Marcos Villeda-Hernandez, Benjamin C. Baker, Christian Romero, Jonathan M. Rossiter, C. Faul
Soft robotics has emerged as a transformative field, leveraging bio-inspired novel actuation mechanisms to enable more adaptable, compliant, and sophisticated robotic systems. However, the portability of soft pneumatic actuators is typically constrained by the tethering to bulky power sources. This review offers a thorough analysis of autonomous power alternatives facilitated by chemical reactions for gas generation and absorption, a concept analogous to biological energy conversion processes. These bio-inspired strategies propel soft pneumatic actuators towards new horizons of autonomy and portability, essential for real-world applications. This comprehensive review explores the critical intersection of gas evolution reactions (GERs) and gas consumption reactions (GCRs) as a power source for pneumatic actuation in soft robotics. We here emphasize the importance and impact of bio-inspired design, control, efficiency, safety, and sustainability within soft robotics to not only mimic biological motions but to enhance them. This review explores the fundamentals of both pneumatic and chemically powered actuation, highlighting the need for careful consideration of reaction kinetics. Additionally, this work highlights key aspects of smart materials that draw from biological structures and response mechanisms, along with state-of-the-art techniques for precise pressure modulation. Finally, we chart prospective development pathways and provide a future outlook for bio-inspired soft robotics, emphasizing the transformative impact of integrating chemical actuation methods. This exploration underlines the quest for further autonomy in soft robotic systems and points towards the future opportunities in this exciting and fast-developing field.
{"title":"Soft alchemy: a comprehensive guide to chemical reactions for pneumatic soft actuation","authors":"Marcos Villeda-Hernandez, Benjamin C. Baker, Christian Romero, Jonathan M. Rossiter, C. Faul","doi":"10.20517/ss.2023.52","DOIUrl":"https://doi.org/10.20517/ss.2023.52","url":null,"abstract":"Soft robotics has emerged as a transformative field, leveraging bio-inspired novel actuation mechanisms to enable more adaptable, compliant, and sophisticated robotic systems. However, the portability of soft pneumatic actuators is typically constrained by the tethering to bulky power sources. This review offers a thorough analysis of autonomous power alternatives facilitated by chemical reactions for gas generation and absorption, a concept analogous to biological energy conversion processes. These bio-inspired strategies propel soft pneumatic actuators towards new horizons of autonomy and portability, essential for real-world applications. This comprehensive review explores the critical intersection of gas evolution reactions (GERs) and gas consumption reactions (GCRs) as a power source for pneumatic actuation in soft robotics. We here emphasize the importance and impact of bio-inspired design, control, efficiency, safety, and sustainability within soft robotics to not only mimic biological motions but to enhance them. This review explores the fundamentals of both pneumatic and chemically powered actuation, highlighting the need for careful consideration of reaction kinetics. Additionally, this work highlights key aspects of smart materials that draw from biological structures and response mechanisms, along with state-of-the-art techniques for precise pressure modulation. Finally, we chart prospective development pathways and provide a future outlook for bio-inspired soft robotics, emphasizing the transformative impact of integrating chemical actuation methods. This exploration underlines the quest for further autonomy in soft robotic systems and points towards the future opportunities in this exciting and fast-developing field.","PeriodicalId":74837,"journal":{"name":"Soft science","volume":"33 5","pages":""},"PeriodicalIF":0.0,"publicationDate":"2024-03-29","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"140368312","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Gabrielle Blewitt, D. Cheneler, Jeremy Andrew, Stephen Monk
In recent years, the development of worm-like robots has increased significantly. These robots use peristaltic motion comprised of radial expansion and axial elongation to move leglessly through their environments. Soft worm-like robots have the advantage of conforming to their environment, making them ideal for confined spaces such as pipelines which are essential to societal infrastructure. Pipeline contamination and corrosion can be detrimental and costly and thus regular checking is vital. Some pipes are difficult to access due to size, access restrictions and harmful waste contamination (such as in nuclear power plants). This has led to an increase of research into soft worm-like robots for pipe inspection. This review will analyse the recent progress in this area to assess current robotic capabilities and where work may be further needed to ensure they are applicable to real-world applications.
{"title":"A review of worm-like pipe inspection robots: research, trends and challenges","authors":"Gabrielle Blewitt, D. Cheneler, Jeremy Andrew, Stephen Monk","doi":"10.20517/ss.2023.49","DOIUrl":"https://doi.org/10.20517/ss.2023.49","url":null,"abstract":"In recent years, the development of worm-like robots has increased significantly. These robots use peristaltic motion comprised of radial expansion and axial elongation to move leglessly through their environments. Soft worm-like robots have the advantage of conforming to their environment, making them ideal for confined spaces such as pipelines which are essential to societal infrastructure. Pipeline contamination and corrosion can be detrimental and costly and thus regular checking is vital. Some pipes are difficult to access due to size, access restrictions and harmful waste contamination (such as in nuclear power plants). This has led to an increase of research into soft worm-like robots for pipe inspection. This review will analyse the recent progress in this area to assess current robotic capabilities and where work may be further needed to ensure they are applicable to real-world applications.","PeriodicalId":74837,"journal":{"name":"Soft science","volume":" 4","pages":""},"PeriodicalIF":0.0,"publicationDate":"2024-03-25","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"140382202","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Recent advancements in materials and mechanics have paved the way for transforming rigid circuits into flexible electronics. Their ability to laminate onto the skin has led to the development of skin-interfaced electronics, including mechano-acoustic sensors and haptic systems. However, the challenges of the coupled mechanics between the skin and skin-interfaced electronics call for further understanding of biomechanics, bioelectronics, and their interactions. This perspective article highlights the emerging trend of employing computer vision methods to optimize the next generation of skin-interfaced electronics by characterizing associated biomechanics and vice versa. The cyclic research process involves the development of soft electronics, the identification of coupled mechanics, and their quantification using computer vision methods. The article describes state-of-the-art computer vision techniques in the context of skin-interfaced electronics and their potential applications in other forms of soft electronics.
{"title":"Coupled mechanics in skin-interfaced electronics via computer vision methods","authors":"Jin-Tae Kim, L. Chamorro","doi":"10.20517/ss.2023.50","DOIUrl":"https://doi.org/10.20517/ss.2023.50","url":null,"abstract":"Recent advancements in materials and mechanics have paved the way for transforming rigid circuits into flexible electronics. Their ability to laminate onto the skin has led to the development of skin-interfaced electronics, including mechano-acoustic sensors and haptic systems. However, the challenges of the coupled mechanics between the skin and skin-interfaced electronics call for further understanding of biomechanics, bioelectronics, and their interactions. This perspective article highlights the emerging trend of employing computer vision methods to optimize the next generation of skin-interfaced electronics by characterizing associated biomechanics and vice versa. The cyclic research process involves the development of soft electronics, the identification of coupled mechanics, and their quantification using computer vision methods. The article describes state-of-the-art computer vision techniques in the context of skin-interfaced electronics and their potential applications in other forms of soft electronics.","PeriodicalId":74837,"journal":{"name":"Soft science","volume":"38 2","pages":""},"PeriodicalIF":0.0,"publicationDate":"2024-02-21","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"140443199","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Flexible and skin-wearable triboelectric nanogenerators (TENGs) have emerged as promising candidates for self-powered tactile and pressure sensors and mechanical energy harvesters due to their compatible design and ability to operate at low frequencies. Most research has focused on improving tribo-negative materials for flexible TENGs, given the limited options for tribo-positive materials. Achieving biocompatibility while maintaining the sensitivity and capability of energy harvesting is another critical issue for wearable sensors. Here, we report a TENG-based biocompatible and self-powered pressure sensor by simple fabrication of layer-by-layer deposition methods. The Laminated Flexible-TENG comprises polytetrafluoroethylene (PTFE) and polymethyl methacrylate (PMMA) films embedded within a flexible and biocompatible polydimethylsiloxane (PDMS) matrix. A nanostructured PDMS surface obtained by oxygen plasma facilitated the sputter deposition of a layered indium tin oxide copper electrode and a tribo-positive PMMA thin layer on top. The addition of the indium tin oxide layer to copper significantly improved the quality and performance of the indium tin oxide-copper electrode. Self-powered Laminated Flexible-TENGs demonstrated impressive pressure-sensing capabilities, featuring dual sensitivity of 7.287 V/kPa for low pressure and 0.663 V/kPa for higher pressure. Moreover, the PDMS-encapsulated TENG sensor effectively traced the physiological motions, such as wrist and finger bending, and efficiently harnessed the waste energy from everyday physical activities, such as walking and jogging. The maximum peak-to-peak voltages of 18.3 and 57.4 V were recorded during these motions. Encapsulated TENGs have broad potential in wearable technology, including healthcare, human-machine interfaces, and energizing microelectronics.
柔性可穿戴皮肤三电纳米发电机（TENGs）因其兼容的设计和低频工作能力，已成为自供电触觉和压力传感器以及机械能收集器的理想候选材料。由于三元正极材料的选择有限，大多数研究都集中在为柔性 TENG 改进三元负极材料上。对于可穿戴传感器来说，在保持灵敏度和能量收集能力的同时实现生物兼容性是另一个关键问题。在此，我们报告了一种基于 TENG 的生物相容性和自供电压力传感器，它采用逐层沉积的简单制造方法。层叠柔性 TENG 由聚四氟乙烯（PTFE）和聚甲基丙烯酸甲酯（PMMA）薄膜组成，嵌入柔性生物相容性聚二甲基硅氧烷（PDMS）基质中。通过氧等离子体获得的纳米结构 PDMS 表面有助于溅射沉积分层的氧化铟锡铜电极和顶部的三正极 PMMA 薄层。在铜上添加氧化铟锡层可显著提高氧化铟锡铜电极的质量和性能。自供电层叠柔性 TENG 展示了令人印象深刻的压力感应能力，具有双重灵敏度，低压灵敏度为 7.287 V/kPa，高压灵敏度为 0.663 V/kPa。此外，PDMS 封装的 TENG 传感器还能有效追踪手腕和手指弯曲等生理运动，并有效利用步行和慢跑等日常体力活动产生的废能。在这些运动中记录到的最大峰峰电压分别为 18.3 和 57.4 V。封装的 TENG 在可穿戴技术领域具有广泛的应用潜力，包括医疗保健、人机界面和增能微电子。
{"title":"A skin-wearable and self-powered laminated pressure sensor based on triboelectric nanogenerator for monitoring human motion","authors":"Agha Aamir Jan, Seungbeom Kim, Seok Kim","doi":"10.20517/ss.2023.54","DOIUrl":"https://doi.org/10.20517/ss.2023.54","url":null,"abstract":"Flexible and skin-wearable triboelectric nanogenerators (TENGs) have emerged as promising candidates for self-powered tactile and pressure sensors and mechanical energy harvesters due to their compatible design and ability to operate at low frequencies. Most research has focused on improving tribo-negative materials for flexible TENGs, given the limited options for tribo-positive materials. Achieving biocompatibility while maintaining the sensitivity and capability of energy harvesting is another critical issue for wearable sensors. Here, we report a TENG-based biocompatible and self-powered pressure sensor by simple fabrication of layer-by-layer deposition methods. The Laminated Flexible-TENG comprises polytetrafluoroethylene (PTFE) and polymethyl methacrylate (PMMA) films embedded within a flexible and biocompatible polydimethylsiloxane (PDMS) matrix. A nanostructured PDMS surface obtained by oxygen plasma facilitated the sputter deposition of a layered indium tin oxide copper electrode and a tribo-positive PMMA thin layer on top. The addition of the indium tin oxide layer to copper significantly improved the quality and performance of the indium tin oxide-copper electrode. Self-powered Laminated Flexible-TENGs demonstrated impressive pressure-sensing capabilities, featuring dual sensitivity of 7.287 V/kPa for low pressure and 0.663 V/kPa for higher pressure. Moreover, the PDMS-encapsulated TENG sensor effectively traced the physiological motions, such as wrist and finger bending, and efficiently harnessed the waste energy from everyday physical activities, such as walking and jogging. The maximum peak-to-peak voltages of 18.3 and 57.4 V were recorded during these motions. Encapsulated TENGs have broad potential in wearable technology, including healthcare, human-machine interfaces, and energizing microelectronics.","PeriodicalId":74837,"journal":{"name":"Soft science","volume":"25 4","pages":""},"PeriodicalIF":0.0,"publicationDate":"2024-01-26","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"139594115","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Ziyang Fan, Min Sang, Xinglong Gong, Ken Cham-Fai Leung, Shouhu Xuan
As a natural material, leather has been widely used in daily life due to its high biocompatibility, wearing comfort, and excellent mechanical strength. However, with the increasing demand for a better life among people, the single function of leather has difficulty in meeting the requirements, which limits its application prospects. It is particularly important to develop multifunctional leather composites with diverse characteristics. Therefore, leather can be modified and functionally designed through physical and chemical methods towards intelligent wearable devices. From this perspective, we review the research progress of intelligent leather-based wearable composites, mainly focusing on the preparation methods and application directions in recent years. Finally, we emphasize the challenges that leather composites will face in practical applications and propose future research directions.
{"title":"From natural leather to intelligent wearable nanocomposite: design and application","authors":"Ziyang Fan, Min Sang, Xinglong Gong, Ken Cham-Fai Leung, Shouhu Xuan","doi":"10.20517/ss.2023.47","DOIUrl":"https://doi.org/10.20517/ss.2023.47","url":null,"abstract":"As a natural material, leather has been widely used in daily life due to its high biocompatibility, wearing comfort, and excellent mechanical strength. However, with the increasing demand for a better life among people, the single function of leather has difficulty in meeting the requirements, which limits its application prospects. It is particularly important to develop multifunctional leather composites with diverse characteristics. Therefore, leather can be modified and functionally designed through physical and chemical methods towards intelligent wearable devices. From this perspective, we review the research progress of intelligent leather-based wearable composites, mainly focusing on the preparation methods and application directions in recent years. Finally, we emphasize the challenges that leather composites will face in practical applications and propose future research directions.","PeriodicalId":74837,"journal":{"name":"Soft science","volume":"92 7","pages":""},"PeriodicalIF":0.0,"publicationDate":"2024-01-18","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"139525991","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Cryosurgery and cryopreservation, as two important categories in cryobiology, have been impeded by the poor thermal conductivity of biological tissues or specimens. To improve this, diverse adjuvants, e.g., carbon-based materials, metallic nanoparticles, metallic oxide nanoparticles, etc ., have been exploited to improve the heat transfer in heat-targeted regions to increase the tumor elimination efficiency as well as the post-thaw viability of cryopreserved specimens. Nevertheless, these materials suffer poor thermal conductivities, controversial biosafety problems, and high expense. Gallium and its alloys, as a class of room-temperature liquid metals (LMs), have been widely studied in the past decade for their low melting point, minor toxicity, outstanding transformability, and conductivity. Integrated with these superior properties, they have been widely applied in multiple fields, such as thermal management, flexible electronics, and soft robotics. Recently, our laboratory has been devoted to fusing LMs with cryobiology and has made a series of progress. In this article, we will first briefly introduce preparation pathways to LM-based functional nanomaterials and composites. Then, how these materials realize improvement in biological heat transfer will be presented, followed by a discussion about the biosafety of these materials, which is an essential concern for the cryobiological field. Recent studies employing LMs in advanced cryosurgery and cryopreservation will also be highlighted. The present challenges and prospects of LMs towards further development in cryobiology will be put forward to point out the possible research direction.
{"title":"Liquid metals enabled advanced cryobiology: development and perspectives","authors":"Fan Yang, Chennan Lu, Wei Rao","doi":"10.20517/ss.2023.43","DOIUrl":"https://doi.org/10.20517/ss.2023.43","url":null,"abstract":"Cryosurgery and cryopreservation, as two important categories in cryobiology, have been impeded by the poor thermal conductivity of biological tissues or specimens. To improve this, diverse adjuvants, e.g., carbon-based materials, metallic nanoparticles, metallic oxide nanoparticles, etc ., have been exploited to improve the heat transfer in heat-targeted regions to increase the tumor elimination efficiency as well as the post-thaw viability of cryopreserved specimens. Nevertheless, these materials suffer poor thermal conductivities, controversial biosafety problems, and high expense. Gallium and its alloys, as a class of room-temperature liquid metals (LMs), have been widely studied in the past decade for their low melting point, minor toxicity, outstanding transformability, and conductivity. Integrated with these superior properties, they have been widely applied in multiple fields, such as thermal management, flexible electronics, and soft robotics. Recently, our laboratory has been devoted to fusing LMs with cryobiology and has made a series of progress. In this article, we will first briefly introduce preparation pathways to LM-based functional nanomaterials and composites. Then, how these materials realize improvement in biological heat transfer will be presented, followed by a discussion about the biosafety of these materials, which is an essential concern for the cryobiological field. Recent studies employing LMs in advanced cryosurgery and cryopreservation will also be highlighted. The present challenges and prospects of LMs towards further development in cryobiology will be put forward to point out the possible research direction.","PeriodicalId":74837,"journal":{"name":"Soft science","volume":"48 14","pages":""},"PeriodicalIF":0.0,"publicationDate":"2024-01-17","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"139526674","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Biao Ma, Ke Huang, Gangsheng Chen, Yingnan Tian, Nan Jiang, Chao Zhao, Hong Liu
Simultaneous monitoring of the body’s biochemical and biophysical signals via wearable devices can provide a comprehensive assessment of an individual’s health state. However, current multifunctional sensors for synchronous biochemical and biophysical sensing rely on discrete sensing units, posing a limitation in increased complexity in device assembly, signal processing, and system integration. In this study, we report a dual-mode and self-powered wearable sensor with ion and pressure-sensing capabilities by interfacing a hydrogel film with a solid ion-selective electrode. The hydrogel film can not only collect natural sweat from the skin but also offer a piezoionic response to pressure. We show that wrist pulse-induced pressure response can be incorporated into the noise of the response to sweat sodium ions, allowing for the simultaneous measurement of heart rate and sweat electrolytes. This work provides an example of simplifying the development of wearable multimode sensors through the rational design of classic electrochemical sensors.
{"title":"A dual-mode wearable sensor with coupled ion and pressure sensing","authors":"Biao Ma, Ke Huang, Gangsheng Chen, Yingnan Tian, Nan Jiang, Chao Zhao, Hong Liu","doi":"10.20517/ss.2023.41","DOIUrl":"https://doi.org/10.20517/ss.2023.41","url":null,"abstract":"Simultaneous monitoring of the body’s biochemical and biophysical signals via wearable devices can provide a comprehensive assessment of an individual’s health state. However, current multifunctional sensors for synchronous biochemical and biophysical sensing rely on discrete sensing units, posing a limitation in increased complexity in device assembly, signal processing, and system integration. In this study, we report a dual-mode and self-powered wearable sensor with ion and pressure-sensing capabilities by interfacing a hydrogel film with a solid ion-selective electrode. The hydrogel film can not only collect natural sweat from the skin but also offer a piezoionic response to pressure. We show that wrist pulse-induced pressure response can be incorporated into the noise of the response to sweat sodium ions, allowing for the simultaneous measurement of heart rate and sweat electrolytes. This work provides an example of simplifying the development of wearable multimode sensors through the rational design of classic electrochemical sensors.","PeriodicalId":74837,"journal":{"name":"Soft science","volume":"50 28","pages":""},"PeriodicalIF":0.0,"publicationDate":"2024-01-16","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"139527851","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Electrochemical glucose sensors that rely on two-dimensional (2D) oxides have attracted significant attention owing to the strong sensing activity of 2D oxides, but their practical application is hindered by the complexity and high cost of fabrication of electrodes and integrated devices. Herein, a convenient and effective fabrication route that includes printing a Ga-based liquid metal (LM) as a current collection electrode, followed by growing electrochemically active 2D oxides directly on the surface of Ga-based LMs under mild conditions, is developed for non-enzyme-based electrochemical sensors. Specifically, 2D annealed Cu-Oxide (ACO) is successfully grown on a printed Ga electrode through a galvanic replacement reaction, resulting in the formation of a mechanically and electrically well-matched interface between the active sensing materials and the current collection substrate. Benefitting from the high quantity of 2D ACO and good charge transfer at the interface, the as-prepared ACO electrode exhibits attractive glucose sensing performance, with a wide linear range (1 μM-10 mM) of effective detection, low detection limit down to 1 μM, and high sensitivity of 0.87 μA·mM-1·cm-2. Our study highlights the potential of using LMs in bio-sensing applications and provides a non-enzyme-based electrochemical biosensor platform for effective glucose detection in diets and clinical diagnostic settings.
{"title":"Printing surface cuprous oxides featured liquid metal for non-enzymatic electrochemical glucose sensor","authors":"Yiyao Luo, Gengcheng Liao, Zixuan Guo, Zongyu Huang, L. Ren, Xiang Qi","doi":"10.20517/ss.2023.40","DOIUrl":"https://doi.org/10.20517/ss.2023.40","url":null,"abstract":"Electrochemical glucose sensors that rely on two-dimensional (2D) oxides have attracted significant attention owing to the strong sensing activity of 2D oxides, but their practical application is hindered by the complexity and high cost of fabrication of electrodes and integrated devices. Herein, a convenient and effective fabrication route that includes printing a Ga-based liquid metal (LM) as a current collection electrode, followed by growing electrochemically active 2D oxides directly on the surface of Ga-based LMs under mild conditions, is developed for non-enzyme-based electrochemical sensors. Specifically, 2D annealed Cu-Oxide (ACO) is successfully grown on a printed Ga electrode through a galvanic replacement reaction, resulting in the formation of a mechanically and electrically well-matched interface between the active sensing materials and the current collection substrate. Benefitting from the high quantity of 2D ACO and good charge transfer at the interface, the as-prepared ACO electrode exhibits attractive glucose sensing performance, with a wide linear range (1 μM-10 mM) of effective detection, low detection limit down to 1 μM, and high sensitivity of 0.87 μA·mM-1·cm-2. Our study highlights the potential of using LMs in bio-sensing applications and provides a non-enzyme-based electrochemical biosensor platform for effective glucose detection in diets and clinical diagnostic settings.","PeriodicalId":74837,"journal":{"name":"Soft science","volume":"47 10","pages":""},"PeriodicalIF":0.0,"publicationDate":"2024-01-15","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"139437440","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Nerve stimulation technology utilizing electricity, magnetism, light, and ultrasound has found extensive applications in biotechnology and medical fields. Neurostimulation devices serve as the crucial interface between biological tissue and the external environment, posing a bottleneck in the advancement of neurostimulation technology. Ensuring safety and stability is essential for their future applications. Traditional rigid devices often elicit significant immune responses due to the mechanical mismatch between their materials and biological tissues. Consequently, there is a growing demand for flexible nerve stimulation devices that offer enhanced treatment efficacy while minimizing irritation to the human body. This review provides a comprehensive summary of the historical development and recent advancements in flexible devices utilizing four neurostimulation techniques: electrical stimulation, magnetic stimulation, optic stimulation, and ultrasonic stimulation. It highlights their potential for high biocompatibility, low power consumption, wireless operation, and superior stability. The aim is to offer valuable insights and guidance for the future development and application of flexible neurostimulation devices.
{"title":"A review: flexible devices for nerve stimulation","authors":"Ze-Qing Liu, Xiang-Yang Yu, Jing Huang, Xin-Yi Wu, Zi-Yu Wang, Ben-Peng Zhu","doi":"10.20517/ss.2023.36","DOIUrl":"https://doi.org/10.20517/ss.2023.36","url":null,"abstract":"Nerve stimulation technology utilizing electricity, magnetism, light, and ultrasound has found extensive applications in biotechnology and medical fields. Neurostimulation devices serve as the crucial interface between biological tissue and the external environment, posing a bottleneck in the advancement of neurostimulation technology. Ensuring safety and stability is essential for their future applications. Traditional rigid devices often elicit significant immune responses due to the mechanical mismatch between their materials and biological tissues. Consequently, there is a growing demand for flexible nerve stimulation devices that offer enhanced treatment efficacy while minimizing irritation to the human body. This review provides a comprehensive summary of the historical development and recent advancements in flexible devices utilizing four neurostimulation techniques: electrical stimulation, magnetic stimulation, optic stimulation, and ultrasonic stimulation. It highlights their potential for high biocompatibility, low power consumption, wireless operation, and superior stability. The aim is to offer valuable insights and guidance for the future development and application of flexible neurostimulation devices.","PeriodicalId":74837,"journal":{"name":"Soft science","volume":"2 10","pages":""},"PeriodicalIF":0.0,"publicationDate":"2024-01-10","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"139439081","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Inorganic p-type Sb2Te3 flexible thin films (f-TFs) with eco-friendly and high thermoelectric performance have attracted wide research interest and potential for commercial applications. This study employs a facile in-situ reaction method to prepare flexible Sb2Te3 thin films by rationally adjusting the synthesized temperature. The prepared thin films show good crystallinity, which enhances the electrical conductivity of ~1,440 S·cm-1 due to the weakened carrier scattering. Simultaneously, the optimized carrier concentration, through adjusting the synthesis temperature, causes the intermediate Seebeck coefficient. Consequently, a high-power factor (16.0 μW·cm-1·K-2 at 300 K) is achieved for Sb2Te3 f-TFs prepared at 623 K. Besides, the f-TFs also exhibit good flexibility due to the slight change in resistance after bending. This study specifies that the in-situ reaction method is an effective route to prepare Sb2Te3 f-TFs with high thermoelectric performance.
具有环保和高热电性能的无机 p 型 Sb2Te3 柔性薄膜（f-TFs）引起了广泛的研究兴趣，并具有商业应用的潜力。本研究采用简便的原位反应方法，通过合理调节合成温度制备柔性 Sb2Te3 薄膜。所制备的薄膜具有良好的结晶性，由于载流子散射减弱，导电性能提高到 ~1,440 S-cm-1。同时，通过调节合成温度，优化了载流子浓度，从而获得了中间塞贝克系数。因此，在 623 K 下制备的 Sb2Te3 f-TFs 实现了较高的功率因数（300 K 时为 16.0 μW-cm-1-K-2）。这项研究表明，原位反应法是制备具有高热电性能的 Sb2Te3 f-TFs 的有效途径。
{"title":"A facile in-situ reaction method for preparing flexible Sb2Te3 thermoelectric thin films","authors":"Dongwei Ao, Bo Wu, Jabar Bushra, Bing Sun, Dong Yang, Yiming Zhong, Zhuanghao Zheng","doi":"10.20517/ss.2023.34","DOIUrl":"https://doi.org/10.20517/ss.2023.34","url":null,"abstract":"Inorganic p-type Sb2Te3 flexible thin films (f-TFs) with eco-friendly and high thermoelectric performance have attracted wide research interest and potential for commercial applications. This study employs a facile in-situ reaction method to prepare flexible Sb2Te3 thin films by rationally adjusting the synthesized temperature. The prepared thin films show good crystallinity, which enhances the electrical conductivity of ~1,440 S·cm-1 due to the weakened carrier scattering. Simultaneously, the optimized carrier concentration, through adjusting the synthesis temperature, causes the intermediate Seebeck coefficient. Consequently, a high-power factor (16.0 μW·cm-1·K-2 at 300 K) is achieved for Sb2Te3 f-TFs prepared at 623 K. Besides, the f-TFs also exhibit good flexibility due to the slight change in resistance after bending. This study specifies that the in-situ reaction method is an effective route to prepare Sb2Te3 f-TFs with high thermoelectric performance.","PeriodicalId":74837,"journal":{"name":"Soft science","volume":"49 51","pages":""},"PeriodicalIF":0.0,"publicationDate":"2024-01-09","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"139442043","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
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