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Studies on DC transport and terahertz conductivity of granular molybdenum thin films for microwave radiation detector applications 微波辐射探测器用颗粒钼薄膜的直流输运和太赫兹电导率研究
Pub Date : 2020-07-26 DOI: 10.1063/5.0013939
Shilpam Sharma, A. Khandelwal, E. Amaladass, A. S, Ramjan Sk, J. J., A. Mani, M. K. Chattopadhyay
The morphological, transport and terahertz optical properties of DC magnetron sputtered granular molybdenum thin-films with nano-grains embedded in an amorphous matrix have been studied in the normal and superconducting states. The superconducting transition temperatures of these films are much higher than that of bulk molybdenum. The optical properties of these thin-films have been studied using terahertz time-domain spectroscopy. Their properties have been compared with the existing materials used for the development of radiation detectors. The resistivity of the films lies in >100 micro-Ohm-cm range which is ideal for making highly sensitive radiation detectors. The Hall measurements indicate the presence of holes as the dominant carriers with very small mean free path and mobility. In the normal state, the films are disordered bad metal but they have large superfluid density and stiffness in their superconducting state. The normal state and superconducting properties of the films are very promising for their use in cryogenic radiation detectors for microwave, terahertz, and far IR frequency ranges.
研究了在正常和超导状态下,在非晶基体中嵌入纳米颗粒的直流磁控溅射颗粒钼薄膜的形态、输运和太赫兹光学性能。这些薄膜的超导转变温度远高于本体钼。利用太赫兹时域光谱技术研究了这些薄膜的光学性质。将它们的性质与现有用于研制辐射探测器的材料进行了比较。薄膜的电阻率在>100微欧姆-厘米范围内,是制作高灵敏度辐射探测器的理想选择。霍尔测量表明,空穴作为主要载流子存在,平均自由程和迁移率非常小。在正常状态下,薄膜是无序的坏金属,但在超导状态下,薄膜具有较大的超流密度和刚度。薄膜的正常状态和超导特性在微波、太赫兹和远红外频率范围的低温辐射探测器中有很大的应用前景。
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引用次数: 1
In-plane electronic anisotropy resulted from ordered magnetic moment in iron-based superconductors 铁基超导体中有序磁矩引起的平面内电子各向异性
Pub Date : 2020-07-24 DOI: 10.1103/PHYSREVRESEARCH.2.033140
S.-F. Wu, W.-L. Zhang, V. Thorsmølle, G. Chen, G. Tan, P. Dai, Y. Shi, C. Jin, T. Shibauchi, S. Kasahara, Y. Matsuda, A. Sefat, H. Ding, P. Richard, G. Blumberg
We used polarization-resolved Raman scattering to study the magneto-elastic coupling in the parent compounds of several families of Fe-based superconductors (BaFe2As2, EuFe2As2, NaFeAs, LiFeAs, FeSe and LaFeAsO). We observe an emergent Ag-symmetry As phonon mode in the XY scattering geometry whose intensity is significantly enhanced below the magneto-structural transition only for compounds showing magnetic ordering. We conclude that the small lattice anisotropy is insufficient to induce the in-plane electronic polarizability anisotropy necessary for the observed phonon intensity enhancement, and interpret this enhancement below the Neel temperature in terms of the anisotropy of the magnetic moment and magneto-elastic coupling. We evidence a Fano line- shape in the XY scattering geometry resulting from a strong coupling between the Ag (As) phonon mode and the B2g symmetry-like electronic continuum. Strong electron-phonon coupling may be relevant to superconductivity.
我们利用偏振分辨拉曼散射研究了几种铁基超导体(BaFe2As2、EuFe2As2、nafea、LiFeAs、FeSe和LaFeAsO)母化合物的磁弹性耦合。我们观察到XY散射几何中出现ag -对称As声子模式,其强度仅在显示磁有序的化合物的磁结构跃迁下显着增强。我们得出结论,小的晶格各向异性不足以诱导所观察到的声子强度增强所必需的平面内电子极化各向异性,并根据磁矩和磁弹性耦合的各向异性来解释尼尔温度以下的这种增强。我们证明了由于Ag (As)声子模式和B2g类对称电子连续体之间的强耦合而导致的XY散射几何中的法诺线形状。强电子-声子耦合可能与超导性有关。
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引用次数: 0
Effect of external electromagnetic radiation on the anomalous metallic behavior in superconducting Ta thin films 外电磁辐射对超导钽薄膜异常金属行为的影响
Pub Date : 2020-07-23 DOI: 10.1103/PHYSREVB.102.184501
Junghyun Shin, Sun-gyu Park, Eunseong Kim
We investigated transport characteristics of superconducting Ta thin films with three configurations in rf radiation filters; no filter, only room-temperature filters, and low-temperature filters in addition to room-temperature filters. The transport properties near the transition temperature are strongly dependent on whether the room-temperature filter is installed or not. The entire transition is shifted to higher temperature with loading layers of the room-temperature filters. Once the zero-resistance state is achieved at B=0, no strong radiation effect is observed even with low-temperature filters installed. When magnetic field is turned on, the nonzero-resistance saturation at low temperatures is revealed without low-temperature filters, which has been considered to be magnetic-field-induced quantum metallic phase. However, the insertion of the additional low-temperature filter weakens the saturation of the resistance, the signature of the metallic behavior. This observation suggests that the previously reported anomalous metallic state in Ta films is mainly induced by the unfiltered radiation and, thus, the intrinsic metallic ground state should be limited to the narrow range of magnetic fields near the critical point, if exists.
研究了三种结构的超导Ta薄膜在射频辐射滤波器中的输运特性;无过滤器,只有室温过滤器,除室温过滤器外还有低温过滤器。在过渡温度附近的传输特性强烈依赖于是否安装了室温过滤器。整个过渡被转移到更高的温度与加载层的室温过滤器。一旦在B=0时达到零电阻状态,即使安装了低温过滤器,也不会观察到强烈的辐射效应。当磁场打开时,在没有低温滤波器的情况下显示出低温下的非零电阻饱和,这被认为是磁场诱导的量子金属相。然而,插入额外的低温滤波器削弱了电阻的饱和,这是金属行为的特征。这一观察结果表明,先前报道的Ta薄膜中的异常金属态主要是由未过滤的辐射引起的,因此,如果存在,则本征金属基态应限制在临界点附近的狭窄磁场范围内。
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引用次数: 1
Thermal fluctuations and vortex lattice structures in chiral p-wave superconductors: Robustness of double-quanta vortices 手性纵波超导体中的热波动和涡旋晶格结构:双量子涡旋的鲁棒性
Pub Date : 2020-07-17 DOI: 10.1103/PhysRevB.103.214517
Fredrik Nicolai Krohg, E. Babaev, J. Garaud, H. H. Haugen, A. Sudbø
We use large-scale Monte-Carlo simulations to study thermal fluctuations in chiral $p$-wave superconductors in an applied magnetic field in three dimensions. We consider the thermal stability of previously predicted unusual double-quanta flux-line lattice ground states in such superconductors. In previous works it was shown that, neglecting thermal fluctuations, a chiral $p$-wave superconductor forms a hexagonal lattice of doubly-quantized vortices, except extremely close vicinity of $H_{c2}$ where double-quanta vortices split apart. We find dissociation of double-quanta vortices driven by thermal fluctuations. However, our calculations also show that the previous predictions of hexagonal doubly-quantized vortices, where thermal fluctuations were ignored, are very robust in the considered model.
本文采用大规模蒙特卡罗模拟方法研究了手性p波超导体在外加磁场中的三维热波动。我们考虑了先前预测的这种超导体中不寻常的双量子通量线晶格基态的热稳定性。在以前的工作中,已经证明,忽略热波动,手性p波超导体形成双量子化涡的六角形晶格,除了在H_{c2}$的极近区域双量子化涡分裂。我们发现由热波动驱动的双量子涡解离。然而,我们的计算也表明,先前对六方双量子化漩涡的预测,在忽略热波动的情况下,在考虑的模型中是非常稳健的。
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引用次数: 0
Visualization by scanning SQUID microscopy of the intermediate state in the superconducting Dirac semimetal PdTe2 用扫描SQUID显微镜观察超导Dirac半金属PdTe2的中间态
Pub Date : 2020-07-16 DOI: 10.1103/PHYSREVB.103.104510
P. Garcia-Campos, Y. Huang, A. de Visser, K. Hasselbach
The Dirac semimetal PdTe${}_2$ becomes superconducting at a temperature $T_{c}=1.6$~K. Thermodynamic and muon spin rotation experiments support type-I superconductivity, which is unusual for a binary compound. A key property of a type-I superconductor is the intermediate state which presents a coexistence of superconducting and normal domains (flux structures) at magnetic fields lower than the thermodynamic critical field $H_{c}$. By means of scanning SQUID microscopy (SSM) we observe flux structures in the superconducting state of PdTe${}_2$. The flux structures are strongly history dependent with a transition from round shapes to laminar shapes as the magnetic field is more and more increased. The field amplitudes measured at the surface are indicative for the presence of Landau branching. The domain wall width in the intermediate state has been determined.
狄拉克半金属PdTe${}_2$在温度$T_{c}=1.6$~K时变为超导。热力学和介子自旋实验支持i型超导性,这对于二元化合物来说是不寻常的。i型超导体的一个关键性质是在低于热力学临界场$H_{c}$的磁场中超导畴和正常畴(通量结构)共存的中间态。利用扫描SQUID显微镜(SSM)观察了PdTe${}_2$超导状态下的磁通结构。磁通结构具有强烈的历史依赖性,随着磁场的增大,磁通结构由圆形向层流形状转变。在地表测得的磁场振幅表明存在朗道分支。确定了中间态的畴壁宽度。
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引用次数: 3
Underlying mechanism of charge transfer in Li-doped MgH16 at high pressure 高压下掺锂MgH16中电荷转移的潜在机制
Pub Date : 2020-07-08 DOI: 10.1103/physrevb.102.184509
Chong Wang, Seho Yi, Shuyuan Liu, Jun-Hyung Cho
A lithium-doped magnesium hydride Li$_2$MgH$_{16}$ was recently reported [Y. Sun $et$ $al$., Phys. Rev. Lett. {bf 123}, 097001 (2019)] to exhibit the highest ever predicted superconducting transition temperature $T_{rm c}$ under high pressure. Based on first-principles density-functional theory calculations, we reveal that the Li dopants locating in the pyroclore lattice sites give rise to the excess electrons distributed in interstitial regions. Such loosely bound anionic electrons are easily captured to stabilize a clathrate structure consisting of H cages. This addition of anionic electrons to H cages enhances the H-derived electronic density of states at the Fermi level, thereby leading to a high-$T_{rm c}$ superconductivity. We thus propose that the electride nature of Li dopants is an essential ingredient in the charge transfer between Li dopants and H atoms. Our findings offer a deeper understanding of the underlying mechanism of charge transfer in Li$_2$MgH$_{16}$ at high pressure.
最近报道了一种掺杂锂的氢化镁Li$_2$MgH$_{16}$ [Y]。Sun $et$ al$。、phy。启。[bf 123}, 097001(2019)]在高压下表现出有史以来预测的最高超导转变温度$T_{rm c}$。基于第一性原理密度泛函理论计算,我们揭示了锂掺杂剂位于焦释石晶格位置导致多余电子分布在间隙区域。这种松散结合的阴离子电子很容易被捕获,以稳定由H笼组成的笼形物结构。在H笼中加入阴离子电子增强了费米能级上H衍生态的电子密度,从而导致高T_{rm c}$超导性。因此,我们认为锂掺杂剂的电性质是锂掺杂剂和氢原子之间电荷转移的重要因素。我们的研究结果对Li$_2$MgH$_{16}$高压下电荷转移的潜在机制有了更深入的了解。
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引用次数: 2
Crystalline anisotropic topological superconductivity in planar Josephson junctions 平面约瑟夫森结的晶体各向异性拓扑超导性
Pub Date : 2020-07-07 DOI: 10.1103/PHYSREVRESEARCH.3.013198
Joseph D. Pakizer, B. Scharf, A. Matos-Abiague
We theoretically investigate the crystalline anisotropy of topological phase transitions in phase-controlled planar Josephson junctions (JJs) subject to spin-orbit coupling and in-plane magnetic fields. It is shown how topological superconductivity (TS) is affected by the interplay between the magnetic field and the orientation of the junction with respect to its crystallographic axes. This interplay can be used to electrically tune between BDI and D symmetry classes in a controlled fashion and thereby optimize the stability and localization of Majorana bound states in planar Josephson junctions. Our findings can be used as a guide for achieving the most favorable conditions when engineering TS in planar JJs and can be particularly relevant for setups containing non-collinear junctions which have been proposed for performing braiding operations on multiple Majorana pairs.
从理论上研究了受自旋轨道耦合和平面磁场影响的相控平面约瑟夫森结(JJs)拓扑相变的晶体各向异性。它显示了拓扑超导性(TS)如何受到磁场和结的取向相对于其晶体轴之间的相互作用的影响。这种相互作用可用于在BDI和D对称类之间以受控的方式进行电调谐,从而优化平面Josephson结中Majorana束缚态的稳定性和局域化。我们的发现可以作为在平面JJs中工程TS时实现最有利条件的指南,并且可以特别适用于包含非共线结的设置,这些连接已被提议用于对多个Majorana对进行编织操作。
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引用次数: 7
Unconventional superconductivity in a strongly correlated band-insulator without doping 非掺杂强相关带绝缘体中的非常规超导性
Pub Date : 2020-07-07 DOI: 10.21468/SCIPOSTPHYSCORE.4.2.009
Anwesha Chattopadhyay, H. R. Krishnamurthy, A. Garg
We present a novel route for attaining unconventional superconductivity (SC) in a strongly correlated system without doping. In a simple model of a correlated band insulator (BI) at half-filling we demonstrate, based on a generalization of the projected wavefunctions method, that SC emerges when e-e interactions and the bare band-gap are both much larger than the kinetic energy, provided the system has sufficient frustration against the magnetic order. As the interactions are tuned, SC appears sandwiched between the correlated BI followed by a paramagnetic metal on one side, and a ferrimagnetic metal, antiferromagnetic (AF) half-metal, and AF Mott insulator phases on the other side.
我们提出了一种在不掺杂的强相关体系中获得非常规超导性(SC)的新途径。在一个简单的半填充相关带绝缘体(BI)模型中,基于投影波函数方法的推广,我们证明了当e-e相互作用和裸带隙都远远大于动能时,只要系统对磁序有足够的挫折,SC就会出现。随着相互作用的调整,SC出现在相关的BI之间,其中一边是顺磁性金属,另一边是铁磁性金属,反铁磁性(AF)半金属和AF莫特绝缘体相。
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引用次数: 2
Designing nickelate superconductors with d8 configuration exploiting mixed-anion strategy 利用混合阴离子策略设计d8结构的镍酸盐超导体
Pub Date : 2020-07-02 DOI: 10.1103/PHYSREVRESEARCH.2.042032
Naoya Kitamine, M. Ochi, K. Kuroki
Inspired by a recently proposed superconducting mechanism for a new cuprate superconductor Ba$_2$CuO$_{3+delta}$, we theoretically design an unconventional nickelate superconductor with $d^8$ electron configuration. Our strategy is to enlarge the on-site energy difference between $3d_{x^2-y^2}$ and other $3d$ orbitals by adopting halogens or hydrogen as out-of-plane anions, so that the $3d$ bands other than $d_{x^-y^2}$ lie just below the Fermi level for the $d^8$ configuration, acting as incipient bands that enhance superconductivity. We also discuss a possible relevance of the present proposal to the recently discovered superconductor (Nd,Sr)NiO$_2$.
受最近提出的一种新型铜超导体Ba$_2$CuO$_{3+delta}$超导机制的启发,我们理论上设计了一种具有$d^8$电子组态的非常规镍酸盐超导体。我们的策略是通过采用卤素或氢作为面外阴离子来扩大$3d_{x^2-y^2}$与其他$3d$轨道之间的场能差,使$d_{x^-y^2}$以外的$3d$能带刚好位于$d^8$结构的费米能级以下,作为增强超导性的初始能带。我们还讨论了本提议与最近发现的超导体(Nd,Sr)NiO$_2$的可能相关性。
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引用次数: 9
Amplitudes of minima in dynamic conductance spectra of the SNS Andreev contact SNS Andreev接触动态电导谱的极小值幅值
Pub Date : 2020-07-01 DOI: 10.1063/5.0010883
Z. Popović, S. Kuzmichev, T. Kuzmicheva
Despite several theoretical approaches describing multiple Andreev reflections (MAR) effect in superconductor-normal metal-superconductor (SNS) junction are elaborated, the problem of comprehensive and adequate description of MAR is highly actual. In particular, a broadening parameter $Gamma$ is still unaccounted at all, whereas a ballistic condition (the mean free path for inelastic scattering $l$ to the barrier width $d$ ratio) is considered only in the framework of Kummel, Gunsenheimer, and Nikolsky (KGN), as well as Gunsenheimer-Zaikin approaches, for an isotropic case and fully-transparent constriction. Nonetheless, an influence of $l/d$ ratio to the dynamic conductance spectrum ($dI/dV$) features remains disregarded, thus being one of the aims of the current work. Our numerical calculations in the framework of an extended KGN approach develop the $l/d$ variation to determine both the number of the Andreev features and their amplitudes in the $dI/dV$ spectrum. We show, in the spectrum of a diffusive SNS junction ($l/d rightarrow 1$) a suppression of the Andreev excess current, dramatic change in the current voltage $I(V)$-curve slope at low bias, with only the main harmonic at $eV=2Delta$ bias voltage remains well-distinguished in the $dI/dV$-spectrum. Additionally, we attempt to make a first-ever comparison between experimental data for the high-transparency SNS junctions (more than $ 85~%$) and theoretical predictions. As a result, we calculate the temperature dependences of amplitudes and areas of Andreev features within the extended KGN approach, which qualitatively agrees with our experimental data obtained using a "break-junction" technique.
尽管有几种理论方法描述了超导体-正常金属-超导体(SNS)结中的多重安德烈夫反射(MAR)效应,但如何全面、充分地描述多重安德烈夫反射是一个非常现实的问题。特别是,展宽参数$Gamma$仍然完全没有考虑,而弹道条件(非弹性散射的平均自由路径$l$与势垒宽度$d$之比)仅在Kummel, Gunsenheimer和Nikolsky (KGN)以及Gunsenheimer- zaikin方法的框架中考虑,用于各向同性情况和全透明缩窄。尽管如此,$l/d$比率对动态电导谱($dI/dV$)特征的影响仍然被忽视,因此是当前工作的目标之一。我们在扩展的KGN方法框架内的数值计算开发了$l/d$变化,以确定$dI/dV$谱中的Andreev特征的数量及其振幅。我们发现,在扩散性SNS结($l/d rightarrow 1$)的频谱中,Andreev过量电流受到抑制,电流电压$I(V)$ -曲线斜率在低偏置下发生了巨大变化,在$dI/dV$ -频谱中,只有$eV=2Delta$偏置电压处的主谐波仍然很好地区分。此外,我们试图对高透明度SNS连接的实验数据(超过$ 85~%$)和理论预测进行首次比较。因此,我们在扩展的KGN方法中计算了Andreev特征的振幅和面积的温度依赖性,这与我们使用“断结”技术获得的实验数据在定性上一致。
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引用次数: 11
期刊
arXiv: Superconductivity
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