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Wafer-scale synthesis of two-dimensional materials for integrated electronics 晶圆级合成二维集成电子材料
Pub Date : 2024-03-01 DOI: 10.1016/j.chip.2023.100080
Zijia Liu , Xunguo Gong , Jinran Cheng , Lei Shao , Chunshui Wang , Jian Jiang , Ruiqing Cheng , Jun He

Two-dimensional (2D) van der Waals materials have attracted great interest and facilitated the development of post-Moore electronics owing to their novel physical properties and high compatibility with traditional microfabrication techniques. Their wafer-scale synthesis has become a critical challenge for large-scale integrated applications. Although the wafer-scale synthesis approaches for some 2D materials have been extensively explored, the preparation of high-quality thin films with well-controlled thickness remains a big challenge. This review focuses on the wafer-scale synthesis of 2D materials and their applications in integrated electronics. Firstly, several representative 2D layered materials including their crystal structures and unique electronic properties were introduced. Then, the current synthesis strategies of 2D layered materials at the wafer scale, which are divided into “top-down” and “bottom-up”, were reviewed in depth. Afterwards, the applications of 2D materials wafer in integrated electrical and optoelectronic devices were discussed. Finally, the current challenges and future prospects for 2D integrated electronics were presented. It is hoped that this review will provide comprehensive and insightful guidance for the development of wafer-scale 2D materials and their integrated applications.

二维(2D)范德华材料因其新颖的物理性质和与传统微加工技术的高度兼容性而备受后摩尔电子技术发展的关注。二维范德华材料的晶圆级合成已成为大规模集成应用的关键挑战。尽管一些二维材料的晶圆级合成方法已得到广泛探索,但如何制备厚度控制良好的高质量薄膜仍是一大挑战。本综述重点介绍二维材料的晶圆级合成及其在集成电子学中的应用。首先,我们介绍了几种具有代表性的二维层状材料,包括它们的晶体结构和独特的电子特性。然后,深入综述了目前在晶圆级合成二维层状材料的策略,分为 "自上而下 "和 "自下而上 "两种。然后,讨论了二维材料晶圆在集成电子和光电器件中的应用。最后,介绍了二维集成电子器件当前面临的挑战和未来的发展前景。我们希望这篇综述能为晶圆级二维材料及其集成应用的发展提供全面而深刻的指导。
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引用次数: 0
Colloidal semiconductor nanocrystals for light emission and photonic integration 用于光发射和光子集成的胶体半导体纳米晶体
Pub Date : 2024-03-01 DOI: 10.1016/j.chip.2023.100073
Huan Liu , Dabin Lin , Puning Wang , Tingchao He , Rui Chen

Solution-processed colloidal semiconductor nanocrystals (NCs) have become attractive materials for the development of optoelectronic and photonic devices due to their inexpensive synthesis and excellent optical properties. Recently, CdSe NCs with different dimensions and structures have achieved significant progress in photonic integrated circuits (PICs), including light generation (laser), guiding (waveguide), modulation, and detection on a chip. This article summarizes the development of CdSe NCs–based lasers and discusses the challenges and opportunities for the application of CdSe NCs in PICs. Firstly, an overview of the optical properties of CdSe-based NCs with different dimensions is presented, with emphasis on the amplified stimulated emission and laser properties. Then, the nanophotonic devices and PICs based on CdSe NCs are introduced and discussed. Finally, the prospects for PICs are addressed.

溶液加工的胶体半导体纳米晶体(NCs)因其低廉的合成成本和优异的光学特性,已成为开发光电和光子器件的极具吸引力的材料。最近,不同尺寸和结构的碲化镉(CdSe)NC 在光子集成电路(PIC)方面取得了重大进展,包括在芯片上实现光的产生(激光)、引导(波导)、调制和检测。本文总结了基于 CdSe NCs 的激光器的发展,并讨论了 CdSe NCs 在 PIC 中应用所面临的挑战和机遇。首先,概述了不同尺寸的镉硒基 NC 的光学特性,重点介绍了放大受激发射和激光特性。然后,介绍并讨论了基于 CdSe NCs 的纳米光子器件和 PIC。最后,探讨了 PIC 的发展前景。
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引用次数: 0
High-performance eight-channel system with fractal superconducting nanowire single-photon detectors 配备分形超导纳米线单光子探测器的高性能八通道系统
Pub Date : 2024-02-27 DOI: 10.1016/j.chip.2024.100087
Zifan Hao , Kai Zou , Yun Meng , Jun-Yong Yan , Fangyuan Li , Yongheng Huo , Chao-Yuan Jin , Feng Liu , Thomas Descamps , Adrian Iovan , Val Zwiller , Xiaolong Hu

Superconducting nanowire single-photon detectors (SNSPDs) have become a mainstream photon-counting technology that has been widely applied in various scenarios. So far, most multi-channel SNSPD systems, either reported in literature or commercially available, are polarization sensitive, that is, the system detection efficiency (SDE) of each channel is dependent on the state of polarization of the to-be-detected photons. Here, we reported an eight-channel system with fractal SNSPDs working in the wavelength range of 930 to 940 nm, which are all featured with low polarization sensitivity. In a close-cycled Gifford-McMahon cryocooler system with the base temperature of 2.2 K, we installed and compared the performance of two types of devices: (1) SNSPD, composed of a single, continuous nanowire and (2) superconducting nanowire avalanche photodetector (SNAP), composed of 16 cascaded units of two nanowires electrically connected in parallel. The highest SDE among the eight channels reaches 965+4%, with the polarization sensitivity of 1.02 and a dark-count rate of 13 counts per second. The average SDE for eight channels for all states of polarization is estimated to be 90 ± 5%. It is concluded that both the SNSPDs and the SNAPs can reach saturated, high SDE at the wavelength of interest, and the SNSPDs show lower dark-count (false-count) rates, whereas the SNAPs show better properties in the time domain. With the adoption of this system, we showcased the measurements of the second-order photon-correlation functions of light emission from a single-photon source based on a semiconductor quantum dot and from a pulsed laser. It is believed that this work will provide new choices of systems with single-photon detectors combining the merits of high SDE, low polarization sensitivity, and low noise that can be tailored for different applications.

超导纳米线单光子探测器(SNSPD)已成为一种主流光子计数技术,并被广泛应用于各种领域。迄今为止,无论是文献报道还是市场上销售的大多数多通道 SNSPD 系统都对偏振敏感,也就是说,每个通道的系统检测效率(SDE)取决于待检测光子的偏振状态。在此,我们报告了一个在 930-940 纳米波长范围内工作的分形 SNSPD 八通道系统,该系统均具有低偏振灵敏度的特点。在基准温度为 2.2 K 的密闭循环 Gifford-McMahon 低温冷却器系统中,我们安装并比较了两种器件的性能:(1) 由单根连续纳米线组成的 SNSPD;(2) 由 16 个由两根纳米线并联组成的级联单元组成的超导纳米线雪崩光电探测器 (SNAP)。八个通道中最高的 SDE 达到 %,偏振灵敏度为 1.02,暗计数率为每秒 13 个计数。在所有偏振状态下,八个通道的平均 SDE 估计为 90 ± 5%。我们的结论是,SNSPD 和 SNAP 在相关波长上都能达到饱和的高 SDE,SNSPD 的暗计数(误计数)率较低,而 SNAP 在时域上表现出更好的特性。利用该系统,我们展示了基于半导体量子点的单光子源和脉冲激光器发出的光的二阶光子相关函数的测量结果。我们相信,我们的工作为具有单光子探测器的系统提供了新的选择,该系统结合了高 SDE、低偏振灵敏度和低噪声等优点,可为不同应用量身定制。
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引用次数: 0
Carbon-based memristors for resistive random access memory and neuromorphic applications 用于 RRAM 和神经形态应用的碳基记忆晶体管
Pub Date : 2024-02-01 DOI: 10.1016/j.chip.2024.100086
Fan Yang , Zhaorui Liu , Xumin Ding , Yang Li , Cong Wang , Guozhen Shen

As a typical representative of nanomaterials, carbon nanomaterials have attracted widespread attention in the construction of electronic devices owing to their unique physical and chemical properties, multi-dimensionality, multi-hybridization methods, and excellent electronic properties. Especially in the recent years, memristors based on carbon nanomaterials have flourished in the field of building non-volatile memory devices and neuromorphic applications. In the current work, the preparation methods and structural characteristics of carbon nanomaterials of different dimensions were systematically reviewed. Afterwards, in depth discussion on the structural characteristics and working mechanism of memristors based on carbon nanomaterials of different dimensions was conducted. Finally, the potential applications of carbon-based memristors in logic operations, neural network construction, artificial vision systems, artificial tactile systems, and multimodal perception systems were also introduced. It is believed that this paper will provide guidance for the future development of high-quality information storage, high-performance neuromorphic applications, and high-sensitivity bionic sensing based on carbon-based memristors.

作为纳米材料的典型代表,碳纳米材料以其独特的物理化学性质、多维性、多杂化方法和优异的电子特性,在电子器件的构建中受到广泛关注。特别是近年来,基于碳纳米材料的忆阻器在构建非易失性存储器件和神经形态应用领域蓬勃发展。本文系统综述了不同尺寸碳纳米材料的制备方法和结构特征。然后,深入讨论了基于不同尺寸碳纳米材料的忆阻器的结构特征和工作机理。最后,介绍了基于碳纳米材料的忆阻器在逻辑运算、神经网络构建、人工视觉系统、人工触觉系统和多模态感知系统中的潜在应用。我们相信,本文将为未来基于碳基忆阻器的高质量信息存储、高性能神经形态应用和高灵敏度仿生传感的发展提供指导。
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引用次数: 0
Coexistence of multiuser entanglement distribution and classical light in optical fiber network with a semiconductor chip 带半导体芯片的光纤网络中的多用户纠缠分布与经典光共存
Pub Date : 2024-01-17 DOI: 10.1016/j.chip.2024.100083
Xu Jing , Cheng Qian , Xiaodong Zheng , Hu Nian , Chenquan Wang , Jie Tang , Xiaowen Gu , Yuechan Kong , Tangsheng Chen , Yichen Liu , Chong Sheng , Dong Jiang , Bin Niu , Liangliang Lu

Building communication links among multiple users in a scalable and robust way is a key objective in achieving large-scale quantum networks. In a realistic scenario, noise from the coexisting classical light is inevitable and can ultimately disrupt the entanglement. The previous significant fully connected multiuser entanglement distribution experiments are conducted using dark fiber links, and there is no explicit relation between the entanglement degradations induced by classical noise and its error rate. Here, a semiconductor chip with a high figure-of-merit modal overlap is fabricated to directly generate broadband polarization entanglement. The monolithic source maintains the polarization entanglement fidelity of above 96% for 42 nm bandwidth, with a brightness of 1.2 × 107 Hz mW−1. A continuously working quantum entanglement distribution are performed among three users coexisting with classical light. Under finite-key analysis, secure keys are established and images encryption are enabled as well as quantum secret sharing between users. This work paves the way for practical multiparty quantum communication with integrated photonic architecture compatible with real-world fiber optical communication network.

以可扩展和稳健的方式在多个用户之间建立通信链路,是实现大规模量子网络的关键目标。在现实场景中,来自共存经典光的噪声是不可避免的,并可能最终破坏纠缠。以往重要的全连接多用户纠缠分发实验都是使用暗光纤链路进行的,经典噪声引起的纠缠退化与其错误率之间没有明确的关系。在这里,我们制造了一种具有高模态重叠系数的半导体芯片,可直接产生宽带偏振纠缠。我们的单片源在 42 nm 带宽和 1.2 × 107 Hz mW-1 的亮度下,偏振纠缠保真度保持在 96% 以上。我们在与经典光共存的三个用户之间进行了连续工作的量子纠缠分配。在有限密钥分析下,我们建立了安全密钥,实现了图像加密以及用户之间的量子秘密共享。我们的工作为采用与现实世界光纤通信网络兼容的集成光子架构的实用多方量子通信铺平了道路。
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引用次数: 0
Cryo-CMOS modeling and a 600 MHz cryogenic clock generator for quantum computing applications 用于量子计算应用的低温-CMOS 建模和 600 MHz 低温时钟发生器
Pub Date : 2023-12-01 DOI: 10.1016/j.chip.2023.100065
Qiwen Xue , Yuanke Zhang , Mingjie Wen , Xiaohu Zhai , Yuefeng Chen , Tengteng Lu , Chao Luo , Guoping Guo

The development of large-scale quantum computing has boosted an urgent desire for the advancement of cryogenic CMOS (cryo-CMOS), which is a promising scalable solution for the control and read-out interface of quantum bits. In the current work, 180 nm CMOS transistors were characterized and modeled down to 4 K, and the impact of low-temperature transistor performance variations on circuit design was also analyzed. Based on the proposed cryogenic model, a 180 nm CMOS-based 450 to 850 MHz clock generator operating at 4 K for quantum computing applications was presented. At the output frequency of 600 MHz, it achieved < 4.8 ps RMS jitter with 30 mW power consumption (with test buffer), corresponding to a211.6 dB jitter-power FOM, which is suitable for providing a stable clock signal for the control and readout electronics of scalable quantum computers.

大规模量子计算的发展推动了人们对低温 CMOS(cryo-CMOS)技术进步的迫切愿望,而低温 CMOS 是量子比特控制和读出接口的一种前景广阔的可扩展解决方案。在目前的工作中,对低至 4 K 的 180 nm CMOS 晶体管进行了表征和建模,并分析了低温晶体管性能变化对电路设计的影响。根据所提出的低温模型,介绍了一种在 4 K 温度下工作的基于 180 nm CMOS 的 450 至 850 MHz 时钟发生器,适用于量子计算应用。在输出频率为 600 MHz 时,它实现了 < 4.8 ps RMS 抖动,功耗为 30 mW(带测试缓冲器),相当于 -211.6 dB 抖动-功耗 FOM,适合为可扩展量子计算机的控制和读出电子设备提供稳定的时钟信号。
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引用次数: 0
Advanced RF filters for wireless communications 用于无线通信的先进射频滤波器
Pub Date : 2023-12-01 DOI: 10.1016/j.chip.2023.100058
Kai Yang , Chenggong He , Jiming Fang , Xinhui Cui , Haiding Sun , Yansong Yang , Chengjie Zuo

This paper provides a comprehensive review of advanced radio frequency (RF) filter technologies available in miniature chip or integrated circuit (IC) form for wireless communication applications. The RF filter technologies were organized according to the timeline of their introduction, in conjunction with each generation of wireless (cellular) communication standards (1G to 5G). This approach enabled a clear explanation of the corresponding invention history, working principles, typical applications and future development trends. The article covered commercially successful acoustic filter technologies, including the widely used surface acoustic wave (SAW) and bulk acoustic wave (BAW) filters, as well as electromagnetic filter technologies based on low-temperature co-fired ceramic (LTCC) and integrated passive device (IPD). Additionally, emerging filter technologies such as IHP-SAW, suspended thin-film lithium niobate (LiNbO3 or LN) resonant devices and hybrid were also discussed. In order to achieve higher performance, smaller form factor and lower cost for the wireless communication industry, it is believed that fundamental breakthroughs in materials and fabrication techniques are necessary for the future development of RF filters.

本文全面回顾了用于无线通信的微型芯片或集成电路(IC)形式的先进射频(RF)滤波器技术。RF滤波器技术是根据其引入的时间线组织的,与每一代无线(蜂窝)通信标准(1G到5G)结合在一起。通过这种方法,可以清楚地说明相应的发明历史、工作原理、典型应用和未来发展趋势。本文涵盖了商业上成功的声学滤波技术,包括广泛使用的表面声波(SAW)和体声波(BAW)滤波器,以及基于低温共烧陶瓷(LTCC)和集成无源器件(IPD)的电磁滤波器技术。此外,还讨论了IHP-SAW、悬浮薄膜铌酸锂(LiNbO3或LN)谐振器件和混合滤波器等新兴滤波技术。为了实现无线通信行业更高的性能,更小的外形尺寸和更低的成本,相信材料和制造技术的根本性突破是射频滤波器未来发展的必要条件。
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引用次数: 1
Corrigendum to “Implementing hardware primitives based on memristive spatiotemporal variability into cryptography applications” [Chip 2 (2023) 100040] 基于记忆时空变异性的硬件基元在密码学应用中的实现"[Chip 2 (2023) 100040]的更正
Pub Date : 2023-12-01 DOI: 10.1016/j.chip.2023.100076
Bo Liu , Yudi Zhao , Hanyuan Liang , Shiwei Feng
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引用次数: 0
Machine learning-accelerated discovery of novel 2D ferromagnetic materials with strong magnetization 机器学习加速发现新型二维强磁铁磁材料
Pub Date : 2023-12-01 DOI: 10.1016/j.chip.2023.100071
Chao Xin , Yaohui Yin , Bingqian Song , Zhen Fan , Yongli Song , Feng Pan

Two-dimensional ferromagnetic (2DFM) semiconductors (metals, half-metals, and so on) are important materials for next-generation nano-electronic and nano-spintronic devices. However, these kinds of materials remain scarce, “trial and error” experiments and calculations are both time-consuming and expensive. In the present work, in order to obtain the optimal 2DFM materials with strong magnetization, a machine learning (ML) framework was established to search the 2D material space containing over 2417 samples and identified 615 compounds whose magnetic orders were then determined via high-throughput first-principles calculations. With the adoption of ML algorithms, two classification models and a regression model were trained. The interpretability of the regression model was evaluated through Shapley Additive exPlanations (SHAP) analysis. Unexpectedly, it is found that Cr2NF2 is a potential antiferromagnetic ferroelectric 2D multiferroic material. More importantly, 60 novel 2DFM candidates were predicted, and among them, 13 candidates have magnetic moments of > 7μB. Os2Cl8, Fe3GeSe2, and Mn4N3S2 were predicted to be novel 2DFM semiconductors, metals, and half-metals, respectively. With the adoption of the ML approach in the current work, the prediction of 2DFM materials with strong magnetization can be accelerated, and the computation time can be drastically reduced by more than one order of magnitude.

二维铁磁(2DFM)半导体(金属、半金属等)是下一代纳米电子和纳米自旋电子器件的重要材料。然而,这类材料仍然稀缺,"试错 "实验和计算既耗时又昂贵。在本研究中,为了获得具有强磁化率的最佳 2DFM 材料,研究人员建立了机器学习(ML)框架,在包含超过 2417 个样品的二维材料空间中进行搜索,并确定了 615 种化合物,然后通过高通量第一原理计算确定了这些化合物的磁阶。通过采用 ML 算法,训练了两个分类模型和一个回归模型。通过 Shapley Additive exPlanations(SHAP)分析评估了回归模型的可解释性。结果意外地发现,Cr2NF2 是一种潜在的反铁磁铁电二维多铁性材料。更重要的是,预测出了 60 种新型二维多铁电体候选材料,其中 13 种候选材料的磁矩为 > 7μB。Os2Cl8、Fe3GeSe2和Mn4N3S2分别被预测为新型2DFM半导体、金属和半金属。在目前的工作中采用 ML 方法,可以加速强磁化 2DFM 材料的预测,计算时间可大幅缩短一个数量级以上。
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引用次数: 0
On-chip single-photon chirality encircling exceptional points 片上单光子手性环绕特殊点
Pub Date : 2023-12-01 DOI: 10.1016/j.chip.2023.100066
Zhen-Nan Tian , Feng Yu , Xu-Lin Zhang , Kai Ming Lau , Li-Cheng Wang , Jensen Li , C.T. Chan , Qi-Dai Chen

Exceptional points (EPs), which are typically defined as the degeneracy points of a non-Hermitian Hamiltonian, have been investigated in various physical systems such as photonic systems. In particular, the intriguing topological structures around EPs have given rise to novel strategies for manipulating photons and the underlying mechanism is especially useful for on-chip photonic applications. Although some on-chip experiments with the adoption of lasers have been reported, EP-based photonic chips working in the quantum regime largely remain elusive. In the current work, a single-photon experiment was proposed to dynamically encircle an EP in on-chip photonic waveguides possessing passive anti-parity-time symmetry. Photon coincidences measurement reveals a chiral feature of transporting single photons, which can act as a building block for on-chip quantum devices that require asymmetric transmissions. The findings in the current work pave the way for on-chip experimental study on the physics of EPs as well as inspiring applications for on-chip non-Hermitian quantum devices.

异常点(EPs)通常被定义为非赫米提哈密顿的退化点,在光子系统等各种物理系统中都得到了研究。特别是,EP 周围引人入胜的拓扑结构催生了操纵光子的新策略,其基本机制尤其适用于片上光子应用。虽然一些采用激光器的片上实验已经有了报道,但基于 EP 的光子芯片在量子体系中的工作在很大程度上仍然难以实现。在目前的工作中,我们提出了一种单光子实验,在具有被动反偶时对称性的片上光子波导中动态环绕 EP。光子重合度测量揭示了单光子传输的手性特征,可作为需要非对称传输的片上量子器件的构件。目前的研究成果为片上 EP 物理实验研究铺平了道路,同时也为片上非赫米提量子器件的应用带来了启发。
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引用次数: 0
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