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Data-Driven Discovery of Robust Materials for Photocatalytic Energy Conversion 数据驱动的光催化能量转换稳健材料的发现
IF 22.6 1区 物理与天体物理 Q1 PHYSICS, CONDENSED MATTER Pub Date : 2022-11-29 DOI: 10.1146/annurev-conmatphys-031620-100957
Arunima K. Singh, R. Gorelik, T. Biswas
The solar–to–chemical energy conversion of Earth-abundant resources like water or greenhouse gas pollutants like CO2 promises an alternate energy source that is clean, renewable, and environmentally friendly. The eventual large-scale application of such photo-based energy conversion devices can be realized through the discovery of novel photocatalytic materials that are efficient, selective, and robust. In the past decade, the Materials Genome Initiative has led to a major leap in the development of materials databases, both computational and experimental. Hundreds of photocatalysts have recently been discovered for various chemical reactions, such as water splitting and carbon dioxide reduction, employing these databases and/or data informatics, machine learning, and high-throughput computational and experimental methods. In this article, we review these data-driven photocatalyst discoveries, emphasizing the methods and techniques developed in the last few years to determine the (photo)electrochemical stability of photocatalysts, leading to the discovery of photocatalysts that remain robust and durable under operational conditions. Expected final online publication date for the Annual Review of Condensed Matter Physics, Volume 14 is March 2023. Please see http://www.annualreviews.org/page/journal/pubdates for revised estimates.
水等地球丰富资源或二氧化碳等温室气体污染物的太阳能转化为化学能有望成为清洁、可再生和环保的替代能源。这种基于光的能量转换装置的最终大规模应用可以通过发现高效、选择性和坚固的新型光催化材料来实现。在过去的十年里,材料基因组计划在计算和实验材料数据库的发展方面取得了重大飞跃。最近,利用这些数据库和/或数据信息学、机器学习以及高通量计算和实验方法,发现了数百种用于各种化学反应的光催化剂,如水分解和二氧化碳还原。在这篇文章中,我们回顾了这些数据驱动的光催化剂的发现,强调了过去几年中开发的确定光催化剂(光)电化学稳定性的方法和技术,从而发现了在操作条件下保持坚固耐用的光催化剂。《凝聚态物理学年度评论》第14卷预计最终在线出版日期为2023年3月。请参阅http://www.annualreviews.org/page/journal/pubdates用于修订估算。
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引用次数: 4
Modeling Active Colloids: From Active Brownian Particles to Hydrodynamic and Chemical Fields 模拟活性胶体:从活性布朗粒子到流体动力学和化学场
IF 22.6 1区 物理与天体物理 Q1 PHYSICS, CONDENSED MATTER Pub Date : 2022-10-20 DOI: 10.1146/annurev-conmatphys-040821-115500
A. Zöttl, H. Stark
Active colloids are self-propelled particles moving in viscous fluids by consuming fuel from their surroundings. Here, we review the numerical and theoretical modeling of active colloids propelled by self-generated near-surface flows. We start with the generic model of an active Brownian particle taking into account potential forces and effective pairwise interaction, which include hydrodynamic and phoretic interactions. Also, the squirmer as a model microswimmer is introduced. We then discuss the explicit modeling of self-generated fluid flow and the full hydrodynamic-chemical coupling. Finally, we discuss recent advances in selected topics in which modeling of active colloids is used to study motion in crowded and complex environments, microrheology in active baths, active colloidal engines, adaptive responses of active colloids with the help of machine learning techniques, as well as effects of colloid and fluid inertia. Expected final online publication date for the Annual Review of Condensed Matter Physics, Volume 14 is March 2023. Please see http://www.annualreviews.org/page/journal/pubdates for revised estimates.
活性胶体是通过消耗周围环境中的燃料在粘性流体中移动的自推进颗粒。在这里,我们回顾了由自发近表面流推动的活性胶体的数值和理论建模。我们从活性布朗粒子的一般模型开始,考虑了势能和有效的成对相互作用,包括流体动力学和电泳相互作用。此外,还介绍了蠕动器作为微型游动器的模型。然后,我们讨论了自生流体流动的显式建模和全流体动力学化学耦合。最后,我们讨论了选定主题的最新进展,其中活性胶体的建模用于研究拥挤和复杂环境中的运动、活性浴中的微流变学、活性胶体发动机、借助机器学习技术的活性胶体的自适应响应,以及胶体和流体惯性的影响。《凝聚态物理学年度评论》第14卷预计最终在线出版日期为2023年3月。请参阅http://www.annualreviews.org/page/journal/pubdates用于修订估算。
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引用次数: 15
A Journey Through Nonlinear Dynamics: The Case of Temperature Gradients 非线性动力学之旅:温度梯度的例子
IF 22.6 1区 物理与天体物理 Q1 PHYSICS, CONDENSED MATTER Pub Date : 2022-09-21 DOI: 10.1146/annurev-conmatphys-040721-023358
A. Libchaber
The overall effect of temperature gradients is stressed for the Earth's core and surface, but also for the Sun's surface. Using Rayleigh–Bénard convection in helium and mercury, we measured all of the scaling properties of the period-doubling cascade and quasiperiodicity. Hard turbulence scaling properties are presented in an experiment using helium gas at low temperature. A 2/7 scaling law is measured and also an exponential distribution for temperature fluctuations is observed. We present a study of a Rayleigh–Bénard convection cell with an open top and a floater. One of the simplest limit cycles is observed for the floater position. It follows a model proposed by Wilson for continents motion. Using the Soret effect, we study how temperature differences lead to strong accumulation of DNA suspensions. Also using polyethylene glycol concentration gradients, we measured local DNA and RNA accumulation. Finally, using thermal convection, we build one of the smallest PCR machines. Expected final online publication date for the Annual Review of Condensed Matter Physics, Volume 14 is March 2023. Please see http://www.annualreviews.org/page/journal/pubdates for revised estimates.
温度梯度的总体影响对地核和地表都很重要,对太阳表面也是如此。利用氦和汞中的Rayleigh–Bénard对流,我们测量了倍周期级联和准周期的所有标度特性。在低温氦气实验中给出了硬湍流标度特性。测量了2/7比例定律,还观察到了温度波动的指数分布。我们研究了一个具有开口顶部和浮子的瑞利-贝纳德对流单元。对于浮子位置,观察到最简单的极限循环之一。它遵循Wilson提出的大陆运动模型。利用Soret效应,我们研究了温度差异如何导致DNA悬浮液的强烈积累。同样使用聚乙二醇浓度梯度,我们测量了局部DNA和RNA的积累。最后,利用热对流,我们建造了一台最小的PCR机器。《凝聚态物理学年度评论》第14卷预计最终在线出版日期为2023年3月。请参阅http://www.annualreviews.org/page/journal/pubdates用于修订估算。
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引用次数: 1
Swimming in Complex Fluids 在复杂流体中游泳
IF 22.6 1区 物理与天体物理 Q1 PHYSICS, CONDENSED MATTER Pub Date : 2022-08-06 DOI: 10.1146/annurev-conmatphys-040821-112149
S. Spagnolie, Patrick T. Underhill
We review the literature on swimming in complex fluids. A classification is proposed by comparing the length and timescales of a swimmer with those of nearby obstacles, interpreted broadly, extending from rigid or soft confining boundaries to molecules that confer the bulk fluid with complex stresses. A third dimension in the classification is the concentration of swimmers, which incorporates fluids whose complexity arises purely by the collective motion of swimming organisms. For each of the eight system classes that we identify, we provide a background and describe modern research findings. Although some classes have seen a great deal of attention for decades, others remain uncharted waters still open and awaiting exploration. Expected final online publication date for the Annual Review of Condensed Matter Physics, Volume 14 is March 2023. Please see http://www.annualreviews.org/page/journal/pubdates for revised estimates.
我们回顾了有关在复杂流体中游泳的文献。通过将游泳者的长度和时间尺度与附近障碍物的长度和时尺度进行比较,提出了一种分类方法,从刚性或软约束边界延伸到赋予大体积流体复杂应力的分子。分类中的第三个维度是游泳者的浓度,它包含了纯粹由游泳生物体的集体运动产生的复杂流体。对于我们确定的八个系统类别中的每一个,我们都提供了背景并描述了现代研究结果。尽管几十年来,一些课程受到了极大的关注,但其他课程仍然是未知的领域,仍在等待探索。《凝聚态物理学年度评论》第14卷预计最终在线出版日期为2023年3月。请参阅http://www.annualreviews.org/page/journal/pubdates用于修订估算。
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引用次数: 8
Random Quantum Circuits 随机量子电路
IF 22.6 1区 物理与天体物理 Q1 PHYSICS, CONDENSED MATTER Pub Date : 2022-07-29 DOI: 10.1146/annurev-conmatphys-031720-030658
M. Fisher, V. Khemani, A. Nahum, S. Vijay
Quantum circuits—built from local unitary gates and local measurements—are a new playground for quantum many-body physics and a tractable setting to explore universal collective phenomena far from equilibrium. These models have shed light on longstanding questions about thermalization and chaos, and on the underlying universal dynamics of quantum information and entanglement. In addition, such models generate new sets of questions and give rise to phenomena with no traditional analog, such as dynamical phase transitions in quantum systems that are monitored by an external observer. Quantum circuit dynamics is also topical in view of experimental progress in building digital quantum simulators that allow control of precisely these ingredients. Randomness in the circuit elements allows a high level of theoretical control, with a key theme being mappings between real-time quantum dynamics and effective classical lattice models or dynamical processes. Many of the universal phenomena that can be identified in this tractable setting apply to much wider classes of more structured many-body dynamics. Expected final online publication date for the Annual Review of Condensed Matter Physics, Volume 14 is March 2023. Please see http://www.annualreviews.org/page/journal/pubdates for revised estimates.
量子电路——由局部酉门和局部测量构建——是量子多体物理学的一个新游乐场,也是探索远离平衡的普遍集体现象的一个容易处理的环境。这些模型揭示了关于热化和混沌的长期问题,以及量子信息和纠缠的潜在普遍动力学。此外,这些模型产生了一系列新的问题,并产生了没有传统模拟的现象,例如由外部观测者监测的量子系统中的动态相变。量子电路动力学也是一个热门话题,因为在构建数字量子模拟器方面取得了实验进展,可以精确控制这些成分。电路元件的随机性允许高水平的理论控制,关键主题是实时量子动力学和有效的经典晶格模型或动力学过程之间的映射。在这种易于处理的环境中可以识别的许多普遍现象适用于更广泛的结构更复杂的多体动力学。《凝聚态物理学年度评论》第14卷预计最终在线出版日期为2023年3月。请参阅http://www.annualreviews.org/page/journal/pubdates用于修订估算。
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引用次数: 119
Odd Viscosity and Odd Elasticity 奇粘度与奇弹性
IF 22.6 1区 物理与天体物理 Q1 PHYSICS, CONDENSED MATTER Pub Date : 2022-07-01 DOI: 10.1146/annurev-conmatphys-040821-125506
Michel Fruchart, C. Scheibner, V. Vitelli
Elasticity typically refers to a material's ability to store energy, whereas viscosity refers to a material's tendency to dissipate it. In this review, we discuss fluids and solids for which this is not the case. These materials display additional linear response coefficients known as odd viscosity and odd elasticity. We first introduce odd viscosity and odd elasticity from a continuum perspective, with an emphasis on their rich phenomenology, including transverse responses, modified dislocation dynamics, and topological waves. We then provide an overview of systems that display odd viscosity and odd elasticity. These systems range from quantum fluids and astrophysical gases to active and driven matter. Finally, we comment on microscopic mechanisms by which odd viscosity and odd elasticity arise.
弹性通常是指材料储存能量的能力,而粘度是指材料耗散能量的倾向。在这篇综述中,我们讨论的流体和固体不是这种情况。这些材料显示出额外的线性响应系数,称为奇粘度和奇弹性。我们首先从连续介质的角度介绍了奇粘度和奇弹性,重点介绍了它们丰富的现象学,包括横向响应、修正位错动力学和拓扑波。然后,我们提供了一个系统的概述,显示奇数粘度和奇数弹性。这些系统的范围从量子流体和天体物理气体到活性和驱动物质。最后,我们评论了奇粘和奇弹性产生的微观机制。
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引用次数: 42
Quantum Many-Body Scars: A Quasiparticle Perspective 量子多体伤痕:准粒子视角
IF 22.6 1区 物理与天体物理 Q1 PHYSICS, CONDENSED MATTER Pub Date : 2022-06-23 DOI: 10.1146/annurev-conmatphys-031620-101617
A. Chandran, Thomas Iadecola, V. Khemani, R. Moessner
Weakly interacting quasiparticles play a central role in the low-energy description of many phases of quantum matter. At higher energies, however, quasiparticles cease to be well defined in generic many-body systems owing to a proliferation of decay channels. In this review, we discuss the phenomenon of quantum many-body scars, which can give rise to certain species of stable quasiparticles throughout the energy spectrum. This goes along with a set of unusual nonequilibrium phenomena including many-body revivals and nonthermal stationary states. We provide a pedagogical exposition of this physics via a simple yet comprehensive example, that of a spin-1 XY model. We place our discussion in the broader context of symmetry-based constructions of many-body scar states, projector embeddings, and Hilbert space fragmentation. We conclude with a summary of experimental progress and theoretical puzzles. Expected final online publication date for the Annual Review of Condensed Matter Physics, Volume 14 is March 2023. Please see http://www.annualreviews.org/page/journal/pubdates for revised estimates.
弱相互作用的准粒子在量子物质许多相的低能描述中起着核心作用。然而,在更高的能量下,由于衰变通道的扩散,准粒子在一般的多体系统中不再有很好的定义。在这篇综述中,我们讨论了量子多体伤痕现象,它可以在整个能谱中产生某些种类的稳定准粒子。这伴随着一系列不同寻常的非平衡现象,包括许多天体复活和非热稳态。我们通过一个简单而全面的例子,即自旋-1 XY模型,对这种物理学进行了教学阐述。我们将我们的讨论放在更广泛的背景下,即许多身体疤痕状态的基于对称的构造、投影嵌入和希尔伯特空间碎片。最后,我们总结了实验进展和理论困惑。《凝聚态物理学年度评论》第14卷预计最终在线出版日期为2023年3月。请参阅http://www.annualreviews.org/page/journal/pubdates用于修订估算。
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引用次数: 68
Learning Without Neurons in Physical Systems 物理系统中没有神经元的学习
IF 22.6 1区 物理与天体物理 Q1 PHYSICS, CONDENSED MATTER Pub Date : 2022-06-13 DOI: 10.1146/annurev-conmatphys-040821-113439
M. Stern, A. Murugan
Learning is traditionally studied in biological or computational systems. The power of learning frameworks in solving hard inverse problems provides an appealing case for the development of physical learning in which physical systems adopt desirable properties on their own without computational design. It was recently realized that large classes of physical systems can physically learn through local learning rules, autonomously adapting their parameters in response to observed examples of use. We review recent work in the emerging field of physical learning, describing theoretical and experimental advances in areas ranging from molecular self-assembly to flow networks and mechanical materials. Physical learning machines provide multiple practical advantages over computer designed ones, in particular by not requiring an accurate model of the system, and their ability to autonomously adapt to changing needs over time. As theoretical constructs, physical learning machines afford a novel perspective on how physical constraints modify abstract learning theory.
学习传统上是在生物或计算系统中研究的。学习框架在解决难逆问题方面的力量为物理学习的发展提供了一个吸引人的案例,在物理学习中,物理系统在没有计算设计的情况下自行采用理想的属性。最近人们意识到,大型物理系统可以通过局部学习规则进行物理学习,根据观察到的使用示例自主调整其参数。我们回顾了最近在新兴物理学习领域的工作,描述了从分子自组装到流动网络和机械材料等领域的理论和实验进展。与计算机设计的机器相比,物理学习机器提供了许多实际优势,特别是不需要系统的精确模型,并且它们能够随着时间的推移自主适应不断变化的需求。作为理论建构,物理学习机提供了物理约束如何修改抽象学习理论的新视角。
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引用次数: 20
Non-Hermitian Topological Phenomena: A Review 非厄米拓扑现象:综述
IF 22.6 1区 物理与天体物理 Q1 PHYSICS, CONDENSED MATTER Pub Date : 2022-05-21 DOI: 10.1146/annurev-conmatphys-040521-033133
N. Okuma, Masatoshi Sato
The past decades have witnessed an explosion of interest in topological materials, and a lot of mathematical concepts have been introduced in condensed matter physics. Among them, the bulk-boundary correspondence is the central topic in topological physics, which has inspired researchers to focus on boundary physics. Recently, the concepts of topological phases have been extended to non-Hermitian Hamiltonians, whose eigenvalues can be complex. Besides the topology, non-Hermiticity can also cause a boundary phenomenon called the non-Hermitian skin effect, which is an extreme sensitivity of the spectrum to the boundary condition. In this article, we review developments in non-Hermitian topological physics by focusing mainly on the boundary problem. As well as the competition between non-Hermitian and topological boundary phenomena, we discuss the topological nature inherent in non-Hermiticity itself. Expected final online publication date for the Annual Review of Condensed Matter Physics, Volume 14 is March 2023. Please see http://www.annualreviews.org/page/journal/pubdates for revised estimates.
在过去的几十年里,人们对拓扑材料的兴趣激增,在凝聚态物理学中引入了许多数学概念。其中,体边界对应关系是拓扑物理学的核心课题,激发了研究者对边界物理学的关注。最近,拓扑相位的概念已经推广到非埃尔米特哈密顿,其特征值可以是复数。除了拓扑之外,非埃尔米特性还可以引起一种称为非埃尔米特皮肤效应的边界现象,这是频谱对边界条件的极端敏感。在这篇文章中,我们通过主要关注边界问题来回顾非埃尔米特拓扑物理学的发展。除了非埃尔米特现象和拓扑边界现象之间的竞争外,我们还讨论了非埃尔米特本身固有的拓扑性质。《凝聚态物理学年度评论》第14卷预计最终在线出版日期为2023年3月。请参阅http://www.annualreviews.org/page/journal/pubdates用于修订估算。
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引用次数: 104
Spin Seebeck Effect: Sensitive Probe for Elementary Excitation, Spin Correlation, Transport, Magnetic Order, and Domains in Solids 自旋塞贝克效应:固体中初等激发、自旋相关、输运、磁序和畴的敏感探针
IF 22.6 1区 物理与天体物理 Q1 PHYSICS, CONDENSED MATTER Pub Date : 2022-05-21 DOI: 10.1146/annurev-conmatphys-040721-014957
T. Kikkawa, E. Saitoh
The spin Seebeck effect (SSE) refers to the generation of a spin current as a result of a temperature gradient in a magnetic material, which can be detected electrically via the inverse spin Hall effect in a metallic contact. Since the discovery of SSE in 2008, intensive studies on the SSE have been conducted to elucidate its origin. SSEs appear in a wide range of magnetic materials including ferro-, ferri-, and antiferromagnets and also paramagnets with classical or quantum spin fluctuation. SSE voltage reflects fundamental properties of a magnet, such as elementary excitation, static magnetic order, spin correlation, and spin transport. In this article, we review recent progress on the SSEs in various systems, with particular emphasis on its emerging role as a probe of these magnetic properties in solids. We also briefly discuss the recently discovered nuclear SSE. Expected final online publication date for the Annual Review of Condensed Matter Physics, Volume 14 is March 2023. Please see http://www.annualreviews.org/page/journal/pubdates for revised estimates.
自旋塞贝克效应(SSE)是指由于磁性材料中的温度梯度而产生的自旋电流,可以通过金属接触中的反向自旋霍尔效应进行电检测。自2008年发现SSE以来,人们对SSE进行了深入的研究,以阐明其起源。SSE出现在广泛的磁性材料中,包括铁磁体、铁磁体和反铁磁体,以及具有经典或量子自旋波动的顺磁体。SSE电压反映了磁体的基本特性,如基本激发、静态磁序、自旋相关和自旋输运。在这篇文章中,我们回顾了SSE在各种系统中的最新进展,特别强调了它作为固体中这些磁性性质的探针的新兴作用。我们还简要讨论了最近发现的核SSE。《凝聚态物理学年度评论》第14卷预计最终在线出版日期为2023年3月。请参阅http://www.annualreviews.org/page/journal/pubdates用于修订估算。
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引用次数: 14
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Annual Review of Condensed Matter Physics
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