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Mechanism of IR assisted charge state conversion of nitrogen vacancy centre in diamond 红外辅助金刚石中氮空位中心电荷态转换的机理
IF 0.9 4区 物理与天体物理 Q3 PHYSICS, MULTIDISCIPLINARY Pub Date : 2025-06-17 DOI: 10.1007/s40042-025-01418-2
Nhu Anh Nguyen, Juil Hwang, Seunghyun Bang, Seonghyeon Kang, Hyunjong Lee, Kwang-Geol Lee, Sangwon Oh

The negatively charged state of nitrogen vacancy centre (NV) in diamond have been exploited in recent studies of magnetometry and quantum information processing. Nevertheless, the useful signal of NV for these applications can be deteriorated by the neutrally charged state (NV0) which acts as backgrounds. In recent studies, it has been reported that simultaneous excitation of green (532 nm) laser combined with infrared (1030, 1040, 1064 nm) laser can enhance the emission from NV while suppressing signal from NV0. Under such laser excitation conditions, however, the underlying mechanism of the photo-induced conversion between two charged states is still not fully understood. In our work, based on multi-photon absorption of IR, we propose a simple model to explain the mutual contribution of green and IR lasers to promote the NV population. Our model recovers the detailed featured observed in our experiment, and also can reconcile the results in previous literatures.

金刚石中氮空位中心(NV -)的负电荷态在磁力学和量子信息处理的研究中得到了广泛的应用。然而,对于这些应用来说,NV -的有用信号可能会因充当背景的中性带电状态(NV0)而恶化。近年来有研究报道,绿色(532 nm)激光与红外(1030、1040、1064 nm)激光同时激发可以增强NV -的发射,同时抑制NV0的信号。然而,在这种激光激发条件下,光诱导两种带电态转换的潜在机制仍未完全了解。在我们的工作中,基于红外的多光子吸收,我们提出了一个简单的模型来解释绿色和红外激光对促进NV -人口的相互贡献。我们的模型恢复了我们实验中观察到的详细特征,也能与以往文献的结果相吻合。
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引用次数: 0
Toxic gas adsorption on in-plane monolayer heterostructure of transition metal dichalcogenide: a first-principles study 过渡金属二硫化物平面内单层异质结构对有毒气体的吸附:第一性原理研究
IF 0.9 4区 物理与天体物理 Q3 PHYSICS, MULTIDISCIPLINARY Pub Date : 2025-06-17 DOI: 10.1007/s40042-025-01414-6
Vipin Kumar, Pushpendra Kumar, Gyanendra Kumar Maurya, Jin Seog Gwag

Heterostructure materials have gained significant research interest due to their distinct physical properties. Toxic gases severely affect the respiratory system of the human body. We propose an in-plane monolayer heterostructure based on transition metal dichalcogenides (TMD) to investigate the effect of toxic gas adsorption. The toxic gas molecules are adsorbed on top of the chalcogen-atom of the in-plane TMD heterostructure. The electronic structure calculations reflect that the band gap of the proposed host material remains almost unchanged upon the adsorption of gas molecules. The gas adsorption leads to the nearly unaltered valance band and conduction band. This is due to the lack of hybridization between the molecular orbitals of the adsorbate and the host material. The Mulliken population method confirms the charge transfer between the host in-plane TMD heterostructure and the adsorbed gas molecules. Furthermore, it is observed that the adsorption of gas molecules significantly changes the dielectric and optical response of the TMD in-plane heterostructure. Our investigations demonstrate that the proposed material has the potential for toxic gas sensing.

异质结构材料由于其独特的物理性质而引起了人们极大的研究兴趣。有毒气体严重影响人体的呼吸系统。我们提出了一种基于过渡金属二硫化物(TMD)的平面内单层异质结构来研究有毒气体吸附的影响。有毒气体分子被吸附在平面内TMD异质结构的硫原子上。电子结构计算表明,在气体分子的吸附作用下,所提出的主体材料的带隙几乎保持不变。气体吸附导致价带和导带几乎没有变化。这是由于在吸附物和宿主物质的分子轨道之间缺乏杂化。Mulliken种群法证实了寄主平面内TMD异质结构与吸附气体分子之间的电荷转移。此外,还观察到气体分子的吸附显著改变了TMD平面异质结构的介电和光学响应。我们的研究表明,所提出的材料具有潜在的有毒气体传感。
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引用次数: 0
Enhanced weak value amplification via photon recycling 通过光子循环增强弱值放大
IF 0.9 4区 物理与天体物理 Q3 PHYSICS, MULTIDISCIPLINARY Pub Date : 2025-06-11 DOI: 10.1007/s40042-025-01401-x
Seung-Yeun Yoo, Dong-Gil Im, U-Shin Kim, Yosep Kim, Yoon-Ho Kim

Weak value amplification (WVA) is a powerful technique in quantum metrology, enabling the detection of small signals that are typically challenging to measure. However, conventional WVA methods often suffer from low post-selection probabilities, which diminish the practical advantages of amplified signals. In this work, we propose and demonstrate an improved WVA scheme using photon recycling, where non-post-selected photons are reused in additional amplification processes. By implementing this recycling-enhanced method with effectively three photon recycling rounds, we achieve improvement of a factor of 1.66 ± 0.01 in post-selection probability and 1.56 ± 0.01 in amplification of the weak value. Additionally, we simulate the impact of optical path losses on the WVA probability. This allows us to determine the saturation limits of our photon recycling approach. This work provides a pathway toward more efficient WVA, significantly advancing precision measurement capabilities in quantum metrology and related sensing applications.

弱值放大(WVA)是量子计量中的一项强大技术,可以检测到通常难以测量的小信号。然而,传统的WVA方法往往存在后选择概率低的问题,这削弱了放大信号的实际优势。在这项工作中,我们提出并演示了一种使用光子回收的改进的WVA方案,其中非后选光子在额外的放大过程中被重复使用。通过有效的三次光子回收,我们将后选择概率提高了1.66±0.01倍,弱值放大提高了1.56±0.01倍。此外,我们还模拟了光路损耗对WVA概率的影响。这使我们能够确定我们的光子回收方法的饱和极限。这项工作为更高效的WVA提供了一条途径,显著提高了量子计量和相关传感应用的精确测量能力。
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引用次数: 0
Analysis of electric field in asymmetrically arranged dielectric media using simple mathematical methods 用简单的数学方法分析非对称排列介质中的电场
IF 0.9 4区 物理与天体物理 Q3 PHYSICS, MULTIDISCIPLINARY Pub Date : 2025-06-11 DOI: 10.1007/s40042-025-01412-8
In-Su Han

Calculations of electric field strength in various structures are essential in the design of most electrical and electronic equipment and devices, because electric field tendencies vary greatly with respect to a given voltage, dielectric constants of insulating media, and the geometry of the structure. Electric field simulation is very convenient to calculate and predict electric field tendencies, but it is time-consuming, expensive, and difficult to understand the physical meaning with. To address this problem in a simpler way than time-consuming and costly electric field simulations, we derive analytical equation-based solutions for pre-designing electrical and electronic devices. In this paper, we consider a simple mathematical model based on Laplace equation, particularly with respect to asymmetrically arranged dielectric structures. In these structures, we analyze electric field tendencies using axis rotation and Legendre polynomials associated with each fitted axis, especially in asymmetrically arranged models.

在大多数电气和电子设备和装置的设计中,计算各种结构中的电场强度是必不可少的,因为电场的趋势随着给定的电压、绝缘介质的介电常数和结构的几何形状而变化很大。电场模拟计算和预测电场趋势非常方便,但耗时长,成本高,且难以理解其物理意义。为了以比耗时和昂贵的电场模拟更简单的方式解决这个问题,我们推导了基于分析方程的预先设计电气和电子设备的解决方案。在本文中,我们考虑了一个基于拉普拉斯方程的简单数学模型,特别是关于不对称排列的介电结构。在这些结构中,我们使用轴旋转和与每个拟合轴相关的勒让德多项式来分析电场趋势,特别是在不对称排列的模型中。
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引用次数: 0
Improvement of dose uniformity using a backscatter plate in a single X-ray source for blood irradiator: Monte Carlo simulation approach 使用后向散射板改善单一x射线血液辐照源的剂量均匀性:蒙特卡罗模拟方法
IF 0.9 4区 物理与天体物理 Q3 PHYSICS, MULTIDISCIPLINARY Pub Date : 2025-06-11 DOI: 10.1007/s40042-025-01413-7
Dung Thi Tran, Minho Kim, Bong hwan Hong, Chawon Park, Seungwoo Park

X-ray irradiators are used to inactivate T-cell function to prevent the risk of transfusion-associated graft-versus-host disease (TA-GVHD). Absorbed dose of 25–50 Gy within 5 min with a dose uniformity ratio (DUR) below 1.5 are recommended for inactivating T cells while sparing other blood components. In this study, different backscatter plate materials were utilized to improve dose uniformity within the entire blood phantom for a single X-ray blood irradiator using Monte Carlo simulation (MCNP6). Based on the simulation results, Be, acrylic, and Al were selected as backscatter plates for their high backscatter ratios. Dose uniformity across the entire blood phantom improved by 29.56%, 21.43%, and 10.44% when using 10 cm Be, 10 cm acrylic, and 4 cm Al as backscatter plates, respectively. Using a backscatter plate improved dose uniformity across the entire blood phantom hence improving blood irradiation efficiency. However, DUR exceeding 1.5 is due to substantial dose difference between the surface and bottom regions of the blood phantom. In future studies, additional filters will be explored to improve DUR and achieve the recommended value.

x射线照射器用于灭活t细胞功能,以防止输血相关移植物抗宿主病(TA-GVHD)的风险。建议在5min内吸收剂量为25 - 50gy,剂量均匀比(DUR)低于1.5,以灭活T细胞,同时保留其他血液成分。在本研究中,采用蒙特卡罗模拟(MCNP6),利用不同的后向散射板材料来改善单个x射线血液辐照器全血模内的剂量均匀性。基于仿真结果,选择Be、丙烯酸和Al等具有高后向散射比的材料作为后向散射板。使用10 cm Be、10 cm丙烯酸和4 cm Al作为后向散射板,整个血模的剂量均匀性分别提高了29.56%、21.43%和10.44%。使用后向散射板改善了整个血模体的剂量均匀性,从而提高了血液辐照效率。然而,DUR超过1.5是由于血幻影的表面和底部区域之间存在巨大的剂量差异。在未来的研究中,将探索额外的滤波器来提高DUR并达到推荐值。
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引用次数: 0
Dependence of ozone concentration on the moisture barrier properties of aluminum oxide using atomic layer deposition 原子层沉积法研究臭氧浓度对氧化铝隔湿性能的影响
IF 0.9 4区 物理与天体物理 Q3 PHYSICS, MULTIDISCIPLINARY Pub Date : 2025-06-10 DOI: 10.1007/s40042-025-01410-w
Yeongtae Choi, Seokyoon Shin, Changwoo Byun, Hee-Soo Kim, Hyeongtag Jeon

As a thin film encapsulation method, atomic layer deposition (ALD) has the potential to provide superior protection for organic light-emitting diodes (OLEDs). However, the application of H2O and O2 plasma in the traditional ALD process has not yet resulted in a successful moisture barrier. The large dipole moment of H2O may result in excess residual hydroxyl groups, and the flux of charged particles from O2 plasma can damage organic materials. Here, we suggest the use of ozone (O3) as an alternative reactant to mitigate these limiting factors. It is a powerful oxidizer and is much more volatile than other oxidizing agents. Thus, O3 is a promising oxygen source to improve moisture barrier properties for OLEDs. This work describes the dependence of O3 concentration on the moisture barrier properties of Al2O3 thin films prepared by ozone-based ALD at 100 °C. Trimethylaluminum and O3 were utilized as aluminum and oxygen precursors, respectively. The O3 concentration varied from 100 to 400 g/m3 in increments of 100 g/m3. An increase in O3 concentration resulted in a significant enhancement in the moisture barrier performance of Al2O3, with values improving from 7.1 × 10⁻4 to 1.9 × 10⁻5 g/m2/day. Further characterization indicated that Al2O3 thin films produced at elevated O3 concentrations exhibited superior physical and chemical properties compared to those generated at lower O3 concentrations.

作为一种薄膜封装方法,原子层沉积(ALD)具有为有机发光二极管(oled)提供优越保护的潜力。然而,H2O和O2等离子体在传统ALD工艺中的应用尚未成功实现水分屏障。H2O的大偶极矩会导致多余的羟基残留,而来自O2等离子体的带电粒子通量会破坏有机材料。在这里,我们建议使用臭氧(O3)作为替代反应物来减轻这些限制因素。它是一种强氧化剂,比其他氧化剂挥发性更强。因此,O3是一种很有前途的氧源,可以改善oled的防潮性能。本工作描述了O3浓度对臭氧基ALD在100°C下制备的Al2O3薄膜防潮性能的依赖关系。以三甲基铝和O3分别作为铝和氧的前驱体。O3浓度变化范围为100 ~ 400 g/m3,每增加100 g/m3。O3浓度的增加导致Al2O3的防潮性能显著增强,其值从7.1 × 10⁻4提高到1.9 × 10⁻5 g/m2/天。进一步的表征表明,在高O3浓度下制备的Al2O3薄膜比在低O3浓度下制备的薄膜具有更好的物理和化学性能。
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引用次数: 0
Dosimetric evaluation of large-area proton minibeam radiation therapy system for clinical applications 大面积质子微束放射治疗系统临床应用的剂量学评价
IF 0.9 4区 物理与天体物理 Q3 PHYSICS, MULTIDISCIPLINARY Pub Date : 2025-06-10 DOI: 10.1007/s40042-025-01387-6
Jusung Kim, Kyeongyun Park, Dohyeon Kim, Hak Soo Kim, Chankyu Kim, Jong Hwi Jeong, Dongho Shin, Se Byeong Lee, Myeongsoo Kim, Tae Hyun Kim, Young Kyung Lim

Proton minibeam radiation therapy (pMBRT) has emerged as a promising radiation treatment modality, offering enhanced tissue-sparing effects compared to conventional proton therapy. For clinical application, we developed a pMBRT system with the largest field size (30 × 40 cm2) in the world, and conducted a comprehensive dosimetric evaluation of its characteristics. Our system consists of a large-area multi-slit collimator (MSC), a depth-dose modulator, a neutron absorber, a range shifter, and a custom snout compatible with the conventional proton therapy machines. We investigated two energy conditions (170 MeV with and 200 MeV without a range shifter), varying air gap and scatterer configurations to simulate clinical treatments. Lateral dose profiles showed peak and valley dose standard deviations below 5.5% of their respective means. Analysis of scatterer characteristics using the peak-to-valley dose ratio (PVDR) showed that as scatterer thickness increased, the PVDR approached 1 just beneath the phantom surface. Conversely, under low-scattering conditions, the PVDR at the phantom surface exceeded 15. For shallow tumors, a high PVDR at the surface is desired, with a rapid decrease near the tumor's depth. The depth-dose modulation effect was analyzed using air gaps and lead scatterers to amplify multiple Coulomb scattering. Monte Carlo simulations confirmed a significant reduction in secondary neutrons due to the neutron absorber. In conclusion, our system generates minibeams with a uniform dose envelope. Excellent depth-dose modulation using scatterers facilitates simultaneous skin protection and shallow-depth tumor treatment. By mitigating secondary neutrons, the system can also reduce radiation toxicity, enhancing its clinical viability.

质子微束放射治疗(pMBRT)已经成为一种很有前途的放射治疗方式,与传统的质子治疗相比,它提供了更好的组织保留效果。为了临床应用,我们开发了世界上最大视野尺寸(30 × 40 cm2)的pMBRT系统,并对其特性进行了全面的剂量学评价。我们的系统由一个大面积多缝准直器(MSC)、一个深度剂量调制器、一个中子吸收器、一个范围移位器和一个与传统质子治疗机兼容的定制喷嘴组成。我们研究了两种能量条件(170 MeV带和200 MeV不带移程器),不同的气隙和散射体配置来模拟临床治疗。横向剂量谱显示峰谷剂量标准差低于各自平均值的5.5%。利用峰谷剂量比(PVDR)分析散射体特性表明,随着散射体厚度的增加,PVDR接近于1。相反,在低散射条件下,模体表面的PVDR大于15。对于浅层肿瘤,需要在表面有较高的PVDR,在肿瘤深度附近迅速降低。利用气隙和铅散射体放大多重库仑散射,分析了深度剂量调制效应。蒙特卡罗模拟证实,由于中子吸收剂,二次中子显著减少。总之,我们的系统产生具有均匀剂量包络的微光束。利用散射体进行出色的深度剂量调制,有助于同时保护皮肤和浅层肿瘤治疗。通过减少次级中子,该系统还可以降低辐射毒性,提高其临床生存能力。
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引用次数: 0
Enhancing gamma-ray shielding performance of HDPE composites using PbO and Bi₂O₃ reinforcements PbO和Bi₂O₃增强HDPE复合材料的γ射线屏蔽性能
IF 0.9 4区 物理与天体物理 Q3 PHYSICS, MULTIDISCIPLINARY Pub Date : 2025-06-06 DOI: 10.1007/s40042-025-01405-7
M. R. Alipoor

The purpose of the research presented is to investigate the protective capacities against gamma-ray and X-ray of high-density polyethylene materials reinforced with different concentrations oxide of lead and bismuth. The materials under study were exposed to a range of gamma ray energy levels and their protective efficiency is quantitatively evaluated through the analytical measurement of several parameters, including mass attenuation coefficient, linear attenuation coefficient and half-value layer. The results derived from both theoretical calculations by Phy-x and simulated outcomes by the Geant4 simulation tool demonstrate a commendable level of correlation and consistency, thereby reinforcing the validity of the findings reported in this study. As photon energy increased, the radiation protection efficiency decreased, while as thickness increased, the radiation protection efficiency increased. It is particularly noteworthy that high-density polyethylene composites, reinforced with specific concentrations of lead and bismuth, exhibit superior radiation shielding properties. This remarkable performance can be attributed to the strategic dispersion of heavy metals as well as their associated density characteristics, which together contribute to the effectiveness of these materials in reducing harmful radiation. Finally, the fast neutron removal cross section was also calculated for polymer composites. In conclusion, these findings emphasize the potential of lead–bismuth-reinforced high-density polyethylene composites as promising materials for radiation shielding applications.

研究了不同浓度的铅铋氧化物增强高密度聚乙烯材料对γ射线和x射线的防护能力。将所研究的材料暴露在一定的伽马射线能级下,通过对质量衰减系数、线性衰减系数和半值层等参数的分析测量,定量评价其防护效率。Phy-x的理论计算结果和Geant4模拟工具的模拟结果都显示出值得称赞的相关性和一致性,从而加强了本研究报告中发现的有效性。随着光子能量的增加,辐射防护效率降低,而随着厚度的增加,辐射防护效率提高。特别值得注意的是,用特定浓度的铅和铋增强的高密度聚乙烯复合材料表现出优越的辐射屏蔽性能。这种卓越的性能可归因于重金属的战略性分散及其相关的密度特性,这些特性共同有助于这些材料在减少有害辐射方面的有效性。最后,计算了聚合物复合材料的快中子去除截面。总之,这些发现强调了铅铋增强高密度聚乙烯复合材料作为辐射屏蔽材料的潜力。
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引用次数: 0
Impact of prior reactions on the recovery behavior of MoS2 transistors 先前反应对二硫化钼晶体管恢复行为的影响
IF 0.9 4区 物理与天体物理 Q3 PHYSICS, MULTIDISCIPLINARY Pub Date : 2025-06-04 DOI: 10.1007/s40042-025-01406-6
Hyunjin Ji

The electrical property changes in monolayer MoS2 transistors were analyzed after bistriflimide (H-TFSI) treatment, which dissociates into hydrogen cations and TFSI anions in solution, followed by intensive acetone rinsing. Charge trapping effects were examined by varying the delay time (0.1, 1, 5 s) between voltage application and current measurement, revealing changes in electrical hysteresis. While degradation in device performance was primarily attributed to TFSI anion adsorbates, a transition to counterclockwise hysteresis was observed as H+ ion effects became more pronounced, leading to a reduction of degradation or slight improvement in performance. To further assess interface trap characteristics, low-frequency noise modeling was conducted for each device condition, enabling the extraction of trap density and Coulomb scattering effects. The reversibility of H-TFSI treatment effects was also evaluated through a 24-h acetone rinse. The results indicated that the impact of H+ ions was almost entirely reversed, restoring the interface trap density to its initial state. However, carrier mobility did not fully recover, suggesting that residual TFSI anion adsorbates remained on the surface, contributing to persistent degradation. These findings demonstrate that hydrogen cations can sufficiently penetrate and exit from both MoS2 and SiO2, allowing defect neutralization to be reset through aggressive rinsing. In contrast, TFSI anions, which adsorb onto the surface, are not fully removable using liquid-phase cleaning methods. This highlights a potential processing strategy in which a passivation layer, impermeable to large molecules, is placed on top of the device before H-TFSI treatment, enabling selective defect passivation solely by H+ ions.

分析了双striflimide (H-TFSI)在溶液中解离成氢阳离子和TFSI阴离子后,经丙酮强烈冲洗后单层MoS2晶体管电学性能的变化。通过改变电压施加和电流测量之间的延迟时间(0.1,1,5 s)来检测电荷捕获效应,揭示电滞后的变化。虽然器件性能的下降主要归因于TFSI阴离子吸附,但随着H+离子效应变得更加明显,观察到向逆时针滞后的转变,导致性能下降或略有改善。为了进一步评估界面陷阱特性,对每种设备条件进行了低频噪声建模,从而提取陷阱密度和库仑散射效应。H-TFSI处理效果的可逆性也通过24小时丙酮冲洗来评估。结果表明,H+离子的影响几乎完全逆转,使界面阱密度恢复到初始状态。然而,载流子迁移率并没有完全恢复,这表明残留的TFSI阴离子吸附物仍然存在于表面,有助于持续降解。这些研究结果表明,氢离子可以充分渗透并从MoS2和SiO2中逸出,从而通过积极的冲洗来重置缺陷中和。相反,吸附在表面的TFSI阴离子不能用液相清洗方法完全去除。这突出了一种潜在的处理策略,即在H- tfsi处理之前,在器件顶部放置一层不渗透大分子的钝化层,从而仅通过H+离子实现选择性缺陷钝化。
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引用次数: 0
T–X phase diagram calculated for the tilted smectic–hexatic transitions in the binary mixtures (THI14 + MPR6) 二元混合物(THI14 + MPR6)中倾斜近六态转变的T-X相图计算
IF 0.9 4区 物理与天体物理 Q3 PHYSICS, MULTIDISCIPLINARY Pub Date : 2025-06-04 DOI: 10.1007/s40042-025-01396-5
Ozlem Tari, Hamit Yurtseven

This study gives our calculation of the (T-X) phase diagram for the mainly smectic–hexatic phase transitions in the binary mixtures of THI14 + MPR6. By expanding the free energy in terms of the order parameters with the biquadratic coupling in the Landau mean field model, the phase line equations are obtained and they are fitted to the experimental (T-X) data from the literature. The first-order and the second-order transitions are considered between the smectic and hexatic phases in the existence of the triple and tricritical (TCP) points in those binary mixtures. Our study indicates that the observed behavior of the first-order and the second-order (smectic–hexatic) transitions can be characterized in the binary mixtures studied by the Landau models given here.

本研究给出了我们计算的THI14 + MPR6二元混合物中主要的近六态相变的(T-X)相图。在朗道平均场模型中,通过双二次耦合将自由能展开为阶参数,得到了相线方程,并与文献中(T-X)实验数据进行了拟合。考虑了二元混合物中存在三临界点和三临界点时的一阶和二阶过渡。我们的研究表明,我们所观察到的一阶和二阶(近六态)跃迁行为可以用本文给出的朗道模型来表征。
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引用次数: 0
期刊
Journal of the Korean Physical Society
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