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Review of the structural properties and interfacial reactions of Al-substituted goethite, hematite and ferrihydrite 评述铝取代的鹅铁矿、赤铁矿和铁酸盐的结构特性和界面反应
IF 5.2 2区 农林科学 Q1 SOIL SCIENCE
Pedosphere
Pub Date : 2025-02-01 DOI: 10.1016/j.pedsph.2024.06.006
Yu LIANG , Hongfeng CHEN , Jinling XU , Mingxia WANG , Wenfeng TAN
Isomorphic substitution of ferric ion (Fe3+) by aluminum ion (Al3+) in iron (hydro)oxides is ubiquitous in natural environments. Aluminum substitution inevitably leads to changes in the microstructures, physicochemical properties, and surface reactions of iron (hydro)oxides, which may have great impacts on the sequestration of nutrients and contaminants in soils and aquatic environments. Over the past decades, the structural properties and surface reactivity of Al-substituted iron (hydro)oxides have been intensively studied. Iron (hydro)oxides in various structural forms and with different Al substitution amounts present high application potentials in addressing environmental issues. A timely summary of the structural properties and interfacial reactions of the most common and representative Al-substituted iron (hydro)oxides is of significance. Herein, the effects of Al substitution on the structural properties and surface activities of iron (hydro)oxides were clarified according to the microstructure, crystal facets, surface site type and density, interfacial reaction mechanisms, and modeling parameters of iron (hydro)oxides. This review systematically elucidates how Al substitution affects the structural properties and surface reactions of iron (hydro)oxides, including the well crystallized goethite and hematite and the poorly crystallized ferrihydrite, providing theoretical guidance for further exploration of the mineralogical characteristics and environmental geochemical behaviors of iron (hydro)oxides.
铁（氢）氧化物中，铁离子（Fe3+）被铝离子（Al3+）同形取代在自然环境中是普遍存在的。铝的取代不可避免地导致铁（氢）氧化物的微观结构、理化性质和表面反应的变化，这可能对土壤和水生环境中营养物质和污染物的固存产生很大影响。在过去的几十年中，人们对铝取代铁（氢）氧化物的结构性质和表面反应性进行了深入的研究。不同结构形式和不同铝取代量的铁（氢）氧化物在解决环境问题方面具有很高的应用潜力。及时总结最常见和最具代表性的铝取代铁（氢）氧化物的结构性质和界面反应是有意义的。本文从铁（氢）氧化物的微观结构、晶面、表面位点类型和密度、界面反应机理和建模参数等方面阐明了Al取代对铁（氢）氧化物结构性能和表面活性的影响。本文系统阐述了Al取代对铁（氢）氧化物（包括晶化良好的针铁矿和赤铁矿以及晶化不良的水合铁）结构性质和表面反应的影响，为进一步探索铁（氢）氧化物的矿物学特征和环境地球化学行为提供了理论指导。
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引用次数: 0
Rice residue management: Alternative strategies and emerging technologies for a sustainable ecosystem 稻草管理：可持续生态系统的替代战略和新兴技术
IF 5.2 2区 农林科学 Q1 SOIL SCIENCE
Pedosphere
Pub Date : 2025-02-01 DOI: 10.1016/j.pedsph.2024.06.004
Jagdish PARSHAD , Ravinder KUMAR , Vinod CHHOKAR , Nagaraj PATIL , Vikas BENIWAL , Namita SINGH , Ajay KUMAR , Nitesh SINGH , Rajesh YOGI , Mukesh KUMAR , Prashant VIKRAM , Avnish CHAUHAN , Anil KUMAR
Rice straw, which is produced after the harvest of rice, is a major agricultural waste in the world. Rice straw has a high carbon/nitrogen ratio and is more resistant to microbial degradation than other straws because its main constituents are cellulose and hemicelluloses encrusted by lignin. When rice straw is burned, hazardous substances such as carbon dioxide, methane, carbon monoxide, and nitrogen monoxide are released into the air as smoke (less than 10 μm-sized particles). The rise in the burning of rice straw has contributed to too many accidents and health issues in the general population residing in Haryana, Punjab, and Uttar Pradesh of India. These states are being urged by the National Green Tribunal to generate money instead of burning rice straw. Even though these lignocellulosic materials might be beneficial, not much has been carried out with them. This overview covers the properties of rice straw and husks, the numerous procedures used to create valuable products, and various applications that may be made for them. These include energy sources, environmental adsorbents, building supplies, and specialist commodities.
水稻收获后产生的秸秆是世界上主要的农业废弃物。由于稻草的主要成分是纤维素和被木质素包裹的半纤维素，因此具有较高的碳氮比，比其他秸秆更耐微生物降解。秸秆燃烧时，二氧化碳、甲烷、一氧化碳、一氧化氮等有害物质以烟雾的形式释放到空气中（颗粒小于10 μm）。焚烧稻草的增加给居住在印度哈里亚纳邦、旁遮普邦和北方邦的普通民众造成了太多的事故和健康问题。国家绿色法庭正在敦促这些邦创收，而不是焚烧稻草。尽管这些木质纤维素材料可能是有益的，但对它们的研究还不多。本综述涵盖了稻秆和稻壳的特性，用于制造有价值产品的众多程序，以及可能为它们制作的各种应用。这些包括能源、环境吸附剂、建筑用品和专业商品。
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引用次数: 0
IF 7.3 2区 农林科学 Q1 SOIL SCIENCE
Pedosphere
Pub Date : 2025-01-01
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引用次数: 0
IF 7.3 2区 农林科学 Q1 SOIL SCIENCE
Pedosphere
Pub Date : 2025-01-01
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引用次数: 0
IF 7.3 2区 农林科学 Q1 SOIL SCIENCE
Pedosphere
Pub Date : 2025-01-01
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引用次数: 0
IF 7.3 2区 农林科学 Q1 SOIL SCIENCE
Pedosphere
Pub Date : 2025-01-01
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引用次数: 0
IF 7.3 2区 农林科学 Q1 SOIL SCIENCE
Pedosphere
Pub Date : 2025-01-01
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引用次数: 0
IF 7.3 2区 农林科学 Q1 SOIL SCIENCE
Pedosphere
Pub Date : 2025-01-01
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引用次数: 0
IF 7.3 2区 农林科学 Q1 SOIL SCIENCE
Pedosphere
Pub Date : 2025-01-01
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引用次数: 0
IF 7.3 2区 农林科学 Q1 SOIL SCIENCE
Pedosphere
Pub Date : 2025-01-01
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引用次数: 0
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