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Multicharged-ion–water-molecule collisions in a classical-trajectory time-dependent mean-field theory 经典轨迹时相关平均场理论中的多电荷离子-水分子碰撞
Pub Date : 2020-01-17 DOI: 10.1103/physreva.102.012808
A. Jorge, M. Horbatsch, T. Kirchner
A recently proposed classical-trajectory dynamical screening model for the description of multiple ionization and capture during ion-water molecule collisions is extended to incorporate dynamical screening on both the multi-center target potential and the projectile ion. Comparison with available experimental data for He$^{2+}$ + H$_2$O collisions at intermediate energies (10-150 keV/u) and Li$^{3+}$ + H$_2$O at higher energies (100-850 keV/u) demonstrates the importance of both screening mechanisms. The question of how to deal with the repartitioning of the capture flux into allowed capture channels is addressed. The model also provides insights for data on highly charged projectile ions (C$^{6+}$, O$^{8+}$, Si$^{13+}$) in the MeV/u range where the question of saturation effects in net ionization was raised in the literature.
最近提出的用于描述离子-水分子碰撞过程中多重电离和捕获的经典轨迹动态筛选模型被扩展到包括多中心靶电位和抛射离子的动态筛选。He$^{2+}$ + H$_2$O中间能量(10-150 keV/u)和Li$^{3+}$ + H$_2$O高能量(100-850 keV/u)的实验数据对比表明了这两种筛选机制的重要性。解决了如何处理捕获通量重新划分为允许的捕获通道的问题。该模型还为MeV/u范围内高电荷抛射离子(C$^{6+}$, O$^{8+}$, Si$^{13+}$)的数据提供了见解,在该范围内,净电离的饱和效应问题在文献中被提出。
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引用次数: 2
Influence of Laser Intensity Fluctuation on Single-Cesium Atom Trapping Lifetime in a 1064-nm Microscopic Optical Tweezer 激光强度波动对1064nm显微光镊中单铯原子捕获寿命的影响
Pub Date : 2020-01-16 DOI: 10.3390/app10020659
R. Sun, Xin Wang, Kong Zhang, Jun He, Junmin Wang
An optical tweezer composed of a strongly focused single-spatial-mode Gaussian beam of a red-detuned 1064-nm laser can confine a single-cesium (Cs) atom at the strongest point of the light intensity. We can use this for coherent manipulation of single-quantum bits and single-photon sources. The trapping lifetime of the atoms in the optical tweezers is very short due to the impact of the background atoms, the laser intensity fluctuation of optical tweezer and the residual thermal motion of the atoms. In this paper, we analyzed the influence of the background pressure, the trap frequency of optical tweezers and the parametric heating of the optical tweezer on the atomic trapping lifetime. Combined with the external feedback loop based on an acousto-optical modulator (AOM), the intensity fluctuation of the 1064-nm laser in the time domain was suppressed from $pm$ 3.360$%$ to $pm$ 0.064$%$, and the suppression bandwidth reached approximately 33 kHz. The trapping lifetime of a single Cs atom in the microscopic optical tweezer was extended from 4.04 s to 6.34 s.
由1064 nm红失谐激光强聚焦单空间模高斯光束组成的光镊可以将单个铯原子限制在光强的最强点。我们可以将其用于单量子比特和单光子源的相干操作。由于背景原子、光镊的激光强度波动和原子的残余热运动的影响,原子在光镊中的捕获寿命很短。本文分析了背景压力、光镊捕获频率和光镊参数加热对原子捕获寿命的影响。结合基于声光调制器(AOM)的外反馈环路,将1064 nm激光器的时域强度波动从$pm$ 3.360$%$抑制到$pm$ 0.064$%$,抑制带宽达到约33 kHz。单Cs原子在显微光镊中的捕获寿命由4.04 s延长至6.34 s。
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引用次数: 2
Nanosecond-timescale development of Faraday rotation in an ultracold gas 超冷气体中法拉第旋转的纳秒级发展
Pub Date : 2019-12-16 DOI: 10.1103/physreva.101.053848
J. Gilbert, Mark Watkins, J. Roberts
When a gas of ultracold atoms is suddenly illuminated by light that is nearly resonant with an atomic transition, the atoms cannot respond instantaneously. This non-instantaneous response means the gas is initially more transparent to the applied light than in steady-state. The timescale associated with the development of light absorption is set by the atomic excited state lifetime. Similarly, the index of refraction in the gas also requires time to reach a steady-state value, but the development of the associated phase response is expected to be slower than absorption effects. Faraday rotation is one manifestation of differing indices of refraction for orthogonal circular light polarization components. We have performed experiments measuring the time-dependent development of polarization rotation in an ultracold gas subjected to a magnetic field. Our measurements match theoretical predictions based on solving optical Bloch equations. We are able to identify how parameters such as steady-state optical thickness and applied magnetic field strength influence the development of Faraday rotation.
当一种由超冷原子组成的气体突然被几乎与原子跃迁共振的光照亮时,原子不能立即做出反应。这种非瞬时响应意味着气体最初对施加的光比在稳态时更透明。与光吸收发展有关的时间标度是由原子激发态寿命决定的。同样,气体中的折射率也需要时间才能达到稳态值,但相关相位响应的发展预计将比吸收效应慢。法拉第旋转是正交圆光偏振分量折射率不同的表现之一。我们进行了实验,测量了磁场作用下超冷气体中极化旋转的随时间发展。我们的测量结果与基于求解光学布洛赫方程的理论预测相符。我们能够确定诸如稳态光学厚度和外加磁场强度等参数如何影响法拉第旋转的发展。
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引用次数: 0
Equation of motion for a bound system of charged particles 带电粒子束缚系统的运动方程
Pub Date : 2019-12-11 DOI: 10.1103/PhysRevA.100.062510
K. Pachucki, V. Yerokhin
We consider a bound system of charged particles moving in an external electromagnetic field, including leading relativistic corrections. The difference from the point particle with a magnetic moment comes from the presence of polarizabilities. Due to the lack of separation of the total momentum from the internal degrees of freedom, the notion of polarizability of the bound state immersed in the continuum spectrum of the global motion is nontrivial. We introduce a bound-continuum perturbation theory and obtain a complete formula for the equation of motion for a polarizable bound system, such as atom, ion, or the nucleus. This formula may find applications when high precision is sought and small effects due polarizabilities are important.
我们考虑一个带电粒子的束缚系统在一个外部电磁场中运动,包括领先的相对论修正。与具有磁矩的点粒子的区别来自于极性的存在。由于总动量与内部自由度之间缺乏分离,因此沉浸在全局运动连续谱中的束缚态极化率的概念是非平凡的。我们引入了一个束缚-连续统摄动理论,并得到了原子、离子或原子核等可极化束缚系统运动方程的完整公式。该公式适用于要求精度高、极化效应小的场合。
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引用次数: 2
Interactions and chemical reactions in ionic alkali-metal and alkaline-earth-metal diatomic AB+ and triatomic A2B+ systems 离子碱金属和碱土金属双原子AB+和三原子A2B+体系中的相互作用和化学反应
Pub Date : 2019-10-30 DOI: 10.1103/physreva.101.012501
Michal 'Smialkowski, M. Tomza
We theoretically characterize interactions, energetics, and chemical reaction paths in ionic two-body and three-body systems of alkali-metal and alkaline-earth-metal atoms in the context of modern experiments with cold hybrid ion-atom mixtures. Using textit{ab initio} techniques of quantum chemistry such as the coupled-cluster method, we calculate ground-state electronic properties of all diatomic $AB^+$ and most of triatomic $A_2B^+$ molecular ions consisting of Li, Na, K, Rb, Cs, Mg, Ca, Sr, Ba, and Yb atoms. Different geometries and wave-function symmetries of the ground state are found for different classes of molecular ions. We analyze intermolecular interactions in the investigated systems including additive two-body and nonadditive three-body ones. As an example we provide two-dimensional interaction potential energy surfaces for KRb$^+$+K and Rb$^+$+Sr$_2$ mixtures. We identify possible channels of chemical reactions based on the energetics of the reactants. The present results may be useful for investigating controlled chemical reactions and other applications of molecular ions formed in cold hybrid ion-atom systems.
在冷杂化离子-原子混合物的现代实验背景下,我们从理论上描述了碱金属和碱土-金属原子的离子二体和三体系统中的相互作用、能量学和化学反应路径。利用量子化学的textit{从头}算技术,如耦合簇方法,我们计算了所有双原子$AB^+$和大多数三原子$A_2B^+$分子离子的基态电子性质,这些分子离子由Li、Na、K、Rb、Cs、Mg、Ca、Sr、Ba和Yb原子组成。不同种类的分子离子具有不同的基态几何形状和波函数对称性。我们分析了所研究系统的分子间相互作用,包括可加性二体和非可加性三体系统。作为例子,我们给出了KRb $^+$ +K和Rb $^+$ +Sr $_2$混合物的二维相互作用势能面。我们根据反应物的能量学来确定化学反应的可能途径。本研究结果可用于研究在冷杂化离子-原子体系中形成的分子离子的受控化学反应和其他应用。
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引用次数: 12
Observation of electric-dipole transitions in the laser-cooling candidate Th− and its application for cooling antiprotons 激光冷却候选者Th -中电偶极子跃迁的观察及其在冷却反质子中的应用
Pub Date : 2019-10-05 DOI: 10.1103/PHYSREVA.103.042817
R. Tang, R. Si, Zejie Fei, Xiaoxi Fu, Yuzhu Lu, T. Brage, Hongtao Liu, Chongyang Chen, C. Ning
Despite the fact that the laser cooling method is a well-established technique to obtain ultra-cold neutral atoms and atomic cations, it has so far never been applied to atomic anions due to the lack of suitable electric-dipole transitions. Efforts of more than a decade currently has La$^-$ as the only promising candidate for laser cooling. Our previous work [Tang et al., Phys. Rev. Lett. 123, 203002(2019)] showed that Th$^-$ is also a potential candidate. Here we report on a combination of experimental and theoretical studies to determine the relevant transition frequencies, transition rates, and branching ratios in Th$^-$. The resonant frequency of the laser cooling transition is determined to be $nu/c$ = 4118.0 (10) cm$^{-1}$. The transition rate is calculated as A=1.17x10^4 s$^{-1}$. The branching fraction to dark states is very small, 1.47x10$^{-10}$, thus this represents an ideal closed cycle for laser cooling. Since Th has zero nuclear spin, it is an excellent candidate to be used to sympathetically cool antiprotons in a Penning trap.
尽管激光冷却方法是一种成熟的获得超冷中性原子和原子阳离子的技术,但由于缺乏合适的电偶极子跃迁,迄今尚未应用于原子阴离子。经过十多年的努力,目前La$^-$是唯一有希望用于激光冷却的候选者。我们之前的工作[Tang et al., Phys.]Rev. Lett. 123, 203002(2019)]表明Th$^-$也是潜在的候选者。在这里,我们报告了实验和理论研究的结合,以确定Th$^-$中的相关跃迁频率,跃迁速率和分支比。确定了激光冷却跃迁的共振频率为$nu/c$ = 4118.0 (10) cm$^{-1}$。跃迁速率计算为A=1.17x10^4 s$^{-1}$。到暗态的分支分数非常小,为1.47x10$^{-10}$,因此这代表了激光冷却的理想闭合循环。由于Th的核自旋为零,因此它是用来冷却潘宁阱中反质子的极好候选者。
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引用次数: 3
Tracing the origins of an asymmetric momentum distribution for polar molecules in strong linearly polarized laser fields 强线偏振激光场中极性分子不对称动量分布的溯源
Pub Date : 2019-09-18 DOI: 10.1103/physreva.102.053103
Shang Wang, J. Che, C. Chen, G. Xin, Yan-jun Chen
We study the ionization dynamics of oriented HeH$^+$ in strong linearly-polarized laser fields by numerically solving the time-dependent Schr"{o}dinger equation. The calculated photoelectron momentum distributions for parallel orientation show a striking asymmetric structure. With a developed model pertinent to polar molecules, we trace the electron motion in real time. We show that this asymmetric structure arises from the interplay of the Coulomb effect and the permanent dipole in strong laser fields. This structure can be used to probe the degree of orientation which is important in ultrafast experiments for polar molecules. we also check our results for other polar molecules such as CO and BF.
通过数值求解随时间变化的薛定谔方程,研究了强线偏振激光场中定向HeH$^+$的电离动力学。计算得到的平行方向的光电子动量分布具有明显的不对称结构。我们开发了一个与极性分子相关的模型,实时跟踪电子运动。我们证明了这种不对称结构是由强激光场中的库仑效应和永久偶极子相互作用引起的。这种结构可以用来探测极性分子的取向程度,这在极性分子的超快实验中是很重要的。我们还检查了其他极性分子(如CO和BF)的结果。
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引用次数: 12
Practical trapped-ion protocols for universal qudit-based quantum computing 通用量子计算的实用俘获离子协议
Pub Date : 2019-07-19 DOI: 10.1103/PHYSREVRESEARCH.2.033128
Pei Jiang Low, Brendan M. White, Andrew Cox, Matthew L. Day, C. Senko
The notion of universal quantum computation can be generalized to multi-level qudits, which offer advantages in resource usage and algorithmic efficiencies. Trapped ions, which are pristine and well-controlled quantum systems, offer an ideal platform to develop qudit-based quantum information processing. Previous work has not fully explored the practicality of implementing trapped-ion qudits accounting for known experimental error sources. Here, we describe a universal set of protocols for state preparation, single-qudit gates, a new generalization of the Mo{}lmer-So{}rensen gate for two-qudit gates, and a measurement scheme which utilizes shelving to a meta-stable state. We numerically simulate known sources of error from previous trapped ion experiments, and show that there are no fundamental limitations to achieving fidelities above (99%) for three-level qudits encoded in (^{137}mathrm{Ba}^+) ions. Our methods are extensible to higher-dimensional qudits, and our measurement and single-qudit gate protocols can achieve (99%) fidelities for five-level qudits. We identify avenues to further decrease errors in future work. Our results suggest that three-level trapped ion qudits will be a useful technology for quantum information processing.
通用量子计算的概念可以推广到多级量子,这在资源利用和算法效率方面具有优势。捕获离子是一种原始且控制良好的量子系统,为开发基于量子位的量子信息处理提供了理想的平台。以前的工作并没有充分探索实现捕获离子量子计算已知实验误差源的实用性。在这里,我们描述了一套用于状态准备的通用协议,单量子位门,M o{} lmer-S o{} rensen门用于双量子位门的新推广,以及一种利用搁置到亚稳定状态的测量方案。我们数值模拟了先前捕获离子实验中已知的误差来源,并表明在(^{137}mathrm{Ba}^+)离子中编码的三能级qudits在达到(99%)以上的保真度方面没有基本限制。我们的方法可扩展到高维量纲,并且我们的测量和单量纲门协议可以实现(99%)五级量纲的保真度。我们确定了在未来工作中进一步减少错误的途径。我们的研究结果表明,三能级阱离子量子将是一种有用的量子信息处理技术。
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引用次数: 59
Symmetric Bloch oscillations of matter waves 物质波的对称布洛赫振荡
Pub Date : 2019-07-13 DOI: 10.1103/physreva.102.053312
Z. Pagel, Weicheng Zhong, Richard H. Parker, Christopher T. Olund, N. Yao, H. Mueller
Cold atoms in an optical lattice provide an ideal platform for studying Bloch oscillations. Here, we extend Bloch oscillations to two superposed optical lattices that are accelerated away from one another, and for the first time show that these symmetric Bloch oscillations can split, reflect and recombine matter waves coherently. Using the momentum parity-symmetry of the Hamiltonian, we map out the energy band structure of the process and show that superpositions of momentum states are created by adiabatically following the ground state of the Hamiltonian. The relative phase and velocity of the two lattices completely determines the trajectories of different branches of the matter wave. Experimentally, we demonstrate symmetric Bloch oscillations using cold Cesium atoms where we form interferometers with up to $240hbar k$ momentum splitting, one of the largest coherent momentum splittings achieved to date. This work has applications in macroscopic tests of quantum mechanics, measurements of fundamental constants, and searches for new physics.
光学晶格中的冷原子为研究布洛赫振荡提供了理想的平台。在这里,我们将布洛赫振荡扩展到两个相互加速远离的叠加光学晶格,并首次表明这些对称的布洛赫振荡可以相干地分裂、反射和重组物质波。利用哈密顿量的动量奇偶对称性,我们绘制了这一过程的能带结构,并证明了动量态的叠加是由哈密顿量的基态绝热地产生的。两个晶格的相对相位和速度完全决定了物质波不同分支的运动轨迹。实验上,我们用冷铯原子证明了对称布洛赫振荡,在那里我们形成了具有高达240 hbar k$动量分裂的干涉仪,这是迄今为止实现的最大的相干动量分裂之一。这项工作在量子力学的宏观测试、基本常数的测量和寻找新物理学中都有应用。
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引用次数: 22
Guidelines for developing optical clocks with 10-18 fractional frequency uncertainty 10-18分数频率不确定度光学钟的研制指南
Pub Date : 2019-06-27 DOI: 10.15488/5553
Moustafa Abdel-Hafiz, P. Ablewski, A. Al-Masoudi, H'ector 'Alvarez Mart'inez, P. Balling, G. Barwood, E. Benkler, M. Bober, M. Borkowski, W. Bowden, R. Ciuryło, H. Cybulski, A. Didier, Miroslav Dolevzal, S. Dorscher, S. Falke, R. Godun, R. Hamid, I. Hill, R. Hobson, N. Huntemann, Y. Coq, R. L. Targat, T. Legero, T. Lindvall, C. Lisdat, J. Lodewyck, H. Margolis, T. Mehlstaubler, E. Peik, L. Pelzer, M. Pizzocaro, B. Rauf, A. Rolland, N. Scharnhorst, M. Schioppo, P. Schmidt, R. Schwarz, cCaugri cSenel, N. Spethmann, U. Sterr, C. Tamm, J. Thomsen, A. Vianello, M. Zawada
There has been tremendous progress in the performance of optical frequency standards since the first proposals to carry out precision spectroscopy on trapped, single ions in the 1970s. The estimated fractional frequency uncertainty of today's leading optical standards is currently in the $10^{-18}$ range, approximately two orders of magnitude better than that of the best caesium primary frequency standards. This exceptional accuracy and stability is resulting in a growing number of research groups developing optical clocks. While good review papers covering the topic already exist, more practical guidelines are needed as a complement. The purpose of this document is therefore to provide technical guidance for researchers starting in the field of optical clocks. The target audience includes national metrology institutes (NMIs) wanting to set up optical clocks (or subsystems thereof) and PhD students and postdocs entering the field. Another potential audience is academic groups with experience in atomic physics and atom or ion trapping, but with less experience of time and frequency metrology and optical clock requirements. These guidelines have arisen from the scope of the EMPIR project "Optical clocks with $1 times 10^{-18}$ uncertainty" (OC18). Therefore, the examples are from European laboratories even though similar work is carried out all over the world. The goal of OC18 was to push the development of optical clocks by improving each of the necessary subsystems: ultrastable lasers, neutral-atom and single-ion traps, and interrogation techniques. This document shares the knowledge acquired by the OC18 project consortium and gives practical guidance on each of these aspects.
自20世纪70年代首次提出对捕获的单离子进行精密光谱学以来,光学频率标准的性能已经取得了巨大的进步。当今领先的光学标准的估计分数频率不确定度目前在$10^{-18}$范围内,大约比最好的铯主频率标准好两个数量级。这种卓越的精度和稳定性导致越来越多的研究小组开发光学时钟。虽然已经存在涵盖该主题的优秀评论论文,但需要更多实用指南作为补充。因此,本文的目的是为从事光学时钟领域的研究人员提供技术指导。目标受众包括想要建立光学时钟(或其子系统)的国家计量研究所(NMIs)以及进入该领域的博士生和博士后。另一个潜在的受众是具有原子物理学和原子或离子捕获经验的学术团体,但在时间和频率计量以及光学时钟要求方面的经验较少。这些准则源自EMPIR项目“1 × 10^{-18}$不确定性的光学时钟”(OC18)的范围。因此,尽管世界各地都在进行类似的工作,但这些例子都来自欧洲的实验室。OC18的目标是通过改进每一个必要的子系统来推动光学时钟的发展:超稳定激光器、中性原子和单离子阱,以及询问技术。本文档分享了OC18项目联盟获得的知识,并就这些方面提供了实际指导。
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引用次数: 17
期刊
arXiv: Atomic Physics
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