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Advancements and applications of smart contact lenses: A comprehensive review 智能隐形眼镜的进步与应用:全面回顾
IF 6 Q1 ENGINEERING, MULTIDISCIPLINARY Pub Date : 2024-11-10 DOI: 10.1016/j.rineng.2024.103268
Abdulamier Ahmed Abdulamier , Lina M. Shaker , Ahmed A. Al-Amiery , Maytham T. Qasim , Wan Nor Roslam Wan Isahak , Abdullah Amru Indera Luthfi
Smart contact lenses are a transformative innovation in wearable technology, combining advanced functionalities like biosensing, drug delivery, and real-time data visualization into a compact form. This review explores recent advancements and applications of smart contact lenses, with a focus on their design principles, key technological components, and potential impact across healthcare, communication, and augmented reality. By examining current research and development, this paper highlights the evolving capabilities of smart contact lenses and their promising future prospects.
智能隐形眼镜是可穿戴技术领域的一项变革性创新,它将生物传感、药物输送和实时数据可视化等先进功能集成到一个小巧的外形中。本综述探讨了智能隐形眼镜的最新进展和应用,重点关注其设计原理、关键技术组件以及对医疗保健、通信和增强现实的潜在影响。通过研究当前的研究与开发,本文强调了智能隐形眼镜不断发展的功能及其充满希望的未来前景。
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引用次数: 0
Transforming food waste into energy: A comprehensive review 将厨余垃圾转化为能源:全面回顾
IF 6 Q1 ENGINEERING, MULTIDISCIPLINARY Pub Date : 2024-11-09 DOI: 10.1016/j.rineng.2024.103376
Shama Kakkar , Nagaraju Dharavat , Suresh Kumar Sudabattula
The proliferation of food waste has emerged as an escalating issue, with forecasts suggesting a persistent increase. Efficient waste management is essential in tackling environmental difficulties, providing a sustainable approach to alleviate these urgent problems. Fruit and vegetable waste (FVW) is notable among waste kinds for its abundant critical nutrients, dietary fibre, bioactive chemicals, and significant energy potential. Establishing an effective system for processing FVW can provide substantial advantages, especially in energy recovery and waste minimisation. The worldwide society is increasingly prioritising renewable energy sources to mitigate the environmental repercussions of fossil fuel consumption. Global initiatives are currently focused on utilising energy from FVW, along with the overarching objective of achieving international energy security. This article investigates the possibilities of power generation from many forms of food waste, analyses prevalent generating methods and their justifications, and addresses the legislation and regulations governing food waste management, as well as prospective pathways for sustainable energy solutions.
食物垃圾的激增已成为一个不断升级的问题,预测显示其数量将持续增加。有效的废物管理对于解决环境问题至关重要,它为缓解这些紧迫问题提供了一种可持续的方法。水果和蔬菜废弃物(FVW)因其丰富的重要营养成分、膳食纤维、生物活性化学物质和巨大的能源潜力而成为废弃物中的佼佼者。建立一个有效的果蔬废料处理系统可以提供巨大的优势,特别是在能源回收和废物最小化方面。全球社会越来越重视可再生能源,以减轻化石燃料消耗对环境造成的影响。目前,全球倡议的重点是利用车用燃料产生的能源,同时实现国际能源安全的总体目标。本文研究了利用多种形式的厨余发电的可能性,分析了普遍采用的发电方法及其理由,探讨了有关厨余管理的法律法规以及可持续能源解决方案的前景。
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引用次数: 0
Thermal management strategies for lithium-ion batteries in electric vehicles: A comprehensive review of nanofluid-based battery thermal management systems 电动汽车中锂离子电池的热管理策略:基于纳米流体的电池热管理系统综述
IF 6 Q1 ENGINEERING, MULTIDISCIPLINARY Pub Date : 2024-11-07 DOI: 10.1016/j.rineng.2024.103339
Abdelrahman Gasmelseed , Mhadi A. Ismael , Mior A. Said , Faiz Ahmad , Sohaib Osman
Electric vehicles have recently experienced rapid growth in battery heat generation rates due to increasing commercial demands for faster vehicle speeds and higher charging rates. This growth intensified the importance of innovative thermal management strategies to ensure safe and efficient vehicle operation. This paper aims to comprehensively review and discuss recent research investigating nanofluid battery thermal management systems (BTMS). Nanofluids are proposed as promising coolants as they possess enhanced thermal performance owing to their higher thermal conductivity compared to conventional fluids. Studies investigating nanofluid BTMSs can be divided into experimental and numerical studies investigating the effects of varying base fluid, nanoparticle type and concentration on thermal performance and pumping power. The overall trend of the reviewed studies displays an improvement in thermal performance with the increase of nanoparticles concentration, coupled with higher pumping power due to the higher viscosity values resulting in higher friction, with reviewed studies demonstrating nanofluids BTMS thermal improvements in the range of 2.9 – 30.5 % with pressure drop increase in the range of 14 – 70 % compared to the base fluid. The most commonly investigated types of nanoparticles are aluminium oxide (Al2O3), copper oxide (CuO), and silver oxide (AgO), with concentrations in the range of 0.1 – 5 %. The review highlighted the lack of long-term stability investigation and hybrid nanofluid BTMS studies in addition to studies evaluating the economic and environmental effects of utilising nanofluids in liquid BTMSs.
由于对更快车速和更高充电率的商业需求不断增加,电动汽车的电池发热量最近出现了快速增长。这种增长加剧了创新热管理策略的重要性,以确保车辆安全高效地运行。本文旨在全面回顾和讨论近期有关纳米流体电池热管理系统(BTMS)的研究。与传统流体相比,纳米流体具有更高的热传导率,因而具有更强的热性能,因此被认为是一种前景广阔的冷却剂。有关纳米流体 BTMS 的研究可分为实验研究和数值研究,以调查不同基液、纳米粒子类型和浓度对热性能和泵功率的影响。与基础流体相比,纳米流体 BTMS 的热性能提高了 2.9 - 30.5%,压降增加了 14 - 70%。最常研究的纳米粒子类型是氧化铝 (Al2O3)、氧化铜 (CuO) 和氧化银 (AgO),浓度范围在 0.1 - 5 % 之间。综述强调,除了评估液体 BTMS 中使用纳米流体的经济和环境影响的研究之外,还缺乏长期稳定性调查和混合纳米流体 BTMS 研究。
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引用次数: 0
A comprehensive recent review and practical insights on the usage of advanced materials and enhancement strategies in thermoelectric applications 有关热电应用中使用先进材料和增强策略的最新综述和实用见解
IF 6 Q1 ENGINEERING, MULTIDISCIPLINARY Pub Date : 2024-11-07 DOI: 10.1016/j.rineng.2024.103354
Mohamad Darwiche , Jalal Faraj , Khaled Chahine , Ali Shaito , Sary Awad , Mehdi Mortazavi , Mahmoud Khaled
Electricity is a critical component of many everyday activities, demanding continuing research to create new or improved techniques for generating electrical power. Thermoelectric generators (TEGs), which work basically on the Seebeck effect can successfully transform input heat from numerous applications into valuable electrical energy, as well as power electronic devices and sensors on their own. However, obstacles include increasing the temperature difference and creating novel materials to improve electrical output and efficiency. Accordingly, this paper discusses these problems by providing a thorough examination of available strategies to enhance the thermoelectric performance. In this study, a variety of materials is presented, starting by the standard used conventional organic and inorganic thermoelectric (TE) materials. Organic materials, such as polyaniline and poly(3,4-ethylenedioxythiophene) polystyrene sulfonate (PEDOT) composites, acquired ZT values ranging from 0.5 to 1.0, demonstrating their promise for versatile and low-cost applications. At extreme temperatures (∼500 K), inorganic materials such as bismuth telluride (Bi2Te3) and lead telluride (PbTe) achieved ZT values around 2.0, indicating great efficiency in power production. Bi2Te3/PEDOT, a hybrid material with organic and inorganic components, demonstrated improved performance with ZT values of 1.5–2.0 due to the synergistic effects of its constituents. Novel composite materials, such as Bi2Te3-carbon nanotube (CNT) composites and using graphene, developed to optimize thermal and electrical characteristics, enhanced device performance by up to 25% over standard materials, with ZT values ranging from 1.8 to 2.2. In addition, in the present study the new recent materials after applying enhancement methods will be presented. These new materials are developed by different methods and synthesis such as doping, superlattice and heterostructure materials and other methods will be discussed. The main findings indicate that the strategic use of these advanced materials may significantly increase the efficiency and output power of TEG devices, making them more practical for a wide variety of applications. As an examples, 2.8 for (GeTe)0.95(Sb2Te3)0.05 alloy, 2.4 for Chalcogenide, ZrS2, Bismuth telluride thin film (p-type Bi2Te3/Sb2Te3 superlattices) and 2.75 for Bismuth telluride thin film (Bi2Se1.2Te1.8). Finally, the present paper investigates on the newest technology and strategies that are applied in this research area in order to enhance the TEG performance enhancement.
电力是许多日常活动的重要组成部分,因此需要不断研究开发新的或改进的发电技术。热电发电机(TEG)主要依靠塞贝克效应工作,能够成功地将许多应用中输入的热量转化为宝贵的电能,还能为电子设备和传感器提供电力。然而,要提高电能输出和效率,还面临着增加温差和创造新型材料等障碍。因此,本文通过深入研究提高热电性能的可用策略来讨论这些问题。本研究介绍了各种材料,首先是标准使用的传统有机和无机热电(TE)材料。聚苯胺和聚(3,4-亚乙二氧基噻吩)聚苯乙烯磺酸盐(PEDOT)复合材料等有机材料的 ZT 值在 0.5 到 1.0 之间,显示了它们在多功能和低成本应用方面的前景。在极端温度(∼500 K)下,碲化铋(Bi2Te3)和碲化铅(PbTe)等无机材料的 ZT 值达到 2.0 左右,显示出极高的发电效率。Bi2Te3/PEDOT 是一种含有有机和无机成分的混合材料,由于其成分的协同效应,其性能得到了改善,ZT 值达到了 1.5-2.0。新型复合材料,如 Bi2Te3-碳纳米管(CNT)复合材料和使用石墨烯的复合材料,是为了优化热和电气特性而开发的,与标准材料相比,器件性能提高了 25%,ZT 值在 1.8 到 2.2 之间。此外,本研究还将介绍应用增强方法后的新型材料。这些新材料是通过掺杂、超晶格和异质结构材料等不同方法和合成技术开发出来的。主要研究结果表明,战略性地使用这些先进材料可以显著提高 TEG 设备的效率和输出功率,使其在各种应用中更加实用。例如,(GeTe)0.95(Sb2Te3)0.05 合金的效率为 2.8,钙钛矿、ZrS2、碲化铋薄膜(p 型 Bi2Te3/Sb2Te3 超晶格)的效率为 2.4,碲化铋薄膜(Bi2Se1.2Te1.8)的效率为 2.75。最后,本文探讨了该研究领域为提高 TEG 性能而采用的最新技术和策略。
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引用次数: 0
Integrating artificial intelligence in nanomembrane systems for advanced water desalination 将人工智能融入纳米膜系统,实现先进的海水淡化
IF 6 Q1 ENGINEERING, MULTIDISCIPLINARY Pub Date : 2024-11-06 DOI: 10.1016/j.rineng.2024.103321
Anbarasu Krishnan , Thanigaivel Sundaram , Beemkumar Nagappan , Yuvarajan Devarajan , Bhumika
The increasing global demand for clean drinking water calls for innovative approaches to optimize desalination processes, making them more sustainable and efficient. The integration of nanotechnology with artificial intelligence (AI)—particularly through machine learning and neural networks—is driving the development of advanced nanomembranes with enhanced performance and reliability. AI algorithms embedded in these nanomembrane systems enable real-time monitoring, adaptive responses to changing conditions, and proactive maintenance strategies. For instance, AI can optimize energy consumption, mitigate membrane fouling, and extend membrane lifespan. As these AI-enhanced systems operate, they continuously learn and improve their efficiency under diverse conditions. This technology also supports decentralized water solutions by enabling remote management, reducing the need for on-site personnel, and expanding access to clean water in remote areas. AI-driven systems can analyze real-time data and make informed decisions, ensuring consistent and sustainable operation. However, challenges remain, such as the development of desalination-specific AI algorithms, ensuring scalability and compatibility, and addressing data privacy and security concerns. While the convergence of AI and nanomembrane technology holds immense potential for revolutionizing water desalination, ongoing research and design efforts are essential to fully realize its capabilities in the coming years.
全球对清洁饮用水的需求日益增长,这就要求采用创新方法来优化海水淡化工艺,使其更具可持续性和效率。纳米技术与人工智能(AI)的结合,特别是通过机器学习和神经网络,推动了性能和可靠性更高的先进纳米膜的发展。嵌入到这些纳米膜系统中的人工智能算法可实现实时监控、对不断变化的条件做出自适应反应,并制定积极主动的维护策略。例如,人工智能可以优化能耗、减少膜堵塞并延长膜的使用寿命。随着这些人工智能增强型系统的运行,它们会不断学习并提高其在各种条件下的效率。这项技术还能实现远程管理,减少对现场人员的需求,扩大偏远地区清洁水的获取范围,从而支持分散式水解决方案。人工智能驱动的系统可以分析实时数据并做出明智决策,从而确保稳定和可持续的运行。然而,挑战依然存在,例如开发海水淡化专用的人工智能算法、确保可扩展性和兼容性,以及解决数据隐私和安全问题。虽然人工智能和纳米膜技术的融合为海水淡化带来了巨大的变革潜力,但要在未来几年充分实现其功能,持续的研究和设计工作至关重要。
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引用次数: 0
Harnessing evacuated tube technology for enhanced solar still: A comprehensive review 利用真空管技术增强太阳能静止:综述
IF 6 Q1 ENGINEERING, MULTIDISCIPLINARY Pub Date : 2024-11-05 DOI: 10.1016/j.rineng.2024.103335
A.S. Abdullah , Abanob Joseph , Gamal B. Abdelaziz , Elbager M.A. Edreis , Mohammed El Hadi Attia , Wissam H. Alawee , Swellam W. Sharshir
The simplest and solar energy-based desalination method, solar still desalination, is presented in response to the expanding need for freshwater. However, as the evaporation process is essential to the functioning of solar stills, effective evaporation upgrades are required to raise the solar desalination ability. Using evacuated tube technology for water heating results in an improved evaporation process that makes solar still desalination replicable. This work conducts a review study on the coupling of this technology with the various types of solar stills. The performance of each type of solar still in conjunction with a solar heater is examined throughout the study, along with the viability of doing so economically. Furthermore, various environmental studies are offered on this kind of assembly to examine how it affects reducing carbon emissions. Additionally, the advantages of combining each form of solar still with the heaters are examined. Moreover, several evacuated tube heater designs, including tank-based, parabolic collector-based, and direct connection to the solar still, also referred to as natural mode, are demonstrated throughout the paper. Proper coupling resulted in yield, energy, and exergetic efficiencies reaching 20.95 L/m2, 65.48, and 6.67 % which were higher than those of basic solar still by 431.7, 57.82, and 74.61 %, respectively. Besides, a bibliometric analysis is conducted using the VOSviewer tool to demonstrate the contribution and trend regarding solar collector-based solar stills.
为满足日益增长的淡水需求,提出了最简单的基于太阳能的海水淡化方法--太阳能蒸馏海水淡化。然而,由于蒸发过程对太阳能蒸馏器的运行至关重要,因此需要对蒸发过程进行有效升级,以提高太阳能海水淡化能力。利用真空管技术加热水可改进蒸发过程,从而使太阳能蒸馏器海水淡化技术具有可复制性。这项工作对该技术与各种类型太阳能蒸馏器的耦合进行了审查研究。在整个研究过程中,对每种类型的太阳能蒸馏器与太阳能加热器结合使用的性能,以及这样做的经济可行性进行了研究。此外,还对这种组合方式进行了各种环境研究,以探讨其对减少碳排放的影响。此外,还研究了每种形式的太阳能蒸发器与加热器相结合的优势。此外,本文还展示了几种真空管加热器的设计,包括水箱式、抛物线集热器式以及直接连接到太阳能蒸馏器(也称为自然模式)的设计。适当的耦合使产量、能量和能效分别达到 20.95 升/平方米、65.48% 和 6.67%,分别比基本太阳能蒸发器高出 431.7%、57.82% 和 74.61%。此外,还使用 VOSviewer 工具进行了文献计量分析,以展示基于太阳能集热器的太阳能蒸馏器的贡献和趋势。
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引用次数: 0
Metallic cutting inserts fabrication by means of additive manufacturing with fused filament fabrication technology 利用熔融长丝制造技术的增材制造方法制造金属切削刀片
IF 6 Q1 ENGINEERING, MULTIDISCIPLINARY Pub Date : 2024-11-04 DOI: 10.1016/j.rineng.2024.103194
Francisco Martín-Fernández , María Jesús Martín-Sánchez , Guillermo Guerrero-Vacas , Óscar Rodríguez-Alabanda
The present work developed a first approach to the manufacturing of turning inserts using the emerging Additive Manufacturing (AM) technology, specifically employing the fused filament fabrication (FFF) process, based on the extrusion of material and deposition layer by layer. Traditionally, this type of cutting tools were manufactured by powder metallurgy and machining processes, but in this instance Additive Manufacturing processes allowed the customisation of the geometries and eliminated the need of dies to manufacture these tools, leading to economic savings. The study analysed, from different perspectives, the viability of these interchangeable inserts as cutting tools. These approaches included qualitative studies of chip formation and cutting-edge wear as well as thermal and roughness analysis of specimens tested under different conditions. The behaviour of H13 Tool Steel cutting inserts on cylindrical specimens of EN AW-2030 aluminium alloy was compared with commercial carbide inserts, being observed that the chip types produced were extremely similar between those obtained by commercial and those from Additive Manufacturing, particularly in dry conditions. The qualitative study of insert wear showed that AM inserts presented overall larger contribution of built-up edge (BUE) and plastic deformation of the tip, with greater incidence at cutting speeds of Vc = 60 m/min and feed rate of fz = 0.1 mm/r. Regarding thermal analysis, the AM inserts revealed a slightly more abrasive behaviour, resulting in a temperature increase throughout the machining process of approximately 70 °C, with no significant influence from the increase in cutting speed. The study of the surface finish offered average roughness results (Ra) of 0.58 µm for commercial inserts, 1.78 µm in AM inserts with dry tests and 2.06 µm in this same type of insert but tested with lubrication. These variations in average roughness were not significant.
本研究利用新兴的增材制造(AM)技术,特别是采用基于材料挤压和逐层沉积的熔融长丝制造(FFF)工艺,开发了第一种制造车削刀片的方法。传统上,这种类型的切削工具是通过粉末冶金和机械加工工艺制造的,但在这种情况下,增材制造工艺允许定制几何形状,并消除了制造这些工具所需的模具,从而节省了经济成本。研究从不同角度分析了这些可互换刀片作为切削工具的可行性。这些方法包括对切屑形成和切削刃磨损的定性研究,以及在不同条件下测试试样的热分析和粗糙度分析。将 H13 工具钢切削刀片在 EN AW-2030 铝合金圆柱形试样上的表现与商用硬质合金刀片进行了比较,发现商用刀片和快速成型制造刀片产生的切屑类型极为相似,尤其是在干燥条件下。对刀片磨损的定性研究表明,AM 刀片的刀尖堆积刃(BUE)和塑性变形总体上更大,在切削速度 Vc = 60 m/min 和进给量 fz = 0.1 mm/r 时发生率更高。在热分析方面,AM 刀片的磨损性稍强,导致整个加工过程中的温度上升约 70 °C,而切削速度的提高对其影响不大。对表面光洁度的研究结果表明,商用刀片的平均粗糙度(Ra)为 0.58 微米,AM 刀片的干燥测试结果为 1.78 微米,同类型刀片的润滑测试结果为 2.06 微米。平均粗糙度的这些变化并不显著。
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引用次数: 0
Critical review on graphene oxide modified geopolymers: Dispersion preparation, mechanical properties, and microscopic mechanisms 氧化石墨烯改性土工聚合物综述:分散制备、力学性能和微观机理
IF 6 Q1 ENGINEERING, MULTIDISCIPLINARY Pub Date : 2024-11-04 DOI: 10.1016/j.rineng.2024.103320
Mengqi Xu , Jiajia Fu , Tianhong Feng , Wei Wang
In recent years, graphene oxide (GO) has been widely used in various fields owing to its high specific surface area and rich oxygen-containing functional groups. Adding an appropriate amount of GO (about 0.01–0.1 wt%) is beneficial to strengthen the soft soil foundation, which can improve the mechanical properties of the geopolymers, promote the hydration reaction, and improve the pore structure. The main mechanisms include the distortion effect, intercalation effect, template effect, bridge effect, active catalytic effect, adsorption cementation effect, and nucleation effect. Currently, GO research on cement materials mainly focuses on mortar and concrete and pays less attention to geotechnical engineering fields, such as cement soil. Therefore, to fully understand the unique advantages of GO, to clarify the method and mechanism of GO strengthening soft soil foundations, and to expand its application in geotechnical engineering, we briefly summarise the characterisation methods, dispersion of GO, analyse the influence of the single incorporation of GO on the mechanical properties of geopolymers, and discuss its microscopic mechanism. The environmental and safety effects are also discussed. Finally, the problems existing in the current research are analysed and future research directions are discussed.
近年来,氧化石墨烯(GO)因其高比表面积和丰富的含氧官能团而被广泛应用于各个领域。添加适量的 GO(约 0.01-0.1 wt%)有利于加固软土地基,可提高土工聚合物的力学性能,促进水化反应,改善孔隙结构。主要机理包括变形效应、插层效应、模板效应、架桥效应、活性催化效应、吸附胶结效应和成核效应等。目前,GO 对水泥材料的研究主要集中在砂浆和混凝土方面,对岩土工程领域(如水泥土)的关注较少。因此,为了充分认识 GO 的独特优势,阐明 GO 加固软土地基的方法和机理,拓展其在岩土工程中的应用,我们简要总结了 GO 的表征方法、分散性,分析了单一掺入 GO 对土工聚合物力学性能的影响,探讨了其微观机理。此外,还讨论了对环境和安全的影响。最后,分析了当前研究中存在的问题,并讨论了未来的研究方向。
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引用次数: 0
Exploring natural plant fiber choices and treatment methods for contemporary composites: A comprehensive review 探索当代复合材料的天然植物纤维选择和处理方法:全面回顾
IF 6 Q1 ENGINEERING, MULTIDISCIPLINARY Pub Date : 2024-11-04 DOI: 10.1016/j.rineng.2024.103270
Muthuselvan Balasubramanian, R. Saravanan, Sathish T
The growing importance of composite materials in engineering is reshaping industries such as automotive, maritime, sports, and aerospace. As industries seek sustainable alternatives to synthetic fibers, natural fibers have emerged as a promising solution due to their abundance, low cost, and biodegradability. Natural fibers not only address environmental concerns but also offer a competitive strength-to-weight ratio, making them an attractive choice for reinforcement in modern composites. They overcome many of the limitations of synthetic fibers and fiberglass, offering enhanced mechanical, thermal, and physical properties while being easier to manufacture. This comprehensive review delves into the latest advancements in natural fiber composites, exploring newly discovered fibers and innovative treatment methods. By examining these natural fiber-based polymers, the review highlights their potential to meet the ever-evolving demands for materials that combine superior performance with affordability and sustainability.
复合材料在工程学中的重要性与日俱增,正在重塑汽车、海事、体育和航空航天等行业。随着各行各业都在寻求合成纤维的可持续替代品,天然纤维因其丰富的资源、低廉的成本和可生物降解性而成为一种前景广阔的解决方案。天然纤维不仅能解决环境问题,还具有极具竞争力的强度重量比,因此成为现代复合材料中极具吸引力的增强材料。它们克服了合成纤维和玻璃纤维的许多局限性,具有更强的机械、热和物理性能,同时更易于制造。本综述深入探讨了天然纤维复合材料的最新进展,探索了新发现的纤维和创新的处理方法。通过研究这些以天然纤维为基础的聚合物,本综述强调了它们在满足不断变化的材料需求方面的潜力,这些材料兼具卓越的性能、经济性和可持续性。
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引用次数: 0
Electrodeposition of nano- and micro-materials: Advancements in electrocatalysts for electrochemical applications 纳米和微米材料的电沉积:电化学应用中的电催化剂研究进展
IF 6 Q1 ENGINEERING, MULTIDISCIPLINARY Pub Date : 2024-11-04 DOI: 10.1016/j.rineng.2024.103285
Mayra S. Tovar-Oliva, Ignacio Tudela
Electrodeposition is an essential technique for the fabrication of nanomaterials and thin films based on passing an electric current through a support electrode in contact with a solution containing a metal salt dissolved in it. Commonly referred to as ‘electroplating’ in industrial settings, this method is extensively used for developing a wide range of electrocatalytic materials due to its simplicity, versatility, cost-effectiveness, and efficiency. Despite its widespread use and growing popularity for electrocatalyst fabrication, electrodeposition processes are often misunderstood, and many research studies have not fully leveraged their potential due to a lack of understanding and optimisation of key aspects of the process; consequently, researchers may miss straightforward opportunities to maximise the performance and functionality of electrodeposited electrocatalysts, as small variations in the electrodeposition process parameters can have significant effects on their activity, selectivity and lifespan. To address these issues, the present review delves deeper into the fundamental principles of electrodeposition, explores the mechanisms of electrodeposited material growth and discusses potentiostatic, galvanostatic and pulse electrodeposition techniques in achieving uniform and high-quality films. Moreover, the review discusses how different operation parameters such as pH, temperature or current density influence the process itself and the properties of deposited materials and films. The use of electrodeposited materials as catalysts in various electrochemical applications such as
reduction, water splitting, pollutant removal and energy storage, among others, is also reviewed, along with a stimulating discussion on challenges faced by the research community and future opportunities for electrodeposition techniques in the area of electrocatalysis. By providing a comprehensive understanding of how process parameters affect the activity, selectivity, stability, and durability of electrodeposited electrocatalysts, this review underscores the importance of electrodeposition in advancing sustainable and efficient energy solutions.
电沉积是一种制造纳米材料和薄膜的基本技术,其原理是将电流通过与含有金属盐溶液接触的支撑电极。这种方法在工业环境中通常被称为 "电镀",因其简单、通用、成本效益高和效率高而被广泛用于开发各种电催化材料。尽管电沉积工艺在电催化剂制造中应用广泛且日益流行,但由于缺乏对该工艺关键环节的了解和优化,电沉积工艺常常被误解,许多研究也未能充分发挥其潜力;因此,研究人员可能会错失将电沉积电催化剂的性能和功能最大化的直接机会,因为电沉积工艺参数的微小变化都会对电催化剂的活性、选择性和寿命产生重大影响。针对这些问题,本综述深入探讨了电沉积的基本原理,探讨了电沉积材料的生长机制,并讨论了实现均匀和高质量薄膜的恒电位、恒电流和脉冲电沉积技术。此外,综述还讨论了 pH 值、温度或电流密度等不同操作参数如何影响工艺本身以及沉积材料和薄膜的特性。此外,还综述了电沉积材料作为催化剂在各种电化学应用(如还原、水分离、污染物去除和能量存储等)中的应用,并就电沉积技术在电催化领域的研究界面临的挑战和未来机遇进行了热烈讨论。通过全面了解工艺参数如何影响电沉积电催化剂的活性、选择性、稳定性和耐久性,本综述强调了电沉积在推进可持续高效能源解决方案方面的重要性。
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引用次数: 0
期刊
Results in Engineering
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