Pub Date : 2024-10-31DOI: 10.1515/nanoph-2024-0454
Oren Goldberg, Noa Mazurski, Uriel Levy
High refractive index dielectric materials like silicon rich nitride (SRN) are critical for constructing advanced dielectric metasurfaces but are limited by transparency and complementary metal oxide semiconductor (CMOS) process compatibility. SRN’s refractive index can be adjusted by varying the silicon to nitride ratio, although this increases absorption, particularly in the blue spectrum. Dielectric metasurfaces, which utilize the material’s high dielectric constant and nano-resonator geometry, experience loss amplification due to resonance, affecting light reflection, light transmission, and quality factor. This study explores the impact of varying the silicon ratio on structural color applications in metasurfaces, using metrics such as gamut coverage, saturation, and reflection amplitude. We found that a higher SRN ratio enhances these metrics, making it ideal for producing vivid structural colors. Our results show that SRN can produce a color spectrum covering up to 166 % of the sRGB space and a resolution of 38,000 dots per inch. Fabricated samples vividly displayed a parrot, a flower, and a rainbow, illustrating SRN’s potential for high-resolution applications. We also show that SRN can provide a better CIE diagram coverage than other popular metasurfaces materials. These findings highlight the advantages of SRN for photonic devices, suggesting pathways for further material and application development.
{"title":"Silicon rich nitride: a platform for controllable structural colors","authors":"Oren Goldberg, Noa Mazurski, Uriel Levy","doi":"10.1515/nanoph-2024-0454","DOIUrl":"https://doi.org/10.1515/nanoph-2024-0454","url":null,"abstract":"High refractive index dielectric materials like silicon rich nitride (SRN) are critical for constructing advanced dielectric metasurfaces but are limited by transparency and complementary metal oxide semiconductor (CMOS) process compatibility. SRN’s refractive index can be adjusted by varying the silicon to nitride ratio, although this increases absorption, particularly in the blue spectrum. Dielectric metasurfaces, which utilize the material’s high dielectric constant and nano-resonator geometry, experience loss amplification due to resonance, affecting light reflection, light transmission, and quality factor. This study explores the impact of varying the silicon ratio on structural color applications in metasurfaces, using metrics such as gamut coverage, saturation, and reflection amplitude. We found that a higher SRN ratio enhances these metrics, making it ideal for producing vivid structural colors. Our results show that SRN can produce a color spectrum covering up to 166 % of the sRGB space and a resolution of 38,000 dots per inch. Fabricated samples vividly displayed a parrot, a flower, and a rainbow, illustrating SRN’s potential for high-resolution applications. We also show that SRN can provide a better CIE diagram coverage than other popular metasurfaces materials. These findings highlight the advantages of SRN for photonic devices, suggesting pathways for further material and application development.","PeriodicalId":19027,"journal":{"name":"Nanophotonics","volume":"7 1","pages":""},"PeriodicalIF":7.5,"publicationDate":"2024-10-31","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142561872","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
We report a transverse optical torque exerted on a conventional isotropic spherical particle in a direction perpendicular to that of the illuminating wave propagation. By using full-wave simulations and deriving an analytical expression of the transverse optical torque for particle of arbitrary size, the origin of this transverse optical torque is traced exclusively to the magnetic part of the spin angular momentum, regardless of the size and composition of the illuminated particle. To our surprise, for a non-magnetic dielectric particle, the transverse optical torque is found to originate mainly from the magnetic response of the particle, even when the particle size is much smaller than the illuminating wavelength. This is contrary to the general intuition that the electric response of a non-magnetic dielectric particle dominates its magnetic response in the mechanical effect of light, especially in the Rayleigh limit.
{"title":"Transverse optical torque from the magnetic spin angular momentum","authors":"Jiquan Wen, Fengling He, Lv Feng, Wanli Lu, Zhifang Lin, Hongxia Zheng, Huajin Chen","doi":"10.1515/nanoph-2024-0406","DOIUrl":"https://doi.org/10.1515/nanoph-2024-0406","url":null,"abstract":"We report a transverse optical torque exerted on a conventional isotropic spherical particle in a direction perpendicular to that of the illuminating wave propagation. By using full-wave simulations and deriving an analytical expression of the transverse optical torque for particle of arbitrary size, the origin of this transverse optical torque is traced exclusively to the magnetic part of the spin angular momentum, regardless of the size and composition of the illuminated particle. To our surprise, for a non-magnetic dielectric particle, the transverse optical torque is found to originate mainly from the magnetic response of the particle, even when the particle size is much smaller than the illuminating wavelength. This is contrary to the general intuition that the electric response of a non-magnetic dielectric particle dominates its magnetic response in the mechanical effect of light, especially in the Rayleigh limit.","PeriodicalId":19027,"journal":{"name":"Nanophotonics","volume":"275 1","pages":""},"PeriodicalIF":7.5,"publicationDate":"2024-10-30","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142555994","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2024-10-30DOI: 10.1515/nanoph-2024-0483
Sahar Behroozinia, Qing Gu
Diffractive Neural Networks (DNNs) leverage the power of light to enhance computational performance in machine learning, offering a pathway to high-speed, low-energy, and large-scale neural information processing. However, most existing DNN architectures are optimized for single tasks and thus lack the flexibility required for the simultaneous execution of multiple tasks within a unified artificial intelligence platform. In this work, we utilize the polarization and wavelength degrees of freedom of light to achieve optical multi-task identification using the MNIST, FMNIST, and KMNIST datasets. Employing bilayer cascaded metasurfaces, we construct dual-channel DNNs capable of simultaneously classifying two tasks, using polarization and wavelength multiplexing schemes through a meta-atom library. Numerical evaluations demonstrate performance accuracies comparable to those of individually trained single-channel, single-task DNNs. Extending this approach to three-task parallel recognition reveals an expected performance decline yet maintains satisfactory classification accuracies of greater than 80 % for all tasks. We further introduce a novel end-to-end joint optimization framework to redesign the three-task classifier, demonstrating substantial improvements over the meta-atom library design and offering the potential for future multi-channel DNN designs. Our study could pave the way for the development of ultrathin, high-speed, and high-throughput optical neural computing systems.
{"title":"Leveraging multiplexed metasurfaces for multi-task learning with all-optical diffractive processors","authors":"Sahar Behroozinia, Qing Gu","doi":"10.1515/nanoph-2024-0483","DOIUrl":"https://doi.org/10.1515/nanoph-2024-0483","url":null,"abstract":"Diffractive Neural Networks (DNNs) leverage the power of light to enhance computational performance in machine learning, offering a pathway to high-speed, low-energy, and large-scale neural information processing. However, most existing DNN architectures are optimized for single tasks and thus lack the flexibility required for the simultaneous execution of multiple tasks within a unified artificial intelligence platform. In this work, we utilize the polarization and wavelength degrees of freedom of light to achieve optical multi-task identification using the MNIST, FMNIST, and KMNIST datasets. Employing bilayer cascaded metasurfaces, we construct dual-channel DNNs capable of simultaneously classifying two tasks, using polarization and wavelength multiplexing schemes through a meta-atom library. Numerical evaluations demonstrate performance accuracies comparable to those of individually trained single-channel, single-task DNNs. Extending this approach to three-task parallel recognition reveals an expected performance decline yet maintains satisfactory classification accuracies of greater than 80 % for all tasks. We further introduce a novel end-to-end joint optimization framework to redesign the three-task classifier, demonstrating substantial improvements over the meta-atom library design and offering the potential for future multi-channel DNN designs. Our study could pave the way for the development of ultrathin, high-speed, and high-throughput optical neural computing systems.","PeriodicalId":19027,"journal":{"name":"Nanophotonics","volume":"7 1","pages":""},"PeriodicalIF":7.5,"publicationDate":"2024-10-30","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142555995","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2024-10-30DOI: 10.1515/nanoph-2024-0391
Donghak Oh, Soojeong Baek, Sangha Lee, Kyungmin Lee, Jagang Park, Zhaowei Liu, Teun-Teun Kim, Bumki Min
Non-Hermitian systems can be tuned to exhibit exceptional points, where both eigenvalues and eigenstates coalesce concurrently. The inherent adaptability of photonic non-Hermitian systems in configuring gain and loss has allowed us to observe a plethora of counterintuitive phenomena, largely as a consequence of the eigenspace reduction at these exceptional points. In this work, we propose a non-Hermitian metasurface that, through the incorporation of gain, enables complete asymmetric polarization conversion at an exceptional point with a zero eigenvalue. Specifically, we provide numerical evidence for this concept by designing a non-Hermitian metasurface that facilitates polarization conversion from right to left circular polarization, while preventing conversion in the reverse direction and co-polarized transmission. Furthermore, our investigation reveals that this specific form of complete asymmetric polarization conversion results in maximum circular dichroism in transmission, thereby eliminating the need for external chirality or three-dimensional helical structures. This non-Hermitian technique offers an intriguing approach to designing polarization-sensitive optical devices and systems, further expanding their functionalities and capabilities.
{"title":"Complete asymmetric polarization conversion at zero-eigenvalue exceptional points of non-Hermitian metasurfaces","authors":"Donghak Oh, Soojeong Baek, Sangha Lee, Kyungmin Lee, Jagang Park, Zhaowei Liu, Teun-Teun Kim, Bumki Min","doi":"10.1515/nanoph-2024-0391","DOIUrl":"https://doi.org/10.1515/nanoph-2024-0391","url":null,"abstract":"Non-Hermitian systems can be tuned to exhibit exceptional points, where both eigenvalues and eigenstates coalesce concurrently. The inherent adaptability of photonic non-Hermitian systems in configuring gain and loss has allowed us to observe a plethora of counterintuitive phenomena, largely as a consequence of the eigenspace reduction at these exceptional points. In this work, we propose a non-Hermitian metasurface that, through the incorporation of gain, enables complete asymmetric polarization conversion at an exceptional point with a zero eigenvalue. Specifically, we provide numerical evidence for this concept by designing a non-Hermitian metasurface that facilitates polarization conversion from right to left circular polarization, while preventing conversion in the reverse direction and co-polarized transmission. Furthermore, our investigation reveals that this specific form of complete asymmetric polarization conversion results in maximum circular dichroism in transmission, thereby eliminating the need for external chirality or three-dimensional helical structures. This non-Hermitian technique offers an intriguing approach to designing polarization-sensitive optical devices and systems, further expanding their functionalities and capabilities.","PeriodicalId":19027,"journal":{"name":"Nanophotonics","volume":"31 1","pages":""},"PeriodicalIF":7.5,"publicationDate":"2024-10-30","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142555996","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2024-10-30DOI: 10.1515/nanoph-2024-0414
Bingbing Liu, Tao Xu, Zhi Hong Hang
Recent research on non-Abelian phenomena has cast a new perspective on controlling light. In this work, we provide a simple and general approach to induce non-Abelian gauge field to tremble the light beam trajectory. With in-plane duality symmetry relaxed, our theoretical analysis finds that non-Abelian electric field can be synthesized through a simple real-space rotation of any biaxial material. With orthogonal optical modes excited, their interference leads to an oscillation of the propagating optical beam, which is a direct consequence of the emergence of non-Abelian electric field, influencing light in a manner similar with how electric fields act on charged particles. Our microwave experiments provide unambiguous evidence to the observation of such an optical Zitterbewegung effect where excellent agreement can be found between theorical derivation, numerical simulations and experiments. By extending the idea to optical regime using natural material, we here provide another example to shake the general intuition that light travels in straight lines in homogeneous media.
{"title":"A general recipe to observe non-Abelian gauge field in metamaterials","authors":"Bingbing Liu, Tao Xu, Zhi Hong Hang","doi":"10.1515/nanoph-2024-0414","DOIUrl":"https://doi.org/10.1515/nanoph-2024-0414","url":null,"abstract":"Recent research on non-Abelian phenomena has cast a new perspective on controlling light. In this work, we provide a simple and general approach to induce non-Abelian gauge field to tremble the light beam trajectory. With in-plane duality symmetry relaxed, our theoretical analysis finds that non-Abelian electric field can be synthesized through a simple real-space rotation of any biaxial material. With orthogonal optical modes excited, their interference leads to an oscillation of the propagating optical beam, which is a direct consequence of the emergence of non-Abelian electric field, influencing light in a manner similar with how electric fields act on charged particles. Our microwave experiments provide unambiguous evidence to the observation of such an optical <jats:italic>Zitterbewegung</jats:italic> effect where excellent agreement can be found between theorical derivation, numerical simulations and experiments. By extending the idea to optical regime using natural material, we here provide another example to shake the general intuition that light travels in straight lines in homogeneous media.","PeriodicalId":19027,"journal":{"name":"Nanophotonics","volume":"27 1","pages":""},"PeriodicalIF":7.5,"publicationDate":"2024-10-30","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142541194","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Structural colors, resulting from the interaction of light with nanostructured materials rather than pigments, present a promising avenue for diverse applications ranging from ink-free printing to optical anti-counterfeiting. Achieving structural colors with high purity and brightness over large areas and at low costs is beneficial for many practical applications, but still remains a challenge for current designs. Here, we introduce a novel approach to realizing large-scale structural colors in layered thin film structures that are characterized by both high brightness and purity. Unlike conventional designs relying on single Fabry–Pérot cavity resonance, our method leverages coupled resonance between adjacent cavities to achieve sharp and intense transmission peaks with significantly suppressed sideband intensity. We demonstrate this approach by designing and experimentally validating transmission-type red, green, and blue colors using an Ag/SiO2/Ag/SiO2/Ag configuration on fused silica substrate. The measured spectra exhibit narrow resonant linewidths (full width at half maximum ∼60 nm), high peak efficiencies (>40 %), and well-suppressed sideband intensities (∼0 %). In addition, the generated color can be easily tuned by adjusting the thickness of SiO2 layer, and the associated color gamut coverage shows a wider range than many existing standards. Moreover, the proposed design method is versatile and compatible with various choices of dielectric and metallic layers. For instance, we demonstrate the production of angle-robust structural colors by utilizing high-index Ta2O5 as the dielectric layer. Finally, we showcase a series of printed color images based on the proposed structures. The coupled-cavity-resonance architecture presented here successfully mitigates the trade-off between color brightness and purity in conventional layered thin film structures and provides a novel and cost-effective route towards the realization of large-scale and high-performance structural colors.
{"title":"Large-scale high purity and brightness structural color generation in layered thin film structures via coupled cavity resonance","authors":"Danyan Wang, Chengang Ji, Moxin Li, Zhenyu Xing, Hao Gao, Xiaochan Li, Huixian Zhou, Yuhui Hu, Zhelin Lin, Cheng Zhang","doi":"10.1515/nanoph-2024-0471","DOIUrl":"https://doi.org/10.1515/nanoph-2024-0471","url":null,"abstract":"Structural colors, resulting from the interaction of light with nanostructured materials rather than pigments, present a promising avenue for diverse applications ranging from ink-free printing to optical anti-counterfeiting. Achieving structural colors with high purity and brightness over large areas and at low costs is beneficial for many practical applications, but still remains a challenge for current designs. Here, we introduce a novel approach to realizing large-scale structural colors in layered thin film structures that are characterized by both high brightness and purity. Unlike conventional designs relying on single Fabry–Pérot cavity resonance, our method leverages coupled resonance between adjacent cavities to achieve sharp and intense transmission peaks with significantly suppressed sideband intensity. We demonstrate this approach by designing and experimentally validating transmission-type red, green, and blue colors using an Ag/SiO<jats:sub>2</jats:sub>/Ag/SiO<jats:sub>2</jats:sub>/Ag configuration on fused silica substrate. The measured spectra exhibit narrow resonant linewidths (full width at half maximum ∼60 nm), high peak efficiencies (>40 %), and well-suppressed sideband intensities (∼0 %). In addition, the generated color can be easily tuned by adjusting the thickness of SiO<jats:sub>2</jats:sub> layer, and the associated color gamut coverage shows a wider range than many existing standards. Moreover, the proposed design method is versatile and compatible with various choices of dielectric and metallic layers. For instance, we demonstrate the production of angle-robust structural colors by utilizing high-index Ta<jats:sub>2</jats:sub>O<jats:sub>5</jats:sub> as the dielectric layer. Finally, we showcase a series of printed color images based on the proposed structures. The coupled-cavity-resonance architecture presented here successfully mitigates the trade-off between color brightness and purity in conventional layered thin film structures and provides a novel and cost-effective route towards the realization of large-scale and high-performance structural colors.","PeriodicalId":19027,"journal":{"name":"Nanophotonics","volume":"35 1","pages":""},"PeriodicalIF":7.5,"publicationDate":"2024-10-29","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142541195","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2024-10-26DOI: 10.1515/nanoph-2024-0437
Lu Sun, Xingfeng Li, Pan Hu, Hongwei Wang, Yong Zhang, Guojing Tang, Xintao He, Jianwen Dong, Yikai Su
Valley photonic crystals (VPCs) provide an intriguing approach to suppress backscattering losses and enable robust transport of light against sharp bends, which could be utilized to realize low-loss and small-footprint devices for on-chip optical communications. However, there are few studies on how to achieve power-efficient tunable devices based on VPCs, which are essential for implementing basic functions such as optical switching and routing. Here, we propose and experimentally demonstrate a thermally tunable add-drop filter (ADF) based on VPCs operating at telecommunication wavelengths. By leveraging the topological protection of the edge state and the distinct property of negligible scattering at sharp bends, a small footprint of 17.4 × 28.2 μm2 and a low insertion loss of 2.7 dB can be achieved for the proposed device. A diamond-shaped microloop resonator is designed to confine the light and enhance its interaction with the thermal field generated by the microheater, leading to a relatively low power of 23.97 mW needed for switching the output signal from one port to the other. Based on the thermally tunable ADF under the protection of band topology, robust data transmission is implemented with an ultrahigh data rate of 132 Gb/s. Our work shows great potential for developing high-performance topological photonic devices with the thermally tunable silicon-based VPCs, which offers unprecedented opportunities for realizing topologically protected and reconfigurable high-speed datalinks on a chip.
{"title":"Thermally tunable add-drop filter based on valley photonic crystals for optical communications","authors":"Lu Sun, Xingfeng Li, Pan Hu, Hongwei Wang, Yong Zhang, Guojing Tang, Xintao He, Jianwen Dong, Yikai Su","doi":"10.1515/nanoph-2024-0437","DOIUrl":"https://doi.org/10.1515/nanoph-2024-0437","url":null,"abstract":"Valley photonic crystals (VPCs) provide an intriguing approach to suppress backscattering losses and enable robust transport of light against sharp bends, which could be utilized to realize low-loss and small-footprint devices for on-chip optical communications. However, there are few studies on how to achieve power-efficient tunable devices based on VPCs, which are essential for implementing basic functions such as optical switching and routing. Here, we propose and experimentally demonstrate a thermally tunable add-drop filter (ADF) based on VPCs operating at telecommunication wavelengths. By leveraging the topological protection of the edge state and the distinct property of negligible scattering at sharp bends, a small footprint of 17.4 × 28.2 μm<jats:sup>2</jats:sup> and a low insertion loss of 2.7 dB can be achieved for the proposed device. A diamond-shaped microloop resonator is designed to confine the light and enhance its interaction with the thermal field generated by the microheater, leading to a relatively low power of 23.97 mW needed for switching the output signal from one port to the other. Based on the thermally tunable ADF under the protection of band topology, robust data transmission is implemented with an ultrahigh data rate of 132 Gb/s. Our work shows great potential for developing high-performance topological photonic devices with the thermally tunable silicon-based VPCs, which offers unprecedented opportunities for realizing topologically protected and reconfigurable high-speed datalinks on a chip.","PeriodicalId":19027,"journal":{"name":"Nanophotonics","volume":"9 1","pages":""},"PeriodicalIF":7.5,"publicationDate":"2024-10-26","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142490780","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2024-10-23DOI: 10.1515/nanoph-2024-0420
Senthil Kuppusamy Kumar, David Hunger, Mario Ruben, Philippe Goldner, Diana Serrano
Efforts to harness quantum hardware relying on quantum mechanical principles have been steadily progressing. The search for novel material platforms that could spur the progress by providing new functionalities for solving the outstanding technological problems is however still active. Any physical property presenting two distinct energy states that can be found in a long-lived superposition state can serve as a quantum bit (qubit), the basic information processing unit in quantum technologies. Molecular systems that can feature electron and/or nuclear spin states together with optical transitions are one of the material platforms that can serve as optically addressable qubits. The attractiveness of molecular systems for quantum technologies relies on the fact that molecular structures of atomically defined nature can be obtained in endless diversity of chemical compositions. Crucially, by harnessing the molecular design protocols, the optical and spin (electronic and nuclear) properties of molecules can be tailored, aiding the design of optically addressable spin qubits and quantum sensors. In this contribution, we present a concise and collective discussion of optically addressable spin-bearing molecules – namely, organic molecules, transition metal (TM) and rare-earth ion (REI) complexes – and highlight recent results such as chemical tuning of optical and electron spin quantum coherence, optical spin initialization and readout, intramolecular quantum teleportation, optical coherent storage, and photonic-enhanced optical addressing. We envision that optically addressable spin-carrying molecules could become a scalable building block of quantum hardware for applications in the fields of quantum sensing, quantum communication and quantum computing.
{"title":"Spin-bearing molecules as optically addressable platforms for quantum technologies","authors":"Senthil Kuppusamy Kumar, David Hunger, Mario Ruben, Philippe Goldner, Diana Serrano","doi":"10.1515/nanoph-2024-0420","DOIUrl":"https://doi.org/10.1515/nanoph-2024-0420","url":null,"abstract":"Efforts to harness quantum hardware relying on quantum mechanical principles have been steadily progressing. The search for novel material platforms that could spur the progress by providing new functionalities for solving the outstanding technological problems is however still active. Any physical property presenting two distinct energy states that can be found in a long-lived superposition state can serve as a quantum bit (qubit), the basic information processing unit in quantum technologies. Molecular systems that can feature electron and/or nuclear spin states together with optical transitions are one of the material platforms that can serve as optically addressable qubits. The attractiveness of molecular systems for quantum technologies relies on the fact that molecular structures of atomically defined nature can be obtained in endless diversity of chemical compositions. Crucially, by harnessing the molecular design protocols, the optical and spin (electronic and nuclear) properties of molecules can be tailored, aiding the design of optically addressable spin qubits and quantum sensors. In this contribution, we present a concise and collective discussion of optically addressable spin-bearing molecules – namely, organic molecules, transition metal (TM) and rare-earth ion (REI) complexes – and highlight recent results such as chemical tuning of optical and electron spin quantum coherence, optical spin initialization and readout, intramolecular quantum teleportation, optical coherent storage, and photonic-enhanced optical addressing. We envision that optically addressable spin-carrying molecules could become a scalable building block of quantum hardware for applications in the fields of quantum sensing, quantum communication and quantum computing.","PeriodicalId":19027,"journal":{"name":"Nanophotonics","volume":"64 1","pages":""},"PeriodicalIF":7.5,"publicationDate":"2024-10-23","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142488923","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2024-10-23DOI: 10.1515/nanoph-2024-0415
Xiaoxiang Dong, Yonglin He, Tao Zhu, Renxian Gao, Lingyun Hu, Jiayu Li, Peiwen Ren, Jian-Feng Li, Ming-De Li, Zhilin Yang
Ultrafast all-optical control has been a subject of wide-spread attention as a method of manipulating optical fields using light excitation on extremely short time scales. As a fundamental form of ultrafast all-optical control, all-optical switching has achieved sub-picosecond switch speeds in the visible, infrared, and terahertz spectral regions. However, due to the lack of suitable materials, ultrafast all-optical control in the ultraviolet range remains in its early stages. We demonstrate sub-picosecond all-optical switching in the ultraviolet wavelength by designing a Si3N4-ITO Fabry–Pérot resonance aligns with the edge of the interband transition region of ITO. The response time of 500 fs achieved at a pump fluence as low as 0.17 mJ/cm2. Notably, unlike conventional binary switches (0, 1), this biphasic all-optical switch enables the modulation of optical intensity with positive, zero, and negative ΔR/R (0, 1, −1) at the same wavelength, all achieved with a switching speed of 680 fs at a pump fluence of 0.45 mJ/cm2. This work establishing a new pathway for all-optical control in the ultraviolet spectrum, the biphasic switch provides an extra degree of freedom for all-optical modulation.
{"title":"Sub-picosecond biphasic ultrafast all-optical switching in ultraviolet band","authors":"Xiaoxiang Dong, Yonglin He, Tao Zhu, Renxian Gao, Lingyun Hu, Jiayu Li, Peiwen Ren, Jian-Feng Li, Ming-De Li, Zhilin Yang","doi":"10.1515/nanoph-2024-0415","DOIUrl":"https://doi.org/10.1515/nanoph-2024-0415","url":null,"abstract":"Ultrafast all-optical control has been a subject of wide-spread attention as a method of manipulating optical fields using light excitation on extremely short time scales. As a fundamental form of ultrafast all-optical control, all-optical switching has achieved sub-picosecond switch speeds in the visible, infrared, and terahertz spectral regions. However, due to the lack of suitable materials, ultrafast all-optical control in the ultraviolet range remains in its early stages. We demonstrate sub-picosecond all-optical switching in the ultraviolet wavelength by designing a Si<jats:sub>3</jats:sub>N<jats:sub>4</jats:sub>-ITO Fabry–Pérot resonance aligns with the edge of the interband transition region of ITO. The response time of 500 fs achieved at a pump fluence as low as 0.17 mJ/cm<jats:sup>2</jats:sup>. Notably, unlike conventional binary switches (0, 1), this biphasic all-optical switch enables the modulation of optical intensity with positive, zero, and negative Δ<jats:italic>R</jats:italic>/<jats:italic>R</jats:italic> (0, 1, −1) at the same wavelength, all achieved with a switching speed of 680 fs at a pump fluence of 0.45 mJ/cm<jats:sup>2</jats:sup>. This work establishing a new pathway for all-optical control in the ultraviolet spectrum, the biphasic switch provides an extra degree of freedom for all-optical modulation.","PeriodicalId":19027,"journal":{"name":"Nanophotonics","volume":"9 1","pages":""},"PeriodicalIF":7.5,"publicationDate":"2024-10-23","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142488924","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2024-10-22DOI: 10.1515/nanoph-2024-0441
Xi Ming Li, Yuan Zhao, Ren Pan Lu, Xiao Feng Sun, Zhao Yang, Hai Dan He, Yan Hui Liu, Guo Hong Du
Flexible and diverse manipulation of electromagnetic (EM) waves in half space (reflection or transmission) has facilitated strong aspiration toward full-space wave control. However, it remains challenging to achieve independent amplitude and phase control, which seriously hinder the real-world applications. Herein, an innovative strategy of trifunctional metasurface is proposed to independently and simultaneously manipulate the amplitude and phase of circular polarized waves in full space. The multifunctional design is composed of double-layer anisotropic metasurface sandwiched with a bandpass frequency selective surface, with a frequency-direction multiplexed paradigm for on-demand control of both amplitude and phase across three independent channels. To validate the concept, a multifunctional metadevice is designed and verified by simulations and experiments, showcasing arbitrary near-field and far-field power modulation in full space. Lateral and axial bifocal metalenses with desired intensity distribution are designed in two reflection channels at 9 GHz, while multibeam generator with desired spatial scatterings and power allocations is designed in transmissive channel at 13 GHz. The finding paves the way for attaining multifunctional metadevices with amplitude and phase modulation in full space, which have potential applications in high-quality imaging and high-capacity communication systems.
{"title":"Full-space trifunctional metasurface with independent control of amplitude and phase for circularly polarized waves","authors":"Xi Ming Li, Yuan Zhao, Ren Pan Lu, Xiao Feng Sun, Zhao Yang, Hai Dan He, Yan Hui Liu, Guo Hong Du","doi":"10.1515/nanoph-2024-0441","DOIUrl":"https://doi.org/10.1515/nanoph-2024-0441","url":null,"abstract":"Flexible and diverse manipulation of electromagnetic (EM) waves in half space (reflection or transmission) has facilitated strong aspiration toward full-space wave control. However, it remains challenging to achieve independent amplitude and phase control, which seriously hinder the real-world applications. Herein, an innovative strategy of trifunctional metasurface is proposed to independently and simultaneously manipulate the amplitude and phase of circular polarized waves in full space. The multifunctional design is composed of double-layer anisotropic metasurface sandwiched with a bandpass frequency selective surface, with a frequency-direction multiplexed paradigm for on-demand control of both amplitude and phase across three independent channels. To validate the concept, a multifunctional metadevice is designed and verified by simulations and experiments, showcasing arbitrary near-field and far-field power modulation in full space. Lateral and axial bifocal metalenses with desired intensity distribution are designed in two reflection channels at 9 GHz, while multibeam generator with desired spatial scatterings and power allocations is designed in transmissive channel at 13 GHz. The finding paves the way for attaining multifunctional metadevices with amplitude and phase modulation in full space, which have potential applications in high-quality imaging and high-capacity communication systems.","PeriodicalId":19027,"journal":{"name":"Nanophotonics","volume":"92 1","pages":""},"PeriodicalIF":7.5,"publicationDate":"2024-10-22","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142487235","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
京公网安备 11010802042870号
京ICP备2023020795号-1
扫码关注我们
求助内容：
应助结果提醒方式：