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High-Numerical-Aperture, 3D-Printed All-Dielectric Harmonic Diffraction Metalens in the Sub-THz Frequency Range 亚太赫兹频率范围内的高数值孔径、3d打印全介电谐波衍射超透镜
IF 3.9 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2025-07-03 DOI: 10.1002/adpr.202500064
Kobi Ben Atar, Jacob Engelberg, Uriel Levy

Terahertz (THz) optical devices have emerged as critical tools across diverse applications, owing to the distinctive properties of THz radiation. The ability of THz waves to penetrate nonconductive materials enables numerous nondestructive testing applications, while their characteristic interaction with molecular vibrations produces unique spectral fingerprints, facilitating precise material identification and quantification. Moreover, the low photon energy of THz radiation makes it particularly suitable for biological inspection without sample damage. Despite these advantages, conventional THz devices, including emitters and detectors, remain bulky, impeding their miniaturization and integration. THz metalenses offer a promising solution by enabling wavefront control in compact, planar architectures. However, their reliance on electromagnetic diffraction introduces significant dispersion, presenting substantial challenges for implementation in the inherently broadband THz regime, which often spans multiple octaves. Herein, an advanced all-dielectric metalens operating at dual-frequency harmonics in the sub-THz regime is demonstrated. The lens, fabricated using commercial 3D printing technology, enables rapid prototyping and cost-effective manufacturing. This metalens achieves a numerical aperture of 0.86 (50 mm diameter, 15 mm focal length) at both 150 and 300 GHz. This development represents a significant advancement toward implementing higher-order metasurface elements in the THz regime.

由于太赫兹(THz)辐射的独特特性,太赫兹(THz)光学器件已成为各种应用的关键工具。太赫兹波穿透非导电材料的能力使许多无损检测应用成为可能,而它们与分子振动的特征相互作用产生独特的光谱指纹,促进精确的材料识别和量化。此外,太赫兹辐射的低光子能量使其特别适合于不损坏样品的生物检测。尽管有这些优点,传统的太赫兹器件,包括发射器和探测器,仍然体积庞大,阻碍了它们的小型化和集成化。太赫兹超透镜通过在紧凑的平面结构中实现波前控制,提供了一个很有前途的解决方案。然而,它们对电磁衍射的依赖会引入明显的色散,这对在固有的宽带太赫兹区域(通常跨越多个八度)中实现提出了实质性的挑战。本文演示了一种工作在亚太赫兹双频谐波下的先进全介电超构透镜。该镜头采用商业3D打印技术制造,可实现快速原型制作和成本效益制造。该超透镜在150 GHz和300 GHz下均实现了0.86 (50 mm直径,15 mm焦距)的数值孔径。这一发展代表了在太赫兹区域实现高阶元表面元素的重大进步。
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引用次数: 0
Realizing Multispectral Fabry–Perot Structural Color Filters Based on Optical Nanostructures on a Complementary Metal Oxide Semiconductor Chip 基于光学纳米结构在互补金属氧化物半导体芯片上实现多光谱法布里-珀罗结构滤色片
IF 3.9 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2025-07-03 DOI: 10.1002/adpr.202500057
Hongwei Gao, Xavier X. Chia, Ruitao Zheng, Sin Heng Lim, Dawn T. H. Tan

A complementary metal oxide semiconductor-compatible transmission filter composed of subwavelength nanostructures is demonstrated through design, numerical modeling, and experimental verification. The tuning of the filters’ peak wavelength via lithographic means in a single dielectric layer, obviating the need for altering the device layer thickness to achieve different filter wavelengths is demonstrated. The FabryPerot function is achieved by sandwiching the nanostructures between a bottom distributed Bragg reflector and a top reflector composed of a layer of silver. A spectral resolution of 10 nm–30 nm full width at half maximum and peak transmission efficiency of ≈70% in the multispectral optical filters in both numerical simulations and experimental characterization is experimentally demonstrated. This approach provides a new paradigm in which to achieve color filters, eliminating the need for multiple mask steps for varied device layer thicknesses conventionally used to achieve FabryPerot filters, greatly reducing the manufacturing process cost and complexity.

通过设计、数值模拟和实验验证,展示了一种由亚波长纳米结构组成的互补金属氧化物半导体兼容透射滤波器。通过光刻方法在单个介质层中调谐滤波器的峰值波长,从而避免了改变器件层厚度以实现不同滤波器波长的需要。法布里-珀罗函数是通过将纳米结构夹在底部分布的布拉格反射器和由银层组成的顶部反射器之间来实现的。在数值模拟和实验表征中,实验证明了该多光谱滤光片的光谱分辨率为10 nm - 30 nm,全宽为一半,峰值透射效率约为70%。这种方法提供了一种实现彩色滤光片的新范例,消除了传统上用于实现Fabry-Perot滤光片的不同器件层厚度的多个掩模步骤的需要,大大降低了制造过程的成本和复杂性。
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引用次数: 0
Switchable Terahertz Beam Steering with Near-Perfect Ordinary Transmission 近乎完美普通传输的可切换太赫兹波束转向
IF 3.9 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2025-07-01 DOI: 10.1002/adpr.202500073
Zhixiang Huang, Jie Ji, Ke Ma, Eric Herrmann, Riad Yahiaoui, S M Jahadun Nobi, Fei Ding, Peter Uhd Jepsen, Thomas A. Searles, Binbin Zhou, Zizwe Chase, Xi Wang

This study introduces a reconfigurable metasurface that achieves transmission control across a broadband terahertz (THz) frequency range by leveraging the phase transition property of vanadium dioxide (VO2) to enable precise beam steering. Designed with a single-layer metasurface composed of VO2 split-ring resonator (SRR) unit structures, this device offers switchable THz beam steering upon actuation with a global temperature change. At high temperatures corresponding to the “ON” state, the metasurface exhibits frequency-dependent THz beam steering at large angles for crosspolarized THz transmission, as demonstrated both numerically and experimentally. At room temperature and in the “OFF” state, it achieves near-perfect ordinary transmission for the incident THz light, without distorting the incoming light. The reconfigurable metasurface demonstrates an average modulation depth of 95% with a maximum value of 99.8% at the designed deflection angles. This innovative approach indicates the potential advanced applications in THz technology, including communications, imaging, and sensing, which require high-performance, efficient, and reconfigurable THz deflectors.

本研究介绍了一种可重构的超表面,通过利用二氧化钒(VO2)的相变特性来实现宽带太赫兹(THz)频率范围内的传输控制,从而实现精确的光束控制。该器件采用由VO2劈裂环谐振器(SRR)单元结构组成的单层超表面设计,在全局温度变化的驱动下提供可切换的太赫兹光束转向。在对应于“开”状态的高温下,超表面显示出频率相关的太赫兹波束在大角度下进行交叉偏振太赫兹传输,数值和实验都证明了这一点。在室温和“关闭”状态下,它实现了入射太赫兹光的近乎完美的普通传输,而不会扭曲入射光。在设计的偏转角度下,可重构超表面的平均调制深度为95%,最大值为99.8%。这种创新的方法表明了太赫兹技术的潜在先进应用,包括通信、成像和传感,这些都需要高性能、高效和可重构的太赫兹偏转器。
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引用次数: 0
Surface Oxidation of 2D γ-Indium Sulfide Nanoplatelets and Its Impact on Photoluminescence 二维γ-硫化铟纳米片的表面氧化及其对光致发光的影响
IF 3.9 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2025-07-01 DOI: 10.1002/adpr.202500017
Leyre Aldaz-Caballero, Nan Liu, Pablo Molina, Antonio Arranz, Eva Hemmer, Antonio Benayas, Riccardo Marin

Two-dimensional (2D) semiconductor materials are being explored for applications including photocatalysis and optoelectronic devices. This class of materials features high surface-to-volume ratio that imparts unique physical properties. Yet, this feature makes 2D semiconductor materials prone to chemical changes that translate to variations in their photophysical behavior. Large-scale application of these materials requires an understanding of degradation processes toward developing strategies to increase their stability. Here, the effect of air exposure on underexplored 2D semiconductor material γ-In2S3 is studied. This In2S3 polymorph is stabilized as nanoplatelets, which are then characterizes before and after exposure to air. A marked surface oxidation , accompanied by drastic variations in photoluminescence is observed. Temperature-dependent spectroscopic measurements show that the emission spectrum of fresh γ-In2S3 nanoplatelets is dominated by two defect-related bands, while oxidation enhances the contribution of a third band. An energy level scheme is proposed based on the analysis of the spectroscopic data. This study finally portrays how a postsynthesis treatment with an oxygen-containing molecule (oleic acid) changes the photoluminescence of γ-In2S3 nanoplatelets similarly to a prolonged air exposure. The work shines light on the optical properties of γ-In2S3, paving the way for their control and the use of this material in luminescence sensing.

二维(2D)半导体材料正在探索用于包括光催化和光电子器件在内的应用。这类材料具有高的表面体积比,赋予其独特的物理性能。然而,这一特性使得二维半导体材料容易发生化学变化,从而导致其光物理行为的变化。这些材料的大规模应用需要对降解过程的理解,以制定增加其稳定性的策略。本文研究了空气暴露对未开发的二维半导体材料γ-In2S3的影响。这种In2S3多晶型被稳定为纳米血小板,然后在暴露于空气前后对其进行表征。观察到明显的表面氧化,并伴有光致发光的剧烈变化。温度相关的光谱测量表明,新鲜γ-In2S3纳米血小板的发射光谱主要由两个缺陷相关的波段主导,而氧化增强了第三个波段的贡献。在对光谱数据进行分析的基础上,提出了一种能级方案。本研究最终描述了含氧分子(油酸)的合成后处理如何改变γ-In2S3纳米血小板的光致发光,类似于长时间暴露在空气中。这项工作揭示了γ-In2S3的光学特性,为它们的控制和在发光传感中使用这种材料铺平了道路。
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引用次数: 0
A Trade-Off between Pulse Energy and Stability in Seeded Free-Electron Lasers 种子自由电子激光器中脉冲能量与稳定性的权衡
IF 3.9 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2025-06-25 DOI: 10.1002/adpr.202400219
Li Zeng, Huaiqian Yi, Xiaofan Wang, Chao Feng, Weiqing Zhang

Over the last decade, external seeded free-electron lasers (FELs) have achieved significant advancements across various disciplines, progressively establishing themselves as indispensable tools in fields ranging from fundamental science to industrial applications. The performance of seeded FELs is critically dependent on the quality of the frequency up-conversion process. Optimized conditions for seeded FELs are typically considered as the maximization of the bunching factor. This article discusses alternative perspectives on the optimization criteria for seeded FELs by analyzing the impact of dispersion strength on their overall performance. This study investigates the differences among the required dispersion strength for achieving the maximum bunching factor, maximum pulse energy, optimal energy stability through theoretical analysis, simulation calculations, and experimental explorations. The direct observation in experiments emphasizes the consideration of trade-off between pulse energy and energy stability in seeded FELs. These results provide valuable insights and practical guidance for controlling the pulse characteristics of seeded FELs, contributing to the tuning and optimization of FEL facilities.

在过去的十年中,外部种子自由电子激光器(FELs)在各个学科领域取得了重大进展,逐渐成为从基础科学到工业应用领域不可或缺的工具。种子FELs的性能很大程度上取决于频率上转换过程的质量。优化条件的种子fel通常被认为是最大的聚束因子。本文通过分析色散强度对其整体性能的影响,讨论了关于种子场的优化标准的不同观点。本研究通过理论分析、模拟计算和实验探索,探讨了实现最大聚束因子、最大脉冲能量和最佳能量稳定性所需的色散强度之间的差异。实验中的直接观察强调了在种子场中考虑脉冲能量和能量稳定性之间的权衡。这些结果为控制种子FEL的脉冲特性提供了有价值的见解和实用指导,有助于FEL设备的调谐和优化。
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引用次数: 0
Improvement of Cu Ablation Efficiency Using GHz-Burst Femtosecond Laser at 515 nm Wavelength 515nm波长GHz-Burst飞秒激光提高Cu烧蚀效率
IF 3.9 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2025-06-25 DOI: 10.1002/adpr.202500002
Ashkan Momeni, Shota Kawabata, Kotaro Obata, Koji Sugioka

In recent years, gigahertz (GHz)-burst-mode femtosecond lasers have revolutionized laser processing by significantly improving processing efficiency and quality. However, the underlying mechanisms are still unclear and experimentally optimizing the processing parameters is difficult due to their huge number. This study implements a theoretical approach based on simulations to investigate the underlying mechanisms of the Cu ablation efficiency enhancement by GHz-burst mode. The simulation results obtained using a two-temperature model suggest that the ablation efficiency is improved due to the interaction of subsequent intra-pulses in a GHz burst with Cu melted by the preceding intra-pulses. It is demonstrated that for GHz-burst mode, a 515 nm wavelength achieves higher Cu ablation performance than when using the infrared wavelength and demonstrates 2.8 times higher ablation efficiency than the single-pulse mode. The simulation results well agree with the experimental results. The approach used here represents a major advance not only in understanding the underlying mechanisms but also in determining the optimal processing conditions for practical applications.

近年来,千兆赫(GHz)突发模式飞秒激光器通过显著提高加工效率和质量,彻底改变了激光加工。然而,其潜在的机制尚不清楚,并且由于其数量众多,实验优化加工参数很困难。本研究采用基于仿真的理论方法研究了GHz-burst模式提高Cu烧蚀效率的潜在机制。采用双温度模型的仿真结果表明,由于在GHz突发中后续的内脉冲与前一个内脉冲熔化的Cu相互作用,提高了烧蚀效率。结果表明,在GHz-burst模式下,515 nm波长的Cu烧蚀性能优于红外模式,烧蚀效率是单脉冲模式的2.8倍。仿真结果与实验结果吻合较好。这里使用的方法不仅在理解潜在机制方面,而且在确定实际应用的最佳处理条件方面都取得了重大进展。
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引用次数: 0
Review of Coherent Anti-Stokes Raman Scattering Nonresonant Background Removal and Phase Retrieval Approaches: From Experimental Methods to Deep Learning Algorithms 相干反斯托克斯拉曼散射非共振背景去除和相位恢复方法综述:从实验方法到深度学习算法
IF 3.9 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2025-06-25 DOI: 10.1002/adpr.202500035
Rajendhar Junjuri, Thomas Bocklitz

Coherent anti-Stokes Raman spectroscopy (CARS) is a nonlinear optical technique widely utilized for vibrational imaging and molecular characterization in fields such as chemistry, biology, medicine, and materials science. Despite the high signal intensity provided by CARS, the nonresonant background (NRB) can obscure valuable molecular fingerprint information. Therefore, effective NRB removal and phase retrieval are essential for achieving precise spectral analysis and accurate material characterization. This review provides a comprehensive overview of the evolution of CARS-NRB removal and phase retrieval methods, tracing the transition from classical experimental techniques and numerical algorithms to cutting-edge deep learning models. The discussion evaluates the strengths and limitations of each approach and explores future directions for integrating deep learning to improve phase retrieval accuracy and NRB removal efficiency in CARS applications.

相干反斯托克斯拉曼光谱(CARS)是一种非线性光学技术,广泛应用于化学、生物、医学和材料科学等领域的振动成像和分子表征。尽管CARS提供了高信号强度,但非共振背景(NRB)会掩盖有价值的分子指纹信息。因此,有效的NRB去除和相位恢复对于实现精确的光谱分析和准确的材料表征至关重要。本文全面概述了CARS-NRB去除和相位恢复方法的发展,追溯了从经典实验技术和数值算法到尖端深度学习模型的转变。讨论评估了每种方法的优势和局限性,并探讨了集成深度学习以提高CARS应用中相位检索精度和NRB去除效率的未来方向。
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引用次数: 0
High-Chroma, High-Contrast Tunable Color Coatings Using Sb2S3 in a Metal-Dielectric Stack 利用Sb2S3在金属-介电层中制备高色度、高对比度可调彩色涂层
IF 3.9 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2025-06-23 DOI: 10.1002/adpr.202400194
Riley Shurvinton, Arjun Karimbana, Priya Dominic, Antonin Moreau, Olivier Hector, Konstantinos Iliopoulos, Fabien Lemarchand, Julien Lumeau

Thin-film coatings are a versatile option for creating color. These coatings can be made tunable by introducing phase-change materials (PCMs), whose optical response changes due to an external signal. However, commonly used PCMs such as Ge2Sb2Te5 (GST) are limited in their applications for color coatings, due to high absorption of visible light. Here, the alternative PCM Sb2S3 is used, and a novel coating design is demonstrated, which incorporates the PCM layer into an asymmetric Fabry–Perot cavity with Ag, SiO2 and Ti layers. Simulations are used to show that this design yields high-chroma colors in a wide range of hues, which exhibit a large tunable hue shift when the phase of the Sb2S3 layer changes. Three coatings are deposited to experimentally verify these results, which give good agreement with the simulations. The phase change of the Sb2S3 layer is demonstrated using direct heating using a hotplate, and also using laser annealing, which allows microscale image writing to be realized on the coatings.

薄膜涂层是创造颜色的通用选择。这些涂层可以通过引入相变材料(PCMs)来实现可调谐,相变材料的光学响应会因外部信号而改变。然而,常用的PCMs,如Ge2Sb2Te5 (GST),由于对可见光的高吸收,在彩色涂料中的应用受到限制。本研究采用了另一种PCM Sb2S3,并展示了一种新的涂层设计,该涂层将PCM层整合到具有Ag、SiO2和Ti层的不对称Fabry-Perot腔中。仿真结果表明,该设计可以在大范围的色调中产生高色度的颜色,当Sb2S3层的相位变化时,其表现出较大的可调色调偏移。通过实验验证了上述结果,结果与模拟结果吻合较好。采用热板直接加热和激光退火的方法对Sb2S3层的相变进行了验证,从而实现了涂层上的微尺度图像写入。
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引用次数: 0
Design Method of Time-Multiplexed Ultrashort Throw Ratio Projection System with Low Distortion and Uniform Resolution 低失真、均匀分辨率时复用超短投比投影系统设计方法
IF 3.9 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2025-06-23 DOI: 10.1002/adpr.202400224
Yuefan Shan, Jiaping Sun, Xilong Dai, Da Wang, Yongqi Liu, Dewen Cheng

Time-multiplexed laser projection is recognized as a promising projection technology owing to its broad color gamut and high energy efficiency. The escalating demands for enhanced laser safety and reduced space occupation necessitate the development of ultrashort throw ratio (UTR) projectors. However, the inherent mechanical deflection limitations and distortions of micro electro mechanical systems (MEMS) scanners pose significant challenges to achieving UTR projection. To address these constraints, trapezoidal distortion is first eliminated by ensuring vertical laser incidence on MEMS mirrors during the initial projection phase. Subsequently, a systematic design methodology for UTR laser MEMS projection systems is proposed, incorporating a miniaturized catadioptric projection objective that maintains uniformly optical étendue distribution. This configuration achieves a throw ratio of 0.27, reduces pillow distortion to 0.4%, and ensures consistent resolution across the entire screen. Segmentation and modular assembly of the catadioptric objective at telecentric intermediate image planes enhances the efficiency of initial structural design phase. The developed projection prototype experimentally validates the efficacy of the projection system designed through the proposed methodology in decreasing the projection ratio, correcting distortion, and maintaining uniform projection resolution across the full field of view.

时间复用激光投影以其广色域和高能效被认为是一种很有前途的投影技术。对提高激光安全性和减少空间占用的日益增长的需求使超短射比(UTR)投影仪的发展成为必要。然而,微机电系统(MEMS)扫描仪固有的机械偏转限制和畸变对实现UTR投影提出了重大挑战。为了解决这些限制,首先通过在初始投影阶段确保垂直激光入射到MEMS反射镜上来消除梯形畸变。随后,提出了一种UTR激光MEMS投影系统的系统设计方法,该系统采用了一种小型化的反射投影物镜,以保持均匀的光学调制调制分布。这种配置实现了0.27的投掷比,将枕头失真降低到0.4%,并确保整个屏幕的分辨率一致。在远心中间像面上对反射物镜进行分割和模块化装配,提高了初始结构设计阶段的效率。通过实验验证了采用该方法设计的投影系统在降低投影比、校正畸变和保持全视场均匀投影分辨率等方面的有效性。
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引用次数: 0
Topological Berry Antenna on a Silicon Chip for Terahertz Wireless Communication 用于太赫兹无线通信的硅晶片拓扑Berry天线
IF 3.9 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2025-06-22 DOI: 10.1002/adpr.202500123
Sonu Kumar, Ridong Jia, Yi Ji Tan, Thomas Caiwei Tan, Pascal Szriftgiser, G. Arun Kumar, Guillaume Ducournau, Arokiaswami Alphones, Ranjan Singh

Nonzero Berry curvature is central to the existence of topological edge states in electronic and photonic valley-Hall systems. While manipulating the Berry curvature in condensed matter systems is challenging, valley-Hall topological photonics offer unprecedented control, where the broken spatial inversion symmetry alters the Berry curvature. Herein, an all-silicon Berry antenna is presented, using a continuously varying geometry corresponding to a gradual change in Berry curvature. The on-chip topological edge mode with a tunable field extent is achieved to enhance effective antenna aperture, creating a high-gain on-chip photonic antenna with perfectly planar wavefronts. Experimentally, a maximum gain of 17 dBi that supports 20 Gbps chip-to-chip wireless communication is demonstrated, with active optical tunability of the antenna gain with modulation depths of 8 dBi. This Berry antenna paves the way for the development of complementary metal-oxide-semiconductor (CMOS) compatible topological Berry devices, with potential applications in integrated micro-/nano-photonics, next-generation wireless communications (6G to Xth generation), and terahertz detection and ranging.

在电子和光子谷-霍尔系统中,非零贝里曲率是拓扑边缘态存在的核心。虽然在凝聚态系统中操纵贝里曲率是具有挑战性的,但谷-霍尔拓扑光子学提供了前所未有的控制,其中空间反演对称性的破坏改变了贝里曲率。本文提出了一种全硅贝里天线,采用连续变化的几何形状,对应于贝里曲率的逐渐变化。实现了具有可调场域的片上拓扑边缘模式,提高了天线的有效孔径,形成了具有完美平面波前的高增益片上光子天线。实验结果表明,该天线的最大增益为17 dBi,支持20 Gbps的片对片无线通信,并且在调制深度为8 dBi的情况下,天线增益具有主动光可调性。这种Berry天线为互补金属氧化物半导体(CMOS)兼容拓扑Berry器件的发展铺平了道路,在集成微/纳米光子学、下一代无线通信(6G到x代)以及太赫兹探测和测距方面具有潜在的应用前景。
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引用次数: 0
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Advanced Photonics Research
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