenges of different PIBs anode materials are pointed out, and the existing modification strategies to improve potassium storage are summarized.

  • The promising research directions of bismuth-based anode materials are proposed.

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引用次数: 0
Novel Cellulosic Fiber Composites with Integrated Multi-Band Electromagnetic Interference Shielding and Energy Storage Functionalities
IF 26.6 1区 材料科学 Q1 Engineering Pub Date : 2025-01-31 DOI: 10.1007/s40820-025-01652-0
Xuewen Han, Cheng Hao, Yukang Peng, Han Yu, Tao Zhang, Haonan Zhang, Kaiwen Chen, Heyu Chen, Zhenxing Wang, Ning Yan, Junwen Pu

Highlights

  • A mild 2,2,6,6-tetramethylpiperidine-1-oxide mediated modification system was applied to improve the reactivity and introduce porous structure of cellulose fiber skeleton.

  • Composite exhibited highly efficient electromagnetic shielding interference performance (> 99.99%) over multi-band.

  • Integrating energy storage, electromagnetic interference shielding, and structural design into bio-based materials.

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Nano-Micro Letters
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