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Large-area fabrication of 2D layered topological semimetal films and emerging applications 二维层状拓扑半金属薄膜的大面积制备及其新兴应用
IF 6 2区 物理与天体物理 Q1 Physics and Astronomy Pub Date : 2022-02-22 DOI: 10.1080/23746149.2022.2034529
Wenzhuo Zhuang, Zhong X. Chen, Xuefeng Wang
ABSTRACT Topological semimetals represent a new class of topological materials, which are highly desirable for both physics frontier and electronics applications owing to their nontrivial band structures and topologically protected surface states. The large-area fabrication of high-quality topological semimetal films is the prerequisite step to realize their practical applications. Its progress has located in its infant period. In this mini-review, we summarize several typical techniques for the fabrication of large-area 2D layered topological semimetal films. The recent progress in these large-area films for electronics, optoelectronics, terahertz, and spintronics applications is briefly reviewed. It is anticipated that with the rapid development of scalable, reliable, and low-cost production techniques and improved functional realization, large-area 2D layered topological semimetals would find the wide commercial applications in electronics, energy and beyond. Graphical Abstract
拓扑半金属是一类新的拓扑材料,由于其非平凡的能带结构和拓扑保护的表面态,在物理前沿和电子学应用中都非常受欢迎。大面积制备高质量拓扑半金属膜是实现其实际应用的前提步骤。它的进步处于萌芽阶段。在这篇小综述中,我们总结了制备大面积二维层状拓扑半金属膜的几种典型技术。简要介绍了这些大面积薄膜在电子、光电子、太赫兹和自旋电子学应用方面的最新进展。预计随着可扩展、可靠、低成本生产技术的快速发展和功能实现的改进,大面积二维层状拓扑半金属将在电子、能源等领域获得广泛的商业应用。图形摘要
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引用次数: 4
Ultrafast dynamics of electrons and phonons: from the two-temperature model to the time-dependent Boltzmann equation 电子和声子的超快动力学:从双温模型到随时间变化的玻尔兹曼方程
IF 6 2区 物理与天体物理 Q1 Physics and Astronomy Pub Date : 2022-02-15 DOI: 10.1080/23746149.2022.2095925
F. Caruso, D. Novko
ABSTRACT The advent of pump-probe spectroscopy techniques paved the way to the exploration of ultrafast dynamics of electrons and phonons in crystalline solids. Following photo-absorption of a pump pulse and the initial electronic thermalization, the dynamics of electronic and vibrational degrees of freedom is dominated by electron-phonon and phonon-phonon scattering processes. The two-temperature model (TTM) and its generalizations provide valuable tools to describe these phenomena and the ensuing coupled dynamics of electrons and phonons. While more sophisticated theoretical approaches are nowadays available, the conceptual and computational simplicity of the TTM makes it the method of choice to model thermalization processes in pump-probe spectroscopy, and it keeps being widely applied in both experimental and theoretical studies. In the domain of ab-initio methods, the time-dependent Boltzmann equation (TDBE) ameliorates many of the shortcomings of the TTM and enables a realistic and parameter-free description of ultrafast phenomena with full momentum resolution. After a pedagogical introduction to the TTM and TDBE, in this manuscript we review their application to the description of ultrafast process in solid-state physics and materials science as well as their theoretical foundation. GRAPHICAL ABSTRACT
摘要泵浦探针光谱技术的出现为探索晶体固体中电子和声子的超快动力学铺平了道路。在泵浦脉冲的光吸收和初始电子热化之后,电子和振动自由度的动力学由电子-声子和声子-声子散射过程主导。双温度模型(TTM)及其推广为描述这些现象以及随之而来的电子和声子的耦合动力学提供了有价值的工具。虽然现在有更复杂的理论方法,但TTM的概念和计算简单性使其成为泵浦探针光谱中模拟热化过程的首选方法,并在实验和理论研究中得到广泛应用。在从头算方法领域,含时玻尔兹曼方程(TDBE)改善了TTM的许多缺点,并能够以全动量分辨率对超快现象进行真实且无参数的描述。在对TTM和TDBE进行了教学介绍后,我们在本文中回顾了它们在固体物理学和材料科学中描述超快过程的应用及其理论基础。图形摘要
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引用次数: 17
Magnetoelectricity in two-dimensional materials 二维材料中的磁电
IF 6 2区 物理与天体物理 Q1 Physics and Astronomy Pub Date : 2022-01-13 DOI: 10.1080/23746149.2022.2032343
Yìlè Yīng, U. Zülicke
ABSTRACT Since the initial isolation of few-layer graphene, a plethora of two-dimensional atomic crystals has become available, covering almost all known materials types including metals, semiconductors, superconductors, ferro- and antiferromagnets. These advances have augmented the already existing variety of two-dimensional materials that are routinely realized by quantum confinement in bulk-semiconductor heterostructures. This review focuses on the type of material for which two-dimensional realizations are still being actively sought: magnetoelectrics. We present an overview of current theoretical expectation and experimental progress towards fabricating low-dimensional versions of such materials that can be magnetized by electric charges and polarized electrically by an applied magnetic field – unusual electromagnetic properties that could be the basis for various useful applications. The interplay between spatial confinement and magnetoelectricity is illustrated using the paradigmatic example of magnetic-monopole fields generated by electric charges in or near magnetoelectric media. For the purpose of this discussion, the image-charge method familiar from electrostatics is extended to solve the boundary-value problem for a magnetoelectric medium in the finite-width slab geometry using image dyons, i.e. point objects having both electric and magnetic charges. We discuss salient features of the magnetoelectrically induced fields arising in the thin-width limit. Graphical abstract
摘要自从最初分离出单层石墨烯以来,大量的二维原子晶体已经问世,几乎涵盖了所有已知的材料类型,包括金属、半导体、超导体、铁磁体和反铁磁体。这些进步增加了已经存在的各种二维材料,这些材料通常通过体半导体异质结构中的量子限制来实现。这篇综述的重点是仍在积极寻求二维实现的材料类型:磁电。我们概述了目前制造低维材料的理论预期和实验进展,这些材料可以通过电荷磁化,并通过施加的磁场进行电极化——这是一种不寻常的电磁特性,可能是各种有用应用的基础。利用磁电介质中或附近电荷产生的磁单极子场的范例,说明了空间约束和磁电之间的相互作用。为了进行讨论,将静电学中常见的图像电荷方法扩展到使用图像dyon(即同时具有电荷和磁电荷的点对象)求解有限宽度平板几何中磁电介质的边值问题。我们讨论了在薄宽度极限下产生的磁电感应场的显著特征。图形摘要
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引用次数: 10
Second order nonlinear frequency generation at the nanoscale in dielectric platforms 介质平台纳米级二阶非线性频率产生
IF 6 2区 物理与天体物理 Q1 Physics and Astronomy Pub Date : 2022-01-13 DOI: 10.1080/23746149.2021.2022992
D. Rocco, R. C. Morales, Lei Xu, A. Zilli, V. Vinel, M. Finazzi, M. Celebrano, G. Leo, M. Rahmani, C. Jagadish, H. Tan, D. Neshev, C. de Angelis
ABSTRACT Nonlinear frequency generation at the nanoscale is a hot research topic which is gaining increasing attention in nanophotonics. The generation of harmonics in subwavelength volumes is historically associated with the enhancement of electric fields in the interface of plasmonic structures. Recently, new platforms based on high-index dielectric nanoparticles have emerged as promising alternatives to plasmonic structures for many applications. By exploiting optically induced electric and magnetic response via multipolar Mie resonances, dielectric nanoelements may lead to innovative opportunities in nanoscale nonlinear optics. Dielectric optical nanoantennas enlarge the volume of light–matter interaction with respect to their plasmonic counterpart, since the electromagnetic field can penetrate such materials, and therefore producing a high throughput of the generated harmonics. In this review, we first recap recent developments obtained in high refractive index structures, which mainly concern nonlinear second order effects. Moreover, we discuss configurations of dielectric nano-devices where reconfigurable nonlinear behavior is achieved. The main focus of this work concerns efficient Sum Frequency Generation in dielectric nano-platforms. The reported results may serve as a reference for the development of new nonlinear devices for nanophotonic applications. GRAPHICAL ABSTRACT
摘要纳米尺度上的非线性频率产生是纳米光子学中一个越来越受到关注的研究热点。亚波长体积中谐波的产生在历史上与等离子体结构界面中电场的增强有关。最近,基于高折射率电介质纳米颗粒的新平台已成为许多应用中等离子体结构的有前途的替代品。通过多极Mie共振利用光学感应的电和磁响应,介电纳米元件可能为纳米非线性光学带来创新机会。电介质光学纳米天线相对于其等离子体对应物扩大了光-物质相互作用的体积,因为电磁场可以穿透这些材料,因此产生高通量的谐波。在这篇综述中,我们首先回顾了高折射率结构的最新进展,主要涉及非线性二阶效应。此外,我们还讨论了实现可重构非线性行为的介电纳米器件的配置。这项工作的主要重点是在介电纳米平台中有效地产生和频。所报道的结果可为开发用于纳米光子应用的新型非线性器件提供参考。图形摘要
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引用次数: 4
Inertial measurement with solid-state spins of nitrogen-vacancy center in diamond 金刚石中氮空位中心的固态自旋惯性测量
IF 6 2区 物理与天体物理 Q1 Physics and Astronomy Pub Date : 2022-01-11 DOI: 10.1080/23746149.2021.2004921
Liye Zhao, Xiang Shen, Lumin Ji, Pu Huang
ABSTRACT The nitrogen-vacancy (NV) center is one of the major platforms in the evolving field of quantum technologies. The inertial surveying technology based on NV centers in diamond is a developing field with both scientific and technological importance. Quantum measurement using the solid-state spin of the NV center has demonstrated potential in both high-precision and small-volume low-cost devices. In terms of rotation measurement, the optically detected magnetic resonance has provided a perspective of the rotation measurement mechanism via the solid-state spin of the NV center. A new type of gyroscope based on the solid-state spin in diamond according to the theory has attracted considerable attention. In addition, combined with the ingenious quantum mechanics manipulation and coupling mechanism, acceleration measurement can be achieved through an efficient quantum detection technology of the NV center. This review summarizes the recent research progress in diamond-based inertial measurement, including sensitivity optimization methods for inertial measurement systems based on the NV center. Graphical abstract
摘要氮空位中心是量子技术发展的主要平台之一。基于金刚石NV中心的惯性测量技术是一个具有重要科学技术意义的发展领域。使用NV中心固态自旋的量子测量在高精度和小体积低成本设备中都显示出了潜力。在旋转测量方面,光学检测的磁共振通过NV中心的固态自旋提供了旋转测量机制的视角。根据该理论,一种基于金刚石中固态自旋的新型陀螺仪引起了人们的广泛关注。此外,结合巧妙的量子力学操纵和耦合机制,可以通过NV中心的高效量子检测技术实现加速度测量。本文综述了金刚石惯性测量的最新研究进展,包括基于NV中心的惯性测量系统灵敏度优化方法。图形摘要
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引用次数: 5
Machine learning in the analysis of biomolecular simulations 生物分子模拟分析中的机器学习
IF 6 2区 物理与天体物理 Q1 Physics and Astronomy Pub Date : 2022-01-10 DOI: 10.1080/23746149.2021.2006080
Shreyas S. Kaptan, I. Vattulainen
ABSTRACT Machine learning has rapidly become a key method for the analysis and organization of large-scale data in all scientific disciplines. In life sciences, the use of machine learning techniques is a particularly appealing idea since the enormous capacity of computational infrastructures generates terabytes of data through millisecond simulations of atomistic and molecular-scale biomolecular systems. Due to this explosion of data, the automation, reproducibility, and objectivity provided by machine learning methods are highly desirable features in the analysis of complex systems. In this review, we focus on the use of machine learning in biomolecular simulations. We discuss the main categories of machine learning tasks, such as dimensionality reduction, clustering, regression, and classification used in the analysis of simulation data. We then introduce the most popular classes of techniques involved in these tasks for the purpose of enhanced sampling, coordinate discovery, and structure prediction. Whenever possible, we explain the scope and limitations of machine learning approaches, and we discuss examples of applications of these techniques. Graphical Abstract
机器学习已迅速成为所有科学学科中分析和组织大规模数据的关键方法。在生命科学中,机器学习技术的使用是一个特别吸引人的想法,因为计算基础设施的巨大容量通过毫秒级的原子和分子尺度的生物分子系统模拟产生tb级的数据。由于数据的爆炸式增长,机器学习方法所提供的自动化、可重复性和客观性在复杂系统的分析中是非常理想的特征。在这篇综述中,我们重点介绍了机器学习在生物分子模拟中的应用。我们讨论了机器学习任务的主要类别,如降维、聚类、回归和用于模拟数据分析的分类。然后,我们介绍了这些任务中涉及的最流行的技术类别,以增强采样,坐标发现和结构预测。只要有可能,我们就会解释机器学习方法的范围和局限性,并讨论这些技术的应用示例。图形抽象
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引用次数: 10
Ultrafast dynamics of helical Dirac fermions in the topological insulators 拓扑绝缘体中螺旋狄拉克费米子的超快动力学
IF 6 2区 物理与天体物理 Q1 Physics and Astronomy Pub Date : 2022-01-06 DOI: 10.1080/23746149.2021.2013134
Y. Bai, Na Li, Ruxin Li, P. Liu
ABSTRACT Three-dimensional topological insulators feature unconventional two-dimensional surface states, the carriers in which are helical Dirac fermions and protected from backscattering. Thus, they exhibit novel electronic response upon illuminate ultrashort and intense laser light. We briefly reviewed recent studies on ultrafast phenomena from the surface of the topological insulators driven by laser pulse ranging from visible to THz frequency. Ultrafast dynamics of Dirac fermions can be excited by helical photons and driven by strong light field. Many unique nonlinear behaviors have been demonstrated, such as the excitation of helicity-dependent photocurrent, the formation of Floquet-Bloch bands, lightwave-driven Dirac currents and the generation of optical high-harmonic emission. This review aimed at understanding the microscopic mechanism of the ultrafast charge and spin dynamics in topological surface states and its prospects for coherent manipulation of Dirac fermions by laser light. GRAPHICAL ABSTRACT
摘要三维拓扑绝缘体具有非常规的二维表面态,其中的载流子是螺旋狄拉克费米子,并受到反向散射的保护。因此,它们在照射超短和强激光时表现出新颖的电子响应。我们简要回顾了最近对拓扑绝缘体表面超快现象的研究,这些现象是由可见光到太赫兹频率的激光脉冲驱动的。狄拉克费米子的超快动力学可以由螺旋光子激发,并由强光场驱动。已经证明了许多独特的非线性行为,如螺旋度相关光电流的激发、Floquet-Bloch带的形成、光波驱动的Dirac电流和光学高次谐波发射的产生。这篇综述旨在了解拓扑表面态中超快电荷和自旋动力学的微观机制及其在激光相干操纵狄拉克费米子方面的前景。图形摘要
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引用次数: 3
Computational methods and theory for ion channel research. 离子通道研究的计算方法与理论。
IF 6 2区 物理与天体物理 Q1 Physics and Astronomy Pub Date : 2022-01-01 DOI: 10.1080/23746149.2022.2080587
C Guardiani, F Cecconi, L Chiodo, G Cottone, P Malgaretti, L Maragliano, M L Barabash, G Camisasca, M Ceccarelli, B Corry, R Roth, A Giacomello, B Roux

Ion channels are fundamental biological devices that act as gates in order to ensure selective ion transport across cellular membranes; their operation constitutes the molecular mechanism through which basic biological functions, such as nerve signal transmission and muscle contraction, are carried out. Here, we review recent results in the field of computational research on ion channels, covering theoretical advances, state-of-the-art simulation approaches, and frontline modeling techniques. We also report on few selected applications of continuum and atomistic methods to characterize the mechanisms of permeation, selectivity, and gating in biological and model channels.

离子通道是基本的生物装置,作为门,以确保选择性离子运输跨细胞膜;它们的运作构成了基本生物功能(如神经信号传递和肌肉收缩)得以实现的分子机制。在这里,我们回顾了离子通道计算研究领域的最新成果,包括理论进展,最先进的模拟方法和前沿建模技术。我们还报道了连续体和原子方法的一些选择应用,以表征生物和模型通道中的渗透,选择性和门控机制。
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引用次数: 5
Intrusion and extrusion of liquids in highly confining media: bridging fundamental research to applications 液体在高度受限介质中的侵入和挤压:连接基础研究与应用
IF 6 2区 物理与天体物理 Q1 Physics and Astronomy Pub Date : 2022-01-01 DOI: 10.1080/23746149.2022.2052353
A. Le Donne, A. Tinti, Eder Amayuelas, Hemant K. Kashyap, G. Camisasca, Richard C. Remsing, R. Roth, Yaroslav Grosu, S. Meloni
ABSTRACT Wetting and drying of pores or cavities, made by walls that attract or repel the liquid, is a ubiquitous process in nature and has many technological applications including, for example, liquid separation, chromatography, energy damping, conversion, and storage. Understanding under which conditions intrusion/extrusion takes place and how to control/tune them by chemical or physical means are currently among the main questions in the field. Historically, the theory to model intrusion/extrusion was based on the mechanics of fluids. However, the discovery of the existence of metastable states, where systems are kinetically trapped in the intruded or extruded configuration, fostered the research based on modern statistical mechanics concepts and more accurate models of the liquid, vapor, and gas phases beyond the simplest sharp interface representation. In parallel, inspired by the growing number of technological applications of intrusion/extrusion, experimental research blossomed considering systems with complex chemistry and pore topology, possessing flexible frameworks, and presenting unusual properties, such as negative volumetric compressibility. In this article, we review recent theoretical and experimental progresses, presenting it in the context of unifying framework. We illustrate also emerging technological applications of intrusion/extrusion and discuss challenges ahead. Graphical Abstract
由吸引或排斥液体的壁面形成的孔隙或空腔的润湿和干燥是自然界中普遍存在的过程,并有许多技术应用,例如液体分离、色谱、能量阻尼、转换和储存。了解在什么条件下发生侵入/挤压以及如何通过化学或物理手段控制/调整它们是目前该领域的主要问题之一。历史上,模拟侵入/挤压的理论是基于流体力学的。然而,亚稳态的存在,即系统在动力学上被困在侵入或挤压的结构中,促进了基于现代统计力学概念的研究,以及更精确的液体、蒸汽和气体相模型,而不是最简单的尖锐界面表示。与此同时,受到越来越多的侵入/挤压技术应用的启发,实验研究蓬勃发展,考虑到具有复杂化学和孔隙拓扑结构、具有柔性框架以及具有不寻常性质(如负体积压缩性)的系统。在本文中,我们回顾了近年来的理论和实验进展,并在统一框架的背景下进行了介绍。我们还说明了侵入/挤压的新兴技术应用,并讨论了未来的挑战。图形抽象
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引用次数: 10
Partially coherent light beam shaping via complex spatial coherence structure engineering 基于复杂空间相干结构工程的部分相干光束整形
IF 6 2区 物理与天体物理 Q1 Physics and Astronomy Pub Date : 2021-12-19 DOI: 10.1080/23746149.2021.2009742
Yahong Chen, Fei Wang, Y. Cai
ABSTRACT The techniques of optical beam shaping have enabled progress in a broad range of interdisciplinary science and engineering, owing to the unique properties and promising applications of their created structured light. However, the conventional methods, which are based on fully coherent optics approaches, introduce several adverse effects such as speckles noise in the generated beams and susceptible to be disturbed in complex environment (e.g. turbulent atmospheres), because of the sensitive coherent light-matter interaction. To overcome those side effects, a new protocol relied on the partially coherent beam shaping has been developed. By elaborately tailoring the complex spatial coherence structure of a partially coherent beam, the desired beam profile and trajectory with high beam quality and robust propagation feature in complex environment can be generated. In this review, we present an overview of such unconventional partially coherent beam shaping with a focus on the important role of the complex spatial coherence structure engineering. Partially coherent beam shaping not only provides an efficient means for resisting the disadvantages in coherent optics methods but also enables new applications in novel optical imaging and tweezers. Graphical abstract
光束整形技术由于其所创造的结构光的独特特性和有前途的应用,使广泛的跨学科科学和工程取得了进展。然而,传统的基于全相干光学方法的方法,由于敏感的相干光-物质相互作用,在复杂的环境(如湍流大气)中,产生的光束容易受到干扰,如斑点噪声。为了克服这些副作用,开发了一种基于部分相干光束整形的新方案。通过对部分相干光束的复杂空间相干结构进行精细裁剪,可以生成在复杂环境中具有高光束质量和鲁棒传播特性的光束轮廓和轨迹。本文对这种非常规的部分相干光束整形技术进行了综述,重点介绍了复杂空间相干结构工程的重要作用。部分相干光束整形不仅为克服相干光学方法的缺点提供了有效的手段,而且在新型光学成像和镊子中有了新的应用。图形抽象
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引用次数: 25
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Advances in Physics: X
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