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Artificial neural network (ANN) vs multilinear regression (MLR) models to predict naturally occurring radioactivity (NORM) in the gold mining area in eastern Sudan 人工神经网络(ANN)与多元线性回归(MLR)模型预测苏丹东部金矿区自然放射性(NORM)
IF 2.8 3区 物理与天体物理 Q3 CHEMISTRY, PHYSICAL Pub Date : 2026-01-22 DOI: 10.1016/j.radphyschem.2026.113656
Tahir E. Adreani , Ibrahim I. Suliman , Hajo Idriss , A. Sulieman , M. Alkhorayef , D. Bradley
Artificial neural network (ANN) and multilinear regression (MLR) models are widely recognized for their effectiveness in predicting the dynamics of industrial and natural phenomena. In this study, both multiple regression and ANN were employed to forecast radioactivity levels in regions affected by gold mining in Eastern Sudan. We developed multi-regression and ANN models using Python scripts in a Linux environment. The results were tested and validated against background radiation measurements in an area with naturally occurring radioactive materials (NORM) in Eastern Sudan. These findings were compared with the activity concentrations of the soil samples measured using high-purity germanium (HPGe) gamma spectrometry. The study revealed that The ANN model demonstrated superior predictive capabilities for 226Ra and 232Th activity concentrations compared to MLR, owing to ANN's ability to model nonlinear relationships in environmental radioactivity data. Although the multilinear regression performed better at 40K because of its linear soil dependency, the ANN achieved higher correlation coefficients overall. These results confirm that ANN-based methodologies can effectively predict radionuclide distributions and improve environmental radiation assessment.
人工神经网络(ANN)和多元线性回归(MLR)模型在预测工业和自然现象的动态方面的有效性得到了广泛的认可。本研究采用多元回归和人工神经网络相结合的方法预测了苏丹东部金矿开采影响地区的放射性水平。我们在Linux环境下使用Python脚本开发了多元回归和人工神经网络模型。在苏丹东部一个有天然放射性物质(NORM)的地区对这些结果进行了本底辐射测量,并加以验证。这些发现与使用高纯度锗(HPGe)伽马能谱法测量的土壤样品的活性浓度进行了比较。研究表明,与MLR相比,由于ANN能够模拟环境放射性数据中的非线性关系,因此ANN模型对226Ra和232Th活性浓度的预测能力优于MLR。虽然多元线性回归在40K时表现较好,但由于其线性土壤依赖性,人工神经网络总体上获得了更高的相关系数。这些结果证实了基于人工神经网络的方法可以有效地预测放射性核素分布,改善环境辐射评价。
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引用次数: 0
Dynamics of neutron-induced water radiolysis in high-temperature, high-pressure water relevant to PWR primary coolant 与压水堆主冷剂有关的高温高压水中中子诱导水辐射分解动力学
IF 2.8 3区 物理与天体物理 Q3 CHEMISTRY, PHYSICAL Pub Date : 2026-01-22 DOI: 10.1016/j.radphyschem.2026.113661
Hui-Chao Li , Dan-Dan Su , Xiao-Bin Li , Jun-Liang Guo , Feng-Chen Li , Shu-Qi Meng
In pressurized water reactors (PWRs), neutron-induced water radiolysis is a key factor in accelerating the oxidation of zirconium alloy cladding. In this study, the neutron-induced water radiolysis process from 1 keV to 5 MeV at 573 K and 15.5 MPa was simulated using the reactive force field molecular dynamics (ReaxFF-MD) method. The results show that the G-values of molecular products (H2, H2O2) decrease with increasing neutron energy, while the G-value of free radicals (•OH, H•) increase, demonstrating the linear energy transfer (LET) effect. The analysis of the microscopic mechanism reveals that low-energy primary knock-on atoms (PKAs) forms a dense track, and the G-value evolution follows a delayed-onset rapid growth pattern. Medium energy PKAs trigger a compression-rebound effect, and forms a transition track. High-energy PKAs penetrate in an inefficient energy-transfer mode with dispersed energy, and the G-value rapidly reaches the peak and then decreases. This study elucidates the intrinsic mechanism of the LET effect from the atomic scale, and provides a theoretical basis for the study of zirconium alloy oxidation and the construction of material damage model.
在压水堆(pwr)中,中子诱导的水辐射是加速锆合金包层氧化的关键因素。本研究采用反应力场分子动力学(ReaxFF-MD)方法模拟了在573 K和15.5 MPa条件下中子诱导水从1 keV到5 MeV的辐射分解过程。结果表明:随着中子能量的增加,分子产物(H2、H2O2)的g值降低,而自由基(•OH、H•)的g值增加,表现出线性能量传递(LET)效应;微观机制分析表明,低能初级敲原子(pka)形成了密集的轨道,g值演化遵循延迟开始的快速增长模式。中等能量的pka触发压缩回弹效应,形成过渡轨迹。高能PKAs以能量分散的低效能量传递方式穿透,g值迅速达到峰值后下降。本研究从原子尺度上阐明了LET效应的内在机理,为锆合金氧化研究和材料损伤模型的构建提供了理论依据。
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引用次数: 0
Standard-less IM-NAA for compositional analysis of nuclear reactor materials: Flux characterization and uncertainty evaluation 核反应堆材料成分分析的无标准IM-NAA:通量表征和不确定度评估
IF 2.8 3区 物理与天体物理 Q3 CHEMISTRY, PHYSICAL Pub Date : 2026-01-21 DOI: 10.1016/j.radphyschem.2026.113657
S.K. Samanta , Purbali Das , Sonika Gupta , Suparna Sodaye
The standard-less IM-NAA approach using research reactors requires characterization of the different irradiation sites with respect to neutron flux parameters, specifically the sub-cadmium to epithermal flux ratio (f) and the epithermal neutron flux shape factor (α). The flux characterization was performed at two research reactor facilities at BARC, Mumbai: the outer core irradiation position (H7) of the Apsara-U reactor and the Pneumatic Carrier Facility (PCF) of the Dhruva reactor. The accuracy and robustness of the developed methodology was validated using certified reference materials (CRMs). The optimized IM-NAA methodology was subsequently employed for the comprehensive chemical characterization of different steel samples relevant to advanced reactor technology. The uncertainty associated with IM-NAA measurements was rigorously evaluated, accounting for nuclear data parameters (e.g., Q0, k0, Er) reactor flux parameters (f, α), and other contributors often neglected in conventional analysis. The work successfully demonstrated that IM-NAA, when implemented with properly characterized flux parameters, provides a reliable, standard-less methodology for the accurate and precise compositional analysis of complex alloys, thereby strengthening quality control and material verification protocols for advanced nuclear technologies.
使用研究堆的无标准IM-NAA方法需要对不同辐照点的中子通量参数进行表征,特别是亚镉与超热中子通量比(f)和超热中子通量形状因子(α)。在孟买BARC的两个研究堆设施进行了通量表征:Apsara-U反应堆的外堆芯辐照位置(H7)和Dhruva反应堆的气动载体设施(PCF)。使用标准物质(crm)验证了所开发方法的准确性和稳健性。优化后的IM-NAA方法随后被用于与先进反应器技术相关的不同钢样品的综合化学表征。与IM-NAA测量相关的不确定度进行了严格的评估,考虑了核数据参数(例如,Q0, k0, Er),反应堆通量参数(f, α),以及在常规分析中经常被忽视的其他贡献者。这项工作成功地证明了IM-NAA,当采用适当的表征通量参数时,为复杂合金的准确和精确的成分分析提供了可靠的、无标准的方法,从而加强了先进核技术的质量控制和材料验证方案。
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引用次数: 0
Beyond CTDIvol: Patient-specific SSDE and organ dose assessment in routine adult CT practice 超越CTDIvol:常规成人CT实践中患者特异性SSDE和器官剂量评估
IF 2.8 3区 物理与天体物理 Q3 CHEMISTRY, PHYSICAL Pub Date : 2026-01-21 DOI: 10.1016/j.radphyschem.2026.113658
Omar Bentiane, Omaima Khettabi, Omar Berradi, El Mehdi Sadiki, Fatimaezzahra Bouzzit, Rodouan Touti
Computed Tomography (CT) is a key diagnostic tool in medical imaging, but concerns persist regarding radiation exposure, particularly in repeat or high-dose examinations. The CTDIvol quantifies scanner output but does not accurately represent the patient dose. The Size-Specific Dose Estimate (SSDE) provides a more clinically relevant patient-specific dose estimate by accounting for body size and composition. This study aims to quantify the differences between CTDIvol and SSDE in adult thoraco-abdominopelvic and abdominopelvic CT scans, compare manual and automatic methods of patient size estimation, and evaluate organ doses. A retrospective review was conducted on 52 adult CT scans (thoraco-abdominopelvic and abdominopelvic). Four patient-size metrics were collected: the manually measured effective diameter (Deff-M), the automatically averaged z-axis effective diameter (Deff-AZ), and two water-equivalent diameters (Dw-E and Dw-AZ). The SSDE values were calculated according to AAPM TG-204 and TG-220. The organ doses were estimated with IndoseCT based on Monte Carlo-derived correlations. The mean CTDIvol was 13.0 ± 3.6 mGy, with SSDE values 31–37 % higher across all methods. Deff-AZ was 4.7 % greater than Deff-M, while Dw-E and Dw-AZ showed near-perfect agreement. The liver, kidneys, and bladder received the highest doses (>15 mGy) as they are directly irradiated, whereas radiosensitive organs outside the primary scan field, such as the thyroid and eyes, received measurable scatter doses. SSDE provides a more accurate representation of patient radiation dose than CTDIvol and should be integrated into routine CT protocols. Among the evaluated size metrics, attenuation-based Dw proved to be the most robust and reproducible. Incorporating organ-dose estimations and SSDE into clinical practice can enhance patient safety, optimize imaging protocols, and support compliance with radiation protection regulations.
计算机断层扫描(CT)是医学成像中的关键诊断工具,但对辐射暴露的担忧持续存在,特别是在重复或高剂量检查中。CTDIvol量化扫描仪输出,但不能准确代表患者剂量。尺寸特异性剂量估计(SSDE)通过考虑身体尺寸和组成提供了更具临床相关性的患者特异性剂量估计。本研究旨在量化CTDIvol和SSDE在成人胸腹骨盆和腹部骨盆CT扫描中的差异,比较人工和自动估计患者大小的方法,并评估器官剂量。回顾性分析了52例成人CT扫描(胸腹骨盆和腹部骨盆)。收集4个患者尺寸指标:人工测量的有效直径(def - m)、自动平均z轴有效直径(def - az)和两个水当量直径(Dw-E和Dw-AZ)。根据AAPM TG-204和TG-220计算SSDE值。使用IndoseCT根据蒙特卡罗导出的相关性估计器官剂量。CTDIvol平均值为13.0±3.6 mGy, SSDE值比所有方法高31 - 37%。def - az比def - m高4.7%,而Dw-E和Dw-AZ表现出近乎完美的一致性。肝脏、肾脏和膀胱受到的辐射剂量最高(15毫戈瑞),因为它们直接受到辐射,而初级扫描场外的辐射敏感器官,如甲状腺和眼睛,则受到可测量的散射剂量。SSDE提供比CTDIvol更准确的患者辐射剂量表示,应纳入常规CT方案。在评估的尺寸指标中,基于衰减的Dw被证明是最稳健和可重复性的。将器官剂量评估和SSDE纳入临床实践可以提高患者安全,优化成像方案,并支持遵守辐射防护法规。
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引用次数: 0
Assessment of mechanical properties and radiation shielding efficiency of fiber-reinforced ultra high-performance concrete: Experimental and simulation analysis 纤维增强高性能混凝土力学性能及辐射屏蔽效能评估:实验与仿真分析
IF 2.8 3区 物理与天体物理 Q3 CHEMISTRY, PHYSICAL Pub Date : 2026-01-21 DOI: 10.1016/j.radphyschem.2026.113640
Ahmed A. Abdou Elabbasy , Ahmed M. El-Khayatt , Mahmoud Elsayed , Hesham M.H. Zakaly , A. Alkaoud , Islam M. Nabil , Islam N. Fathy , Alaa M. Rashad , Manar Ali
This study examined the mechanical properties and γ-ray radiation shielding performance of different ultra high-performance concrete (UHPC) mixes incorporating individual and hybrid combinations of steel (SF), polyvinyl alcohol (PVA), polypropylene (PP), and natural jute fibers (JF). Radiation attenuation was assessed through experimental testing and validated using Monte Carlo (MC) simulations and Phy-X software. Results indicated that the control UHPC mix with steel fibers alone achieved the highest compressive strength of 140 MPa at curing age of 28 days. In comparison with this SF-reinforced control mix, the hybrid fiber mixtures (SF + PVA, SF + PP, SF + JF, and SF + PP + PVA + JF) exhibited reductions in compressive strength of approximately 12.4 %, 11.6 %, 15.7 %, and 21.1 %, respectively, at the same age. Tensile and flexural strengths followed a similar trend of reduction with hybrid fiber incorporation. Relative to the tensile strength value of the control mix (10 MPa), hybrid fiber combinations (SF + PVA, SF + PP, SF + JF, and SF + PP + PVA + JF) resulted in tensile strength reductions of approximately 4 %, 5 %, 8 %, and 8 %. Similarly, their flexural strengths were notably decreased by about 9.6 %, 18.4 %, 22 %, and 24.4 %, respectively, when compared to the control mix that achieved 25 MPa with only SF. While steel fibers remain the most effective, incorporating natural or synthetic fibers like jute and polypropylene can provide acceptable γ-attenuation performance, with potential advantages in cost, flexibility, and sustainability. Hybrid combinations offer a promising balance, especially when multi-functionality (e.g., mechanical strength and γ-radiation shielding) is desired. The key novelty aspect of this work lies in examining fiber type as the main affecting variable on the radiation shielding behavior of UHPC, while combining experimental testing with MC simulation and Phy-X software for radiation shielding assessment.
本研究考察了不同的超高性能混凝土(UHPC)混合材料的力学性能和γ射线屏蔽性能,这些混合材料包括钢(SF)、聚乙烯醇(PVA)、聚丙烯(PP)和天然黄麻纤维(JF)的单独和混合组合。通过实验测试评估辐射衰减,并使用蒙特卡罗(MC)模拟和Phy-X软件进行验证。结果表明,单独加入钢纤维的UHPC混合料在养护28 d时抗压强度最高,达到140 MPa。在相同龄期,与SF增强对照相比,混杂纤维混合物(SF + PVA、SF + PP、SF + JF和SF + PP + PVA + JF)的抗压强度分别降低了12.4%、11.6%、15.7%和21.1%。混合纤维掺入后,拉伸和弯曲强度也有类似的降低趋势。与对照纤维的抗拉强度值(10 MPa)相比,混合纤维组合(SF + PVA、SF + PP、SF + JF和SF + PP + PVA + JF)的抗拉强度降低了约4%、5%、8%和8%。同样,它们的抗弯强度分别显著下降了约9.6%,18.4%,22%和24.4%,与仅使用SF达到25 MPa的对照混合物相比。虽然钢纤维仍然是最有效的,但结合天然或合成纤维,如黄麻和聚丙烯,可以提供可接受的γ衰减性能,在成本、灵活性和可持续性方面具有潜在优势。混合组合提供了一种有希望的平衡,特别是当需要多功能(例如,机械强度和γ辐射屏蔽)时。本工作的关键新颖之处在于将光纤类型作为影响UHPC辐射屏蔽性能的主要变量,并将实验测试与MC模拟和Phy-X软件相结合进行辐射屏蔽评估。
{"title":"Assessment of mechanical properties and radiation shielding efficiency of fiber-reinforced ultra high-performance concrete: Experimental and simulation analysis","authors":"Ahmed A. Abdou Elabbasy ,&nbsp;Ahmed M. El-Khayatt ,&nbsp;Mahmoud Elsayed ,&nbsp;Hesham M.H. Zakaly ,&nbsp;A. Alkaoud ,&nbsp;Islam M. Nabil ,&nbsp;Islam N. Fathy ,&nbsp;Alaa M. Rashad ,&nbsp;Manar Ali","doi":"10.1016/j.radphyschem.2026.113640","DOIUrl":"10.1016/j.radphyschem.2026.113640","url":null,"abstract":"<div><div>This study examined the mechanical properties and γ-ray radiation shielding performance of different ultra high-performance concrete (UHPC) mixes incorporating individual and hybrid combinations of steel (SF), polyvinyl alcohol (PVA), polypropylene (PP), and natural jute fibers (JF). Radiation attenuation was assessed through experimental testing and validated using Monte Carlo (MC) simulations and Phy-X software. Results indicated that the control UHPC mix with steel fibers alone achieved the highest compressive strength of 140 MPa at curing age of 28 days. In comparison with this SF-reinforced control mix, the hybrid fiber mixtures (SF + PVA, SF + PP, SF + JF, and SF + PP + PVA + JF) exhibited reductions in compressive strength of approximately 12.4 %, 11.6 %, 15.7 %, and 21.1 %, respectively, at the same age. Tensile and flexural strengths followed a similar trend of reduction with hybrid fiber incorporation. Relative to the tensile strength value of the control mix (10 MPa), hybrid fiber combinations (SF + PVA, SF + PP, SF + JF, and SF + PP + PVA + JF) resulted in tensile strength reductions of approximately 4 %, 5 %, 8 %, and 8 %. Similarly, their flexural strengths were notably decreased by about 9.6 %, 18.4 %, 22 %, and 24.4 %, respectively, when compared to the control mix that achieved 25 MPa with only SF. While steel fibers remain the most effective, incorporating natural or synthetic fibers like jute and polypropylene can provide acceptable γ-attenuation performance, with potential advantages in cost, flexibility, and sustainability. Hybrid combinations offer a promising balance, especially when multi-functionality (e.g., mechanical strength and γ-radiation shielding) is desired. The key novelty aspect of this work lies in examining fiber type as the main affecting variable on the radiation shielding behavior of UHPC, while combining experimental testing with MC simulation and Phy-X software for radiation shielding assessment.</div></div>","PeriodicalId":20861,"journal":{"name":"Radiation Physics and Chemistry","volume":"243 ","pages":"Article 113640"},"PeriodicalIF":2.8,"publicationDate":"2026-01-21","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"146014443","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Determination of lead isotopic ratios for nuclear forensic signatures from Mpumalanga Province, South Africa 南非姆普马兰加省核法医特征中铅同位素比率的测定
IF 2.8 3区 物理与天体物理 Q3 CHEMISTRY, PHYSICAL Pub Date : 2026-01-21 DOI: 10.1016/j.radphyschem.2026.113659
Murorunkwere Beatrice, Noxolo Manyoba, Manny Mathuthu
South Africa has seven uranium provinces scattered across different national provinces and consisting of different ore deposits. As a signatory to the Pelindaba NPT Treaty, the country is required by the International Atomic Energy Agency (IAEA) to develop its own National Nuclear Forensics Library (NNFL). Nuclear forensic science provides an essential tool to examine nuclear and other radioactive materials, as well as provide evidence that the material was out of regulatory control and was being trafficked. Once the nuclear or radioactive material is seized, the identification of the material and determination of its source is of prime importance. One of the key signatures in nuclear forensics is the isotopic analysis of lead (Pb), which can serve as a fingerprint for nuclear materials. The lead isotopic composition varies between the mining locations, depending on the geological settings. In this study, samples were collected from different mines of Mpumalanga Province. Lead isotopic ratios of the uranium ore were determined using inductively coupled plasma mass spectrometer (ICP-MS) PerkinElmer NexION 2000. According to the results of the lead-lead (Pb–Pb) geochemistry, detrital pyrites make up the mineralization of the uranium ore. The isotopic ratios differed among various ore bodies, which could act as their distinct fingerprints. Additionally, this study provided compelling evidence of the differences between BT and ET, and BT and WT samples. But for the ET-WT pair, it suggested that samples were most likely taken from the same mine shaft.
南非有七个铀矿省,分布在不同的国家省份,由不同的矿床组成。作为《佩林达巴核不扩散条约》的签署国,国际原子能机构(IAEA)要求该国发展自己的国家核法医图书馆(NNFL)。核法医科学是检查核材料和其他放射性材料的重要工具,并提供证据证明这些材料已脱离监管控制并正在被贩运。一旦核材料或放射性材料被扣押,材料的鉴定和其来源的确定是至关重要的。核取证的关键特征之一是铅(Pb)的同位素分析,它可以作为核材料的指纹。铅的同位素组成在不同的采矿地点有所不同,这取决于地质环境。在本研究中,样本采集自姆普马兰加省的不同矿山。采用PerkinElmer NexION 2000电感耦合等离子体质谱仪(ICP-MS)测定铀矿石的铅同位素比值。铅-铅(Pb-Pb)地球化学结果表明,碎屑黄铁矿构成了铀矿石的成矿作用,不同矿体的同位素比值不同,可以作为其独特的指纹。此外,本研究提供了令人信服的证据,证明BT和ET以及BT和WT样本之间存在差异。但对于ET-WT对,它表明样本很可能取自同一个矿井。
{"title":"Determination of lead isotopic ratios for nuclear forensic signatures from Mpumalanga Province, South Africa","authors":"Murorunkwere Beatrice,&nbsp;Noxolo Manyoba,&nbsp;Manny Mathuthu","doi":"10.1016/j.radphyschem.2026.113659","DOIUrl":"10.1016/j.radphyschem.2026.113659","url":null,"abstract":"<div><div>South Africa has seven uranium provinces scattered across different national provinces and consisting of different ore deposits. As a signatory to the Pelindaba NPT Treaty, the country is required by the International Atomic Energy Agency (IAEA) to develop its own National Nuclear Forensics Library (NNFL). Nuclear forensic science provides an essential tool to examine nuclear and other radioactive materials, as well as provide evidence that the material was out of regulatory control and was being trafficked. Once the nuclear or radioactive material is seized, the identification of the material and determination of its source is of prime importance. One of the key signatures in nuclear forensics is the isotopic analysis of lead (Pb), which can serve as a fingerprint for nuclear materials. The lead isotopic composition varies between the mining locations, depending on the geological settings. In this study, samples were collected from different mines of Mpumalanga Province. Lead isotopic ratios of the uranium ore were determined using inductively coupled plasma mass spectrometer (ICP-MS) PerkinElmer NexION 2000. According to the results of the lead-lead (Pb–Pb) geochemistry, detrital pyrites make up the mineralization of the uranium ore. The isotopic ratios differed among various ore bodies, which could act as their distinct fingerprints. Additionally, this study provided compelling evidence of the differences between BT and ET, and BT and WT samples. But for the ET-WT pair, it suggested that samples were most likely taken from the same mine shaft.</div></div>","PeriodicalId":20861,"journal":{"name":"Radiation Physics and Chemistry","volume":"242 ","pages":"Article 113659"},"PeriodicalIF":2.8,"publicationDate":"2026-01-21","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"146014447","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
On equivalence of metal-dielectric and single-layer dielectric waveguides in the problems of accelerator physics 加速器物理问题中金属介质波导与单层介质波导的等价性
IF 2.8 3区 物理与天体物理 Q3 CHEMISTRY, PHYSICAL Pub Date : 2026-01-21 DOI: 10.1016/j.radphyschem.2026.113644
M.I. Ivanyan , B.A. Grigoryan , A.H. Grigoryan , L.V. Aslyan , A.S. Vardanyan , V.G. Khachatryan , M.Z. Karalyan , V. Sh Avagyan
The impedance characteristics of a cylindrical waveguide with a two-layer wall are compared with similar characteristics both an open dielectric waveguide and a waveguide with a perfectly conducting wall inside coated by a dielectric layer. Based on the analysis, a conclusion is made about their interchangeability, and in some important cases – about the preference for using an open dielectric waveguide when solving problems of particle radiation in waveguides and their application.
将两层壁圆柱波导的阻抗特性与开放介质波导和内壁涂有介质层的波导的阻抗特性进行了比较。在分析的基础上,得出了它们的互换性,以及在一些重要的情况下,在解决波导中的粒子辐射问题及其应用时,更倾向于使用开放介质波导的结论。
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引用次数: 0
Intra-pulse sub-structure sensing of accelerated electrons 加速电子的脉冲内子结构传感
IF 2.8 3区 物理与天体物理 Q3 CHEMISTRY, PHYSICAL Pub Date : 2026-01-20 DOI: 10.1016/j.radphyschem.2026.113653
D.A. Bradley , A. Basaif , A. Oresegun , H.T. Zubair , H.M. Zin , K.Y. Choo , S.A. Ibrahim , F. Moradi , M. Alkhorayef , Tingyu Wang , Jianxiang Wen , E. Lewis , H.A. Abdul-Rashid
Examination is made of the temporal pattern of 6–15 MeV electrons, specifically at the dose-rates familiar in use of conventional linacs. The observed intra-pulse sub-structure variations are a manifestation of linac power modifications (modulation occurring within the duration of a single accelerator pulse) and inter-bunch electron repulsion. The measurement system, focal in providing sub-μs temporal resolution as well as capability in covering the dose per pulse dynamic range, comprises an in-house fabricated Ge-doped fiber-sensor, a photon-counting circuit, a multi-pixel photon counter (MPPC), and a fast digital oscilloscope. Together with the observed pulse decay-time and magnitude of afterglow, the variations in intra-pulse sub-structure captured by the system can be expected to have influence upon the accuracy of dose deposition. The measurement capability of the optical fiber scintillator system is shown to be sufficient to serve present needs, largely negating a desire for more sophisticated systems offering superior temporal resolution.
检查了6 - 15mev电子的时间模式,特别是在使用传统直线加速器时熟悉的剂量率下。观察到的脉冲内子结构变化是直线功率变化(在单个加速器脉冲持续时间内发生的调制)和束间电子排斥的表现。该测量系统的重点是提供亚μs的时间分辨率以及覆盖每脉冲剂量动态范围的能力,包括一个自制的掺锗光纤传感器、一个光子计数电路、一个多像素光子计数器(MPPC)和一个快速数字示波器。与观测到的脉冲衰减时间和余辉大小一起,系统捕获的脉冲内子结构的变化可以预期对剂量沉积的准确性产生影响。光纤闪烁体系统的测量能力被证明足以满足目前的需要,在很大程度上否定了对提供优越时间分辨率的更复杂系统的渴望。
{"title":"Intra-pulse sub-structure sensing of accelerated electrons","authors":"D.A. Bradley ,&nbsp;A. Basaif ,&nbsp;A. Oresegun ,&nbsp;H.T. Zubair ,&nbsp;H.M. Zin ,&nbsp;K.Y. Choo ,&nbsp;S.A. Ibrahim ,&nbsp;F. Moradi ,&nbsp;M. Alkhorayef ,&nbsp;Tingyu Wang ,&nbsp;Jianxiang Wen ,&nbsp;E. Lewis ,&nbsp;H.A. Abdul-Rashid","doi":"10.1016/j.radphyschem.2026.113653","DOIUrl":"10.1016/j.radphyschem.2026.113653","url":null,"abstract":"<div><div>Examination is made of the temporal pattern of 6–15 MeV electrons, specifically at the dose-rates familiar in use of conventional linacs. The observed intra-pulse sub-structure variations are a manifestation of linac power modifications (modulation occurring within the duration of a single accelerator pulse) and inter-bunch electron repulsion. The measurement system, focal in providing sub-μs temporal resolution as well as capability in covering the dose per pulse dynamic range, comprises an in-house fabricated Ge-doped fiber-sensor, a photon-counting circuit, a multi-pixel photon counter (MPPC), and a fast digital oscilloscope. Together with the observed pulse decay-time and magnitude of afterglow, the variations in intra-pulse sub-structure captured by the system can be expected to have influence upon the accuracy of dose deposition. The measurement capability of the optical fiber scintillator system is shown to be sufficient to serve present needs, largely negating a desire for more sophisticated systems offering superior temporal resolution.</div></div>","PeriodicalId":20861,"journal":{"name":"Radiation Physics and Chemistry","volume":"242 ","pages":"Article 113653"},"PeriodicalIF":2.8,"publicationDate":"2026-01-20","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"146014452","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Growth and scintillation performance of Tb/Dy: YAG, Tb/Dy/Lu: YAG and Tb/Dy/Ce: YAG crystals for X-ray imaging applications 用于x射线成像的Tb/ Dy: YAG、Tb/ Dy/ Lu: YAG和Tb/ Dy/ Ce: YAG晶体的生长和闪烁性能
IF 2.8 3区 物理与天体物理 Q3 CHEMISTRY, PHYSICAL Pub Date : 2026-01-20 DOI: 10.1016/j.radphyschem.2026.113655
Longxing Zheng , Linchao Mei , Zhaojie Zhu , Yizhi Huang , Chaoyang Tu , G. Lakshminarayana , Qianqian Lin , Yan Wang
In response to the environmental concerns and limited stability of traditional scintillators for current-mode radiation detectors, which are often used in computed tomography, baggage screening, and non-destructive testing, this study used the Czochralski method to successfully grow YAG-based crystals doped with trivalent rare-earth ions, including Tb/Dy: YAG, Tb/Dy/Ce: YAG, and Tb/Dy/Lu: YAG crystals. Their X-ray scintillation properties and imaging performance were comprehensively investigated. The results reveal that Tb/Dy/Ce: YAG and Tb/Dy/Lu: YAG exhibit radioluminescence intensities exceeding those of commercial Ce: GAGG and Ce: LuAG crystals, demonstrating high sensitivity to X-ray irradiation. The minimum detectable doses for Tb/Dy/Ce: YAG and Tb/Dy/Lu: YAG were measured to be as low as 173.65 nGy s−1 and 211 nGy s−1, respectively—both significantly below the typical diagnostic dose of 5.5 μGy s−1. Moreover, these crystals exhibit excellent radiation stability. X-ray imaging tests further confirm that Tb/Dy/Ce: YAG and Tb/Dy/Lu: YAG offer high spatial resolution limits of 10.17 lp mm−1 and 19.4 lp mm−1, respectively, delivering high-quality imaging results. These findings underscore the superior scintillation performance of Tb/Dy/Ce: YAG and Tb/Dy/Lu: YAG crystals, and highlight their strong potential for advanced X-ray detection and imaging applications.
针对当前模式辐射探测器的传统闪烁体(常用于计算机断层扫描、行李筛查和无损检测)的环境问题和有限的稳定性问题,本研究使用Czochralski方法成功生长了掺杂三价稀土离子的YAG基晶体,包括Tb/Dy: YAG、Tb/Dy/Ce: YAG和Tb/Dy/Lu: YAG晶体。对其x射线闪烁特性和成像性能进行了全面研究。结果表明,Tb/Dy/Ce: YAG和Tb/Dy/Lu: YAG晶体的辐射发光强度超过了商用Ce: GAGG和Ce: LuAG晶体,对x射线辐射具有较高的灵敏度。Tb/Dy/Ce: YAG和Tb/Dy/Lu: YAG的最低检测剂量分别为173.65 μGy s−1和211 μGy s−1,均显著低于典型诊断剂量5.5 μGy s−1。此外,这些晶体表现出优异的辐射稳定性。x射线成像测试进一步证实,Tb/Dy/Ce: YAG和Tb/Dy/Lu: YAG分别提供10.17 lp mm−1和19.4 lp mm−1的高空间分辨率限制,提供高质量的成像结果。这些发现强调了Tb/Dy/Ce: YAG和Tb/Dy/Lu: YAG晶体优越的闪烁性能,并突出了它们在先进x射线探测和成像应用中的强大潜力。
{"title":"Growth and scintillation performance of Tb/Dy: YAG, Tb/Dy/Lu: YAG and Tb/Dy/Ce: YAG crystals for X-ray imaging applications","authors":"Longxing Zheng ,&nbsp;Linchao Mei ,&nbsp;Zhaojie Zhu ,&nbsp;Yizhi Huang ,&nbsp;Chaoyang Tu ,&nbsp;G. Lakshminarayana ,&nbsp;Qianqian Lin ,&nbsp;Yan Wang","doi":"10.1016/j.radphyschem.2026.113655","DOIUrl":"10.1016/j.radphyschem.2026.113655","url":null,"abstract":"<div><div>In response to the environmental concerns and limited stability of traditional scintillators for current-mode radiation detectors, which are often used in computed tomography, baggage screening, and non-destructive testing, this study used the Czochralski method to successfully grow YAG-based crystals doped with trivalent rare-earth ions, including Tb/Dy: YAG, Tb/Dy/Ce: YAG, and Tb/Dy/Lu: YAG crystals. Their X-ray scintillation properties and imaging performance were comprehensively investigated. The results reveal that Tb/Dy/Ce: YAG and Tb/Dy/Lu: YAG exhibit radioluminescence intensities exceeding those of commercial Ce: GAGG and Ce: LuAG crystals, demonstrating high sensitivity to X-ray irradiation. The minimum detectable doses for Tb/Dy/Ce: YAG and Tb/Dy/Lu: YAG were measured to be as low as 173.65 nGy s<sup>−1</sup> and 211 nGy s<sup>−1</sup>, respectively—both significantly below the typical diagnostic dose of 5.5 μGy s<sup>−1</sup>. Moreover, these crystals exhibit excellent radiation stability. X-ray imaging tests further confirm that Tb/Dy/Ce: YAG and Tb/Dy/Lu: YAG offer high spatial resolution limits of 10.17 lp mm<sup>−1</sup> and 19.4 lp mm<sup>−1</sup>, respectively, delivering high-quality imaging results. These findings underscore the superior scintillation performance of Tb/Dy/Ce: YAG and Tb/Dy/Lu: YAG crystals, and highlight their strong potential for advanced X-ray detection and imaging applications.</div></div>","PeriodicalId":20861,"journal":{"name":"Radiation Physics and Chemistry","volume":"242 ","pages":"Article 113655"},"PeriodicalIF":2.8,"publicationDate":"2026-01-20","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"146014453","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Quantification of ionic migration in TlBr gamma-ray detector via temperature-dependent conductivity measurements 通过温度相关电导率测量的TlBr伽玛射线探测器中离子迁移的量化
IF 2.8 3区 物理与天体物理 Q3 CHEMISTRY, PHYSICAL Pub Date : 2026-01-20 DOI: 10.1016/j.radphyschem.2026.113652
Beomjun Park , Jiwon Seo , Ill Hyuk Han , Jihwan Boo , Jangwon Byun , Seungho Song , Dakyoung Lee , Joo-Hong Lee , Jin-Wook Lee , Jung-Yeol Yeom , Geehyun Kim
Thallium bromide (TlBr) is a promising room-temperature gamma-ray detector material owing to its high atomic number, wide bandgap, and relatively simpler crystal growth process than CdTe-based crystals. However, its practical application is hindered by ionic migration and polarization effects that degrade long-term stability under high bias voltages. In this work, we present a quantitative methodology to evaluate ionic transport in TlBr detectors through temperature-dependent conductivity measurements in the 193–323 K range. By separating electronic and ionic contributions under both current- and voltage-bias conditions, we extracted ionic conductivity values and determined the activation energy of ion migration. The activation energy varied with the vertical position of zone-refined TlBr ingots. These values were correlated with device performance, including photocurrent degradation under X-ray irradiation and peak channel shifts in gamma-ray spectra. The results reveal that ionic migration critically impacts charge collecting ability and spectral stability. This study proposed a standardized framework for quantifying ionic migration in TlBr detectors, offering valuable guidance for evaluating the operational stability in TlBr detectors. The activation energy of ion migration can serve as a robust metric for quantitatively comparing compound semiconductor detectors, whose ions migrate.
溴化铊(TlBr)具有原子序数高、带隙宽、晶体生长过程相对简单等优点,是一种很有前途的室温伽马射线探测器材料。然而,它的实际应用受到离子迁移和极化效应的阻碍,这些效应会降低高偏置电压下的长期稳定性。在这项工作中,我们提出了一种定量方法,通过在193-323 K范围内的温度相关电导率测量来评估TlBr探测器中的离子传输。通过分离电流和电压偏置条件下的电子和离子贡献,我们提取了离子电导率值,并确定了离子迁移的活化能。区域精炼TlBr坯料的活化能随其垂直位置的变化而变化。这些值与器件性能相关,包括x射线照射下的光电流退化和伽马射线能谱中的峰值通道移位。结果表明,离子迁移严重影响电荷收集能力和光谱稳定性。本研究提出了一种量化TlBr探测器中离子迁移的标准化框架,为评价TlBr探测器的运行稳定性提供了有价值的指导。离子迁移活化能可以作为定量比较离子迁移的化合物半导体探测器的可靠指标。
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Radiation Physics and Chemistry
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