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A Trade-Off between Pulse Energy and Stability in Seeded Free-Electron Lasers 种子自由电子激光器中脉冲能量与稳定性的权衡
IF 3.9 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2025-06-25 DOI: 10.1002/adpr.202400219
Li Zeng, Huaiqian Yi, Xiaofan Wang, Chao Feng, Weiqing Zhang

Over the last decade, external seeded free-electron lasers (FELs) have achieved significant advancements across various disciplines, progressively establishing themselves as indispensable tools in fields ranging from fundamental science to industrial applications. The performance of seeded FELs is critically dependent on the quality of the frequency up-conversion process. Optimized conditions for seeded FELs are typically considered as the maximization of the bunching factor. This article discusses alternative perspectives on the optimization criteria for seeded FELs by analyzing the impact of dispersion strength on their overall performance. This study investigates the differences among the required dispersion strength for achieving the maximum bunching factor, maximum pulse energy, optimal energy stability through theoretical analysis, simulation calculations, and experimental explorations. The direct observation in experiments emphasizes the consideration of trade-off between pulse energy and energy stability in seeded FELs. These results provide valuable insights and practical guidance for controlling the pulse characteristics of seeded FELs, contributing to the tuning and optimization of FEL facilities.

在过去的十年中,外部种子自由电子激光器(FELs)在各个学科领域取得了重大进展,逐渐成为从基础科学到工业应用领域不可或缺的工具。种子FELs的性能很大程度上取决于频率上转换过程的质量。优化条件的种子fel通常被认为是最大的聚束因子。本文通过分析色散强度对其整体性能的影响,讨论了关于种子场的优化标准的不同观点。本研究通过理论分析、模拟计算和实验探索,探讨了实现最大聚束因子、最大脉冲能量和最佳能量稳定性所需的色散强度之间的差异。实验中的直接观察强调了在种子场中考虑脉冲能量和能量稳定性之间的权衡。这些结果为控制种子FEL的脉冲特性提供了有价值的见解和实用指导,有助于FEL设备的调谐和优化。
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引用次数: 0
Improvement of Cu Ablation Efficiency Using GHz-Burst Femtosecond Laser at 515 nm Wavelength 515nm波长GHz-Burst飞秒激光提高Cu烧蚀效率
IF 3.9 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2025-06-25 DOI: 10.1002/adpr.202500002
Ashkan Momeni, Shota Kawabata, Kotaro Obata, Koji Sugioka

In recent years, gigahertz (GHz)-burst-mode femtosecond lasers have revolutionized laser processing by significantly improving processing efficiency and quality. However, the underlying mechanisms are still unclear and experimentally optimizing the processing parameters is difficult due to their huge number. This study implements a theoretical approach based on simulations to investigate the underlying mechanisms of the Cu ablation efficiency enhancement by GHz-burst mode. The simulation results obtained using a two-temperature model suggest that the ablation efficiency is improved due to the interaction of subsequent intra-pulses in a GHz burst with Cu melted by the preceding intra-pulses. It is demonstrated that for GHz-burst mode, a 515 nm wavelength achieves higher Cu ablation performance than when using the infrared wavelength and demonstrates 2.8 times higher ablation efficiency than the single-pulse mode. The simulation results well agree with the experimental results. The approach used here represents a major advance not only in understanding the underlying mechanisms but also in determining the optimal processing conditions for practical applications.

近年来,千兆赫(GHz)突发模式飞秒激光器通过显著提高加工效率和质量,彻底改变了激光加工。然而,其潜在的机制尚不清楚,并且由于其数量众多,实验优化加工参数很困难。本研究采用基于仿真的理论方法研究了GHz-burst模式提高Cu烧蚀效率的潜在机制。采用双温度模型的仿真结果表明,由于在GHz突发中后续的内脉冲与前一个内脉冲熔化的Cu相互作用,提高了烧蚀效率。结果表明,在GHz-burst模式下,515 nm波长的Cu烧蚀性能优于红外模式,烧蚀效率是单脉冲模式的2.8倍。仿真结果与实验结果吻合较好。这里使用的方法不仅在理解潜在机制方面,而且在确定实际应用的最佳处理条件方面都取得了重大进展。
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引用次数: 0
Review of Coherent Anti-Stokes Raman Scattering Nonresonant Background Removal and Phase Retrieval Approaches: From Experimental Methods to Deep Learning Algorithms 相干反斯托克斯拉曼散射非共振背景去除和相位恢复方法综述:从实验方法到深度学习算法
IF 3.9 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2025-06-25 DOI: 10.1002/adpr.202500035
Rajendhar Junjuri, Thomas Bocklitz

Coherent anti-Stokes Raman spectroscopy (CARS) is a nonlinear optical technique widely utilized for vibrational imaging and molecular characterization in fields such as chemistry, biology, medicine, and materials science. Despite the high signal intensity provided by CARS, the nonresonant background (NRB) can obscure valuable molecular fingerprint information. Therefore, effective NRB removal and phase retrieval are essential for achieving precise spectral analysis and accurate material characterization. This review provides a comprehensive overview of the evolution of CARS-NRB removal and phase retrieval methods, tracing the transition from classical experimental techniques and numerical algorithms to cutting-edge deep learning models. The discussion evaluates the strengths and limitations of each approach and explores future directions for integrating deep learning to improve phase retrieval accuracy and NRB removal efficiency in CARS applications.

相干反斯托克斯拉曼光谱(CARS)是一种非线性光学技术,广泛应用于化学、生物、医学和材料科学等领域的振动成像和分子表征。尽管CARS提供了高信号强度,但非共振背景(NRB)会掩盖有价值的分子指纹信息。因此,有效的NRB去除和相位恢复对于实现精确的光谱分析和准确的材料表征至关重要。本文全面概述了CARS-NRB去除和相位恢复方法的发展,追溯了从经典实验技术和数值算法到尖端深度学习模型的转变。讨论评估了每种方法的优势和局限性,并探讨了集成深度学习以提高CARS应用中相位检索精度和NRB去除效率的未来方向。
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引用次数: 0
High-Chroma, High-Contrast Tunable Color Coatings Using Sb2S3 in a Metal-Dielectric Stack 利用Sb2S3在金属-介电层中制备高色度、高对比度可调彩色涂层
IF 3.9 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2025-06-23 DOI: 10.1002/adpr.202400194
Riley Shurvinton, Arjun Karimbana, Priya Dominic, Antonin Moreau, Olivier Hector, Konstantinos Iliopoulos, Fabien Lemarchand, Julien Lumeau

Thin-film coatings are a versatile option for creating color. These coatings can be made tunable by introducing phase-change materials (PCMs), whose optical response changes due to an external signal. However, commonly used PCMs such as Ge2Sb2Te5 (GST) are limited in their applications for color coatings, due to high absorption of visible light. Here, the alternative PCM Sb2S3 is used, and a novel coating design is demonstrated, which incorporates the PCM layer into an asymmetric Fabry–Perot cavity with Ag, SiO2 and Ti layers. Simulations are used to show that this design yields high-chroma colors in a wide range of hues, which exhibit a large tunable hue shift when the phase of the Sb2S3 layer changes. Three coatings are deposited to experimentally verify these results, which give good agreement with the simulations. The phase change of the Sb2S3 layer is demonstrated using direct heating using a hotplate, and also using laser annealing, which allows microscale image writing to be realized on the coatings.

薄膜涂层是创造颜色的通用选择。这些涂层可以通过引入相变材料(PCMs)来实现可调谐,相变材料的光学响应会因外部信号而改变。然而,常用的PCMs,如Ge2Sb2Te5 (GST),由于对可见光的高吸收,在彩色涂料中的应用受到限制。本研究采用了另一种PCM Sb2S3,并展示了一种新的涂层设计,该涂层将PCM层整合到具有Ag、SiO2和Ti层的不对称Fabry-Perot腔中。仿真结果表明,该设计可以在大范围的色调中产生高色度的颜色,当Sb2S3层的相位变化时,其表现出较大的可调色调偏移。通过实验验证了上述结果,结果与模拟结果吻合较好。采用热板直接加热和激光退火的方法对Sb2S3层的相变进行了验证,从而实现了涂层上的微尺度图像写入。
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引用次数: 0
Design Method of Time-Multiplexed Ultrashort Throw Ratio Projection System with Low Distortion and Uniform Resolution 低失真、均匀分辨率时复用超短投比投影系统设计方法
IF 3.9 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2025-06-23 DOI: 10.1002/adpr.202400224
Yuefan Shan, Jiaping Sun, Xilong Dai, Da Wang, Yongqi Liu, Dewen Cheng

Time-multiplexed laser projection is recognized as a promising projection technology owing to its broad color gamut and high energy efficiency. The escalating demands for enhanced laser safety and reduced space occupation necessitate the development of ultrashort throw ratio (UTR) projectors. However, the inherent mechanical deflection limitations and distortions of micro electro mechanical systems (MEMS) scanners pose significant challenges to achieving UTR projection. To address these constraints, trapezoidal distortion is first eliminated by ensuring vertical laser incidence on MEMS mirrors during the initial projection phase. Subsequently, a systematic design methodology for UTR laser MEMS projection systems is proposed, incorporating a miniaturized catadioptric projection objective that maintains uniformly optical étendue distribution. This configuration achieves a throw ratio of 0.27, reduces pillow distortion to 0.4%, and ensures consistent resolution across the entire screen. Segmentation and modular assembly of the catadioptric objective at telecentric intermediate image planes enhances the efficiency of initial structural design phase. The developed projection prototype experimentally validates the efficacy of the projection system designed through the proposed methodology in decreasing the projection ratio, correcting distortion, and maintaining uniform projection resolution across the full field of view.

时间复用激光投影以其广色域和高能效被认为是一种很有前途的投影技术。对提高激光安全性和减少空间占用的日益增长的需求使超短射比(UTR)投影仪的发展成为必要。然而,微机电系统(MEMS)扫描仪固有的机械偏转限制和畸变对实现UTR投影提出了重大挑战。为了解决这些限制,首先通过在初始投影阶段确保垂直激光入射到MEMS反射镜上来消除梯形畸变。随后,提出了一种UTR激光MEMS投影系统的系统设计方法,该系统采用了一种小型化的反射投影物镜,以保持均匀的光学调制调制分布。这种配置实现了0.27的投掷比,将枕头失真降低到0.4%,并确保整个屏幕的分辨率一致。在远心中间像面上对反射物镜进行分割和模块化装配,提高了初始结构设计阶段的效率。通过实验验证了采用该方法设计的投影系统在降低投影比、校正畸变和保持全视场均匀投影分辨率等方面的有效性。
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引用次数: 0
Topological Berry Antenna on a Silicon Chip for Terahertz Wireless Communication 用于太赫兹无线通信的硅晶片拓扑Berry天线
IF 3.9 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2025-06-22 DOI: 10.1002/adpr.202500123
Sonu Kumar, Ridong Jia, Yi Ji Tan, Thomas Caiwei Tan, Pascal Szriftgiser, G. Arun Kumar, Guillaume Ducournau, Arokiaswami Alphones, Ranjan Singh

Nonzero Berry curvature is central to the existence of topological edge states in electronic and photonic valley-Hall systems. While manipulating the Berry curvature in condensed matter systems is challenging, valley-Hall topological photonics offer unprecedented control, where the broken spatial inversion symmetry alters the Berry curvature. Herein, an all-silicon Berry antenna is presented, using a continuously varying geometry corresponding to a gradual change in Berry curvature. The on-chip topological edge mode with a tunable field extent is achieved to enhance effective antenna aperture, creating a high-gain on-chip photonic antenna with perfectly planar wavefronts. Experimentally, a maximum gain of 17 dBi that supports 20 Gbps chip-to-chip wireless communication is demonstrated, with active optical tunability of the antenna gain with modulation depths of 8 dBi. This Berry antenna paves the way for the development of complementary metal-oxide-semiconductor (CMOS) compatible topological Berry devices, with potential applications in integrated micro-/nano-photonics, next-generation wireless communications (6G to Xth generation), and terahertz detection and ranging.

在电子和光子谷-霍尔系统中,非零贝里曲率是拓扑边缘态存在的核心。虽然在凝聚态系统中操纵贝里曲率是具有挑战性的,但谷-霍尔拓扑光子学提供了前所未有的控制,其中空间反演对称性的破坏改变了贝里曲率。本文提出了一种全硅贝里天线,采用连续变化的几何形状,对应于贝里曲率的逐渐变化。实现了具有可调场域的片上拓扑边缘模式,提高了天线的有效孔径,形成了具有完美平面波前的高增益片上光子天线。实验结果表明,该天线的最大增益为17 dBi,支持20 Gbps的片对片无线通信,并且在调制深度为8 dBi的情况下,天线增益具有主动光可调性。这种Berry天线为互补金属氧化物半导体(CMOS)兼容拓扑Berry器件的发展铺平了道路,在集成微/纳米光子学、下一代无线通信(6G到x代)以及太赫兹探测和测距方面具有潜在的应用前景。
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引用次数: 0
Terahertz Spoof Surface Plasmon Polariton Structure for High-Precision Gas Sensor Technology 高精度气体传感器技术的太赫兹欺骗表面等离子体激元结构
IF 3.9 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2025-06-17 DOI: 10.1002/adpr.202400163
Vahid Najafy, Bijan Abbasi-Arand, Maryam Hesari-Shermeh

It is a significant challenge to accurately identify and differentiate sample materials in the gas phase, especially when they have closely similar refractive indices. A promising solution in the THz range is to use plasmonic spoof surface structures configured in an Otto arrangement. Here, this study proposes a multilevel meta-grating structure sensor that achieves a remarkable improvement over the conventional binary-grating structure model. The proposed setup has been meticulously designed to maximize reflectance within the sensor's reflectance spectrum. This has been achieved by precisely adjusting the air gap distance, effectively minimizing the impact of sample material density. An in-depth analysis of gas samples with this structure shows a considerable increase in sensitivity with a small refractive index change up to 11.4 (TH/RIU), and the results are validated by simulating the reflection spectrum using the semi-analytical rigorous coupled wave analysis method. Moreover, the eigenmode solver in the CST Studio software is used to generate dispersion curves. The newly proposed design is particularly suitable for effectively detecting different gases with closely spaced refractive indices, making the proposed structure very useful in high-precision sensors that discern small refractive index changes.

准确识别和区分气相样品材料是一项重大挑战,特别是当它们具有非常相似的折射率时。在太赫兹范围内,一个有希望的解决方案是使用以奥托排列配置的等离子体欺骗表面结构。在此,本研究提出了一种多层元光栅结构传感器,它比传统的二元光栅结构模型有了显著的改进。所提出的设置经过精心设计,以最大限度地提高传感器反射光谱内的反射率。这是通过精确调节气隙距离来实现的,有效地减少了样品材料密度的影响。对气体样品的深入分析表明,该结构的灵敏度显著提高,折射率变化很小,可达11.4 (TH/RIU),并通过半解析严格耦合波分析方法模拟反射光谱验证了结果。利用CST Studio软件中的本征模求解器生成色散曲线。新提出的设计特别适合于有效地检测具有紧密间隔折射率的不同气体,使所提出的结构在识别微小折射率变化的高精度传感器中非常有用。
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引用次数: 0
High-Quality-Factor, Compact Nanoplasmonic Filter Utilizing Graphene Metasurface at Near-Infrared Range 在近红外范围内利用石墨烯超表面的高质量因数,紧凑的纳米等离子体滤波器
IF 3.9 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2025-06-17 DOI: 10.1002/adpr.202400186
Mohammad Sadegh Zare, Asma Attariabad, Sevda Seyedmasoumian, Ali Farmani

A plasmonic reflective filter (PRF) based on monolayer graphene and four nanoscale cylindrical silica grooves inside a silver film is suggested and theoretically analyzed. The designed filter has a dual-band reflection and absorption spectra with a near-unity absorption value at resonance wavelengths located in near-infrared region. Furthermore, the two reflection dips can be tuned via harnessing graphene chemical potential. Application of subwavelength metallic structure as well as graphene layer contributes to the increased light–matter interactions and reinforces the light confinement in the nanoscale regions in the cylindrical grooves. As a result, near-zone electric field is highly enhanced and leads to the strong optical absorption of the filter. Also, the optical response of the proposed PRF is independent from the polarization of the incident light due to the symmetrical geometry of the structure. The suggested filter can be utilized in photonic integrated circuits.

提出了一种基于单层石墨烯和四个纳米圆柱形硅沟槽的等离子体反射滤光片(PRF),并进行了理论分析。所设计的滤波器具有双波段反射和吸收光谱,在近红外共振波长处吸收值接近一致。此外,这两个反射衰减可以通过利用石墨烯的化学势来调节。亚波长金属结构和石墨烯层的应用有助于增加光与物质的相互作用,并加强了圆柱形凹槽中纳米级区域的光约束。因此,近区电场被大大增强,导致滤光片的强光吸收。此外,由于结构的对称几何,所提出的PRF的光学响应与入射光的偏振无关。该滤波器可用于光子集成电路。
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引用次数: 0
Imaging Photonic Resonances within an All-Dielectric Metasurface via Photoelectron Emission Microscopy 利用光电子发射显微镜成像全介电超表面内的光子共振
IF 3.9 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2025-06-12 DOI: 10.1002/adpr.70022
Andrew R. Kim, Chloe F. Doiron, Fernando J. Vega, Jaeyeon Yu, Alex M. Boehm, Joseph P. Klesko, Igal Brener, Raktim Sarma, Alexander Cerjan, Taisuke Ohta

All-Dielectric Metasurfaces

Confinement of light within nanostructures of increasingly smaller sizes has resulted in ever more precise control of light-matter interactions. In article number 2400223, Taisuke Ohta and co-workers demonstrate near-field imaging of volume-type photonic resonances within a dielectric metasurface using photoelectron emission microscopy. This imaging approach, utilizing far-field excitation and sub-optical wavelength spatial resolution, offers a new avenue for examining light–matter interactions within dielectric nanophotonic systems.

将光限制在尺寸越来越小的纳米结构中,可以更精确地控制光与物质的相互作用。在第2400223号文章中,Taisuke Ohta及其同事使用光电子发射显微镜演示了介质超表面内体积型光子共振的近场成像。这种成像方法利用远场激发和亚光学波长空间分辨率,为研究介电纳米光子系统中的光-物质相互作用提供了新的途径。
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引用次数: 0
Q-Switched Mode-Locking in Er-Doped ZrF4-BaF2-LaF3-AlF3-NaF Fiber Lasers Using Carbon Nanotube–Saturable Absorber and GaSb-Based Semiconductor-Saturable Absorber Mirror 利用碳纳米管可饱和吸收镜和基于气体的半导体可饱和吸收镜实现掺铒ZrF4-BaF2-LaF3-AlF3-NaF光纤激光器的调q锁模
IF 3.9 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2025-06-12 DOI: 10.1002/adpr.202500065
Boris Perminov, Aram Mkrtchyan, Yuriy Gladush, Dmitry V. Krasnikov, Albert G. Nasibulin, Maria Chernysheva

Mid-infrared (IR) fiber lasers are crucial for applications in spectroscopy, medical diagnostics, and environmental sensing, owing to their ability to interact with fundamental molecular vibrational bands. However, achieving stable ultrafast pulse generation in this spectral range remains challenging due to the limited availability of robust saturable absorbers. For the first time, we demonstrate Q-switched mode-locking in an all-fiber Er-doped ZrF4-BaF2-LaF3-AlF3-NaF laser employing an aerosol-synthesized carbon nanotube (CNT) film. Furthermore, we compare the laser performance with pulse generation using a state-of-the-art GaSb-based semiconductor-saturable absorber mirror (SESAM) in an identical cavity design. The CNT-saturable absorber enables pulse generation with a minimum duration of 1.32 μs and a pulse energy of 1.4 μJ at an average output power of 63.1 mW. In contrast, the SESAM-based laser produces 345-ns pulses with a pulse energy reaching 3.84 μJ and an average power of 202 mW. These results provide new insights into the interplay between saturable absorber properties and mid-IR fiber laser performance, paving the way for next-generation compact ultrafast sources for scientific and industrial applications.

中红外(IR)光纤激光器由于能够与基本分子振动带相互作用,在光谱学、医学诊断和环境传感等领域的应用至关重要。然而,在这个光谱范围内实现稳定的超快脉冲产生仍然具有挑战性,因为强大的饱和吸收剂的可用性有限。我们首次在采用气溶胶合成碳纳米管(CNT)薄膜的全光纤掺铒ZrF4-BaF2-LaF3-AlF3-NaF激光器中证明了q开关模式锁定。此外,我们在相同的腔体设计中使用最先进的基于gasb的半导体可饱和吸收镜(SESAM)来比较激光性能和脉冲产生。碳纳米管可饱和吸收体产生脉冲的最小持续时间为1.32 μs,脉冲能量为1.4 μJ,平均输出功率为63.1 mW。而sesam激光器产生的脉冲功率为345 ns,脉冲能量为3.84 μJ,平均功率为202 mW。这些结果为饱和吸收特性和中红外光纤激光器性能之间的相互作用提供了新的见解,为科学和工业应用的下一代紧凑型超快光源铺平了道路。
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引用次数: 0
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Advanced Photonics Research
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