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Super Depth‐of‐Field Snapshot Light‐Field Microscopy 超景深快照光场显微镜
IF 11 1区 物理与天体物理 Q1 OPTICS Pub Date : 2026-01-30 DOI: 10.1002/lpor.202502750
Zhi‐Yong Hu, Chang Qiao, Jian‐Yu Dou, Ming‐Ze Zhao, Zhen‐Nan Tian, Yue‐Ying Zhang, Yan‐Hao Yu, Chong Pan, Yong‐Lai Zhang, Qi‐Dai Chen, Din Ping Tsai, Hong‐Bo Sun
Snapshot light‐field microscopes (SLFMs) enable high‐speed 3D observation (4D imaging) of dynamic micro‐targets. However, their performance is fundamentally restricted by the inherent planar structure of microlens arrays (MLAs), which leads to tradeoffs among resolution, depth of field (DOF), and depth perception, making large DOF light‐field detection extremely challenging. Here, we propose a paradigm in curved MLA with a logarithmic profile, featuring extreme depth of focus (>346λ), enhanced parallax (273%), and near‐diffraction‐limited resolution, outperforming conventional planar counterparts. Integrated into a commercial microscope and combined with neural network‐based reconstruction, this architecture yields a super depth‐of‐field snapshot light‐field microscope (SDOF‐SLFM), achieving over 15 times improvement in DOF (>3 mm) and enabling in situ stereo imaging of micro‐pyramids and 4D tracking of micro‐particles in flow fields. This study offers a practical pathway for upgrading SLFMs without complex system assembly or sample processing, facilitating the adaptation of conventional commercial microscopes to dynamic 4D imaging applications such as biological laboratories and microfluidic flow monitoring.
快照光场显微镜(SLFMs)能够对动态微目标进行高速3D观察(4D成像)。然而,它们的性能从根本上受到微透镜阵列(mla)固有的平面结构的限制,这导致了分辨率,景深(DOF)和深度感知之间的权衡,使得大DOF光场检测极具挑战性。在这里,我们提出了一个具有对数轮廓的弯曲MLA范例,具有极端聚焦深度(>346λ),增强视差(273%)和近衍射极限分辨率,优于传统的平面对偶。集成到商用显微镜中,并结合基于神经网络的重建,该架构产生了超景深快照光场显微镜(SDOF - SLFM),实现了超过15倍的DOF (> 3mm)改进,并实现了微金字塔的原位立体成像和流场中微颗粒的4D跟踪。该研究为SLFMs的升级提供了一种实用的途径,无需复杂的系统组装或样品处理,促进了传统商用显微镜适应生物实验室和微流体流动监测等动态四维成像应用。
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引用次数: 0
Optical Topological Differentiation Cryptography 光学拓扑微分密码学
IF 11 1区 物理与天体物理 Q1 OPTICS Pub Date : 2026-01-30 DOI: 10.1002/lpor.202502957
Yanliang He, Yuanfeng Zhu, Haimei Luo, Wen Yuan, Guiqiang Liu, Zhengqi Liu, Xianping Wang, Junxiao Zhou
Optical encryption provides an effective way to secure confidential information, featuring low energy consumption, parallel operation, high speed, and the ability to process multidimensional data. However, a unified framework that can encrypt and decrypt optical information across the fundamental spatial physical dimensions (amplitude, phase, and polarization) is still lacking. Here, we present an optical cryptography approach based on topological differentiation via Pancharatnam–Berry (PB) phase liquid crystal optical elements. By leveraging the spin‐dependent phase modulation of the PB phase, binary‐encoded optical images in any physical dimension are encrypted into an identical ciphertext, effectively hiding the information by converting it into edge‐based representations. Decryption is accomplished through a conjugate topological differentiation operation, which precisely reverses the process by redistributing energy from the edge back to the center, thereby restoring the original image. As a proof of concept, we successfully demonstrated the encryption and decryption of the plaintext information “LIGHT” across the spatial dimensions of amplitude, phase, and polarization. This work introduces a new paradigm in optical information security by innovatively applying optical differentiation to physical‐layer encryption and decryption, providing a robust and unified approach for the protection of multidimensional optical data.
光加密具有低能耗、并行运行、速度快、能够处理多维数据等特点,是保护机密信息安全的有效手段。然而,目前还缺乏一个统一的框架,可以跨基本空间物理维度(振幅、相位和偏振)对光学信息进行加密和解密。在这里,我们提出了一种基于拓扑分化的基于Pancharatnam-Berry (PB)相位液晶光学元件的光学密码方法。通过利用PB相位的自旋相关相位调制,任何物理维度的二进制编码光学图像都被加密成相同的密文,通过将其转换为基于边缘的表示有效地隐藏信息。解密是通过共轭拓扑微分操作完成的,该操作通过将能量从边缘重新分配到中心来精确地逆转这一过程,从而恢复原始图像。作为概念验证,我们成功地演示了跨幅度、相位和极化空间维度的明文信息“LIGHT”的加密和解密。这项工作通过创新地将光差分应用于物理层加密和解密,引入了光信息安全的新范式,为多维光学数据的保护提供了一种强大而统一的方法。
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引用次数: 0
Dynamic and Underwater X‐ray Imaging Enabled by Instant Ion Exchange of Copper Halide Scintillators 通过卤化铜闪烁体的即时离子交换实现动态和水下X射线成像
IF 11 1区 物理与天体物理 Q1 OPTICS Pub Date : 2026-01-30 DOI: 10.1002/lpor.202503085
Xinjiang Zhan, Jie Cao, Le Dong, Ye Xun, Ya Chen, Yulong Wang, Bing Chen, Shujuan Liu, Xiuwen Xu, Qiang Zhao
Organic–inorganic hybrid copper halides, with exceptional optoelectronic properties encoded in their highly tunable crystal structure, are emerging as promising candidates for next‐generation scintillators. However, achieving both high light yield and fast luminescence decay in copper halides remains a significant challenge, limiting their application in real‐time X‐ray imaging. Here, a simple yet effective ion exchange approach is developed to enable rapid conversion of (MeEn) 2 Cu 4 Br 6 (MeEn = 3‐methylbut‐2‐enyl(triphenyl)phosphanium) to (MeEn) 2 Cu 4 I 6 , resulting in a near‐unity photoluminescence quantum yield (PLQY), a 1.7‐fold increase in light yield (39700 photons MeV −1 ), and a 15‐fold reduction in luminescence decay time (2.4 µs). Mechanistic investigations reveal that the enhanced scintillation properties arise from reduced lattice distortion, appropriately weakened electron‐phonon coupling, and strong spin–orbit coupling induced by the heavy iodine atom. Beyond (MeEn) 2 Cu 4 X 6 , this approach is applicable to a variety of copper halides, leading to consistent improvements in photophysical performance. Finally, by embedding (MeEn) 2 Cu 4 I 6 with a polymer matrix, the resulting scintillation film is further entailed with desired flexibility and water resistance, demonstrating its capability in static, dynamic, curved, and underwater X‐ray imaging.
有机-无机杂化卤化铜在其高度可调的晶体结构中具有特殊的光电特性,正在成为下一代闪烁体的有希望的候选者。然而,在卤化铜中实现高产光率和快速发光衰减仍然是一个重大挑战,限制了它们在实时X射线成像中的应用。在这里,我们开发了一种简单而有效的离子交换方法,使(MeEn) 2 Cu 4 Br 6 (MeEn = 3‐methylbut‐2‐enyl(triphenyl) phospium)快速转化为(MeEn) 2 Cu 4 I 6,从而产生接近统一的光致发光量子产率(PLQY),光产率增加1.7倍(39700光子MeV−1),发光衰减时间减少15倍(2.4µs)。机制研究表明,增强的闪烁特性是由于减少了晶格畸变,适当减弱了电子-声子耦合,以及由重碘原子引起的强自旋-轨道耦合。除了(MeEn) 2 Cu 4 X 6之外,这种方法适用于各种卤化铜,从而导致光物理性能的持续改进。最后,通过在聚合物基体中嵌入(MeEn) 2 Cu 4 i6,所得到的闪烁膜进一步具有所需的柔韧性和耐水性,展示了其在静态、动态、弯曲和水下X射线成像方面的能力。
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引用次数: 0
Chiral Quantum Optics With Topological Photonic Crystal Waveguide of Triangular Lattice 具有三角形晶格拓扑光子晶体波导的手性量子光学
IF 11 1区 物理与天体物理 Q1 OPTICS Pub Date : 2026-01-30 DOI: 10.1002/lpor.202501893
Hancong Li, Sai Yan, Zhikai Ma, Rui Zhu, Hanqing Liu, Xiqing Chen, Yu Yuan, Longlong Yang, Haiqiao Ni, Zhichuan Niu, Qihuang Gong, Xiulai Xu
We present a versatile dielectric platform for studying chiral light–matter interaction and cavity quantum electrodynamics, based on high bend transmittance waveguide (HBT WG) modes of triangular‐lattice photonic crystals (Tri‐PhCs). The demonstration of chiral coupling is realized by employing two Tri‐PhC zigzag interface waveguides which offer a simplified geometry in the first place. Compared to previous honeycomb‐lattice systems, Tri‐PhC zigzag waveguides provide at least twice the effective chiral area for quantum dot (QD) interaction and support accessible slow‐light modes that are crucial for light–matter interaction. Integrating self‐assembled QDs, we experimentally demonstrate chiral photon routing in Z‐shaped Tri‐PhC HBT WGs, confirming robust directional photon transport. Additionally, we incorporate a whispering‐gallery‐mode cavity‐waveguide structure to achieve Purcell‐enhanced on‐chip single‐photon emission, with a Purcell factor of 4 and spin‐dependent directional contrast of 82%. Our results show the potential of Tri‐PhC‐based topological waveguides as a promising, scalable platform for low‐loss, high‐chirality quantum photonic devices.
基于三角晶格光子晶体(Tri - PhCs)的高弯曲透射波导(HBT WG)模式,我们提出了一个用于研究手性光-物质相互作用和腔量子电动力学的通用介电平台。手性耦合的演示是通过使用两个Tri - PhC之字形界面波导来实现的,这首先提供了一个简化的几何结构。与之前的蜂窝晶格系统相比,Tri - PhC之字形波导为量子点(QD)相互作用提供了至少两倍的有效手性面积,并支持对光-物质相互作用至关重要的可访问的慢光模式。整合自组装量子点,我们实验证明了Z形Tri - PhC HBT WGs中的手性光子路由,证实了强大的定向光子传输。此外,我们结合了一个窃窃私语走廊模式腔波导结构,以实现Purcell增强的片上单光子发射,Purcell因子为4,自旋相关的方向对比度为82%。我们的研究结果表明,基于三PhC的拓扑波导作为一个有前途的、可扩展的低损耗、高手性量子光子器件平台的潜力。
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引用次数: 0
Inverse Design of Mirror‐Symmetric Disordered Systems for Broadband Perfect Transmission 宽带完美传输的镜像对称无序系统的反设计
IF 11 1区 物理与天体物理 Q1 OPTICS Pub Date : 2026-01-30 DOI: 10.1002/lpor.202501055
Zhazira Zhumabay, Clément Ferise, Vincent Pagneux, Stefan Rotter, Matthieu Davy
We present a framework for achieving broadband perfect wave transmission in complex systems by optimizing symmetric disordered media via inverse design. We show that leveraging symmetry of complex media reduces the optimization's complexity enabling the incorporation of additional constraints in the parameter space. Starting from a single perfectly transmitting state with predefined input and output wavefronts at a specific frequency, we progressively broaden the bandwidth — from a reflectionless exceptional point with a flattened lineshape to narrowband filters and ultimately to broadband quasi‐perfect transmission exhibiting a rainbow effect. Numerical simulations based on the coupled dipole approximation are validated experimentally in a multichannel microwave waveguide with dielectric and metallic scatterers. Finally, we demonstrate broadband enhanced wave transmission through barriers highlighting the potential for advanced wave control applications.
我们提出了一种通过逆设计优化对称无序介质实现复杂系统宽带完美波传输的框架。我们表明,利用复杂介质的对称性可以在参数空间中加入额外的约束,从而降低优化的复杂性。从具有特定频率的预定义输入和输出波前的单一完美传输状态开始,我们逐步拓宽带宽-从具有平坦线形的无反射异常点到窄带滤波器,最终到具有彩虹效应的宽带准完美传输。在具有介质和金属散射体的多通道微波波导中,实验验证了基于耦合偶极子近似的数值模拟。最后,我们展示了通过屏障的宽带增强波传输,突出了先进波控制应用的潜力。
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引用次数: 0
Monolithically Integrated Silicon Photonic Local Oscillator‐Free Homodyne Receiver 单片集成硅光子本振-自由纯差接收机
IF 11 1区 物理与天体物理 Q1 OPTICS Pub Date : 2026-01-30 DOI: 10.1002/lpor.202502793
Jingchi Li, Hua Zhong, Yixiao Zhu, Yu He, Zhen Wang, Xiong Ni, Xingchen Ji, Qian Hu, Haoshuo Chen, Nicolas K. Fontaine, Roland Ryf, William Shieh, Yikai Su
The exponential growth of global data traffic driven by artificial intelligence and cloud computing necessitates cost‐efficient, ultrahigh‐capacity optical interconnects. Integrated photonic interconnect offers a promising solution but faces critical bottlenecks: integrated coherent receivers require local oscillator (LO) lasers, resulting in material incompatibility and cost challenges for monolithic integration, while integrated self‐coherent schemes fundamentally suffer from nonlinear distortions induced by the nonlinear beating process between signal inputs during optical‐to‐electrical mapping, which limits both capacity and spectral efficiency. Here, we present an integrated LO‐free homodyne detection scheme with superior linearity enabled by a micro‐ring filter. The Si 3 N 4 micro‐ring resonator effectively filters out the optical carrier for homodyne detection, saving the LO in coherent receivers and eliminating the second‐order nonlinear distortions commonly encountered in self‐coherent schemes. Our fabricated monolithically integrated silicon photonic receiver enables single‐polarization 600‐Gb/s 16‐ary quadrature amplitude modulated orthogonal frequency division multiplexing signal transmission over an 80‐km fiber, achieving a net 480‐Gb/s per polarization. This represents an 86% improvement over previous integrated self‐coherent detection records and matches that of state‐of‐the‐art integrated coherent systems. Multichannel validation across the C band further confirms the dense wavelength‐division multiplexing compatibility. This work provides an Optical communication, dense wavelength division multiplexing, direct detection, integrated photonic interconnects, silicon photonicsscalable and cost‐effective solution essential for future 1.6 Tb/s per lane optical interconnects.
在人工智能和云计算的驱动下,全球数据流量呈指数级增长,这就需要具有成本效益、超高容量的光互连。集成光子互连提供了一个有前途的解决方案,但面临着关键的瓶颈:集成相干接收器需要本振(LO)激光器,这导致材料不兼容和单片集成的成本挑战,而集成自相干方案从根本上遭受由光-电映射过程中信号输入之间的非线性加热过程引起的非线性扭曲,这限制了容量和频谱效率。在这里,我们提出了一个集成的无LO差检测方案,该方案通过微环滤波器实现了良好的线性度。si3n4微环谐振器有效滤除光载流子用于零差检测,节省了相干接收器中的LO,消除了自相干方案中常见的二阶非线性失真。我们制造的单片集成硅光子接收器能够在80公里光纤上实现600 Gb/s的单极化16正交调幅正交频分复用信号传输,达到480 Gb/s的极化速率。这比以前的集成自相干检测记录提高了86%,并与最先进的集成相干系统相匹配。跨C波段的多通道验证进一步证实了密集波分复用的兼容性。这项工作为未来1.6 Tb/s每通道光互连提供了光通信、密集波分复用、直接检测、集成光子互连、硅光子可扩展和成本效益的解决方案。
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引用次数: 0
Information Metasurface‐Enabled Dynamically Reconfigurable Radar Electromagnetic Phantoms 信息metassurface - Enabled动态可重构雷达电磁模型
IF 11 1区 物理与天体物理 Q1 OPTICS Pub Date : 2026-01-30 DOI: 10.1002/lpor.202502619
Shijian Yu, Jinxing Guo, Dongfang Guan, Zhen Liu, Yongxiang Liu
Radar electromagnetic phantoms aim to deceive radar systems by introducing virtual targets—entities that do not physically exist—into radar imagery, thereby inducing erroneous recognition. Information metasurfaces, functioning as digitally reconfigurable electromagnetic reflectors, offer unprecedented capabilities in multidimensional radar target signatures control. Nevertheless, existing space‐coding‐based techniques are constrained by static phantom image templates, limiting their ability to generate dynamically reconfigurable radar phantoms. Temporal modulation strategies are susceptible to synchronization errors under non‐cooperative scenarios. To address these challenges, this paper proposes a novel method for generating image‐level, dynamically stable, and reconfigurable radar electromagnetic phantoms via information metasurfaces. The proposed approach leverages the geometric theory of diffraction (GTD) to extract characteristic parameters oftargets. These parameters subsequently guide the design of asynchronous frequency‐modulated sequences implemented on the metasurface. A 1‐bit information metasurface prototype was developed and experimentally validated. The results demonstrate its capability to generate a variety of reconfigurable radar phantoms in high‐resolution range profiles (HRRPs) in real time. Furthermore, both human radar image interpretation and artificial neural network (ANN)‐based classification exhibit high confidence in identifying the modulated imagery as authentic targets, thereby confirming the effectiveness of deception. The developed metasurface and its associated modulation strategy hold significant promise for critical target protection in electronic warfare scenarios.
雷达电磁幽灵旨在通过将虚拟目标(物理上不存在的实体)引入雷达图像来欺骗雷达系统,从而诱导错误识别。信息元表面作为数字可重构电磁反射器,在多维雷达目标特征控制方面提供了前所未有的能力。然而,现有的基于空间编码的技术受到静态幻像模板的限制,限制了它们生成动态可重构雷达幻像的能力。在非合作情况下,时间调制策略容易受到同步误差的影响。为了解决这些挑战,本文提出了一种通过信息元表面生成图像级、动态稳定和可重构的雷达电磁幻影的新方法。该方法利用几何衍射理论提取目标的特征参数。这些参数随后指导了在元表面上实现的异步调频序列的设计。开发了一个1比特的信息超表面原型并进行了实验验证。结果表明,它能够在高分辨率距离剖面(hrrp)中实时生成各种可重构雷达幻影。此外,人类雷达图像解释和基于人工神经网络(ANN)的分类在识别调制图像为真实目标方面表现出很高的置信度,从而证实了欺骗的有效性。所开发的超表面及其相关调制策略对电子战场景中的关键目标保护具有重要的前景。
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引用次数: 0
One-Step In Situ Synthesis of Carbon Dot-Based Nanospheres With Underwater Color-Tunable, Dual-Mode Long-Afterglow Emission 具有水下可调色双模长余辉发射的碳点基纳米球的一步原位合成
IF 11 1区 物理与天体物理 Q1 OPTICS Pub Date : 2026-01-29 DOI: 10.1002/lpor.202502697
Tengyang Cao, Lei Chen, Helang Li, Zinan Jiang, Jiawen Li, Jijun Huang, Caiqi Wang
Carbon dot (CD)-based afterglow materials have recently proliferated in various areas, but color-tunable, carbon dot-based underwater afterglow nanomaterials remain largely unexplored. Moreover, the existing synthesis methods are generally complex, and there has been a notable lack of efficient, one-step preparation techniques. We present a simple one-step hydrothermal method to synthesize CD-based nanomaterials that exhibit stable dual-mode underwater emission comprising room-temperature phosphorescence (RTP) and thermally activated delayed fluorescence (TADF). Using 3-aminopropyltriethoxysilane, a densely cross-linked SiO2 matrix forms, embedding in situ generated CDs. This confined structure stabilizes triplet excitons, enabling an ultra-long underwater afterglow lifetime of 1218 ms and a quantum yield of 46.7%. By doping with halide ions, the afterglow wavelength was tuned from 402 to 560 nm, achieving multicolor emission. The nanocomposites maintain stable afterglow performance in harsh conditions, including strong acids, alkalis, oxidants, and polar solvents. Given its exceptional stability and multicolor afterglow, the material was used to construct a sophisticated triple anti-counterfeiting system, demonstrating great potential for advanced information encryption.
碳点(CD)基余辉材料最近在各个领域得到了广泛的应用,但颜色可调的碳点基水下余辉纳米材料在很大程度上仍未被开发。此外,现有的合成方法一般都很复杂,并且明显缺乏高效的一步制备技术。我们提出了一种简单的一步水热法来合成具有室温磷光(RTP)和热激活延迟荧光(TADF)的稳定双模水下发射的cd基纳米材料。使用3-氨基丙基三乙氧基硅烷,形成密集交联的SiO2基质,包埋在原位生成的CDs中。这种受限结构稳定了三重态激子,使水下余辉寿命达到1218 ms,量子产率达到46.7%。通过掺杂卤化物离子,使余辉波长从402 nm调整到560 nm,实现了多色发射。纳米复合材料在强酸、强碱、氧化剂和极性溶剂等恶劣条件下保持稳定的余辉性能。由于其优异的稳定性和多色余辉,该材料被用于构建复杂的三重防伪系统,显示出先进信息加密的巨大潜力。
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引用次数: 0
High‐Brightness and Fast‐Response in Cerium‐Doped Halide Double Perovskite Scintillators Based on Defect‐Suppressed Strategies for High‐Speed X‐Ray Imaging 高速X射线成像中基于缺陷抑制策略的掺铈卤化物双钙钛矿闪烁体的高亮度和快速响应
IF 11 1区 物理与天体物理 Q1 OPTICS Pub Date : 2026-01-27 DOI: 10.1002/lpor.202503264
Peiyang Li, Wei Xiong, Laishun Qin, Ji‐Guang Li, Qi Zhu
High‐performance scintillators play a core role in the development of advanced medical imaging technologies, particularly in complex detection scenarios requiring both high sensitivity and high temporal resolution. However, developing a scintillator that simultaneously combines outstanding radioluminescence (RL) efficiency with fast decay characteristics remains a formidable challenge. Here, Ce 3+ ‐doped Cs 2 NaGdCl 6 (CNGC) double perovskite is designed to regulate the luminescence efficiency feature of the scintillator by introducing Br to suppress the formation of Cl vacancy defects. Notably, the doping of Br significantly reduces the defect density in CNGC:Ce 3+ , decreases non‐radiative recombination, and achieves a high photoluminescence quantum yield (PLQY) of 90.2%. Based on its outstanding scintillation performance, including a high light yield (LY) of 47637 photons MeV −1 , a short RL decay time of 153 ns, and a low detection limit of 74.95 nGy s −1 , the CNGC:15%Ce 3+ ,3%Br scintillator film can capture clear high‐speed X‐ray imaging of the flowing contrast agents in simulated angiography. This work develops a novel scintillator material that not only holds immense potential as a candidate material for diverse ultrafast radiation detection applications, but also establishes a foundation for designing scintillators that simultaneously exhibit high LY and rapid RL decay characteristics.
高性能闪烁体在先进医学成像技术的发展中发挥着核心作用,特别是在需要高灵敏度和高时间分辨率的复杂检测场景中。然而,开发一种同时结合出色的辐射发光(RL)效率和快速衰减特性的闪烁体仍然是一个艰巨的挑战。本文设计了ce3 +掺杂c2nagdcl6 (CNGC)双钙钛矿,通过引入Br−抑制Cl空位缺陷的形成来调节闪烁体的发光效率特性。值得注意的是,Br−的掺杂显著降低了CNGC: ce3 +的缺陷密度,减少了非辐射复合,实现了90.2%的高光致发光量子产率(PLQY)。基于其出色的闪烁性能,包括47637光子MeV−1的高光产率(LY), 153 ns的短RL衰减时间和74.95 nGy s−1的低检测限,CNGC:15%Ce 3+,3%Br−闪烁体薄膜可以在模拟血管造影中捕获流动造影剂的高速X射线成像。这项工作开发了一种新型闪烁体材料,它不仅作为各种超快辐射探测应用的候选材料具有巨大的潜力,而且为设计同时具有高LY和快速RL衰减特性的闪烁体奠定了基础。
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引用次数: 0
Engineering Localized Surface Plasmon Resonance of Nanoparticles in Transparent Materials for Advanced Optical Applications 工程定域表面等离子体共振纳米粒子在透明材料中的先进光学应用
IF 11 1区 物理与天体物理 Q1 OPTICS Pub Date : 2026-01-27 DOI: 10.1002/lpor.202502571
Chi Pang, Rang Li, Xia Wang, Weijin Kong, Feng Chen
Localized surface plasmon resonance (LSPR) of nanoparticles embedded in transparent solid‐state materials provides a robust platform for integrated photonic and optoelectronic devices requiring precise spectral positioning, strong field localization, and long‐term stability. This review links fundamentals to engineering strategies and applications for plasmonic nanostructures in transparent hosts. We summarize the formation and evolution of metallic species in solids and the resulting optical properties across size regimes, covering both linear and nonlinear responses. We identify three energy‐transduction mechanisms that connect nanostructure properties to device functionality: (i) near‐field enhancement, (ii) hot‐carrier processes, and (iii) photothermal effects. Building on these foundations, we emphasize post‐fabrication morphology reconfiguration of pre‐embedded nanostructures as a primary route to programmable LSPR control, and organize representative approaches by actuation mode (thermal, electric‐field–driven, and chemistry‐based) and stimulus modality (photons, electrons, ions, or external fields). We then review applications in nonlinear and integrated photonics and optoelectronic energy conversion, highlighting how embedded plasmonic resonances improve device performance. Finally, we discuss practical challenges and emerging opportunities toward scalable, spatially programmable plasmonics, including control of buried interfaces and reproducible processing enabled by coordinated beam/laser/thermal/chemical routes.
嵌入透明固态材料中的纳米粒子的局部表面等离子体共振(LSPR)为集成光子和光电子器件提供了一个强大的平台,这些器件需要精确的光谱定位、强场定位和长期稳定性。本文综述了透明宿主中等离子体纳米结构的基本原理、工程策略和应用。我们总结了固体中金属物种的形成和演变以及由此产生的光学性质,涵盖了线性和非线性响应。我们确定了将纳米结构特性与器件功能联系起来的三种能量转导机制:(i)近场增强,(ii)热载流子过程和(iii)光热效应。在此基础上,我们强调预嵌入纳米结构的制造后形态重构是可编程LSPR控制的主要途径,并通过驱动模式(热、电场驱动和化学驱动)和刺激模式(光子、电子、离子或外场)组织了具有代表意义的方法。然后,我们回顾了非线性和集成光子学和光电子能量转换的应用,重点介绍了嵌入式等离子体共振如何提高器件性能。最后,我们讨论了可扩展、空间可编程等离子体的实际挑战和新机遇,包括埋藏界面的控制和通过协调光束/激光/热/化学路线实现的可重复处理。
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引用次数: 0
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Laser & Photonics Reviews
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