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Parameter optimization of light outcoupling structures for high-efficiency organic light-emitting diodes 高效有机发光二极管光解耦结构参数优化
Pub Date : 2020-07-17 DOI: 10.1063/5.0022497
Dinara Samigullina, P. Will, L. Galle, Simone Lenk, J. Grothe, S. Kaskel, S. Reineke
Organic light-emitting diodes (OLEDs) have successfully entered the display market and continue to be attractive for many other applications. As state-of-the-art OLEDs can reach an internal quantum efficiency (IQE) of almost 100 %, light outcoupling remains one of the major screws left to be turned. The fact that no superior outcoupling structure has been found underlines that further investigations are needed to understand their prospect. In this paper, we use two-dimensional titanium dioxide (2D TiO$_2$) block arrays as a model of an internal light outcoupling structure and investigate the influence of its geometrical parameters on achieving the highest external quantum efficiency (EQE) for OLEDs. The multivariable problem is evaluated with the visual assistance of scatter plots, which enables us to propose an optimal period range and block width-to-distance ratio. The highest EQE achieved is 45.2 % with internal and external structures. This work contributes to the highly desired prediction of ideal light outcoupling structures in the future.
有机发光二极管(oled)已成功进入显示市场,并继续吸引许多其他应用。由于最先进的oled可以达到几乎100%的内部量子效率(IQE),光脱耦仍然是剩下的主要问题之一。没有发现更好的脱耦结构这一事实表明,需要进一步的研究来了解它们的前景。本文采用二维二氧化钛(2D TiO$_2$)块阵列作为内部光解耦结构的模型,研究了其几何参数对oled实现最高外量子效率(EQE)的影响。用散点图的视觉辅助来评估多变量问题,这使我们能够提出最优的周期范围和块宽距离比。内部和外部结构实现的最高EQE为45.2%。这项工作有助于预测未来理想的光脱耦结构。
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引用次数: 3
Perfect Absorption in Mirror-Symmetric Acoustic Metascreens 镜面对称声学元屏的完美吸收
Pub Date : 2020-07-16 DOI: 10.1103/physrevapplied.14.054055
V. Romero-Garc'ia, N. Jim'enez, J. Groby, A. Merkel, Vincent Tournat, G. Theocharis, O. Richoux, V. Pagneux
Mirror-symmetric acoustic metascreens producing perfect absorption independently of the incidence side are theoretically and experimentally reported in this work. The mirror-symmetric resonant building blocks of the metascreen support symmetric and antisymmetric resonances that can be tuned to be at the same frequency (degenerate resonances). The geometry of the building blocks is optimized to critically couple both the symmetric and the antisymmetric resonances at the same frequency allowing perfect absorption of sound from both sides of the metascreen. A hybrid analytical model based on the transfer matrix method and the modal decomposition of the exterior acoustic field is developed to analyze the scattering properties of the metascreen. The resulting geometry is 3D printed and experimentally tested in an impedance tube. Experimental results agree well with the theoretical predictions proving the efficiency of these metascreens for the perfect absorption of sound in the ventilation problems.
在理论上和实验上,本研究报告了镜面对称声超屏产生独立于入射侧的完美吸收。元屏幕的镜像对称共振构建块支持对称和反对称共振,可以调谐到相同的频率(简并共振)。构建块的几何结构经过优化,可以在同一频率上严格耦合对称和反对称共振,从而完美地吸收来自元屏两侧的声音。建立了基于传递矩阵法和外声场模态分解的混合解析模型来分析元屏的散射特性。所得到的几何形状是3D打印的,并在阻抗管中进行实验测试。实验结果与理论预测吻合较好,证明了在通风问题中,这些超滤屏具有较好的吸声效果。
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引用次数: 17
High Contrast Probe Cleavage Detection 高对比度探针解理检测
Pub Date : 2020-07-15 DOI: 10.1364/FIO.2020.JTU7C.3
M. Dubrovsky, Morgan G. Blevins, S. Boriskina, Diedrik Vermeulen SiPhox Inc., Cambridge, Ma, Usa, M. I. O. Technology
Photonic biosensors that use optical resonances to amplify biological signals associated with the adsorption of low-index biological markers offer high-sensitivity detection capability, real-time readout, and scalable low-cost fabrication. However, they lack inherent target specificity and can be sensitive to temperature variations and other noise sources. In this letter, we introduce a concept of the High Contrast Probe Cleavage Detection (HCPCD) mechanism, which makes use of the dramatic optical signal amplification caused by cleavage of large numbers of high-contrast nanoparticle labels instead of the adsorption of low-index biological molecules. We illustrate numerically the HCPCD detection mechanism with an example of a silicon ring resonator as an optical transducer with gold and silicon nanoparticles as high-contrast labels. Simulations show that it is possible to detect a single cleavage-event by monitoring spectral shifts of micro-ring resonances. Furthermore, detection specificity and signal amplification can be achieved through the use of collateral nucleic acid cleavage caused by enzymes such as CAS12a and CAS13 after binding to a target DNA/RNA sequence.
光子生物传感器利用光学共振来放大与低指数生物标记物吸附相关的生物信号,提供高灵敏度检测能力、实时读数和可扩展的低成本制造。然而,它们缺乏固有的目标特异性,并且可能对温度变化和其他噪声源敏感。在这封信中,我们介绍了高对比度探针解理检测(High Contrast Probe Cleavage Detection, HCPCD)机制的概念,该机制利用大量高对比度纳米颗粒标签解理引起的显著光信号放大,而不是吸附低指数的生物分子。我们用一个硅环谐振器作为光学换能器,用金纳米粒子和硅纳米粒子作为高对比度标签,数值说明了HCPCD检测机制。模拟表明,通过监测微环共振的光谱位移,可以检测到单个解理事件。此外,利用CAS12a和CAS13等酶与靶DNA/RNA序列结合后引起的侧链核酸裂解,可以实现检测特异性和信号扩增。
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引用次数: 2
Communication—Conductive Paintable 2D Layered MoS2 Inks 通信导电可涂二维层状MoS2油墨
Pub Date : 2020-07-15 DOI: 10.1149/2162-8777/abc1c0
Elaine Carroll, Darragh Buckley, D. McNulty, C. O’Dwyer
Conductive and paintable inks of 2D layered MoS2 with aspect ratio-dependent conductivity are demonstrated. Using ultrasonically assisted solvent-exfoliation of MoS2, 2D and few-layer suspensions become inks that provide smooth films when painted. Conductivity of painted 2D MoS2 inks can be modulated by length and width, where the aspect ratio dependence of conductivity is linked to the painting direction. Inks of solvent-exfoliated MoS2 can be painted as conductive films without polymeric additives.
演示了具有纵横比相关电导率的二维层状二硫化钼的导电和可涂油墨。使用超声波辅助的二硫化钼溶剂剥离,2D和几层悬浮液成为油墨,在涂漆时提供光滑的薄膜。绘制的二维MoS2油墨的电导率可以通过长度和宽度来调节,其中电导率的纵横比依赖于绘制方向。溶剂剥离的二硫化钼油墨可以涂成导电薄膜,不需要聚合物添加剂。
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引用次数: 2
Temperature dependence of reconfigurable bandstop filters using vanadium dioxide switches 使用二氧化钒开关的可重构带阻滤波器的温度依赖性
Pub Date : 2020-07-14 DOI: 10.1063/5.0021942
A. Muller, M. Cavalieri, A. Ionescu
In this letter we report and investigate the temperature dependency of various radio frequency parameters (RF) for a fabricated reconfigurable bandstop filter with vanadium dioxide (VO2) switches measured up to 55 GHz. Here the insulator to metal (ITM) and metal to insulator transition (MIT) hysteresis of the VO2 thin film influence on the RF characteristics of the filters is analyzed from 25 °C and 120 °C in heating and cooling. The resonance frequency and maximum insertion loss (IL) stability and sensitivity with temperature variations are explored. It is noticed that increasing the temperature with 50 °C from 25 °C (or decreasing it with 50 °C from 120 °C) will result in a less than 1% fractional frequency shift in respect to the off and on resonance frequencies. The sharp DC conductivity levels variations of the VO2 thin film around the transition temperatures translate into sharp effects on the resonance characteristics of the filters. On the contrary, the maximum IL levels are less sensitive to the DC films sharp conductivity changes around the VO2 transition temperature. Last, we see that the RF parameters in heating and cooling at 80 °C, above (but close to) the DC transition temperatures of VO2 exhibit completely different resonance frequencies. The RF results reported close to the transition temperatures for the VO2 thin films can diverge in heating and cooling, thus of a more insightful understanding of VO2 reconfigurable RF devices has to include temperature dependent measurements at various temperatures below MIT and ITM in the RF ranges too
在这封信中,我们报告并研究了各种射频参数(RF)对制造的可重构带阻滤波器的温度依赖性,其中二氧化钒(VO2)开关的测量频率高达55 GHz。本文分析了在25°C和120°C加热和冷却条件下,VO2薄膜的绝缘体到金属(ITM)和金属到绝缘体转变(MIT)迟滞对滤波器射频特性的影响。探讨了谐振频率和最大插入损耗随温度变化的稳定性和灵敏度。值得注意的是,温度从25°C增加50°C(或从120°C降低50°C)将导致相对于关闭和打开谐振频率的分数频率移位小于1%。VO2薄膜在转变温度附近的直流电导率水平的急剧变化转化为对滤波器谐振特性的急剧影响。相反,在VO2转变温度附近,最大IL电平对直流薄膜电导率的急剧变化不太敏感。最后,我们看到在80°C加热和冷却时,高于(但接近)VO2的直流转变温度的RF参数表现出完全不同的谐振频率。报告的射频结果接近VO2薄膜的转变温度,在加热和冷却时可能会出现分歧,因此,为了更深刻地理解VO2可重构射频器件,必须包括在RF范围内低于MIT和ITM的各种温度下的温度相关测量
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引用次数: 2
Isotropic conduction and negative photoconduction in ultrathin PtSe2 films 超薄PtSe2薄膜的各向同性导电和负光导
Pub Date : 2020-07-11 DOI: 10.1063/5.0021009
F. Urban, F. Gity, P. Hurley, N. McEvoy, A. Di Bartolomeo
PtSe$_2$ ultrathin films are used as the channel of back-gated field-effect transistors (FETs) that are investigated at different temperatures and under super-continuous white laser irradiation. The temperature-dependent behavior confirms the semiconducting nature of multilayer PtSe$_2$, with p-type conduction, a hole field-effect mobility up to 40 cm2/(Vs) and significant gate modulation. Electrical conduction measured along different directions shows isotropic transport. A reduction of PtSe$_2$ channel conductance is observed under exposure to light. Such negative photoconductivity is explained by a photogating effect caused by photo-charge accumulation in SiO$_2$ and at the Si/SiO$_2$ interface.
利用PtSe$_2$超薄膜作为背控场效应晶体管(fet)的通道,研究了在不同温度和超连续白光照射下的场效应晶体管(fet)。温度相关的行为证实了多层PtSe$_2$的半导体性质,具有p型导电性,空穴场效应迁移率高达40 cm2/(Vs)和显著的栅极调制。沿不同方向测量的电导率显示各向同性传输。在光照下观察到PtSe$_2$通道电导的降低。这种负的光电导率是由SiO$_2$和Si/SiO$_2$界面上的光电荷积累引起的光门效应所解释的。
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引用次数: 18
Slow propagation of 2 GHz acoustical waves in a suspended GaAs phononic waveguide on insulator 绝缘体上悬浮式砷化镓声子波导中2ghz声波的慢传播
Pub Date : 2020-07-10 DOI: 10.1063/5.0019949
G. Modica, R. Zhu, R. Horváth, G. Beaudoin, I. Sagnes, R. Braive
Optoelectronic oscillators have dominated the scene of microwave oscillators in the last few years thanks to their great performances regarding frequency stability and phase noise. However, miniaturization of such a device is an up to date challenge. Recently, devices based on phonon-photon interaction gather a lot of interest thanks to their extreme compactness and working frequency directly in the GHz. In this frame, a still missing element to obtain long-term frequency stability performances is an on-chip delay within the feedback loop. Here, we experimentally show filtering and slow propagation of 2 GHz acoustic waves on a Gallium Arsenide membrane heterogeneously integrated on silicon wafer. By engineering the dispersion of an acoustical waveguide, we evidence a group velocity below 1000 m/s for the mode able to propagate. Thus, an integrated delay implementation is at reach for potential improvement of opto-acoustic devices such as optomechanical oscillators or wireless applications.
光电子振荡器由于其在频率稳定性和相位噪声方面的优异性能,近年来在微波振荡器领域占据主导地位。然而,这种设备的小型化是一个最新的挑战。最近,基于声子-光子相互作用的器件由于其极端紧凑和工作频率直接在GHz而引起了人们的极大兴趣。在这个框架中,仍然缺少获得长期频率稳定性能的元素是反馈回路中的片上延迟。在这里,我们实验展示了2 GHz声波在硅片上非均匀集成的砷化镓膜上的滤波和慢传播。通过设计声波导的色散,我们证明了能够传播的模式的群速度低于1000米/秒。因此,集成延迟实现可用于光声设备(如光机械振荡器或无线应用)的潜在改进。
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引用次数: 6
Gigahertz Phononic Integrated Circuits on Thin-Film Lithium Niobate on Sapphire 蓝宝石上铌酸锂薄膜的千兆赫声子集成电路
Pub Date : 2020-07-09 DOI: 10.1103/PHYSREVAPPLIED.15.014039
Felix M. Mayor, Wentao Jiang, Christopher J. Sarabalis, T. McKenna, J. Witmer, A. Safavi-Naeini
Acoustic devices play an important role in classical information processing. The slower speed and lower losses of mechanical waves enable compact and efficient elements for delaying, filtering, and storing of electric signals at radio and microwave frequencies. Discovering ways of better controlling the propagation of phonons on a chip is an important step towards enabling larger scale phononic circuits and systems. We present a platform, inspired by decades of advances in integrated photonics, that utilizes the strong piezoelectric effect in a thin film of lithium niobate on sapphire to excite guided acoustic waves immune from leakage into the bulk due to the phononic analogue of index-guiding. We demonstrate an efficient transducer matched to 50 ohm and guiding within a 1-micron wide mechanical waveguide as key building blocks of this platform. Putting these components together, we realize acoustic delay lines, racetrack resonators, and meander line waveguides for sensing applications. To evaluate the promise of this platform for emerging quantum technologies, we characterize losses at low temperature and measure quality factors on the order of 50,000 at 4 kelvin. Finally, we demonstrate phononic four-wave mixing in these circuits and measure the nonlinear coefficients to provide estimates of the power needed for relevant parametric processes.
声学器件在经典信息处理中起着重要的作用。机械波的速度较慢,损耗较低,这使得在无线电和微波频率上延迟、滤波和存储电信号的元件紧凑而有效。发现更好地控制声子在芯片上传播的方法是实现更大规模声子电路和系统的重要一步。受集成光子学数十年进步的启发,我们提出了一个平台,该平台利用蓝宝石上铌酸锂薄膜中的强压电效应来激发引导声波,从而避免由于声子模拟的指数引导而泄漏到体中。我们展示了一个匹配50欧姆的高效换能器,并在1微米宽的机械波导内引导,作为该平台的关键组成部分。将这些组件组合在一起,我们实现了用于传感应用的声学延迟线,赛道谐振器和曲线波导。为了评估该平台对新兴量子技术的前景,我们表征了低温下的损耗,并在4开尔文下测量了50,000数量级的质量因子。最后,我们演示了这些电路中的声子四波混频,并测量了非线性系数,以提供相关参数过程所需功率的估计。
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引用次数: 28
Charge-pumping with finger capacitance in a custom electrostatic energy harvesting ASIC 一种定制静电能量收集专用集成电路中带指电容的电荷泵送
Pub Date : 2020-07-09 DOI: 10.1063/5.0014008
A. Y. Zhou, M. Maharbiz
We present an integrated circuit capable of scavenging energy from repetitive changes in finger touch capacitance. A finger tapping on this ASIC generates a capacitive change of approximately 770pF. These changes feed into a charge-pump circuit which stores 320pJ of energy on a 1nF storage capacitor. We present measurement results and simulations that demonstrate operation. As a proof-of-concept, we also demonstrate that the harvested energy can power a ring oscillator which outputs a series of chirps with frequencies ranging from 80Hz to 30kHz as the storage capacitor voltage charges and discharges.
我们提出了一种能够从手指触摸电容的重复变化中清除能量的集成电路。手指轻敲ASIC会产生大约770pF的电容变化。这些变化输入到电荷泵电路中,该电路在1nF存储电容上存储320pJ的能量。我们给出了测试结果和仿真,以验证该方法的有效性。作为概念验证,我们还证明了所收集的能量可以为环形振荡器供电,该振荡器在存储电容器电压充电和放电时输出一系列频率范围为80Hz至30kHz的啁啾。
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引用次数: 1
Extended Short-Wave Infrared Absorption in Group-IV Nanowire Arrays 四族纳米线阵列中短波红外吸收的扩展
Pub Date : 2020-07-07 DOI: 10.1103/PHYSREVAPPLIED.15.014034
A. Attiaoui, É. Bouthillier, G. Daligou, A. Kumar, S. Assali, O. Moutanabbir
Engineering light absorption in the extended short-wave infrared (e-SWIR) range using scalable materials is a long-sought-after capability that is crucial to implement cost-effective and high-performance sensing and imaging technologies. Herein, we demonstrate enhanced, tunable e-SWIR absorption using silicon-integrated platforms consisting of ordered arrays of metastable GeSn nanowires with Sn content reaching 9 at.% and variable diameters. Detailed simulations were combined with experimental analyses to systematically investigate light-GeSn nanowire interactions to tailor and optimize the nanowire array geometrical parameters and the corresponding optical response. The diameter-dependent leaky mode resonance peaks are theoretically predicted and experimentally confirmed with a tunable wavelength from 1.5 to 2.2 {mu}m. A three-fold enhancement in the absorption with respect to GeSn layers at 2.1 {mu}m was achieved using nanowires with a diameter of 325 nm. Finite difference time domain simulations unraveled the underlying mechanisms of the e-SWIR enhanced absorption. Coupling of the HE11 and HE12 resonant modes to nanowires is observed at diameters above 325 nm, while at smaller diameters and longer wavelengths the HE11 mode is guided into the underlying Ge layer. The presence of tapering in NWs further extends the absorption range while minimizing reflection. This ability to engineer and enhance e-SWIR absorption lays the groundwork to implement novel photonic devices exploiting all-group IV platforms.
在扩展短波红外(e-SWIR)范围内使用可扩展材料的工程光吸收是一种长期追求的能力,对于实现成本效益和高性能传感和成像技术至关重要。在这里,我们展示了增强的、可调谐的e-SWIR吸收,使用由有序阵列的亚稳GeSn纳米线组成的硅集成平台,Sn含量达到9 at。%和可变直径。详细的模拟与实验分析相结合,系统地研究了光- gesn纳米线的相互作用,以定制和优化纳米线阵列的几何参数和相应的光学响应。理论上预测了与直径相关的漏模共振峰,并在1.5 ~ 2.2 {mu}m的波长范围内进行了实验验证。使用直径为325 nm的纳米线,相对于2.1 {mu}m的GeSn层的吸收增强了三倍。时域有限差分模拟揭示了e-SWIR增强吸收的潜在机制。在直径大于325 nm处,HE11和HE12谐振模式与纳米线耦合,而在直径较小、波长较长的纳米线处,HE11模式被引导到其下的Ge层。NWs中逐渐变细的存在进一步扩大了吸收范围,同时使反射最小化。这种设计和增强e-SWIR吸收的能力为实现利用全IV群平台的新型光子器件奠定了基础。
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引用次数: 3
期刊
arXiv: Applied Physics
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