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Achievement of Sub-Diffractive Detection Depth in Absorption Spectroscopy Using Excitation from an Upconverting Particle 利用上转换粒子的激发实现吸收光谱的亚衍射探测深度
IF 3.7 Pub Date : 2024-04-10 DOI: 10.1002/adpr.202300292
Jayesh Goswami, Snigdhadev Chakraborty, Gokul Nalupurackal, Srestha Roy, Basudev Roy

Conventionally, a collimated visible laser beam can only be focused to a transverse region volume with a waist of about 200 nm and an axial waist of about 1200 nm due to the wave nature of light. Several techniques have been used to bypass the diffraction limit, including a recently developed one using the emission from an optically trapped upconverting nanoparticle. This nanoparticle has a diameter smaller than 200 nm, such that it emits like a dipole into a 45° cone. Thus, not only is the emission coming from a particle smaller in size than the waist of the diffraction-limited spot but also the cone is smaller than that of the volume of a very tightly focused beam. Here, the technique is developed even further where the emission coming from a specific region of the cone is selected by an optical fiber-based pinhole in the detection path. Using this technique, a confocal depth of about 200 nm is achieved as the overlap between the emission cone and the detection volume. This would correspond to a volume of about 250 attoliters for a 1.5 μm diameter particle which can be reduced to 40 attoliters by using a 500 nm diameter particle.

传统上,由于光的波特性,准直的可见激光束只能聚焦到一个横向区域,其腰围约为 200 纳米,轴向腰围约为 1200 纳米。有几种技术被用来绕过衍射极限,包括最近开发的一种利用光捕获上转换纳米粒子发射的技术。这种纳米粒子的直径小于 200 纳米,因此它能像偶极子一样发射出 45° 锥形光。因此,不仅粒子的发射尺寸小于衍射极限光斑的腰部,而且锥体的尺寸也小于非常紧密聚焦光束的体积。在这里,该技术得到了进一步发展,即通过检测路径上的光纤针孔来选择来自锥体特定区域的发射。利用这种技术,发射锥和检测体积之间的重叠部分可达到约 200 nm 的共焦深度。这相当于直径为 1.5 μm 的微粒的体积约为 250 阿托立特,而使用直径为 500 nm 的微粒则可减少到 40 阿托立特。
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引用次数: 0
hBN-Encapsulated Graphene Coupled to a Plasmonic Metasurface via 1D Electrodes for Photodetection Applications 通过一维电极耦合到等离子体元表面的 hBN 封装石墨烯用于光探测应用
IF 3.7 Pub Date : 2024-04-08 DOI: 10.1002/adpr.202470010
Christian Frydendahl, Sita Rama Krishna Chaitanya Indukuri, Taget Raghavendran Devidas, Zhengli Han, Noa Mazurski, Kenji Watanabe, Takashi Taniguchi, Hadar Steinberg, Uriel Levy

In article number 2300192, Christian Frydendahl, Uriel Levy, and co-workers demonstrate a new approach where plasmonic nanostructures are pierced through the hexagonal boron nitride layers to make atomic edge contacts to the graphene, thus maintaining the advantages of encapsulation, while enabling strong enhancement of the optical response of graphene from charge transfer from plasmonic decay in the nanocavities.

在编号为 2300192 的文章中,Christian Frydendahl、Uriel Levy 及其合作者展示了一种新方法,即穿透六方氮化硼层使等离子体纳米结构与石墨烯产生原子边缘接触,从而保持封装的优势,同时使石墨烯的光学响应因纳米腔中等离子衰减产生的电荷转移而得到有力增强。
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引用次数: 0
Electromagnetic Waves in Crystals: The Presence of Exceptional Points 晶体中的电磁波:异常点的存在
IF 3.7 Pub Date : 2024-04-08 DOI: 10.1002/adpr.202470012
Chris Sturm

In article number 2300235, Chris Sturm presents a comprehensive discussion on exceptional points (EPs) in optically anisotropic materials, their occurrence, and properties as well as the properties of the electromagnetic waves propagating along such EPs. The presence of such EPs, their spatial and spectral distribution in bulk, and semi-infinite and finite crystals are discussed.

在编号为 2300235 的文章中,Chris Sturm 全面论述了光学各向异性材料中的特殊点 (EP)、它们的出现、特性以及沿这些特殊点传播的电磁波的特性。文章讨论了这种 EP 的存在、它们在块体、半无限和有限晶体中的空间和光谱分布。
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引用次数: 0
Exploring the Regulatory Mechanism of ZnS Materials under Stress and Re Doping: Insights from Density Functional Theory 探索应力和再掺杂条件下 ZnS 材料的调控机制:密度泛函理论的启示
IF 3.7 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-04-03 DOI: 10.1002/adpr.202300347
Benle Dou, Yi Li, Shuangqiang Fang, Qiangqiang Zhao, Haoliang Cheng, Pei Liang, Le Wang

The application prospects of ZnS stress luminescent materials cover many fields such as high-precision structural monitoring, smart materials, biomedical imaging, and new sensor technologies, which bring broad application prospects and significance to them in the fields of engineering, medicine, and scientific research. In this article, the electronic structure and optical properties of ZnS materials are successfully regulated by applying pressure and doping rare earth metals (Re), and it is found that the regulation of the luminescence properties of ZnS is the result of stress and doping interactions. Specifically, when pressure is applied or Re metal doping, the lattice structure is deformed and the atomic spacing is adjusted, which affects the electronic energy level distribution and optical properties of ZnS materials. Computational analysis of density functional theory (DFT) reveals the microscopic mechanisms behind these changes, including changes in lattice parameters, adjustment of bond length, and changes in band structure. This study provides theoretical guidance for the design and synthesis of high-performance and high-stability ZnS light-emitting materials, and is of great significance for expanding the application of ZnS in the field of lasers and sensors.

ZnS应力发光材料的应用前景涉及高精度结构监测、智能材料、生物医学成像、新型传感技术等多个领域,在工程、医学、科研等领域具有广阔的应用前景和重要意义。本文通过施加压力和掺杂稀土金属(Re)成功调控了 ZnS 材料的电子结构和光学特性,发现 ZnS 发光特性的调控是应力和掺杂相互作用的结果。具体来说,当施加压力或掺杂 Re 金属时,晶格结构会发生变形,原子间距会发生调整,从而影响 ZnS 材料的电子能级分布和光学特性。密度泛函理论(DFT)的计算分析揭示了这些变化背后的微观机制,包括晶格参数变化、键长调整和能带结构变化。该研究为设计和合成高性能、高稳定性的 ZnS 发光材料提供了理论指导,对拓展 ZnS 在激光器和传感器领域的应用具有重要意义。
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引用次数: 0
Integrated Electro-Optically Tunable Narrow-Linewidth III–V Laser 集成式电光可调谐窄线宽 III-V 激光器
IF 3.7 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-03-30 DOI: 10.1002/adpr.202400018
Yiran Zhu, Shupeng Yu, Zhiwei Fang, Difeng Yin, Jian Liu, Zhe Wang, Yuan Zhou, Yu Ma, Haisu Zhang, Min Wang, Ya Cheng

Herein, an integrated electro-optically tunable narrow-linewidth III–V laser with an output power of 738.8 μW and an intrinsic linewidth of 45.55 kHz at the C band is demonstrated. The laser cavity is constructed using a fiber Bragg grating (FBG) and a tunable Sagnac loop reflector (TSLR) fabricated on thin-film lithium niobate. The combination of the FBG and the electro-optically tunable TSLR offers the advantages of single spatial mode, single frequency, narrow linewidth, and wide wavelength tunability for the electrically pumped hybrid integrated laser, which features a frequency tuning range of 20 GHz and a tuning efficiency of 0.8 GHz V−1.

本文展示了一种集成的电光可调谐窄线宽 III-V 激光器,其输出功率为 738.8 μW,C 波段固有线宽为 45.55 kHz。激光腔由光纤布拉格光栅(FBG)和在铌酸锂薄膜上制造的可调谐萨格纳克环形反射器(TSLR)构成。FBG 和电光可调谐 TSLR 的组合为电泵浦混合集成激光器提供了单空间模式、单频率、窄线宽和宽波长可调谐的优势,其频率调谐范围为 20 GHz,调谐效率为 0.8 GHz V-1。
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引用次数: 0
Silicon Photonic Filters: A Pathway from Basics to Applications 硅光子滤波器:从基础到应用的途径
IF 3.7 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-03-30 DOI: 10.1002/adpr.202300343
Nabarun Saha, Giuseppe Brunetti, Annarita di Toma, Mario Nicola Armenise, Caterina Ciminelli

Silicon photonics has found a profound place among emerging technologies in the past few decades due to several advantages. Due to a series of breakthroughs and increased funding from private and government sectors, the development of silicon photonics has accelerated especially starting from the two years 2004–2005 with a persisting and ever-growing momentum. Among various components, the silicon photonic filters that selectively pass or block particular wavelengths with a finite bandwidth have found particular interest as they are useful in signal processing in different fields ranging from optical communication to microwave photonics and quantum photonics. Herein, a comprehensive review of silicon photonic filters focusing on the four most commonly used architectures, such as microring resonators, waveguide Bragg grating, Mach–Zehnder interferometers, and arrayed waveguide grating, encapsulating basics, and guidelines, in terms of simulating tools and topologies, of realizing reconfigurable and high-performing filters for several applications, is provided. The novelty of this review relies on the fact that it summarizes these filter architectures covering a broad range of applications concisely and constructively and includes the basics, growth, and future trends, providing a clear understanding and importance of silicon photonic filters from research to commercialization perspective.

在过去的几十年中,硅光子技术凭借其多项优势在新兴技术中占据了重要地位。由于硅光子技术的一系列突破以及私人和政府部门资金的增加,硅光子技术的发展速度加快,特别是从 2004-2005 年两年开始,发展势头持续不断。在各种元件中,以有限带宽选择性通过或阻断特定波长的硅光子滤波器尤其受到关注,因为它们在从光通信到微波光子学和量子光子学等不同领域的信号处理中都非常有用。本文对硅光子滤波器进行了全面综述,重点介绍了四种最常用的架构,如微波谐振器、波导布拉格光栅、马赫-泽恩德干涉仪和阵列波导光栅,封装基础知识,以及在模拟工具和拓扑结构方面的指导原则,以实现可重新配置的高性能滤波器的多种应用。这篇综述的新颖之处在于,它简明扼要、富有建设性地总结了这些涵盖广泛应用的滤波器架构,并介绍了其基本原理、发展和未来趋势,从研究到商业化的角度,让人们清楚地了解硅光子滤波器的重要性。
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引用次数: 0
An Integrated All-Optical Ising Machine with Unlimited Spin Array Size and Coupling 具有无限自旋阵列尺寸和耦合的集成式全光等效机
IF 3.7 Pub Date : 2024-03-26 DOI: 10.1002/adpr.202400004
Yuchi Lan, Guanyu Chen, Yuan Gao, Wujie Fu, Aaron J. Danner

Artificial spin systems are used to solve combinatorial optimization problems by mapping them to the ground state search of the Ising model. Ising machines of various designs, in fields as diverse as photonics and electronics, have been proposed and demonstrated in recent years. One important mathematical operation required in photonic Ising machines for nearly all Hamiltonian minimization algorithms is repeated matrix–vector multiplication with the vector size limited by the physical size of the optical system. Herein, an integrated photonic Ising machine based on matrix partitioning and phase encoding, which effectively allows the use of physically small optical circuits to handle arbitrarily large spin vectors, is proposed. All the complicated calculations are carried out optically, rather than electronically, in this approach. How the required surface area of a hypothetical chip-based photonic Ising machine can be resized according to convenience, with the trade-off being the solution time, and that this trade-off can be done in a way that does not impact the algorithm's efficacy, is shown. Through simulation, the system is predicted to have a high success rate, high noise tolerance, and high error tolerance.

人工自旋系统通过映射伊辛模型的基态搜索来解决组合优化问题。近年来,在光子学和电子学等不同领域提出并展示了各种设计的伊辛机。在光子伊辛机中,几乎所有哈密顿最小化算法都需要进行一个重要的数学运算,那就是重复矩阵-矢量乘法,而矢量的大小受到光学系统物理尺寸的限制。在这里,我们提出了一种基于矩阵分割和相位编码的集成光子伊辛机,它能有效地利用物理尺寸较小的光路来处理任意大的自旋矢量。在这种方法中,所有复杂的计算都是通过光学而非电子方式进行的。图中展示了如何根据方便程度调整假想的芯片式光子伊辛机所需的表面积,而折衷的办法是缩短求解时间,并且这种折衷可以在不影响算法功效的情况下完成。通过仿真预测,该系统具有高成功率、高噪音容限和高误差容限。
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引用次数: 0
Enhancing Triplet–Triplet Annihilation Upconversion Performance Through Anthracene–Carbazole Interactions for Organic Optoelectronic Applications 通过蒽-咔唑相互作用提高三重-三重湮没上转换性能,实现有机光电应用
IF 3.7 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-03-25 DOI: 10.1002/adpr.202300344
Kai-Hong Hsieh, Yuan-Zhen Zhuang, Jing-Xiang Huang, Zheng-Yu Wei, Yong-Yun Zhang, Jiun-Haw Lee, Tien-Lung Chiu, Man-kit Leung

Three carbazole-substituted anthracene 2CbzAn, 26CbzAn, and 246CbzAn have been developed. The introduction of these carbazole substituents could generate more triplet states with energy levels close to 2× E(T1) that could successfully facilitate the triplet-triplet annihilation upconversion (TTA-UC) process to achieve high upconversion quantum yield (UCQY). This observation aligns with the Adachi theory about TTA-UC mechanisms. In organic light-emitting diode (OLED) device investigation, in a non-doped state show an external quantum efficiency (EQEmax) of 5.82% with exceptional pure-blue emission (CIEy of 0.101), and the DPaNIF doped DMPPP/26CbzAn bilayer structure reaches an impressive EQEmax of 11.12%.

目前已开发出三种咔唑取代的蒽 2CbzAn、26CbzAn 和 246CbzAn。这些咔唑取代基的引入可以产生更多能级接近 2× E(T1)的三重态,从而成功促进三重态-三重态湮灭上转换(TTA-UC)过程,实现高上转换量子产率(UCQY)。这一观察结果与有关 TTA-UC 机制的 Adachi 理论相吻合。在有机发光二极管(OLED)器件的研究中,无掺杂状态下的外部量子效率(EQEmax)为 5.82%,具有特殊的纯蓝色发射(CIEy 为 0.101),而掺杂 DPaNIF 的 DMPPP/26CbzAn 双层结构的外部量子效率(EQEmax)达到了惊人的 11.12%。
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引用次数: 0
Electromagnetic Waves in Crystals: The Presence of Exceptional Points 晶体中的电磁波:异常点的存在
IF 3.7 Pub Date : 2024-03-19 DOI: 10.1002/adpr.202300235
Chris Sturm

Although the investigation of the propagation of electromagnetic waves in crystals dates back to the 19th century, the presence of singular optic axes in optically anisotropic materials has not been fully explored until now. Along such an axis, either a left or a right circular polarized wave can propagate without changing its polarization state. More generally, these singular optic axes belong to exceptional points (EPs) in the momentum space and correspond to a simultaneous degeneration of the eigenmodes and their propagation properties. Herein, a comprehensive discussion on EPs in optically anisotropic materials, their occurrence, and properties as well as the properties of the electromagnetic waves propagating along such EPs is presented. The presence of such EPs, their spatial and spectral distribution in bulk, and semi-infinite and finite crystals are discussed. It is shown that the presence of interfaces has a strong impact on the presence of the EPs and their spatial distribution. At an EP, the propagation of an arbitrarily polarized wave cannot be described by a superposition of two eigenmodes, as typically described in textbooks. This leads to singularities if the reflection and transmission coefficients have to be calculated. Here, two approaches are presented to overcome these limitations.

尽管对电磁波在晶体中传播的研究可以追溯到 19 世纪,但对光学各向异性材料中存在的奇异光轴的研究至今仍未全面展开。沿着这样的轴线,左旋或右旋圆极化波可以在不改变其极化状态的情况下传播。一般来说,这些奇异的光轴属于动量空间中的异常点(EP),同时对应于特征模式及其传播特性的退化。本文全面讨论了光学各向异性材料中的例外点、例外点的出现、例外点的特性以及沿例外点传播的电磁波的特性。本文讨论了这种 EP 的存在,以及它们在块体、半无限和有限晶体中的空间和光谱分布。研究表明,界面的存在对 EP 的存在及其空间分布有很大影响。在 EP 处,任意极化波的传播不能用教科书中通常描述的两个特征模的叠加来描述。如果要计算反射和透射系数,就会出现奇异现象。这里介绍两种克服这些限制的方法。
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引用次数: 0
Dispersion-Engineered Super-Gain Parametric Amplification in Nanoscale Optical Cavities 纳米级光腔中的弥散工程超增益参量放大
IF 3.7 Pub Date : 2024-03-17 DOI: 10.1002/adpr.202300247
Özüm Emre Aşırım

The gain factor of the optical parametric amplification (OPA) process is known to be negligible in the small scale due to low-interaction-medium length. Hence, in the nanoscale, OPA is deemed as infeasible. Therefore, in small-scale-integrated optical devices, stimulated-emission-based amplifiers (lasers) are employed instead of OPAs. In contrast, the major advantage of OPAs over lasers is that unlike lasers which only provide amplification over a narrow spectral band, OPAs provide high-gain amplification over a very large, user-controlled spectral band. In this article, it is shown that OPA can yield wideband high-gain amplification over a nanoscale beam propagation distance through dispersion engineering. This is achieved by a proper tuning of the pump (source) wave frequency, which can maximize the effective medium nonlinearity by a few orders of magnitude, while concurrently maximizing the intracavity energy density, thereby compensating for the small co-propagation distance for the input (signal) and pump beams. In this study, it is shown that an input wave can be amplified by a factor 108$left(10right)^{8}$ in a nanoscale cavity via precise dispersion engineering. Both empirical and computational formulations are used for the investigation, which display a reasonable agreement.

众所周知,光参量放大(OPA)过程的增益因数在小尺度上可以忽略不计,这是由于低交互介质长度造成的。因此,在纳米尺度上,OPA 被认为是不可行的。因此,在小尺度集成光学设备中,人们采用基于受激发射的放大器(激光器)来代替 OPA。相比之下,与激光器相比,OPA 的主要优势在于激光器只能提供窄光谱带的放大,而 OPA 则能在用户控制的很大光谱带内提供高增益放大。本文表明,OPA 可通过色散工程在纳米级光束传播距离上产生宽带高增益放大。这是通过适当调整泵(源)波频率实现的,这可以将有效介质非线性最大化几个数量级,同时将腔内能量密度最大化,从而补偿输入(信号)光束和泵光束较小的共传播距离。本研究表明,通过精确的色散工程,输入波可以在纳米级腔内放大一个系数。研究采用了经验公式和计算公式,两者显示出合理的一致性。
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引用次数: 0
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Advanced Photonics Research
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