In response to the demands of electrochromic devices, the advantages and designs of the corresponding multifunctional integrated gel polymer electrolytes were discussed.
Through reviewing the applications of electrochromic devices based on gel polymer electrolytes, the remarkable advantages that gel polymer electrolytes bring to electrochromic devices and their practical applications in electrochromic devices were analyzed.
The future research directions of gel polymer electrolytes for electrochromic devices were explored, thereby facilitating their further development and commercial application.
Sucralose (SCL) has been unveiled as an electrolyte additive to promote the exposure of the Zn(002) texture.
SCL has been verified to disrupt the solvation structure around zinc ions and reduce water activity on Zn anode.
After adding SCL additives, Zn//Zn battery achieves the cycling lifespan of 171 h at 30 mA cm−2–30 mAh cm−2 (DOD = 73.3%). Zn//Cu battery achieves a high Coulombic efficiency of 99.61% at 0.2 mA cm−2 with 0.2 mAh cm−2.
A multi-cycle growth and flame annealing strategy was developed to construct textured and hierarchically porous Ti-doped hematite (tp-Fe2O3) photoanodes with enhanced charge transport and surface kinetics.
The hydrazine oxidation reaction was introduced as a fast and thermodynamically favorable alternative to the oxygen evolution reaction, enabling the simultaneous production of hydrogen and the remediation of toxic hydrazine.
The tp-Fe2O3-based bias-free photovoltaic-photoelectrochemical tandem device achieved a record solar-to-hydrogen efficiency of 8.7%, demonstrating excellent stability and scalability for sustainable solar fuel generation.
A novel coplanar structure design is proposed for floating-gate antiferroelectric field-effect transistor (FG AFeFET) demonstration with enhanced design flexibility and vertical scalability.
Multifunctionality is achieved within a single coplanar FG AFeFET via area ratio engineering, including volatile neuronal behavior, fading memory dynamics, and nonvolatile synaptic function. Systematic investigations into its detailed operating principles are conducted.
Seamless integration of a full analog reservoir computing system is demonstrated based on a unified coplanar FG AFeFET architecture, realizing satisfactory accuracies for pattern recognition tasks.
The precise tuning of magnetic nanoparticle size and spacing directly influences the alignment of intrinsic magnetic moments and magnetic domains, thereby shaping magnetic properties. However, the dynamic evolution mechanisms of magnetic domain configurations in relation to electromagnetic (EM) attenuation behavior remain poorly understood. To address this gap, a thermodynamically controlled periodic coordination strategy is proposed to achieve precise modulation of magnetic nanoparticle spacing. This approach unveils the evolution of magnetic domain configurations, progressing from individual to coupled and ultimately to crosslinked domain configurations. A unique magnetic coupling phenomenon surpasses the Snoek limit in low-frequency range, which is observed through micromagnetic simulation. The crosslinked magnetic configuration achieves effective low-frequency EM wave absorption at 3.68 GHz, encompassing nearly the entire C-band. This exceptional magnetic interaction significantly enhances radar camouflage and thermal insulation properties. Additionally, a robust gradient metamaterial design extends coverage across the full band (2-40 GHz), effectively mitigating the impact of EM pollution on human health and environment. This comprehensive study elucidates the evolution mechanisms of magnetic domain configurations, addresses gaps in dynamic magnetic modulation, and provides novel insights for the development of high-performance, low-frequency EM wave absorption materials.
Layered oxides have attracted significant attention as cathodes for sodium-ion batteries (SIBs) due to their compositional versatility and tuneable electrochemical performance. However, these materials still face challenges such as structural phase transitions, Na+/vacancy ordering, and Jahn-Teller distortion effect, resulting in severe capacity decay and sluggish ion kinetics. We develop a novel Cu/Y dual-doping strategy that leads to the formation of "Na-Y" interlayer aggregates, which act as structural pillars within alkali metal layers, enhancing structural stability and disrupting the ordered arrangement of Na+/vacancies. This disruption leads to a unique coexistence of ordered and disordered Na+/vacancy states with near-zero strain, which significantly improves Na+ diffusion kinetics. This structural innovation not only mitigates the unfavorable P2-O2 phase transition but also facilitates rapid ion transport. As a result, the doped material demonstrates exceptional electrochemical performance, including an ultra-long cycle life of 3000 cycles at 10 C and an outstanding high-rate capability of ~70 mAh g-1 at 50 C. The discovery of this novel interlayer pillar, along with its role in modulating Na⁺/vacancy arrangements, provides a fresh perspective on engineering layered oxides. It opens up promising new pathways for the structural design of advanced cathode materials toward efficient, stable, and high-rate SIBs.
High-entropy layered hydroxides (HELHs), an emerging frontier in entropy-stabilized materials derived from layered double hydroxides (LDHs), have captivated attention with their unparalleled tunability, thermodynamic stability, and electrochemical performance. The integration of the high-entropy concept into LDHs empowers HELHs to surmount the constraints of conventional materials through compositional diversity, structurally disordered configurations, and synergistic multi-element interactions. This review systematically embarks on their synthesis methodologies, functional mechanisms, and applications in energy conversion/storage and biomedicine. Advanced synthesis strategies, such as plasma-assisted hydrothermal methods, facilitate precise control over HELH architectures while supporting scalable production. HELHs demonstrate superior electrochemical performance in critical reactions, including oxygen evolution reaction, water oxidation, hydrogen evolution, and glucose electrooxidation. Future directions encompass integrating in situ characterization with simulations, leveraging machine learning for composition screening, and expanding HELHs application through interdisciplinary collaborations. This work establishes a comprehensive roadmap for advancing HELHs as next-generation multifunctional platforms for sustainable energy and biomedical technologies.
PKT-TENG woven with K-MXene/PEDOT:PSS integrated bacterial cellulose (BC) via polydimethylsiloxane (PDMS) coating (PKMPBC) macrofibers were fabricated by bridging K-MXene/PEDOT:PSS ink with aligned BC macrofibers, then dip-coated with PDMS, showing high conductivity (10.05 S cm−1), high mechanical strength (433.8 MPa) and superior Young’s modules (25.9 GPa).
PKT-TENG integrated with PKMPBC macrofiebrs shows excellent triboelectric response and stability, delivering 86.29 mW m−2 power density to power an electronic watch and capacitors.
Resistance-sensitive PKMPBC macrofibers proved the capability of recognition for diverse liquid with precisely detection and fed back multifactor behaviors.
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