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Time-domain oscillations between distant spin qubits coupled via virtual photons 通过虚光子耦合的远距离自旋量子位之间的时域振荡
IF 17.6 1区 物理与天体物理 Q1 PHYSICS, MULTIDISCIPLINARY Pub Date : 2024-12-09 DOI: 10.1038/s41567-024-02706-7
In a device comprising two double quantum dots separated by a 250-μm-long superconducting resonator, virtual photons in the resonator are shown to mediate the coupling of electron spins between the quantum dots. When the spin–spin coupling is activated for a controlled duration, oscillations between the spins are observed.
在一个由250 μm长的超导谐振腔分隔的双量子点组成的装置中,谐振腔中的虚光子介导了量子点之间电子自旋的耦合。当自旋-自旋耦合在控制的持续时间内被激活时,观察到自旋之间的振荡。
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引用次数: 0
Cavity-mediated iSWAP oscillations between distant spins 远距离自旋间腔介导的iSWAP振荡
IF 17.6 1区 物理与天体物理 Q1 PHYSICS, MULTIDISCIPLINARY Pub Date : 2024-12-09 DOI: 10.1038/s41567-024-02694-8
Jurgen Dijkema, Xiao Xue, Patrick Harvey-Collard, Maximilian Rimbach-Russ, Sander L. de Snoo, Guoji Zheng, Amir Sammak, Giordano Scappucci, Lieven M. K. Vandersypen
Direct interactions between quantum particles naturally fall off with distance. However, future quantum computing architectures are likely to require interaction mechanisms between qubits across a range of length scales. In this work, we demonstrate a coherent interaction between two semiconductor spin qubits 250 μm apart using a superconducting resonator. This separation is several orders of magnitude larger than for the commonly used direct interaction mechanisms in this platform. We operate the system in a regime in which the resonator mediates a spin–spin coupling through virtual photons. We report the anti-phase oscillations of the populations of the two spins with controllable frequency. The observations are consistent with iSWAP oscillations of the spin qubits, and suggest that entangling operations are possible in 10 ns. These results hold promise for scalable networks of spin qubit modules on a chip. Coupling semiconductor spin qubits over long distances using a superconducting resonator makes different quantum architectures possible. Now, the coherent swapping of quantum states has been observed between qubits coupled using this design.
量子粒子之间的直接相互作用自然会随着距离的增加而减弱。然而,未来的量子计算架构可能需要量子位之间跨越一定长度尺度的相互作用机制。在这项工作中,我们使用超导谐振器演示了两个相距250 μm的半导体自旋量子比特之间的相干相互作用。这种分离比该平台中常用的直接交互机制要大几个数量级。我们在谐振器通过虚光子介导自旋-自旋耦合的状态下操作系统。我们报道了频率可控的两个自旋居群的反相位振荡。观测结果与自旋量子位的iSWAP振荡一致,并表明纠缠操作可能在10 ns内发生。这些结果为芯片上自旋量子比特模块的可扩展网络带来了希望。
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引用次数: 0
Signatures of two gaps in the spin susceptibility of a cuprate superconductor 铜超导体自旋磁化率的两个间隙特征
IF 17.6 1区 物理与天体物理 Q1 PHYSICS, MULTIDISCIPLINARY Pub Date : 2024-12-05 DOI: 10.1038/s41567-024-02692-w
Rui Zhou, Igor Vinograd, Michihiro Hirata, Tao Wu, Hadrien Mayaffre, Steffen Krämer, W. N. Hardy, Ruixing Liang, D. A. Bonn, Toshinao Loew, Juan Porras, Bernhard Keimer, Marc-Henri Julien
A fundamental obstacle to understanding high-temperature superconducting cuprates is that the occurrence of superconductivity hinders the observation of the normal-state properties at low temperature. One important property illustrating this issue is the spin susceptibility: its decrease upon cooling in the normal state is considered as evidence of pseudogap behaviour. However, unambiguous interpretation of this decrease has been impossible, as the crucial low-temperature data inevitably reflect the superconducting pairing rather than the normal state. Here we measure the spin susceptibility of YBa2Cu3Oy at low temperature while suppressing superconductivity in high magnetic field. We found that there are two thermally activated contributions, each of which comes from a different gap, alongside a residual component due to gapless excitations. We relate these two distinct gaps to short-range charge density waves and to the formation of singlets, as occurs in certain quantum spin systems. Both phenomena contribute to the pseudogap at low temperature, supplementing the short-lived antiferromagnetism that initiates pseudogap behaviour at high temperatures. We, therefore, propose that the pseudogap should be regarded as a composite property and that, when not undergoing spin-stripe ordering, underdoped cuprates tend to form short-range spin singlets. Measurements of the spin susceptibility in a model cuprate reveal the presence of two distinct gaps underlying the pseudogap behaviour. One gap is attributed to charge density waves and the other to the predicted formation of spin singlets.
理解高温超导铜酸盐的一个根本障碍是超导性的发生阻碍了低温下正常状态性质的观察。说明这个问题的一个重要性质是自旋磁化率:它在正常状态下冷却时的减少被认为是赝隙行为的证据。然而,对这种减少的明确解释是不可能的,因为关键的低温数据不可避免地反映了超导配对而不是正常状态。本文测量了YBa2Cu3Oy在低温下的自旋磁化率,同时抑制了高磁场下的超导性。我们发现有两种热激活的贡献,每一种都来自不同的间隙,以及由于无间隙激励而产生的残余成分。我们将这两个不同的间隙与短程电荷密度波和单重态的形成联系起来,就像在某些量子自旋系统中发生的那样。这两种现象都有助于低温下的赝隙,补充了在高温下引发赝隙行为的短暂反铁磁性。因此,我们提出赝隙应被视为一种复合性质,并且当不进行自旋条纹排序时,欠掺杂铜酸盐倾向于形成短程自旋单重态。
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引用次数: 0
Observation of the Schmid–Bulgadaev dissipative quantum phase transition Schmid-Bulgadaev耗散量子相变的观察
IF 17.6 1区 物理与天体物理 Q1 PHYSICS, MULTIDISCIPLINARY Pub Date : 2024-12-02 DOI: 10.1038/s41567-024-02695-7
Roman Kuzmin, Nitish Mehta, Nicholas Grabon, Raymond A. Mencia, Amir Burshtein, Moshe Goldstein, Vladimir E. Manucharyan
A classical particle moving in a periodic potential can localize inside a single potential minimum, but a quantum particle forms extended states by tunnelling to neighbouring minima. These two limits are separated by a quantum Schmid–Bulgadaev phase transition driven by a viscous friction force. This physics has implications for Josephson junction devices, which feature superconducting phase dynamics that can be modelled by a fictitious particle in a periodic potential. As a result, it has been anticipated that any junction of two superconductors connected to a resistor can undergo a Schmid–Bulgadaev transition when the value of the resistor exceeds a threshold. Here we observe this transition by implementing the ohmic environment as a massively multimode cavity and probing the effect of the junction on the standing-wave mode spectrum of the cavity. We find that, depending on the characteristic impedance of the cavity, sufficiently weak junctions scatter cavity photons as either inductors or capacitors. These regimes correspond to the superconducting and insulating phases, respectively, and the critical impedance matches the expected value. At the phase boundary, quantum fluctuations boost the junction nonlinearity so that the junction behaves as a resistor. This loss mechanism reconciles the superconducting and insulating phases and provides a possibly useful indication of quantum-critical dynamics. Josephson junctions are expected to transition from superconducting to insulating behaviour depending on the impedance of their environment. This Schmid–Bulgadaev transition has now been observed by probing the effect of a junction on its environment.
在周期势中运动的经典粒子可以定位在单个势最小值内,但量子粒子通过隧穿到邻近的最小值形成扩展状态。这两个极限被一个由粘性摩擦力驱动的量子Schmid-Bulgadaev相变所分隔。这一物理学对约瑟夫森结器件具有重要意义,该器件具有超导相动力学,可以通过周期势中的虚拟粒子来模拟。因此,当电阻的值超过阈值时,两个超导体连接到一个电阻的任何结都可以经历Schmid-Bulgadaev跃迁。在这里,我们通过将欧姆环境实现为大规模多模腔,并探测结对腔驻波模式频谱的影响来观察这种转变。我们发现,根据腔的特性阻抗,足够弱的结散射腔光子作为电感或电容器。这些状态分别对应于超导相和绝缘相,临界阻抗符合期望值。在相边界处,量子涨落增强了结的非线性,使结表现为电阻器。这种损耗机制调和了超导相和绝缘相,并提供了可能有用的量子临界动力学指示。
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引用次数: 0
Electronic dynamics created at conical intersections and its dephasing in aqueous solution 锥形交叉点产生的电子动力学及其在水溶液中的消相现象
IF 17.6 1区 物理与天体物理 Q1 PHYSICS, MULTIDISCIPLINARY Pub Date : 2024-11-27 DOI: 10.1038/s41567-024-02703-w
Yi-Ping Chang, Tadas Balciunas, Zhong Yin, Marin Sapunar, Bruno N. C. Tenorio, Alexander C. Paul, Shota Tsuru, Henrik Koch, Jean-Pierre Wolf, Sonia Coriani, Hans Jakob Wörner
A dynamical rearrangement in the electronic structure of a molecule can be driven by different phenomena, including nuclear motion, electronic coherence or electron correlation. Recording such electronic dynamics and identifying its fate in an aqueous solution has remained a challenge. Here, we reveal the electronic dynamics induced by electronic relaxation through conical intersections in both isolated and solvated pyrazine molecules using X-ray spectroscopy. We show that the ensuing created dynamics corresponds to a cyclic rearrangement of the electronic structure around the aromatic ring. Furthermore, we found that such electronic dynamics were entirely suppressed when pyrazine was dissolved in water. Our observations confirm that conical intersections can create electronic dynamics that are not directly excited by the pump pulse and that aqueous solvation can dephase them in less than 40 fs. These results have implications for the investigation of electronic dynamics created during light-induced molecular dynamics and shed light on their susceptibility to aqueous solvation. Tracking ultrafast electronic changes in molecules is challenging, especially in liquids. An X-ray spectroscopy study in pyrazine now shows electronic dynamics created at conical intersections that are rapidly suppressed when the molecule is in water.
分子电子结构的动态重排可以由不同的现象驱动,包括核运动、电子相干性或电子相关性。记录这种电子动力学并确定其在水溶液中的命运一直是一个挑战。在这里,我们利用 X 射线光谱揭示了孤立的吡嗪分子和溶解的吡嗪分子中通过锥形交叉点的电子弛豫引起的电子动力学。我们发现,随之产生的动态与围绕芳香环的电子结构的循环重排相对应。此外,我们还发现,当吡嗪溶于水时,这种电子动力学完全被抑制。我们的观察结果证实,锥形交叉点可以产生不被泵脉冲直接激发的电子动力学,而水溶解可以在不到 40 fs 的时间内消除这些电子动力学。这些结果对研究光诱导分子动力学过程中产生的电子动力学具有重要意义,并揭示了它们对水溶解的敏感性。
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引用次数: 0
Quantum geometry in solids measured using photo-emitted electrons 使用光发射电子测量固体中的量子几何学
IF 17.6 1区 物理与天体物理 Q1 PHYSICS, MULTIDISCIPLINARY Pub Date : 2024-11-25 DOI: 10.1038/s41567-024-02681-z
Quantum geometry gives rise to many fascinating phenomena in solids that go beyond Landau theory. A general framework is now introduced to measure the quantum geometric tensor in solids — a fundamental physical quantity that encodes the complete geometric information of the Bloch state.
量子几何在固体中产生了许多超越朗道理论的迷人现象。现在介绍一种测量固体量子几何张量的通用框架--这是一种基本物理量,它编码了布洛赫态的完整几何信息。
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引用次数: 0
Measurements of the quantum geometric tensor in solids 测量固体中的量子几何张量
IF 17.6 1区 物理与天体物理 Q1 PHYSICS, MULTIDISCIPLINARY Pub Date : 2024-11-25 DOI: 10.1038/s41567-024-02678-8
Mingu Kang, Sunje Kim, Yuting Qian, Paul M. Neves, Linda Ye, Junseo Jung, Denny Puntel, Federico Mazzola, Shiang Fang, Chris Jozwiak, Aaron Bostwick, Eli Rotenberg, Jun Fuji, Ivana Vobornik, Jae-Hoon Park, Joseph G. Checkelsky, Bohm-Jung Yang, Riccardo Comin
Understanding the geometric properties of quantum states and their implications in fundamental physical phenomena is a core aspect of contemporary physics. The quantum geometric tensor (QGT) is a central physical object in this regard, encoding complete information about the geometry of the quantum state. The imaginary part of the QGT is the well-known Berry curvature, which plays an integral role in the topological magnetoelectric and optoelectronic phenomena. The real part of the QGT is the quantum metric, whose importance has come to prominence recently, giving rise to a new set of quantum geometric phenomena such as anomalous Landau levels, flat band superfluidity, excitonic Lamb shifts and nonlinear Hall effect. Despite the central importance of the QGT, its experimental measurements have been restricted only to artificial two-level systems. Here, we develop a framework to measure the QGT in crystalline solids using polarization-, spin- and angle-resolved photoemission spectroscopy. Using this framework, we demonstrate the effective reconstruction of the QGT in the kagome metal CoSn, which hosts topological flat bands. Establishing this momentum- and energy-resolved spectroscopic probe of the QGT is poised to significantly advance our understanding of quantum geometric responses in a wide range of crystalline systems. Experiments that directly probe the quantum geometric tensor in solids have not been reported. Now, the quantum metric and spin Berry curvature—dual components of the quantum geometric tensor—have been simultaneously measured in reciprocal space.
理解量子态的几何特性及其对基本物理现象的影响是当代物理学的核心内容。量子几何张量(QGT)是这方面的核心物理对象,它完整地编码了量子态的几何信息。QGT 的虚部是著名的贝里曲率,在拓扑磁电和光电现象中发挥着不可或缺的作用。QGT 的实部是量子度量,其重要性近来逐渐凸显,引发了一系列新的量子几何现象,如反常朗道水平、平带超流、激子兰姆位移和非线性霍尔效应。尽管 QGT 非常重要,但其实验测量却仅限于人工两级系统。在这里,我们建立了一个框架,利用偏振、自旋和角度分辨光发射光谱测量晶体固体中的 QGT。利用这一框架,我们展示了在含有拓扑扁平带的卡戈米金属 CoSn 中有效重建 QGT 的方法。建立这种动量和能量分辨的 QGT 光谱探针,将极大地推动我们对各种晶体系统中量子几何响应的理解。
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引用次数: 0
Super- and subradiant dynamics of quantum emitters mediated by atomic matter waves 原子物质波介导的量子发射器的超辐射和亚辐射动力学
IF 17.6 1区 物理与天体物理 Q1 PHYSICS, MULTIDISCIPLINARY Pub Date : 2024-11-18 DOI: 10.1038/s41567-024-02676-w
Youngshin Kim, Alfonso Lanuza, Dominik Schneble
The cooperative modification of spontaneous radiative decay exemplifies a many-emitter effect in quantum optics. So far, its experimental realizations have relied on interactions mediated by rapidly escaping photons, which do not play an active role in the emitter dynamics. Here we use a platform of ultracold atoms in a one-dimensional optical lattice geometry to explore cooperative non-Markovian dynamics of synthetic quantum emitters that decay by radiating slow atomic matter waves. By preparing and manipulating arrays of emitters hosting weakly and strongly interacting many-body phases of excitations, we demonstrate directional collective emission and study the interplay between retardation and super- and subradiant dynamics. Moreover, we directly observe the spontaneous buildup of coherence among emitters. Our results on collective radiative dynamics establish ultracold matter waves as a versatile tool for studying many-body quantum optics in spatially extended and ordered systems. Experiments on cooperative radiative decay typically involve rapidly escaping photons. Collective emission dynamics have now been studied in an array of quantum emitters interacting via atomic matter waves in a novel regime of slow propagation.
自发辐射衰变的合作修正是量子光学中多发射极效应的典范。迄今为止,其实验实现依赖于由快速逃逸光子介导的相互作用,而这些光子在发射器动力学中并不发挥积极作用。在这里,我们利用一维光学晶格几何中的超冷原子平台,探索通过辐射缓慢原子物质波衰变的合成量子发射器的合作非马尔可夫动力学。通过制备和操纵承载弱和强相互作用多体激发相的发射体阵列,我们展示了定向集体发射,并研究了迟滞与超辐射和亚辐射动力学之间的相互作用。此外,我们还直接观察到发射体之间自发建立的相干性。我们在集体辐射动力学方面的研究成果确立了超冷物质波作为研究空间扩展和有序系统中多体量子光学的多功能工具的地位。
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引用次数: 0
Universal dynamics exposed by interaction quenches 相互作用淬火所揭示的普遍动力学
IF 17.6 1区 物理与天体物理 Q1 PHYSICS, MULTIDISCIPLINARY Pub Date : 2024-11-14 DOI: 10.1038/s41567-024-02704-9
Chandrasekhar Ramanathan
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引用次数: 0
Nematic fluctuations shape Cooper pairs 向列波动形成库珀对
IF 17.6 1区 物理与天体物理 Q1 PHYSICS, MULTIDISCIPLINARY Pub Date : 2024-11-13 DOI: 10.1038/s41567-024-02693-9
Lingyuan Kong
Experimental evidence of nematic-fluctuation-mediated superconductivity has been observed in an iron-based superconductor near the quantum critical point.
在一种接近量子临界点的铁基超导体中观察到了由向列波动介导的超导现象的实验证据。
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引用次数: 0
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