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From air to water: Regulation-induced pollution substitution across media 从空气到水:监管引发的跨媒介污染替代
IF 13.2 1区 环境科学与生态学 Q1 ENGINEERING, ENVIRONMENTAL Pub Date : 2026-03-19 DOI: 10.1016/j.resconrec.2026.108909
Lin Xiang, Ying Fan, Xueying Yu
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引用次数: 0
Climate stability hinges on energy-material feedback dynamics: Aluminum perspectives 气候稳定性取决于能量-物质反馈动力学:铝的观点
IF 13.2 1区 环境科学与生态学 Q1 ENGINEERING, ENVIRONMENTAL Pub Date : 2026-03-18 DOI: 10.1016/j.resconrec.2026.108911
Harald Desing, Marinella Passarella, Romain G. Billy, Alexander Griebler, Moritz Langhorst, Stefan Pogatscher, Dierk Raabe, Kirsten Remmen, Sebastian Samberger, Hauke Schlesier, Daniel B. Müller, Michael Tost
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引用次数: 0
Recycled content and recycling of electric vehicle batteries in the context of EU battery regulation: Methodological deficits and strategic approaches for sustainable battery materials 在欧盟电池法规的背景下,电动汽车电池的回收内容和回收:可持续电池材料的方法缺陷和战略途径
IF 13.2 1区 环境科学与生态学 Q1 ENGINEERING, ENVIRONMENTAL Pub Date : 2026-03-18 DOI: 10.1016/j.resconrec.2026.108903
Daniel Philipp Müller, Michael Hiete
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引用次数: 0
One-step conversion into Al2O3 coated Si nanowire anode from photovoltaic silicon waste wafers through electrothermal shock for excellent capacity retention 光伏废硅片经电热冲击一步转化为Al2O3包覆的硅纳米线阳极,具有优异的容量保持性能
IF 13.2 1区 环境科学与生态学 Q1 ENGINEERING, ENVIRONMENTAL Pub Date : 2026-03-17 DOI: 10.1016/j.resconrec.2026.108884
Qiushi Chen, Xuzhong Gong, Wenhui Fu, Xiaorui Wang, Junhao Liu, Zhi Wang
Upcycling photovoltaic waste silicon wafers into Si-based anode for lithium-ion batteries offers a promising solution to both the recycling of retired photovoltaic components and the growing demand for high-energy-density batteries driven by new energy development, but current capacity retention remain suboptimal. To address this, we leverage the intrinsic properties of photovoltaic waste silicon wafers and the ease of oxidation of their primary impurity Al to synthesize Al₂O₃-coated core-shell Si nanowires in a single step using the electrothermal shock method. By integrating Vapor-Liquid-Solid (VLS) and Oxidation-Assisted Growth (OAG) growth mechanisms, a one-step synthesis of Si nanowires and the Al2O3 coatings are achieved. The resulting Si/Al2O3 core-shell nanowires demonstrate a capacity retention of nearly 100% at 0.5 A g−1 and over 70% at 15 A g−1 both after 500 cycles. Full cell assembled with the commercial NCM811 cathode retains a capacity retention rate of 88% after 350 cycles at 0.5 C. Experimental and simulation results demonstrate that Al₂O₃ suppresses silicon expansion through its high mechanical strength and enhances lithium-ion mobility by generating oxygen vacancies as it lithiates to form LiAlO₂ during cycling. This work offers a promising approach for recycling photovoltaic waste silicon wafers into high-performance Si-based anode for lithium-ion batteries.
对于退役光伏组件的回收利用,以及新能源发展对高能量密度电池日益增长的需求,将光伏废旧硅片升级为锂离子电池的硅基负极,都是一种很有前景的解决方案,但目前的容量保持能力仍不理想。为了解决这个问题,我们利用光伏废硅片的固有特性及其主要杂质Al的易氧化性,利用电热冲击法一步合成了Al₂O₃涂层的核壳硅纳米线。通过整合气液固(VLS)和氧化辅助生长(OAG)生长机制,实现了硅纳米线和Al2O3涂层的一步合成。结果表明,经过500次循环后,Si/Al2O3核壳纳米线在0.5 a g−1下的容量保持率接近100%,在15 a g−1下的容量保持率超过70%。实验和模拟结果表明,Al₂O₃通过其高机械强度抑制硅的膨胀,并在循环过程中形成LiAlO₂,从而产生氧空位,从而提高锂离子的迁移率。这项工作为回收光伏废硅片制成高性能锂离子电池硅基阳极提供了一种有前途的方法。
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引用次数: 0
Unveiling potential water and land resource pressures under the electrolytic hydrogen boom in China 揭示中国电解氢热潮下潜在的水资源和土地资源压力
IF 13.2 1区 环境科学与生态学 Q1 ENGINEERING, ENVIRONMENTAL Pub Date : 2026-03-16 DOI: 10.1016/j.resconrec.2026.108910
Yilin Li, Jichao Fu, Mingkai Liu, Bin Chen, Xingying Lan, Chunming Xu
China’s future large-scale electrolytic green hydrogen deployment faces significant water and land constraints. Regional disparities in green hydrogen demand, electricity mix, and resource endowments lead to highly heterogeneous provincial pressures. Thus, this study quantifies water and land pressures from green hydrogen demand as feedstock and fuel in 30 provinces for 2030 under four deployment scenarios, using a nested model integrating demand forecasting and life-cycle accounting. Relative to the baseline scenario, water use may rise by up to 6-fold and land occupation by >12-fold. Polyester fiber shows the highest green hydrogen coupling potential but the greatest water and land pressures of 45.34 ton and 0.58 hectare-year per ton of product. Off-grid deployment amplifies land stress in already land-scarce eastern provinces, whereas grid-connected deployment exacerbates water stress in inherently water-scarce northwestern provinces. Multi-scale governance measures are proposed to balance China’s hydrogen transition ambitions with the constraints of water and land resource sustainability.
中国未来的大规模电解绿色氢部署面临着严重的水和土地限制。绿色氢需求、电力结构和资源禀赋的区域差异导致了高度异质性的省级压力。因此,本研究使用需求预测和生命周期会计相结合的嵌套模型,量化了2030年30个省份在四种部署情景下,绿色氢作为原料和燃料的需求对水和土地的压力。与基线情景相比,用水量可能最多增加6倍,土地占用可能增加12倍。聚酯纤维表现出最高的绿色氢偶联潜力,但最大的水和土地压力为45.34吨和0.58公顷/年每吨产品。离网部署加剧了土地本已稀缺的东部省份的土地压力,而并网部署则加剧了本来缺水的西北省份的水资源压力。提出了多尺度治理措施,以平衡中国的氢转型雄心与水资源和土地资源可持续性的限制。
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引用次数: 0
Sustainable food waste valorization pathways through co-treatment with wastewater: A bench-scale study 通过与废水共处理的可持续食物垃圾增值途径:一个实验规模的研究
IF 13.2 1区 环境科学与生态学 Q1 ENGINEERING, ENVIRONMENTAL Pub Date : 2026-03-16 DOI: 10.1016/j.resconrec.2026.108882
Zhenjun Tian, Caili Du, Yanyan Jia, Zhongzhi Chen, Baoshan Xing, Shengwang Gao, Yangwei Bai, Yimei Wei, Xuezheng Huang, Lieyu Zhang
The accelerating generation of food waste (FW) and the shortage of carbon sources in wastewater treatment pose dual challenges to sustainable urban waste management. A promising solution lies in transforming FW’s carbon-rich organics into a value-added resource. This study systematically evaluated the long-term performance of food waste hydrolysis acidification liquid (FWHAL) as a sustainable carbon source for denitrification, comparing it with commercial carbon sources (glucose and sodium acetate) in a sequencing batch reactor (SBR) under varying temperatures (10–20 °C). The assessment focused on denitrification efficiency, sludge properties, microbial community dynamics, and economic viability. Results showed that FWHAL achieved comparable denitrification efficiency, with stable nitrogen removal even at 10 °C (resulting in an average effluent nitrate nitrogen (NO₃⁻-N) concentration of 12.21–12.35 mg/L from an influent ammonium nitrogen (NH₄⁺-N) concentration of 40 mg/L). Furthermore, FWHAL had minimal impact on sludge settleability, evidenced by a significantly lower (P < 0.05) settled volume after 30 min (SV30) of 22.38% compared to glucose (27.89%) and sodium acetate (25.17%). Microbial analysis revealed that FWHAL enriched key denitrifiers, such as Dokdonella, and promoted synergistic microbial interactions. An economic assessment confirmed the viability of FWHAL, with a unit COD production cost of 0.47 USD/kg, significantly lower than the purchase cost of glucose (0.74 USD/kg) and sodium acetate (0.96 USD/kg). These findings demonstrate that FWHAL is a sustainable, cost-effective carbon source that supports the co-treatment of FW and wastewater, offering a practical strategy for integrated waste management and advancing circular economy objectives.
食物垃圾的加速产生和废水处理中碳源的短缺给可持续城市废物管理带来了双重挑战。一个有希望的解决方案是将FW富含碳的有机物转化为增值资源。本研究系统评估了食物垃圾水解酸化液(FWHAL)作为可持续反硝化碳源的长期性能,并将其与商业碳源(葡萄糖和乙酸钠)在顺序间歇反应器(SBR)中在不同温度(10-20°C)下进行了比较。评估的重点是反硝化效率、污泥特性、微生物群落动态和经济可行性。结果表明,FWHAL达到了相当的反硝化效率,即使在10°C下也能稳定地去除氮(导致流出的硝酸盐氮(NO₃⁻-N)平均浓度为12.21-12.35 mg/L,而流出的铵态氮(NH₄+ -N)浓度为40 mg/L)。此外,FWHAL对污泥沉降性的影响最小,与葡萄糖(27.89%)和乙酸钠(25.17%)相比,30分钟后的沉降体积(SV30)显著降低(P < 0.05),为22.38%。微生物分析表明,FWHAL富集了关键的反硝化菌,如Dokdonella,并促进了微生物的协同相互作用。经济评估证实了FWHAL的可行性,单位COD生产成本为0.47美元/kg,显著低于葡萄糖(0.74美元/kg)和乙酸钠(0.96美元/kg)的采购成本。这些发现表明,FWHAL是一种可持续的、具有成本效益的碳源,支持FW和废水的共同处理,为综合废物管理和推进循环经济目标提供了实用的策略。
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引用次数: 0
A systematic review of the soil C, N, and P cycles mediated by microplastics: Enzyme activities, greenhouse gas emissions and plant growth 微塑料介导的土壤碳、氮、磷循环:酶活性、温室气体排放和植物生长的系统综述
IF 10.9 1区 环境科学与生态学 Q1 ENGINEERING, ENVIRONMENTAL Pub Date : 2026-03-15 Epub Date: 2026-01-14 DOI: 10.1016/j.resconrec.2026.108788
Xianliang Wu , Jinfa Chen , Yaoyue Su , Zhenming Zhang , Jun Wang
Microplastics (MPs) are generally considered biologically inert and do not participate in element cycling in soil because microorganisms in nature lack enzyme systems that can effectively cut off these artificially synthesized polymer chains. However, an increasing number of studies have confirmed that MPs entering the soil can interfere with the stability of the microbial community structure and affect the nutrient cycling processes driven by microorganisms in the soil, thereby affecting greenhouse gas emissions and plant growth. Our understanding concerning the effects of MPs on element cycling, enzyme activity, and microbial gene expression remains unclear. The present review focuses mainly on the effects of MPs on carbon (C), nitrogen (N), and phosphorus (P) cycling on soil and plant responses and introduces related advancements, challenges, limitations, and future directions. MPs can significantly affect soil C, N and P cycles and functional microorganisms in soil and correspondingly alter enzyme activities and gene expression related to greenhouse gas emissions (CH4 and N2O), depending on the interactions between the characteristics of the MPs themselves and the soil environment (e.g., moisture status, redox potential, and the microbial community). Despite the rapid development of life cycle assessment, carbon footprint and sustainable development goals related to MPs, this is still a challenging frontier field, reflected mainly in data gaps and standardization, indistinction of the carrier effect, and incompletion of the impact assessment model. Currently, several controversies remain concerning whether the same MPs have varying effects across different soil types; findings from short-term laboratory experiments often conflict with long-term field data, and MPs ultimately enhance or suppress plant absorption of N and P. This review proposes several valuable suggestions for future research, including long-term field experiments, multifactor interactions, molecular ecology techniques, standardized research methods, and coregulatory effects of viruses and hosts, which will narrow the knowledge gap concerning MPs-mediated element cycles in soil.
微塑料(MPs)通常被认为是生物惰性的,不参与土壤中的元素循环,因为自然界的微生物缺乏能够有效切断这些人工合成的聚合物链的酶系统。然而,越来越多的研究证实,MPs进入土壤会干扰微生物群落结构的稳定性,影响土壤中微生物驱动的养分循环过程,从而影响温室气体排放和植物生长。我们对MPs对元素循环、酶活性和微生物基因表达的影响的理解尚不清楚。本文主要综述了MPs对土壤和植物碳(C)、氮(N)和磷(P)循环的影响,并介绍了相关进展、挑战、局限性和未来发展方向。MPs可以显著影响土壤C、N、P循环和土壤中功能微生物,并相应地改变与温室气体排放(CH4和N2O)相关的酶活性和基因表达,这取决于MPs本身的特征与土壤环境(如水分状况、氧化还原电位和微生物群落)之间的相互作用。尽管与MPs相关的生命周期评估、碳足迹和可持续发展目标发展迅速,但这仍然是一个具有挑战性的前沿领域,主要表现在数据的空白和标准化、载体效应的不清晰、影响评估模型的不完善等方面。目前,关于相同的MPs是否在不同的土壤类型中具有不同的效果,仍然存在一些争议;本文对今后的研究提出了一些有价值的建议,包括长期的田间实验、多因素相互作用、分子生态学技术、标准化研究方法以及病毒和宿主的协同调节作用,这将缩小MPs介导土壤元素循环的知识差距。
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引用次数: 0
Reducing embodied carbon in steel modules through end-of-life circular economy systems 通过报废循环经济系统减少钢模块的碳含量
IF 10.9 1区 环境科学与生态学 Q1 ENGINEERING, ENVIRONMENTAL Pub Date : 2026-03-15 Epub Date: 2026-01-14 DOI: 10.1016/j.resconrec.2026.108786
Vorada Kosajan, Wei Pan, Yang Zhang
This study examined the potential of End-of-Life circular economy systems to reduce embodied carbon in steel modular buildings. A multicycle life cycle assessment framework integrating material flow analysis and time-specific impact factors was developed. A case study involving a typical steel module in Hong Kong showed that landfilling generated 154.9 t CO2 eq. over the period 2020–2070, whereas recycle-priority and reuse-priority scenarios achieved 123.1 t CO2 eq. and 47.2 t CO2 eq., respectively. Reusing the steel module up to ten times reduced embodied carbon by 4.1 t CO2 eq./m2. Component-level analysis revealed that architectural components could significantly contribute to embodied carbon reductions. However, decarbonisation of the upstream industry (steel, aluminium, and electricity) reduced the benefits of multiple reuses by 24.2 %. This paper provides a comprehensive and flexible framework for multiple lifecycle assessment and offers valuable insights into how steel modular construction can enhance decarbonisation through End-of-Life circular economy systems.
本研究考察了报废循环经济系统的潜力,以减少钢模块建筑的隐含碳。建立了一个集物料流分析和时间影响因子于一体的多周期生命周期评价框架。一项涉及香港典型钢组件的个案研究显示,在2020-2070年期间,堆填区产生的二氧化碳当量为154.9吨,而优先循环再造和优先再用的方案则分别产生123.1吨和47.2吨二氧化碳当量。重复使用钢模块多达10次,减少了4.1吨二氧化碳当量/平方米的隐含碳。构件级分析表明,建筑构件可以显著减少碳排放。然而,上游工业(钢铁、铝和电力)的脱碳使多次再利用的效益降低了24.2%。本文为多个生命周期评估提供了一个全面而灵活的框架,并就钢模块结构如何通过生命周期结束循环经济系统加强脱碳提供了有价值的见解。
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引用次数: 0
Toward circular, value-added recycling of modified-poly(ethylene terephthalate): Microstructure and performance across multiple fused particle fabrication cycles 改性聚对苯二甲酸乙酯的循环增值回收:在多个熔合颗粒制造周期中的微观结构和性能
IF 10.9 1区 环境科学与生态学 Q1 ENGINEERING, ENVIRONMENTAL Pub Date : 2026-03-15 Epub Date: 2026-01-09 DOI: 10.1016/j.resconrec.2026.108781
Mohammad Sagor Hosen , Heon E. Park , Mark P. Staiger
Dimensional instability remains a principal concern in extrusion-based additive manufacturing, driven by volumetric shrinkage stemming from microstructural changes, especially throughout closed-loop recycling of semicrystalline polymers such as poly(ethylene terephthalate) (PET). The present study investigates the microstructural evolution and corresponding volumetric shrinkage of modified-PET (mPET) quantifying key microstructural contents (i.e., degree of crystallinity, and mobile and rigid amorphous fractions) across 4 fused particle fabrication cycles for the first time. The results reveal proto-spherullite formation in recycled mPET microstructure and associated microstructural changes that cause progressive volumetric shrinkage. The degree of crystallinity and rigid amorphous content are found to vary as a function of the FPF cycle number. Notably, recycled mPET exhibited an increase in density from 1.23 to 1.30 g/cm³ and volumetric shrinkage from 0 to 4.8 % following 4 FPF cycles. The study observations have important implications for predicting dimensional accuracy in 3D-printed parts manufactured from both virgin and recycled semicrystalline polymers using extrusion-based additive manufacturing.
尺寸不稳定性仍然是基于挤压的增材制造的主要问题,由微观结构变化引起的体积收缩驱动,特别是在半晶聚合物(如聚对苯二甲酸乙酯)(PET)的闭环回收过程中。本研究研究了改性pet (mPET)的微观结构演变和相应的体积收缩率,首次量化了4个熔融颗粒制造周期中的关键微观结构含量(即结晶度、可移动和刚性非晶部分)。结果揭示了再生mPET微观结构中原始球晶的形成和相关的微观结构变化导致了渐进的体积收缩。发现结晶度和刚性非晶含量随FPF循环数的变化而变化。值得注意的是,经过4次FPF循环后,再生mPET的密度从1.23 g/cm³增加到1.30 g/cm³,体积收缩率从0增加到4.8%。研究结果对于预测3d打印部件的尺寸精度具有重要意义,这些部件是使用基于挤压的增材制造技术由原始和回收的半晶聚合物制造的。
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引用次数: 0
PRecTimber 2.0: Forecasting quantitative and qualitative potentials for wood circularity in Germany, Finland, and Sweden pretimber 2.0:预测德国、芬兰和瑞典木材循环的数量和质量潜力
IF 10.9 1区 环境科学与生态学 Q1 ENGINEERING, ENVIRONMENTAL Pub Date : 2026-03-15 Epub Date: 2026-01-30 DOI: 10.1016/j.resconrec.2026.108813
Vijhay Krisshna Mahenthren , Gabriele Weber-Blaschke , Mark Hughes , Michael Risse
National bioeconomy strategies in Germany, Finland, and Sweden are expected to increase wood demand, putting pressure on already strained forest resources. Circularity of wood products can reduce this demand by improving resource efficiency, but barriers like uncertain availability and quality of post-consumer wood hinder implementation. This study optimizes and extends the PRecTimber model to forecast post-consumer wood quantities and qualities in Germany (revised with quality information), Finland, and Sweden. By 2050, predicted post-consumer wood volumes are 14.11 Mt in Germany, 1.64 Mt in Finland, and 2.74 Mt in Sweden, mainly from the construction sector. Our quality assessment methodology with scenario analysis (status quo S0 and improved scenarios S1–S2 with +10 and +20 percentage-point gains in key quality factors) reveals that the shares of post-consumer construction sawnwood suitable for lifespan extension and material recycling, respectively, are 25 % and 59 % under S0, 36 % and 50 % under S1, and 49 % and 38 % under S2. Leveraging these quantity and quality insights, policy reforms can support industries and technological innovation to optimize the use of post-consumer wood.
德国、芬兰和瑞典的国家生物经济战略预计将增加木材需求,给已经紧张的森林资源带来压力。木材产品的循环利用可以通过提高资源效率来减少这种需求,但消费后木材的可得性和质量不确定等障碍阻碍了实施。本研究优化并扩展了PRecTimber模型,以预测德国(根据质量信息修订)、芬兰和瑞典的消费后木材数量和质量。到2050年,预计消费后的木材量在德国为1411万吨,芬兰为164万吨,瑞典为274万吨,主要来自建筑部门。我们的质量评估方法与情景分析(现状S0和改进情景S1 - S2,关键质量因素提高10个百分点和20个百分点)显示,消费后建筑锯木适用于延长使用寿命和材料回收的比例分别为S0下的25%和59%,S1下的36%和50%,S2下的49%和38%。利用这些数量和质量的见解,政策改革可以支持行业和技术创新,以优化消费后木材的使用。
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引用次数: 0
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Resources Conservation and Recycling
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