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Accurate identification and formation mechanism unraveling of radicals in UV-induced peracetic acid activation system using in-situ electron paramagnetic resonance.
IF 18.8 1区 综合性期刊 Q1 MULTIDISCIPLINARY SCIENCES Pub Date : 2025-03-08 DOI: 10.1016/j.scib.2025.03.008
Long Chen, Ruohan Zhang, Zhaoli Liu, Fan Li, Boyu Huang, Wen Liu
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引用次数: 0
Great Oxidation Event was caused by Neoarchean global cratonization: opportunity and challenge from rock and sedimentary records in China. 新元古代全球克拉通化导致的大氧化事件:中国岩石和沉积记录带来的机遇与挑战。
IF 18.8 1区 综合性期刊 Q1 MULTIDISCIPLINARY SCIENCES Pub Date : 2025-03-08 DOI: 10.1016/j.scib.2025.03.020
Li-Gang Zhou, Jun-Ping Liu, Jing Li, Zai-Bo Sun, Lu Xiang, Yan-Yan Zhou, Hao-Shu Tang, Yan-Bin Zhang, Xi-Yan Zhu, Hai-Long He, Ming-Guo Zhai
{"title":"Great Oxidation Event was caused by Neoarchean global cratonization: opportunity and challenge from rock and sedimentary records in China.","authors":"Li-Gang Zhou, Jun-Ping Liu, Jing Li, Zai-Bo Sun, Lu Xiang, Yan-Yan Zhou, Hao-Shu Tang, Yan-Bin Zhang, Xi-Yan Zhu, Hai-Long He, Ming-Guo Zhai","doi":"10.1016/j.scib.2025.03.020","DOIUrl":"https://doi.org/10.1016/j.scib.2025.03.020","url":null,"abstract":"","PeriodicalId":421,"journal":{"name":"Science Bulletin","volume":" ","pages":""},"PeriodicalIF":18.8,"publicationDate":"2025-03-08","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143630120","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"综合性期刊","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Towards rational design of high-performance anion exchange membranes.
IF 18.8 1区 综合性期刊 Q1 MULTIDISCIPLINARY SCIENCES Pub Date : 2025-03-05 DOI: 10.1016/j.scib.2025.03.004
Licheng Sun
{"title":"Towards rational design of high-performance anion exchange membranes.","authors":"Licheng Sun","doi":"10.1016/j.scib.2025.03.004","DOIUrl":"https://doi.org/10.1016/j.scib.2025.03.004","url":null,"abstract":"","PeriodicalId":421,"journal":{"name":"Science Bulletin","volume":" ","pages":""},"PeriodicalIF":18.8,"publicationDate":"2025-03-05","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143672898","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"综合性期刊","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Abrupt loss of species richness caused by ecosystem transition.
IF 18.8 1区 综合性期刊 Q1 MULTIDISCIPLINARY SCIENCES Pub Date : 2025-03-03 DOI: 10.1016/j.scib.2025.03.001
Li Fu, Jianping Huang, Guolong Zhang, Dongliang Han, Lei Ding, Yun Wei, Xiaoyue Liu, Changyu Li, Haipeng Yu

Ecosystem transition occurs when ecological thresholds are crossed, causing ecosystems to irreversibly shift from secure to insecure states. However, how ecosystem transition exacerbates species richness loss remains poorly understood. This hinders the effective protection of species richness, which is an urgent global priority. In this study, we integrated multiple ecosystem variables to elucidate ecosystem transition and its impacts on species richness loss. Our findings reveal that species richness declines abruptly following ecosystem transition, as insecure ecosystems are characterized by reduced plant cover and productivity, intensified warming and drying, and diminished oxygen production. Insecure ecosystems imperil the survival of all species, including 39.4% of threatened birds and 29.2% of threatened mammal species. We project that by 2100, the ecosystem areas considered insecure will encompass 40.4% of the global land areas under the RCP8.5 scenario, contributing to 51.6% of species richness loss. In contrast, hyper-secure ecosystems are projected to account for 18.1% of species richness loss. This study identifies ecosystem transition as a critical driver of species richness loss that should be accounted for by policymakers in designing targeted conservation strategies.

{"title":"Abrupt loss of species richness caused by ecosystem transition.","authors":"Li Fu, Jianping Huang, Guolong Zhang, Dongliang Han, Lei Ding, Yun Wei, Xiaoyue Liu, Changyu Li, Haipeng Yu","doi":"10.1016/j.scib.2025.03.001","DOIUrl":"https://doi.org/10.1016/j.scib.2025.03.001","url":null,"abstract":"<p><p>Ecosystem transition occurs when ecological thresholds are crossed, causing ecosystems to irreversibly shift from secure to insecure states. However, how ecosystem transition exacerbates species richness loss remains poorly understood. This hinders the effective protection of species richness, which is an urgent global priority. In this study, we integrated multiple ecosystem variables to elucidate ecosystem transition and its impacts on species richness loss. Our findings reveal that species richness declines abruptly following ecosystem transition, as insecure ecosystems are characterized by reduced plant cover and productivity, intensified warming and drying, and diminished oxygen production. Insecure ecosystems imperil the survival of all species, including 39.4% of threatened birds and 29.2% of threatened mammal species. We project that by 2100, the ecosystem areas considered insecure will encompass 40.4% of the global land areas under the RCP8.5 scenario, contributing to 51.6% of species richness loss. In contrast, hyper-secure ecosystems are projected to account for 18.1% of species richness loss. This study identifies ecosystem transition as a critical driver of species richness loss that should be accounted for by policymakers in designing targeted conservation strategies.</p>","PeriodicalId":421,"journal":{"name":"Science Bulletin","volume":" ","pages":""},"PeriodicalIF":18.8,"publicationDate":"2025-03-03","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143646758","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"综合性期刊","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Direct synthesis of millimeter-sized hexagonal diamond from graphite 从石墨中直接合成毫米级六角金刚石。
IF 18.8 1区 综合性期刊 Q1 MULTIDISCIPLINARY SCIENCES Pub Date : 2025-03-03 DOI: 10.1016/j.scib.2025.03.003
Xiaohong Yuan , Guwen Chen , Yong Cheng , Shengcai Zhu , Fuyang Liu , Yujiao Ke , Kuo Hu , Yue Pan , Ming-Sheng Wang , Zhaodong Liu , Hu Tang , Bingbing Liu
Diamond has the strongest three-dimensional network structure and its cubic configuration is extremely stable under high pressure, thus limiting the experimental synthesis of diamond polymorphs. Hexagonal diamond, a typical polymorph of diamond, has attracted considerable attention in recent decades, yet synthesizing pure and large-sized hexagonal diamond remains technically challenging, preventing an accurate understanding of its properties and formation mechanism. Here, we report the direct synthesis of millimeter-sized, nearly pure hexagonal diamond from graphite under high-pressure and high-temperature conditions using our developed high-pressure technique in a multi-anvil press. The synthesized hexagonal diamond is highly oriented polycrystalline, exhibiting an ultrahard hardness (165 ± 4 GPa) on (100) planes, which is ∼50% harder than single-crystal cubic diamond. Structural characterizations and molecular dynamics simulations indicate that hexagonal diamond is formed through a martensitic transformation process whereby hexagonal graphite is transformed into hexagonal diamond by sliding and then direct bonding between graphite sheets. Furthermore, we show that the transformations from graphite to cubic or hexagonal diamonds are strongly temperature-pressure dependent. With this understanding, we further synthesized cubic/hexagonal diamond composites with unusual heterostructures at a lower pressure. This work not only established a fundamental framework for high-pressure phase transformations in graphite but also provided insight into the structural evolution of two-dimensional materials at high pressures and a potent strategy for exploring their new high-pressure phases.
金刚石具有最强的三维网络结构,其立方构型在高压下极其稳定,因此限制了金刚石多晶体的实验合成。六方金刚石是金刚石的一种典型多晶体,近几十年来一直备受关注,然而合成纯净的大尺寸六方金刚石在技术上仍然具有挑战性,这阻碍了人们对其性质和形成机理的准确理解。在此,我们报告了在高压和高温条件下,利用我们开发的多钒压机高压技术,从石墨中直接合成出毫米大小、近乎纯净的六方金刚石。合成的六方金刚石是高度取向的多晶体,在(100)平面上表现出超高硬度(165 ± 4 GPa),比单晶立方金刚石的硬度高出 50%。结构表征和分子动力学模拟表明,六方金刚石是通过马氏体转变过程形成的,即六方石墨通过滑动转变为六方金刚石,然后在石墨片之间直接结合。此外,我们还发现,从石墨到立方或六方金刚石的转变与温度压力密切相关。基于这一认识,我们进一步合成了立方/六方金刚石复合材料,并在较低的压力下获得了不同寻常的异质结构。这项工作不仅建立了石墨高压相变的基本框架,还深入了解了二维材料在高压下的结构演变,并为探索其新的高压相提供了有力的策略。
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引用次数: 0
A PLA2-responsive nanoagonist to boost immunotherapy via targeted release of lipid mediators in cold tumor microenvironment.
IF 18.8 1区 综合性期刊 Q1 MULTIDISCIPLINARY SCIENCES Pub Date : 2025-03-03 DOI: 10.1016/j.scib.2025.03.002
Hui-Ping Wen, Meng-Die Zhu, Di Ning, Zhi-Gang Wang, Yusi Hu, Chuan-Ming Yu, Dai-Wen Pang, Shu-Lin Liu
{"title":"A PLA2-responsive nanoagonist to boost immunotherapy via targeted release of lipid mediators in cold tumor microenvironment.","authors":"Hui-Ping Wen, Meng-Die Zhu, Di Ning, Zhi-Gang Wang, Yusi Hu, Chuan-Ming Yu, Dai-Wen Pang, Shu-Lin Liu","doi":"10.1016/j.scib.2025.03.002","DOIUrl":"https://doi.org/10.1016/j.scib.2025.03.002","url":null,"abstract":"","PeriodicalId":421,"journal":{"name":"Science Bulletin","volume":" ","pages":""},"PeriodicalIF":18.8,"publicationDate":"2025-03-03","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143612936","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"综合性期刊","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
New insights on carbon forms in China's rivers and lakes.
IF 18.8 1区 综合性期刊 Q1 MULTIDISCIPLINARY SCIENCES Pub Date : 2025-03-01 DOI: 10.1016/j.scib.2025.02.040
Dong Liu, Kun Shi, Nuoxiao Yan, Evangelos Spyrakos, Andrew N Tyler, R Iestyn Woolway, Hongtao Duan
{"title":"New insights on carbon forms in China's rivers and lakes.","authors":"Dong Liu, Kun Shi, Nuoxiao Yan, Evangelos Spyrakos, Andrew N Tyler, R Iestyn Woolway, Hongtao Duan","doi":"10.1016/j.scib.2025.02.040","DOIUrl":"https://doi.org/10.1016/j.scib.2025.02.040","url":null,"abstract":"","PeriodicalId":421,"journal":{"name":"Science Bulletin","volume":" ","pages":""},"PeriodicalIF":18.8,"publicationDate":"2025-03-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143612947","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"综合性期刊","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Pivotal roles of intracellular Cl- in COVID-19: pathogenesis and therapeutic targets.
IF 18.8 1区 综合性期刊 Q1 MULTIDISCIPLINARY SCIENCES Pub Date : 2025-02-28 DOI: 10.1016/j.scib.2025.02.035
Su Qu, Lei Chen, Jie Sheng, Xiao-Chun Hou, Wen-Liang Zhou, Nan-Shan Zhong, Yi-Lin Zhang
{"title":"Pivotal roles of intracellular Cl<sup>-</sup> in COVID-19: pathogenesis and therapeutic targets.","authors":"Su Qu, Lei Chen, Jie Sheng, Xiao-Chun Hou, Wen-Liang Zhou, Nan-Shan Zhong, Yi-Lin Zhang","doi":"10.1016/j.scib.2025.02.035","DOIUrl":"https://doi.org/10.1016/j.scib.2025.02.035","url":null,"abstract":"","PeriodicalId":421,"journal":{"name":"Science Bulletin","volume":" ","pages":""},"PeriodicalIF":18.8,"publicationDate":"2025-02-28","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143584199","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"综合性期刊","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
A 300-km fully-connected quantum secure direct communication network.
IF 18.8 1区 综合性期刊 Q1 MULTIDISCIPLINARY SCIENCES Pub Date : 2025-02-27 DOI: 10.1016/j.scib.2025.02.038
Yilin Yang, Yuanhua Li, Hao Li, Chennan Wu, Yuanlin Zheng, Xianfeng Chen

Transmission distance and number of users limit the realization of large-scale scalable quantum communication networks, as existing quantum network construction techniques struggle to address these two important factors simultaneously. In this paper, we propose a long-distance large-scale and scalable fully-connected quantum secure direct communication (QSDC) network, which employs a double-pumped structure and the introduction of extra noise to successfully realize QSDC over 300 km between four users in the network in pairs. The results demonstrate that the fidelity of the entangled state shared between users following communication remains above 85%. The results of our research demonstrate the viability of this quantum communication network, offering a novel foundation for the future realization of long-distance large-scale quantum communication.

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引用次数: 0
D/V Meng Xiang is coming to revive the 60-year-old dream of Moho drilling and enter a new phase of international scientific ocean drilling.
IF 18.8 1区 综合性期刊 Q1 MULTIDISCIPLINARY SCIENCES Pub Date : 2025-02-26 DOI: 10.1016/j.scib.2025.02.039
Yue Xu, Yaoling Niu, Xia Zhang, Tienan Chen, Tingting Wang, Pengyuan Guo, Pu Sun, Xiaohong Wang, Meng Duan, Yanhong Chen
{"title":"D/V Meng Xiang is coming to revive the 60-year-old dream of Moho drilling and enter a new phase of international scientific ocean drilling.","authors":"Yue Xu, Yaoling Niu, Xia Zhang, Tienan Chen, Tingting Wang, Pengyuan Guo, Pu Sun, Xiaohong Wang, Meng Duan, Yanhong Chen","doi":"10.1016/j.scib.2025.02.039","DOIUrl":"https://doi.org/10.1016/j.scib.2025.02.039","url":null,"abstract":"","PeriodicalId":421,"journal":{"name":"Science Bulletin","volume":" ","pages":""},"PeriodicalIF":18.8,"publicationDate":"2025-02-26","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143555430","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"综合性期刊","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
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