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Inelastic thermoelectric transport and fluctuations in mesoscopic systems 介观系统中的非弹性热电输运和涨落
IF 6 2区 物理与天体物理 Q1 Physics and Astronomy Pub Date : 2021-12-17 DOI: 10.1080/23746149.2022.2082317
Rongqian Wang, Chen Wang, Jincheng Lu, Jian‐Hua Jiang
ABSTRACT In the past decade, a new research frontier emerges at the interface between physics and renewable energy, termed as inelastic thermoelectric effects, where inelastic transport processes play a key role. The study of inelastic thermoelectric effects broadens our understanding of thermoelectric phenomena and provides new routes towards high-performance thermoelectric energy conversion. Here, we review the main progress in this field, with a particular focus on inelastic thermoelectric effects induced by the electron-phonon and electron–photon interactions. We introduce the motivations, the basic pictures, and prototype models, as well as the unconventional effects induced by inelastic thermoelectric transport. These unconventional effects include the separation of heat and charge transport, the cooling by heating effect, the linear thermal transistor effect, nonlinear enhancement of performance, Maxwell demons, and cooperative effects. We find that elastic and inelastic thermoelectric effects are described by significantly different microscopic mechanisms and belong to distinct linear thermodynamic classes. We also pay special attention to the unique aspect of fluctuations in small mesoscopic thermoelectric systems. Finally, we discuss the challenges and future opportunities in the field of inelastic thermoelectrics. Graphical Abstract
在过去的十年中,在物理和可再生能源的界面上出现了一个新的研究前沿,即非弹性热电效应,其中非弹性输运过程起着关键作用。非弹性热电效应的研究拓宽了我们对热电现象的认识,为高性能热电能量转换提供了新的途径。本文综述了这一领域的主要进展,重点介绍了电子-声子和电子-光子相互作用引起的非弹性热电效应。我们介绍了非弹性热电输运的动机、基本图像和原型模型,以及非弹性热电输运引起的非常规效应。这些非常规效应包括热和电荷输运的分离、加热效应的冷却、线性热晶体管效应、性能的非线性增强、麦克斯韦魔和合作效应。我们发现弹性和非弹性热电效应是由不同的微观机制描述的,属于不同的线性热力学类。我们还特别注意小介观热电系统波动的独特方面。最后,讨论了非弹性热电学领域面临的挑战和未来的机遇。图形抽象
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引用次数: 9
Recent trends in high-order harmonic generation in solids 固体中高次谐波产生的最新趋势
IF 6 2区 物理与天体物理 Q1 Physics and Astronomy Pub Date : 2021-12-05 DOI: 10.1080/23746149.2021.2003244
Jongkyoon Park, Amutha V. Subramani, Seungchul Kim, M. Ciappina
ABSTRACT High-order harmonic generation in solids, the nonlinear up-conversion of coherent radiation resulting from the interaction of a strong and short laser pulse with a solid sample, has come to age. Since the first experiments and theoretical developments, there has been a constant and steady interest in this topic. In this paper, we summarize the progress made so far and propose new possibilities for the generation of high-order harmonics with the aid of plasmonic fields. The driven fields could be adequately engineered both spatially and temporally with nanometric and attosecond resolution, offering to the conventional solid-HHG novel and exciting coherent sources. Just to cite an example, the generation of attosecond pulses using bulk matter is strongly linked to the appropriate manipulation of the driven field to avoid, for instance, reaching the damage threshold of the material. Plasmonics fields as an alternative to conventional laser beams could open new avenues in the development of table-top sources of ultrashort and strong coherent radiation. Graphical abstract
摘要固体中的高次谐波产生,即强激光脉冲和短激光脉冲与固体样品相互作用产生的相干辐射的非线性上转换,已经过时。自从第一次实验和理论发展以来,人们一直对这个话题感兴趣。在本文中,我们总结了迄今为止取得的进展,并提出了借助等离子体场产生高次谐波的新可能性。驱动场可以在空间和时间上以纳米和阿秒的分辨率进行充分的设计,为传统的固体HHG提供了新颖而令人兴奋的相干源。举个例子,使用大块物质产生阿秒脉冲与适当操纵驱动场密切相关,以避免达到材料的损伤阈值。等离子体场作为传统激光束的替代品,可以为开发超短强相干辐射的桌面源开辟新的途径。图形摘要
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引用次数: 18
Flame assisted synthesis of nanostructures for device applications 用于器件应用的纳米结构的火焰辅助合成
IF 6 2区 物理与天体物理 Q1 Physics and Astronomy Pub Date : 2021-11-11 DOI: 10.1080/23746149.2021.1997153
Alishba T. John, A. Tricoli
ABSTRACT Development of fabrication technologies for three-dimensional structuring and integration of nanomaterials in devices is important for a broad range of applications, including next-generation high energy density batteries, super(de)wetting and biomedical coatings, and miniaturized biomedical diagnostics. Amongst various nanofabrication approaches, the flame synthesis route accounts for some of the first man-made nanomaterials and industrial production of various nanoparticle commodities such as carbon black, fumed silica, and pigmentary titania. In the past two decades, flexibility in nanomaterials and facile fabrication of nanostructured films by aerosol self-assembly has motivated the exploration of this technology for device applications. In this review, we present a perspective of recent progress in flame-assisted nanofabrication and its application to emerging technologies. The fundamentals of flame synthesis will be briefly reviewed to evaluate trends in flame reactor designs and directions for improvements. A selection of exemplary flame-made nanostructures will be presented across the major categories of catalysis, energy conversion devices, membranes and sensors, highlighting weakness and strengths of this synthesis route. We will conclude with an outlook towards possible implementation of flame-assisted self-assembly as a scalable tool for nanofabrication in emerging devices and a critical assessment of the persisting challenges for its broader industrial uptake. Graphical Abstract
纳米材料在器件中的三维结构和集成制造技术的发展对于下一代高能量密度电池、超(去)湿和生物医学涂层以及小型化生物医学诊断等广泛应用具有重要意义。在各种纳米制造方法中,火焰合成路线是最早的人造纳米材料和工业生产各种纳米颗粒商品,如炭黑、气相二氧化硅和颜料二氧化钛。在过去的二十年中,纳米材料的灵活性和通过气溶胶自组装制备纳米结构薄膜的便利性推动了该技术在器件应用中的探索。在这篇综述中,我们介绍了火焰辅助纳米制造的最新进展及其在新兴技术中的应用。本文将简要回顾火焰合成的基本原理,以评价火焰反应器设计的趋势和改进方向。在催化、能量转换装置、膜和传感器的主要类别中,将展示一些典型的火焰纳米结构,突出这种合成路线的优缺点。最后,我们将展望火焰辅助自组装作为新兴设备中纳米制造的可扩展工具的可能实现,并对其更广泛的工业应用所面临的持续挑战进行关键评估。图形抽象
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引用次数: 2
Electroosmosis in nanopores: computational methods and technological applications 纳米孔中的电渗:计算方法和技术应用
IF 6 2区 物理与天体物理 Q1 Physics and Astronomy Pub Date : 2021-11-10 DOI: 10.1080/23746149.2022.2036638
A. Gubbiotti, Matteo Baldelli, Giovanni Di Muccio, P. Malgaretti, S. Marbach, M. Chinappi
ABSTRACT Electroosmosis is a fascinating effect where liquid motion is induced by an applied electric field. Counter ions accumulate in the vicinity of charged surfaces, triggering a coupling between liquid mass transport and external electric field. In nanofluidic technologies, where surfaces play an exacerbated role, electroosmosis is thus of primary importance. Its consequences on transport properties in biological and synthetic nanopores are subtle and intricate. Thorough understanding is therefore challenging yet crucial to fully assess the mechanisms at play. Here, we review recent progress on computational techniques for the analysis of electroosmosis and discuss technological applications, in particular for nanopore sensing devices. Graphical Abstract
电渗透是一种由外加电场诱导液体运动的奇妙效应。反离子聚集在带电表面附近,引发液体质量输运和外电场之间的耦合。在纳米流体技术中,表面起着更大的作用,因此电渗透是最重要的。它对生物和合成纳米孔中的输运特性的影响是微妙而复杂的。因此,透彻理解对充分评估起作用的机制具有挑战性,但又至关重要。在这里,我们回顾了电渗透分析的计算技术的最新进展,并讨论了技术应用,特别是纳米孔传感装置。图形抽象
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引用次数: 14
Experimental challenges in ion channel research: uncovering basic principles of permeation and gating in potassium channels 离子通道研究中的实验挑战:揭示钾通道中渗透和门控的基本原理
IF 6 2区 物理与天体物理 Q1 Physics and Astronomy Pub Date : 2021-10-15 DOI: 10.1080/23746149.2021.1978317
J. Carvalho-de-Souza, A. Saponaro, C. Bassetto, O. Rauh, I. Schroeder, F. Franciolini, L. Catacuzzeno, F. Bezanilla, G. Thiel, A. Moroni
ABSTRACT Biological ion channels precisely control the flow of ions across membranes in response to a range of physical and chemical stimuli. With their ability of transporting ions in a highly selective manner and of integrating regulatory cues, they are a source of inspiration for the construction of solid-state nanopores as sensors or switches for practical applications. Here, we summarize recent advancements in understanding the mechanisms of ion permeation and gating in channel proteins with a focus on the elementary steps of ion transport through the pore and on non-canonical modes of intramolecular communication between peripheral sensory domains and the central channel pore. Graphical Abstract
生物离子通道在一系列物理和化学刺激下精确控制离子在膜上的流动。由于它们具有以高度选择性的方式运输离子和整合调节信号的能力,它们是构建固态纳米孔作为实际应用的传感器或开关的灵感来源。在这里,我们总结了离子在通道蛋白中渗透和门控机制的最新进展,重点介绍了离子通过孔运输的基本步骤以及外周感觉域与中央通道孔之间的分子内通信的非规范模式。图形抽象
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引用次数: 4
Strong-field physics with nanospheres 纳米球的强场物理
IF 6 2区 物理与天体物理 Q1 Physics and Astronomy Pub Date : 2021-09-06 DOI: 10.1080/23746149.2021.2010595
L. Seiffert, S. Zherebtsov, M. Kling, T. Fennel
ABSTRACT When intense laser fields interact with nanoscale targets, strong-field physics meets plasmonic near-field enhancement and subwavelength localization of light. Photoemission spectra reflect the associated attosecond optical and electronic response and encode the collisional and collective dynamics of the solid. Nanospheres represent an ideal platform to explore the underlying attosecond nanophysics because of their particularly simple geometry. This review summarizes key results from the last decade and aims to provide the essential stepping stones for students and researchers to enter this field. Graphical abstract
摘要当强激光场与纳米级目标相互作用时,强场物理会遇到等离子体近场增强和光的亚波长局域化。光发射光谱反映了相关的阿秒光学和电子响应,并编码了固体的碰撞和集体动力学。纳米球是探索阿秒纳米物理的理想平台,因为它们的几何形状特别简单。这篇综述总结了过去十年的主要成果,旨在为学生和研究人员进入这一领域提供重要的垫脚石。图形摘要
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引用次数: 5
Prospects and applications of photonic neural networks 光子神经网络的展望与应用
IF 6 2区 物理与天体物理 Q1 Physics and Astronomy Pub Date : 2021-05-20 DOI: 10.1080/23746149.2021.1981155
Chaoran Huang, V. Sorger, M. Miscuglio, M. Al-Qadasi, Avilash Mukherjee, S. Shekhar, L. Chrostowski, L. Lampe, Mitchell Nichols, M. Fok, D. Brunner, A. Tait, T. F. D. Lima, B. Marquez, P. Prucnal, B. Shastri
ABSTRACT Neural networks have enabled applications in artificial intelligence through machine learning, and neuromorphic computing. Software implementations of neural networks on conventional computers that have separate memory and processor (and that operate sequentially) are limited in speed and energy efficiency. Neuromorphic engineering aims to build processors in which hardware mimics neurons and synapses in the brain for distributed and parallel processing. Neuromorphic engineering enabled by photonics (optical physics) can offer sub-nanosecond latencies and high bandwidth with low energies to extend the domain of artificial intelligence and neuromorphic computing applications to machine learning acceleration, nonlinear programming, intelligent signal processing, etc. Photonic neural networks have been demonstrated on integrated platforms and free-space optics depending on the class of applications being targeted. Here, we discuss the prospects and demonstrated applications of these photonic neural networks. Graphical Abstract
神经网络通过机器学习和神经形态计算在人工智能中实现了应用。神经网络在传统计算机上的软件实现具有独立的存储器和处理器(并按顺序运行),在速度和能源效率方面受到限制。神经形态工程旨在制造处理器,其中的硬件模仿大脑中的神经元和突触,以进行分布式和并行处理。光子神经网络已经在集成平台和自由空间光学上进行了演示,具体取决于所针对的应用类别。在这里,我们讨论了这些光子神经网络的前景和演示应用。图形抽象
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引用次数: 63
High bandwidth temporal RF photonic signal processing with Kerr micro-combs: integration, fractional differentiation and Hilbert transforms 克尔微梳的高带宽时域射频光子信号处理:积分、分数阶微分和希尔伯特变换
IF 6 2区 物理与天体物理 Q1 Physics and Astronomy Pub Date : 2021-02-17 DOI: 10.1080/23746149.2020.1838946
M. Tan, Xingyuan Xu, Jiayang Wu, D. Moss
Integrated Kerr micro-combs, a powerful source of many wavelengths for photonic RF and microwave signal processing, are particularly useful for transversal filter systems. They have many advantages including a compact footprint, high versatility, large numbers of wavelengths, and wide bandwidths. We review recent progress on photonic RF and microwave high bandwidth temporal signal processing based on Kerr micro-combs with spacings from 49-200GHz. We cover integral and fractional Hilbert transforms, differentiators as well as integrators. The potential of optical micro-combs for RF photonic applications in functionality and ability to realize integrated solutions is also discussed.
集成克尔微梳,一个强大的许多波长的光子射频和微波信号处理源,是特别有用的横向滤波系统。它们具有许多优点,包括占地面积小、通用性强、波长数量多和带宽宽。本文综述了基于49 ~ 200ghz克尔微梳的光子射频和微波高带宽时域信号处理的最新进展。我们涵盖了积分和分数希尔伯特变换,微分和积分器。讨论了光学微梳在射频光子应用中的功能和集成解决方案的潜力。
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引用次数: 15
Future applications of the high-flux thermal neutron spectroscopy: the ever-green case of collective excitations in liquid metals 高通量热中子能谱的未来应用:液态金属中集体激发的绿色案例
IF 6 2区 物理与天体物理 Q1 Physics and Astronomy Pub Date : 2021-01-01 DOI: 10.1080/23746149.2021.1871862
C. Petrillo, F. Sacchetti
ABSTRACT The European landscape of neutron sources for research applications is changing and the major European joint effort, the European Spallation Source (ESS) currently under construction in Lund (Sweden), is progressing. The high flux source ESS is designed to deliver slow neutrons with a long-pulse time structure, a rather unique feature, with characteristics optimised to maximise the instrument performances and the experimental throughput. This is expected to result in unprecedented scientific capability over broad research areas. Major breakthroughs are likely to take place in the understanding of complex, strongly interacting and disordered systems, more specifically on their dynamical response. This will have an impact on the development of novel theories to cover some of the presently existing knowledge gaps and will prompt advanced applications of the investigated materials. Liquid metals are a prototypical example of complex systems extensively studied from the sixties on, now re-emerging as powerful functional materials for unconventional and broad spectrum applications. Research on liquid metal composites will benefit of the new experimental possibilities available at the ESS. We review the status of the experiments on liquid metals dynamics, focusing on a selected set of systems, and discuss the perspectives for cutting-edge experiments at the new sources. Graphical abstract
摘要欧洲用于研究应用的中子源格局正在发生变化,欧洲的主要合作项目——目前正在瑞典隆德建造的欧洲散裂源(ESS)正在取得进展。高通量源ESS设计用于输送具有长脉冲时间结构的慢中子,这是一个相当独特的特征,其特性经过优化以最大限度地提高仪器性能和实验吞吐量。预计这将在广泛的研究领域产生前所未有的科学能力。在理解复杂、强相互作用和无序系统方面,特别是在其动力学响应方面,可能会取得重大突破。这将对新理论的发展产生影响,以弥补目前存在的一些知识空白,并将促进所研究材料的先进应用。液态金属是从60年代开始广泛研究的复杂系统的典型例子,现在又重新成为非常规和广谱应用的强大功能材料。对液态金属复合材料的研究将受益于ESS提供的新的实验可能性。我们回顾了液体金属动力学实验的现状,重点关注一组选定的系统,并讨论了在新来源进行尖端实验的前景。图形摘要
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引用次数: 5
Disorder effects on quantum transport and quantum phase transition in low-dimensional superconducting and topological systems 无序对低维超导和拓扑系统中量子输运和量子相变的影响
IF 6 2区 物理与天体物理 Q1 Physics and Astronomy Pub Date : 2021-01-01 DOI: 10.1080/23746149.2021.1884133
Haijiao Ji, Haiwen Liu, Hua Jiang, Xincheng Xie
ABSTRACT Disorder effects inevitably exist in realistic samples, manifesting in various physical properties. In this paper, we review the recent progress in understanding the disorder effects on quantum transport and quantum phase transition properties in low-dimensional superconducting and topological systems. As a consequence of the pronounced quantum fluctuation in low-dimensional systems, rare events drastically change the physical characteristics and underlying microscopic transport process in these systems, which are beyond the traditional paradigms. Associating with recent experimental observations, we emphasize the microscopic mechanism for disordered Ising superconductivity, the quantum Griffiths singularity of superconductor metal transition and the discrete scale invariance in topological materials. GRAPHICAL ABSTRACT
无序效应不可避免地存在于现实样品中,表现为各种物理性质。在本文中,我们回顾了在理解低维超导和拓扑系统中无序对量子输运和量子相变性质的影响方面的最新进展。由于低维系统中明显的量子涨落,罕见事件极大地改变了这些系统中的物理特性和潜在的微观输运过程,这超出了传统的范式。结合最近的实验观察,我们强调了无序伊辛超导的微观机制、超导体-金属跃迁的量子Griffiths奇异性以及拓扑材料中的离散尺度不变性。图形摘要
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引用次数: 5
期刊
Advances in Physics: X
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