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Ferroelectric and ferroionic multifunctional quantum sensors: Incursion into applications 铁电和铁离子多功能量子传感器:进入应用领域
IF 15 1区 物理与天体物理 Q1 PHYSICS, APPLIED Pub Date : 2026-01-09 DOI: 10.1063/5.0251263
Beatriz M. Gomes, Tomás Prior, Ângela Freitas, António B. Vale, Beatriz A. Maia, Hugo Lebre, Manuela C. Baptista, Raquel Dantas, M. Helena Braga
Ferroelectric materials are poised to drive the next technological leap through their emergent functionalities, including negative capacitance and resistance, charge accumulation without transport, and spontaneous polarization switching. The discovery of ferroionic material-systems that combine room-temperature ferroelectricity and fast ionic conductivity has opened an unprecedented avenue for multifunctional devices that merge the territories of electronics and ionics. These hybrid materials enable the direct coupling of ionic and electronic order parameters, allowing long-range electrostatic interactions, wireless field communication, and energy transduction across solid–solid and solid–air interfaces. Such capabilities offer potential solutions to long-standing challenges, including the Boltzmann limit in transistor subthreshold operation, voltage amplification without power dissipation, and nonvolatile polarization states with ionic reconfigurability. Beyond conventional applications, ferroionics support a new generation of quantum sensors and adaptive devices, spanning optical, electrical, mechanical, thermal, and magnetic domains. This review provides a comprehensive overview of the conceptual foundations, theoretical frameworks, and experimental progress underlying ferroionic systems, highlighting their role as a bridge between ferroelectrics, solid electrolytes, and correlated quantum materials. Finally, perspectives are offered on how ferroionic coupling may reshape device physics and enable sustainable, self-powered information and energy technologies.
铁电材料有望通过其新兴功能推动下一个技术飞跃,包括负电容和电阻、无输运的电荷积累和自发极化开关。铁离子材料系统的发现结合了室温铁电性和快速离子电导率,为融合电子和离子领域的多功能设备开辟了前所未有的途径。这些杂化材料能够实现离子和电子序参数的直接耦合,从而实现远距离静电相互作用、无线场通信和跨越固体-固体和固体-空气界面的能量转导。这种能力为长期存在的挑战提供了潜在的解决方案,包括晶体管亚阈值操作中的玻尔兹曼极限,无功耗的电压放大,以及具有离子可重构性的非易失性极化状态。除了传统应用之外,铁离子支持新一代量子传感器和自适应设备,跨越光学,电气,机械,热和磁领域。本文综述了铁离子系统的概念基础、理论框架和实验进展,重点介绍了铁电体、固体电解质和相关量子材料之间的桥梁作用。最后,提出了铁离子耦合如何重塑设备物理并实现可持续、自供电的信息和能源技术的观点。
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引用次数: 0
Quantum sensing with cavity optomechanics 基于腔光力学的量子传感
IF 15 1区 物理与天体物理 Q1 PHYSICS, APPLIED Pub Date : 2026-01-09 DOI: 10.1063/5.0237048
Zeng-Xing Liu, Xiao-Jie Zuo, Jia-Xin Peng, Hao Xiong
Quantum sensing, leveraging the principles of quantum mechanics, has revolutionized the field of precision measurement by achieving sensitivities beyond the classical limits. Among the various platforms for quantum sensing, cavity optomechanics has emerged as a particularly promising field. It studies the interaction between light and mechanical resonators within high-Q optical cavities, providing unique opportunities for enhancing measurement precision and sensitivity in quantum sensing. With advancements in technology, the range of applications for cavity optomechanics in quantum sensing is expanding rapidly. Particularly, the integration of optoelectronic technologies and miniaturization techniques holds promise for the development of more compact, efficient, and scalable quantum sensors. Quantum sensing with cavity optomechanics has been extensively studied and has progressed enormously over the past decades. This paper provides a systematic review of research on quantum sensing with cavity optomechanics, starting from the fundamental principles of optomechanical coupling, to the achievement of quantum ground-state cooling of mechanical oscillators and the preparation of basic quantum states, and then to the mechanisms of quantum sensing based on cavity optomechanics. Furthermore, we survey recent advancements in quantum sensing utilizing cavity optomechanics, including the enhancement of optomechanical sensing through the use of entanglement, squeezing, and quantum exceptional points. Finally, perspectives and opportunities for future developments of this field are provided.
量子传感利用量子力学原理,通过实现超越经典极限的灵敏度,彻底改变了精密测量领域。在各种量子传感平台中,腔光力学已成为一个特别有前途的领域。它研究了高q光腔内光与机械谐振器之间的相互作用,为提高量子传感的测量精度和灵敏度提供了独特的机会。随着技术的进步,腔光力学在量子传感中的应用范围正在迅速扩大。特别是,光电技术和小型化技术的集成为开发更紧凑、高效和可扩展的量子传感器带来了希望。近几十年来,基于腔光力学的量子传感技术得到了广泛的研究,并取得了巨大的进展。本文从光力学耦合的基本原理,到机械振子的量子基态冷却的实现和基本量子态的制备,再到基于腔光力学的量子传感机理,对腔光力学的量子传感研究进行了系统的综述。此外,我们调查了利用腔光力学的量子传感的最新进展,包括通过使用纠缠、挤压和量子异常点来增强光力学传感。最后,对该领域的未来发展提出了展望和机遇。
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引用次数: 0
Triplet-mediated waveguiding and energy transfer in organic phosphors on cellulose 纤维素上有机荧光粉的三重介质波导和能量传递
IF 15 1区 物理与天体物理 Q1 PHYSICS, APPLIED Pub Date : 2026-01-02 DOI: 10.1063/5.0302351
Seokho Kim, Jiyoun Kim, Jiyoung Boo, Junsung Lee, Bo Hyun Kim, Bong Sup Shim, Jinho Choi, Dong Hyuk Park, Healin Im
Purely organic emitters can generate long-lived phosphorescence at room temperature. With their extremely low toxicity and environmentally friendly processes, their extended emissive decay, often lasting several milliseconds, combined with high quantum yields makes them promising for a range of emission and sensory platforms. Room temperature phosphorescence (RTP) is highly dependent on both the crystallinity and geometry of organic crystals, which are significantly influenced by the surrounding environments. Key factors include organic solvents in which organic emitters are dissolved or dispersed, the surface properties where the organic crystal is grown, and nearby adjacent emitters. This work presents a strategy for forming nanorod-shaped purely organic chromophores that exhibit RTP through hybridization with host molecules on an eco-friendly cellulose membrane. Tuning the crystal morphology significantly influences the photophysical properties and enhances phosphorescence efficiency while enabling waveguided emission along a one-dimensional geometry. Finally, to exploit the ultralong phosphorescent lifetime in the millisecond regime, phosphorescence resonance energy transfer was achieved by coupling with Rhodamine B, an organic fluorophore, highlighting the potential for tunable emission through the formation of an amorphous interface at the contact region.
纯有机发射体可以在室温下产生长寿命的磷光。由于其极低的毒性和对环境友好的过程,其延长的发射衰变通常持续几毫秒,再加上高量子产率,使它们有望用于一系列发射和感官平台。室温磷光(RTP)高度依赖于有机晶体的结晶度和几何形状,而晶体的结晶度和几何形状又受周围环境的显著影响。关键因素包括溶解或分散有机发射体的有机溶剂、生长有机晶体的表面性质以及附近邻近的发射体。这项工作提出了一种通过与生态友好型纤维素膜上的宿主分子杂交形成纳米棒状纯有机发色团的策略。调整晶体形态显著影响光物理性质,提高磷光效率,同时实现沿一维几何形状的波导发射。最后,为了利用毫秒级的超长磷光寿命,通过与罗丹明B(一种有机荧光团)耦合实现磷光共振能量转移,突出了通过在接触区域形成无定形界面而可调谐发射的潜力。
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引用次数: 0
Effect of polarization Coulomb field scattering on GaN devices 极化库仑场散射对GaN器件的影响
IF 15 1区 物理与天体物理 Q1 PHYSICS, APPLIED Pub Date : 2026-01-02 DOI: 10.1063/5.0273085
Zhaojun Lin, Heng Zhou, Yuanjie Lv, Peng Cui, Mingyan Wang, Chongbiao Luan, Jianzhi Zhao, Ming Yang, Chen Fu
We present a comprehensive review and analysis of the polarization Coulomb field (PCF) scattering theory in GaN heterostructure field-effect transistors (GaN HFETs), which include AlGaN/GaN HFETs and InAlN/GaN HFETs. This paper develops a theoretical framework for understanding PCF scattering in GaN HFETs and explores its application in various areas, including device modeling, channel electron velocity modulation, circuit performance optimization, and the analysis of split-gate AlGaN/GaN HFETs. Additionally, we investigate the potential applications of PCF scattering theory in polar dielectric semiconductor devices and underscore its broader scientific significance.
本文对氮化镓异质结构场效应晶体管(GaN hfet)中的极化库仑场(PCF)散射理论进行了全面的综述和分析,包括AlGaN/GaN hfet和InAlN/GaN hfet。本文建立了理解GaN hfet中PCF散射的理论框架,并探讨了其在器件建模、通道电子速度调制、电路性能优化以及分栅AlGaN/GaN hfet分析等各个领域的应用。此外,我们还研究了PCF散射理论在极性介电半导体器件中的潜在应用,并强调了其更广泛的科学意义。
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引用次数: 0
Programmable magnetized pillars enabled self-powered, single-channel and identity identifiable handwritten e-skin 可编程磁化柱使自供电,单通道和身份识别手写电子皮肤
IF 15 1区 物理与天体物理 Q1 PHYSICS, APPLIED Pub Date : 2026-01-02 DOI: 10.1063/5.0301455
Qian Zhou, Yongchao Li, Yiwei Wang, Hui Zhou, Pei He, Bing Ji, Bingpu Zhou, Junliang Yang
Human–machine interaction (HMI) interfaces capable of conveniently transmitting massive human-made information and conversely recognizing the identity (ID) of individuals are highly desired while remaining challenging. Herein, a programmable self-powered handwritten e-skin consisted of soft magnetized pillars (MPs) and an underneath flexible coil electrode for convenient, efficient and ID identifiable HMI applications is presented. With the built-in magnetic moment alignment, the deflection and elastic recovery (ER) of the soft MPs triggered by sliding operations can induce the sequential generation of sliding-adaptive negative voltage signals and fixed ER-induced positive voltage signals. The sliding-adaptive signals can originally serve as the bio-mechanical information of individuals to recognize the habit-related sliding speeds for ID identification. The sliding-irrelevant ER-induced signals can be further programmed into a variety of non-overlapping levels by customizing the MPs with different elastic and magnetic properties. Such programmable non-overlapping ER-induced signals not only ensure the capability of encoding massive information, but also endow the function of single-channel addressing of the e-skin. With these distinctive features, the potential applications of high-capacity commands output for game character controlling, single-channel handwritten transmission of alphabet information, and password/ID dual decoding (with an average accuracy rate of 99.5%) are successfully demonstrated.
人机交互(HMI)界面能够方便地传输大量的人造信息,并反过来识别个人的身份(ID),这是非常需要的,但仍然具有挑战性。本文提出了一种可编程的自供电手写电子皮肤,该电子皮肤由软磁柱(MPs)和下方柔性线圈电极组成,用于方便,高效和ID可识别的HMI应用。通过内置磁矩对准,滑动操作触发软MPs的挠曲和弹性恢复(ER)可以诱导顺序产生滑动自适应负电压信号和固定ER诱导的正电压信号。滑动自适应信号可以作为个体的生物力学信息,识别与习惯相关的滑动速度,用于身份识别。通过定制具有不同弹性和磁性质的MPs,可以将与滑动无关的er诱导信号进一步编程为各种不重叠的电平。这种可编程的无重叠er诱导信号不仅保证了海量信息的编码能力,而且赋予了电子皮肤的单通道寻址功能。在此基础上,成功展示了游戏角色控制大容量命令输出、字母信息单通道手写传输、密码/ID双解码(平均准确率99.5%)的潜在应用。
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引用次数: 0
Advances in fluorescence lifetime imaging microscopy: Techniques and biomedical applications 荧光寿命成像显微镜的研究进展:技术和生物医学应用
IF 15 1区 物理与天体物理 Q1 PHYSICS, APPLIED Pub Date : 2026-01-02 DOI: 10.1063/5.0300853
Fangrui Lin, Chenshuang Zhang, Zhenlong Huang, Yiqiang Wang, Min Yi, Jia Li, Xiaoyu Weng, Yu Chen, Puxiang Lai, Junle Qu
Fluorescence lifetime imaging microscopy (FLIM) has emerged as a powerful biomedical imaging technique for the quantitative visualization of intricate molecular and cellular processes. Significant advancements in photonics, sensor technology, data acquisition systems, and computational algorithms have substantially improved the spatiotemporal resolution, imaging depth, and analytical throughput of FLIM. These developments have diversified FLIM methodologies, including time-domain techniques such as time-correlated single-photon counting (TCSPC), time-gated detection, streak cameras, and direct pulse-recording systems, as well as frequency-domain approaches. Concurrently, FLIM has been successfully integrated with advanced imaging modalities, such as multiphoton microscopy, light-sheet imaging, and endoscopy. This review provides a comprehensive synthesis of advanced FLIM technologies. We present in-depth discussions on the principles of lifetime quantification, recent innovations in hardware and algorithms for lifetime recovery, and state-of-the-art strategies to accelerate imaging speed while maintaining resolution and sensitivity. Moreover, we explore FLIM's unique capability to investigate dynamic metabolic states through endogenous autofluorescent cofactors, quantify physicochemical parameters of the cellular microenvironment (e.g., pH, polarity, viscosity, and ion concentrations), and facilitate the diagnosis of diseases such as cancer and neurodegeneration. Finally, we discuss future directions for FLIM development, including integration with deep learning, miniaturized hardware for point-of-care applications, and real-time clinical translation. Collectively, this review aims to provide researchers, clinicians, and engineers with both fundamental knowledge and forward-looking perspectives to further unlock the potential of FLIM in advancing biomedical science.
荧光寿命成像显微镜(FLIM)已成为一种强大的生物医学成像技术,用于复杂的分子和细胞过程的定量可视化。光子学、传感器技术、数据采集系统和计算算法的重大进步大大提高了FLIM的时空分辨率、成像深度和分析吞吐量。这些发展使FLIM方法多样化,包括时域技术,如时间相关单光子计数(TCSPC)、时间门控检测、条纹相机和直接脉冲记录系统,以及频域方法。同时,FLIM已经成功地集成了先进的成像模式,如多光子显微镜、光片成像和内窥镜。本文综述了先进的FLIM技术的全面综合。我们深入讨论了生命周期量化的原理,生命周期恢复的硬件和算法的最新创新,以及在保持分辨率和灵敏度的同时加快成像速度的最先进策略。此外,我们还探索了FLIM通过内源性自荧光辅助因子研究动态代谢状态的独特能力,量化细胞微环境的理化参数(如pH、极性、粘度和离子浓度),并促进癌症和神经变性等疾病的诊断。最后,我们讨论了FLIM发展的未来方向,包括与深度学习的集成,用于护理点应用的小型化硬件,以及实时临床翻译。总的来说,这篇综述旨在为研究人员、临床医生和工程师提供基础知识和前瞻性观点,以进一步释放FLIM在推进生物医学科学方面的潜力。
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引用次数: 0
Topological insulator materials for optics: Research progress and prospects 光学用拓扑绝缘体材料:研究进展与展望
IF 15 1区 物理与天体物理 Q1 PHYSICS, APPLIED Pub Date : 2026-01-02 DOI: 10.1063/5.0271855
Xin Li, Hua Lu, Runze Li, Zhengfen Wan, Xiaolin Wang, Salvatore Macis, Stefano Lupi, Min Gu, Hongxia Wang, Zengji Yue
Topological insulators (TIs) are emerging quantum materials with insulating bulk and topologically protected metallic surface states. The electrons in the surface state are massless Dirac fermions with full spin polarization and are protected from backscattering. Due to this unique electronic structure, they exhibit novel optoelectronic properties and a variety of quantum effects. These distinctive properties make TIs potential candidates for applications in low-energy-consumption electronic devices, quantum computing, and low-loss optoelectronic devices. The unique optical properties of TIs have advanced considerably the development of plasmon-enhanced photovoltaic devices, ultrathin holograms, optical angular momentum nanometrology, and planar lenses. These developments underscore how TIs are setting new benchmarks in the optoelectronic domain and demonstrate the broad applicability of these materials. This comprehensive overview of recent progress in the field of TI optics emphasizes the wide range of applications of various compounds and showcases their exceptional performance. We introduce the optical properties of TIs and explore the performances of many devices based on these materials. On the latter subject, we discuss the innovative structures on which they are based, highlight potential directions for experimental innovations and device development, and consider their significance in both fundamental research and practical applications.
拓扑绝缘体是一种具有绝缘体和拓扑保护金属表面态的新型量子材料。表面态的电子是具有全自旋极化的无质量狄拉克费米子,并且不受后向散射的影响。由于这种独特的电子结构,它们表现出新的光电特性和各种量子效应。这些独特的特性使其成为低能耗电子器件、量子计算和低损耗光电器件应用的潜在候选者。ti独特的光学特性极大地推动了等离子体增强光伏器件、超薄全息、光学角动量纳米测量和平面透镜的发展。这些发展强调了ti如何在光电领域设定新的基准,并证明了这些材料的广泛适用性。这全面概述了TI光学领域的最新进展,强调了各种化合物的广泛应用,并展示了它们的卓越性能。我们介绍了ti的光学特性,并探讨了基于这些材料的许多器件的性能。关于后者,我们讨论了它们所基于的创新结构,强调了实验创新和器件开发的潜在方向,并考虑了它们在基础研究和实际应用中的意义。
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引用次数: 0
Quantum sensing using atomic clocks for nuclear and particle physics 核物理和粒子物理中使用原子钟的量子传感
IF 15 1区 物理与天体物理 Q1 PHYSICS, APPLIED Pub Date : 2025-12-30 DOI: 10.1063/5.0273813
Akio Kawasaki
Technologies for manipulating single atoms have advanced drastically in the past decades. Due to their excellent controllability of internal states, atoms serve as one of the ideal platforms for quantum systems. One major research direction in atomic systems is the precise determination of physical quantities using atoms, which is included in the field of precision measurements. One of such precisely measured physical quantities is the energy differences between two energy levels in atoms, which is symbolized by the remarkable fractional uncertainty of 10−18 or lower achieved in the state-of-the-art atomic clocks. Two-level systems in atoms are sensitive to various external fields and can, therefore, function as quantum sensors. The effect of these fields manifests as energy shifts in the two-level system. Traditionally, such shifts are induced by electric or magnetic fields, as recognized even before the advent of precision spectroscopy with lasers. With high-precision measurements, tiny energy shifts caused by hypothetical fields weakly coupled to ordinary matter or by small effects mediated by massive particles can be potentially detectable, which are conventionally dealt with in the field of nuclear and particle physics. In most cases, the atomic systems as quantum sensors have not been sensitive enough to detect such effects. Instead, experiments searching for these interactions have placed constraints on coupling constants, except in a few cases where the effects are predicted by the Standard Model of particle physics. Nonetheless, measurements and searches for these effects in atomic systems have led to the emergence of a new field of physics. In some cases, they open new parameter spaces to explore in conventionally investigated topics, e.g., dark matter, fifth force, and other physics beyond the Standard Model. In other cases, these measurements provide alternative experimental approaches to established topics, e.g., variations of fundamental constants searched for astronomically and nuclear structure studied in high-energy scattering experiments. The use of atomic clocks as quantum sensors for phenomena originating from nuclear and particle physics evolved significantly in the past decades. This paper highlights the recent developments in the field.
操纵单个原子的技术在过去几十年里取得了巨大的进步。由于原子具有优异的内部状态可控性,是量子系统的理想平台之一。原子系统的一个主要研究方向是利用原子精确测定物理量,这属于精密测量领域。这种精确测量的物理量之一是原子中两个能级之间的能量差,这是由最先进的原子钟所达到的10−18或更低的显著分数不确定度来表示的。原子中的二能级系统对各种外部场都很敏感,因此可以作为量子传感器。这些场的影响表现为两能级系统中的能量转移。传统上,这种变化是由电场或磁场引起的,甚至在激光精密光谱学出现之前就已经认识到这一点。通过高精度测量,由与普通物质弱耦合的假想场或由大质量粒子介导的小效应引起的微小能量转移可以被潜在地探测到,这通常是在核物理和粒子物理领域处理的。在大多数情况下,作为量子传感器的原子系统还不够灵敏,无法探测到这种效应。相反,寻找这些相互作用的实验对耦合常数施加了限制,除了粒子物理学标准模型预测的几种情况。尽管如此,在原子系统中对这些效应的测量和研究已经导致了一个新的物理学领域的出现。在某些情况下,它们开辟了新的参数空间来探索传统研究的主题,例如暗物质、第五力和其他超出标准模型的物理。在其他情况下,这些测量为既定主题提供了替代的实验方法,例如,在高能散射实验中为天文和核结构研究而寻找的基本常数的变化。在过去的几十年里,原子钟作为源自核物理和粒子物理现象的量子传感器的使用取得了重大进展。本文重点介绍了该领域的最新进展。
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引用次数: 0
Atomic layer deposition (ALD) of passivating, carrier-selective oxides for silicon photovoltaics 用于硅光电器件的钝化、载流子选择性氧化物的原子层沉积(ALD)
IF 15 1区 物理与天体物理 Q1 PHYSICS, APPLIED Pub Date : 2025-12-29 DOI: 10.1063/5.0275420
Chien-Hsuan Chen, Gouri Syamala Rao Mullapudi, Kristopher O. Davis, Parag Banerjee
Crystalline silicon (c-Si) photovoltaics dominate the solar industry, yet further advancements hinge on passivating and carrier-selective contacts to overcome efficiency limitations. This review explores the pivotal role of atomic layer deposition (ALD) in enabling metal oxide films for high-performance c-Si solar cells, bridging material innovation with industrial scalability. Historically, ALD-grown Al2O3 enabled the effective passivation of p-type Si surfaces via its high negative fixed charge, which made localized rear contacts viable and facilitated the transition from aluminum back surface field to passivated emitter rear contact architectures, ultimately lowering J0 and boosting efficiency. However, emerging carrier-selective contacts demand materials that simultaneously minimize recombination and resistive losses while avoiding parasitic absorption. Metal oxides, leveraging tunable optoelectronic properties and ALD's atomic-scale precision, offer a promising alternative to conventional silicon-based films (e.g., a-Si:H and poly-Si). We analyzed 373 studies to map trends in ALD metal oxide applications, highlighting the dominance of Al2O3 and TiO2, alongside growing interest in multi-metal oxides. The review underscores ALD's unique ability to tailor chemical and field-effect passivation mechanisms while addressing challenges in stoichiometric control and interfacial engineering. Targeting both ALD specialists and PV engineers, we propose standardized metrics for evaluating passivating contacts, aiming to accelerate cross-disciplinary innovation. Finally, we outline future opportunities for ALD-derived metal oxide in next-generation photovoltaics, including tandem and thin-film technologies, advocating for systematic research to unlock their full potential.
晶体硅(c-Si)光伏电池在太阳能产业中占据主导地位,但进一步的发展取决于钝化和载流子选择性接触来克服效率限制。这篇综述探讨了原子层沉积(ALD)在高性能c-Si太阳能电池的金属氧化物膜中的关键作用,将材料创新与工业可扩展性联系起来。从历史上看,ald生长的Al2O3通过其高负电荷能够有效地钝化p型Si表面,这使得局部后触点可行,并促进了从铝后表面场到钝化发射极后触点结构的转变,最终降低了J0并提高了效率。然而,新兴的载流子选择性触点要求材料同时最小化重组和电阻损失,同时避免寄生吸收。金属氧化物,利用可调谐的光电特性和ALD的原子尺度精度,为传统的硅基薄膜(例如,a- si:H和多晶硅)提供了一个有前途的替代品。我们分析了373项研究,绘制了ALD金属氧化物应用的趋势图,突出了Al2O3和TiO2的主导地位,以及对多金属氧化物的兴趣日益增长。该综述强调了ALD在解决化学计量控制和界面工程方面的挑战时,定制化学和场效应钝化机制的独特能力。针对ALD专家和光伏工程师,我们提出了评估钝化接触的标准化指标,旨在加速跨学科创新。最后,我们概述了下一代光伏电池中ald衍生金属氧化物的未来机会,包括串联和薄膜技术,倡导系统研究以释放其全部潜力。
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引用次数: 0
Stable multi-level quantum conductance in an optically tunable ITO/MoS2-Ag/Pt memristor 光学可调谐ITO/MoS2-Ag/Pt记忆电阻器中稳定的多层量子电导
IF 15 1区 物理与天体物理 Q1 PHYSICS, APPLIED Pub Date : 2025-12-24 DOI: 10.1063/5.0296500
Yuyang Zhang, Kang'an Jiang, Anhua Dong, Ke Chang, Xian-Min Jin, Hui Wang
While classical memristors demonstrate reliable binary switching, multi-level states remain constrained by scalability and mechanism variability. Quantum conductance memristors, with discrete quantized conductance steps, offer a promising alternative. However, achieving stable quantized states requires precise atomic-scale filament control and quantum state stability, posing even greater challenges. Here, we address these challenges by constructing a multilayer MoS2/MoS2:Ag structure that stably yields previously elusive conductance steps. Combined with a non-reset voltage scanning method and supported by a scattering center model, our approach markedly improves reproducibility. Moreover, we observe light-induced half-integer conductance states in a non-magnetic system. Such phenomena, previously reported only in oxygen-vacancy-based devices, are here realized for the first time in a cation-migration-based quantum conductance memristor. This arises from the strong photoresponse of MoS2 and the offset between the Ag work function and the MoS2 conduction band minimum, which together enable spin-selective transport. This finding surpasses classical multi-level limits and opens new paths for optoelectronic quantum conductance control.
虽然经典的忆阻器表现出可靠的二进制开关,但多级状态仍然受到可扩展性和机制可变性的限制。具有离散量子化电导步骤的量子电导忆阻器提供了一个有希望的替代方案。然而,实现稳定的量子化状态需要精确的原子尺度灯丝控制和量子态稳定性,这带来了更大的挑战。在这里,我们通过构建多层MoS2/MoS2:Ag结构来解决这些挑战,该结构稳定地产生以前难以捉摸的电导步骤。结合非复位电压扫描方法,在散射中心模型的支持下,我们的方法显著提高了再现性。此外,我们在非磁性系统中观察到光诱导的半整数电导态。这种现象以前只在基于氧空位的器件中报道过,现在首次在基于阳离子迁移的量子电导忆阻器中实现。这是由于MoS2的强光响应和银功函数与MoS2导带最小值之间的偏移,这两者共同使自旋选择性输运成为可能。这一发现超越了经典的多级限制,为光电量子电导控制开辟了新的途径。
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引用次数: 0
期刊
Applied physics reviews
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