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Implementation and optimisation of cosmic veto system using digital electronics in an environmental gamma-spectrometry laboratory 在环境伽马能谱仪实验室利用数字电子技术实施和优化宇宙否决系统
IF 1.6 3区 物理与天体物理 Q2 NUCLEAR SCIENCE & TECHNOLOGY Pub Date : 2024-09-20 DOI: 10.1016/j.radmeas.2024.107302
Luka Bakrač , Tomislav Ilievski , Nikola Marković , Damir Bosnar , Ivana Tucaković
This paper presents a detailed description of construction and introduction of an assembly for cosmic veto system at the Laboratory for radioecology of the Ruđer Bošković Institute in Zagreb. It is a typical surface laboratory for environmental radioactivity measurements using HPGe detectors. In surface level laboratories a large part of the background signal is caused by radiation produced by cosmic radiation, mostly by muons. It leads to limiting factors for reaching low detection limits, essential in environmental sample measurements, where relatively low activity concentrations are expected. Thus, reduction of cosmic component of background becomes a requirement, but also a challenge and an expense for already set routine gamma spectrometric laboratories. This paper offers a detailed description of materials and steps needed for construction and implementation of such an assembly as a guideline for other laboratories. The homebuilt veto system presented here is based on large scintillator plates covering the existing passive lead shielding. For the easy and rapid characterization of the veto system, a newly acquired digitizer was used. More specifically, the timestamping capabilities of the CAEN DT5781 MCA were used to identify the coincidences caused by muons between the scintillators and the HPGe. With the 3 plates added, a reduction factor of 2.4 was achieved, reducing the count rate between 40 keV and 2700 keV from 0.58 cps to 0.27 cps. After the full characterization of the veto system, the setup was transferred back to the previously used Canberra DSA, more suitable for routine measurements. This step and its description are lacking in the existing literature, while it is very valuable for the laboratories already set up for the environmental measurement. The additional advantages of a homebuilt system are the modularity and multi-purpose of the system which can later be used for different applications.
本文详细介绍了萨格勒布鲁杰尔-博什科维奇研究所放射生态学实验室宇宙否决系统组件的建造和引进情况。这是一个使用 HPGe 探测器进行环境放射性测量的典型地面实验室。在地表实验室中,很大一部分本底信号是由宇宙辐射(主要是μ介子)产生的。这导致了达到低检测限的限制因素,而低检测限对于环境样品测量是至关重要的,因为环境样品的放射性浓度相对较低。因此,减少本底中的宇宙成分就成了一项要求,同时也是一项挑战,对已经建立的常规伽马能谱实验室来说也是一笔开支。本文详细介绍了建造和实施这种装置所需的材料和步骤,为其他实验室提供指导。本文介绍的自制否决系统是以覆盖现有被动铅屏蔽的大型闪烁板为基础的。为了简便快速地鉴定否决系统,使用了新购置的数字转换器。更具体地说,CAEN DT5781 MCA 的时间戳功能被用来识别闪烁体和 HPGe 之间μ介子引起的重合。由于增加了 3 块板,减少系数达到了 2.4,使 40 keV 至 2700 keV 之间的计数率从 0.58 cps 降至 0.27 cps。在对否决系统进行全面鉴定之后,该装置被转回先前使用的堪培拉 DSA,因为它更适合常规测量。现有文献中缺乏对这一步骤及其说明的介绍,而这一步骤对于已经建立的环境测量实验室来说非常有价值。自制系统的额外优势在于系统的模块化和多用途性,日后可用于不同的应用领域。
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引用次数: 0
Single-photon elimination in liquid scintillation counting with pulse shape discrimination and delayed coincidence 利用脉冲形状判别和延迟重合在液体闪烁计数中消除单光子
IF 1.6 3区 物理与天体物理 Q2 NUCLEAR SCIENCE & TECHNOLOGY Pub Date : 2024-09-20 DOI: 10.1016/j.radmeas.2024.107299
Pengpeng Zhang , Deyuan Li , Hui Li , Hui Zhang , Xuanru Zhang , Yan Ma , Linjing Wang , Hua Li , Xuewen Yan
Liquid scintillation counting is widely used in the rapid measurement of beta activity in environmental and biological samples. However, the single-photons generated by chemiluminescence and photoluminescence in liquid scintillation cocktails seriously affect the measurement accuracy of low-energy beta activity. A novel method based on the combination of the signal characteristic analysis and selective gate to eliminate the single-photon signal was developed. A preprocessing circuit made of a fast response time photomultiplier tube (PMT, Hamamatsu R9420), two charge-sensitive preamplifiers (CSP), two comparators, an analog switch and delay-line devices were designed and developed to verify the feasibility and effectiveness. The output signals from the last dynode were characterized in the pulse time and were used to discriminate the beta signals from the single-photon ones. The beta signals were “tagged” through pulse width detection, pulse width-amplitude transform and pulse-height discrimination with the first comparator, the first CSP and the second comparator. The “tagged” beta signal were applied to control the analog switch. The anode signals were specially delayed and then selected by the analog switch to achieve the single-photon signal elimination. Liquid scintillation cocktails containing 14C or NaOH used as beta or single-photon sources were provided to verify the feasibility of the principle. The results showed that the typical fall time of the single-photon and beta signal was 16.05 ns and 43.17 ns. The single-photon rejection ratio is 2.76 × 103 ± 3.89 × 105, and the detection efficiency is up to 93.02%±0.59%.
液体闪烁计数被广泛用于快速测量环境和生物样品中的β活度。然而,液体闪烁鸡尾酒中化学发光和光致发光产生的单光子严重影响了低能贝塔活度的测量精度。研究人员开发了一种基于信号特征分析和选择性门相结合的消除单光子信号的新方法。为了验证这种方法的可行性和有效性,我们设计并开发了一个由快速响应时间光电倍增管(PMT,滨松 R9420)、两个电荷敏感前置放大器(CSP)、两个比较器、一个模拟开关和延迟线器件组成的预处理电路。最后一个 dynode 的输出信号具有脉冲时间特征,用于从单光子信号中分辨出贝塔信号。通过第一个比较器、第一个 CSP 和第二个比较器的脉宽检测、脉宽-脉幅变换和脉高分辨,对贝塔信号进行 "标记"。标记 "的贝塔信号用于控制模拟开关。阳极信号经过特殊延迟后由模拟开关选择,以实现单光子信号消除。为了验证该原理的可行性,我们提供了含有 14C 或 NaOH 的液体闪烁鸡尾酒作为贝塔源或单光子源。结果表明,单光子和贝塔信号的典型下降时间分别为 16.05 ns 和 43.17 ns。单光子抑制比为 2.76 × 10-3 ± 3.89 × 10-5,探测效率高达 93.02%±0.59%。
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引用次数: 0
3D printed microcrystalline CsI:Tl composite scintillating thin films for X-ray imaging 用于 X 射线成像的 3D 打印微晶 CsI:Tl 复合闪烁薄膜
IF 1.6 3区 物理与天体物理 Q2 NUCLEAR SCIENCE & TECHNOLOGY Pub Date : 2024-09-19 DOI: 10.1016/j.radmeas.2024.107301
Divya Pandya , Nisha Oad , Sheetal Rawat , Brijesh Tripathi , Pavan Gurrala , Partha Sarathi Sarkar , Mohit Tyagi , Apoorva Bhatt
The utilization of additive manufacturing techniques, especially Digital Light Printing (DLP), in fabricating CsI:Tl scintillator films demonstrates considerable potential for streamlining the production of scintillators tailored for X-ray imaging applications. This research focuses on the fabrication of CsI:Tl-based composite plastic scintillator thin films. In this study, circular films measuring 1-inch in diameter and 0.1 mm & 0.2 mm in thickness are being produced and tested for gamma photon counts under alpha and gamma radiation. To establish the stopping power range of the films, a Monte Carlo based GEANT4 simulation has been carried out. Additionally, investigations into their suitability for X-ray imaging applications are being conducted, revealing the spatial resolution of the films (0.2 and 0.1 mm) between 100 and 130 μm and 1.26 lp/mm with a contrast range of 4.0–12.3 %. The observed decrease in spatial resolution and contrast for the 0.2 mm thick film is attributed to the thickness increase exacerbating the scattering phenomenon while simultaneously enhancing the X-ray stopping power. This highlights the significance of inherent trade-off between maximizing spatial resolution and compromising light yield of 0.1 mm films compared to the 0.2 mm thick film. By utilizing 3D printing, this approach offers a cost-effective and time-efficient method for producing thin-film scintillators with enhanced flexibility and customization options compared to conventional methods.
利用增材制造技术,特别是数字光打印(DLP)技术来制造铯钛闪烁体薄膜,对于简化 X 射线成像应用闪烁体的生产具有相当大的潜力。本研究的重点是铯钛基复合塑料闪烁体薄膜的制造。在这项研究中,我们制作了直径为 1 英寸、直径为 0.1 毫米、厚度为 0.2 毫米的圆形薄膜,并在阿尔法和伽马射线辐射下进行了伽马光子计数测试。为了确定薄膜的阻挡功率范围,我们进行了基于蒙特卡罗的 GEANT4 模拟。此外,还对薄膜在 X 射线成像应用中的适用性进行了研究,结果显示薄膜(0.2 和 0.1 毫米)的空间分辨率在 100 和 130 μm 之间,对比度范围为 4.0-12.3 %,对比度为 1.26 lp/mm。观察到 0.2 毫米厚薄膜的空间分辨率和对比度下降,这是因为厚度增加加剧了散射现象,同时增强了 X 射线阻挡能力。这突出表明,与 0.2 毫米厚的薄膜相比,0.1 毫米厚的薄膜在最大限度提高空间分辨率和降低光产率之间的内在权衡意义重大。通过利用三维打印技术,这种方法为生产薄膜闪烁体提供了一种具有成本效益和时间效率的方法,与传统方法相比,它具有更高的灵活性和定制选项。
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引用次数: 0
Study of thermoluminescence characteristics of quartz for high radiation doses (>1kGy): Implications for extending the luminescence dating range 高辐射剂量(>1kGy)石英热发光特性研究:对扩大发光测年范围的影响
IF 1.6 3区 物理与天体物理 Q2 NUCLEAR SCIENCE & TECHNOLOGY Pub Date : 2024-09-18 DOI: 10.1016/j.radmeas.2024.107300
Malika Singhal , Madhusmita Panda , S.H. Shinde , Sandip Mondal , O. Annalakshmi , Naveen Chauhan
Quartz is an omnipresent abundant natural mineral, used for luminescence dating. Lately, quartz optically stimulated luminescence (OSL) technique is widely used to estimate the equivalent doses (De) for dating geological events (up to 250 Gy, limited by saturation). Some works report thermoluminescence (TL) saturation around ∼ (10–40) kGy. Still dose estimates for such high radiation dose (HRD) range are not achieved. Significant research exists about luminescence response for low dose ranges (<250 Gy) but limited studies are done for HRDs (>1 kGy). This work characterizes the luminescence response of quartz for HRDs (1–21 kGy) to improve existing understanding of luminescence mechanism. Results show that the characteristics of the trap (<200 °C) differ significantly at HRDs than low doses. TL in multi-spectral detection (UV–Visible) band suggest an increase in 340–380 °C peak intensity up to 11 kGy dose. The measurements of saturation dose suggest that it depends on the trapping centres but is independent of recombination centres for the samples used for study. The traps are found bleachable by sunlight, reducing TL signal to residual levels in 1 h. Further, the bleachability is found to be anti-correlated with luminescence emission wavelength. At HRDs luminescence sensitivity is influenced by dose given in previous cycle which is difficult to correct by routine normalization procedures. The work also explores the various normalization methods to find appropriate method for HRD estimation and recommends the use of mass normalization as other normalization methods do not correct the sensitivity changes at HRDs adequately.
石英是一种无处不在的丰富天然矿物,可用于发光测年。最近,石英光激发发光(OSL)技术被广泛用于估算地质事件年代的当量剂量(De)(最高可达 250 Gy,受饱和度限制)。一些研究报告称,热释光(TL)的饱和度约为∼ (10-40) kGy。但对这种高辐射剂量(HRD)范围的剂量估计仍未实现。关于低剂量范围(250 Gy)的发光响应已有大量研究,但针对高辐射剂量(1 kGy)的研究却十分有限。这项研究描述了石英对 HRDs(1-21 kGy)的发光响应,以加深对发光机制的理解。结果表明,与低剂量相比,HRDs 时陷阱(<200 °C)的特性有很大不同。多光谱检测(紫外-可见光)波段的 TL 表明,在 11 kGy 剂量以下,340-380 ℃ 峰值强度会增加。饱和剂量的测量结果表明,它取决于捕获中心,但与用于研究的样品的重组中心无关。此外,还发现漂白性与发光发射波长无关。在 HRDs 中,发光灵敏度受前一周期所给剂量的影响,这很难通过常规归一化程序来纠正。这项研究还探讨了各种归一化方法,以找到合适的方法来估算 HRD,并建议使用质量归一化,因为其他归一化方法不能充分纠正 HRD 的灵敏度变化。
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引用次数: 0
Microdosimetry for BNCT: First measurements at different site sizes 用于 BNCT 的显微模拟技术:不同部位尺寸的首次测量
IF 1.6 3区 物理与天体物理 Q2 NUCLEAR SCIENCE & TECHNOLOGY Pub Date : 2024-09-14 DOI: 10.1016/j.radmeas.2024.107298
A. Selva, A. Bianchi, L. Bellan, E. Fagotti, A. Pisent, V. Conte

Microdosimetric techniques are a valuable tool for beam quality monitoring in BNCT, due to their capability to distinguish different contributions to the total dose and provide physics-based quantities related to biological effectiveness of this composite radiation field. To this aim, measurements are generally performed with gas detectors simulating a tissue-equivalent site size between 0.5 and 2 μm. This work presents instead measurements for site sizes up to 10 μm, performed in the thermal neutron field produced by the accelerator-based MUNES source available at INFN-LNL. An avalanche-confinement TEPC with boron doping in the cathode walls was used. Photon and neutron dose fractions were discriminated in the measured dose-weighted distributions based on their different lineal energy range. In the neutron component two separate peaks could be distinguished for site sizes of 5 μm and greater, the origin of which was tentatively related to contributions due to protons and alpha particles. These results allow to assess the impact of increasing site diameter on the measured relative dose contributions and provide valuable reference data for biological modelling and for comparison with solid-state microdosimeters.

微剂量测定技术是监测 BNCT 射束质量的重要工具,因为它能够区分对总剂量的不同贡献,并提供与这种复合辐射场的生物有效性有关的物理量。为此,通常使用气体探测器模拟 0.5 至 2 μm 的组织等效部位进行测量。这项工作介绍的是在 INFN-LNL 的 MUNES 加速器源产生的热中子场中对最大 10 μm 的位点尺寸进行的测量。使用的是阴极壁中掺有硼的雪崩抵消 TEPC。在测量的剂量加权分布中,根据不同的线能量范围对光子和中子剂量分数进行了区分。在中子分量中,5 μm 或更大的位点尺寸可区分出两个单独的峰值,其来源初步与质子和阿尔法粒子的贡献有关。通过这些结果,可以评估点直径增大对所测相对剂量贡献的影响,并为生物建模和与固态微剂量计进行比较提供有价值的参考数据。
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引用次数: 0
Use of a Machine Learning based method to detect anomalous Thermoluminescence Glow Curves (TL-GC) in routine Dosimetry Services 在常规剂量测定服务中使用基于机器学习的方法检测异常热释光辉光曲线 (TL-GC)
IF 1.6 3区 物理与天体物理 Q2 NUCLEAR SCIENCE & TECHNOLOGY Pub Date : 2024-09-10 DOI: 10.1016/j.radmeas.2024.107293
O. Arquero , J. Berenguer-Antequera , J.F. Benavente

This contribution describes the development of a set of numerical methods based on Machine Learning algorithms to generate an automated classification of experimental Thermoluminescence (TL) Glow Curves obtained routinely by Dosimetry Services. This classification will use experimental data historically recorded by Thermoluminescence Dosimeter (TLD) devices and will be based on the search for possible anomalies in the curves. The classifier tool will ease the labelling of experimental data and the detection of anomalies without previous supervision, implying an improvement in the control evaluations in Quality Guarantee Systems often implemented by Dosimetry Services. Furthermore, this study shows that each curve provides information about the status of each dosimeter, and can be used to perform unsupervised classifications of the measurements.

本论文介绍了一套基于机器学习算法的数值方法的开发过程,该方法可对剂量测定服务部门日常获得的实验性热释光(TL)辉光曲线进行自动分类。该分类将使用热释光剂量计(TLD)设备历史记录的实验数据,并基于对曲线中可能存在的异常情况的搜索。分类器工具将简化实验数据的标注和异常检测,而无需事先监督,这意味着剂量测定服务部门通常实施的质量保证体系中的控制评估将得到改进。此外,这项研究还表明,每条曲线都提供了有关每个剂量计状态的信息,可用于对测量结果进行无监督分类。
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引用次数: 0
Thermoluminescence properties of β-ray irradiated LuAGG:Ce nanophosphors prepared by sol-gel method for potential applications in dosimetry 溶胶-凝胶法制备的 β 射线辐照 LuAGG:Ce 纳米磷的热致发光特性在剂量测定中的潜在应用
IF 1.6 3区 物理与天体物理 Q2 NUCLEAR SCIENCE & TECHNOLOGY Pub Date : 2024-09-10 DOI: 10.1016/j.radmeas.2024.107296
S. Saadi , D.E. Kdib , A. Boukerika , R. Berreksi , A. Bentabet , S. Mahtout , Z. L Mokrani

In this paper, Lu2.97Al5–xGaxO12:Ce0.03 (x = 0, 1, 2, 3) nanophosphors were synthesized using sol-gel method and calcined at 1100 °C for 3 h. The effect of Ga content on the structural, photoluminescence (PL), and notably thermoluminescence (TL) glow curve, dose response, repeatability and fading properties were investigated. X-ray diffraction (XRD) results indicated that all synthesized samples were crystallized in a pure garnet phase. The PL emission spectra exhibited a broad emission band corresponding to the 5 d → 4f (2F5/2, 2F7/2) transition of Ce3+ ions in the garnet lattice. Furthermore, a significant decrease in emission intensity was observed upon increasing Ga content. The TL characteristics of nanopowders irradiated with β-rays revealed a significant effect of Ga content on the peak position, shape and intensities of TL Glow curves, which can be explained by the reduction of the energy gap and the distribution of trap levels. The dose response linearity in the range of 0.125–100 Gy was examined for different Ga content, revealing a good linear behavior for x = 0 and 1 Ga. Additionally, samples prepared with x = 0, 1, and 2 Ga exhibited a high level of repeatability across a batch of 10 samples. Also, fading studies were performed for 128 h and revealed strong fading in samples synthesized with x = 0 and 1 Ga. These results suggest potential applications of Lu3Al5O12:Ce and Lu3Al4Ga1O12:Ce in ionizing radiation dosimetry.

本文采用溶胶-凝胶法合成了 Lu2.97Al5-xGaxO12:Ce0.03(x = 0、1、2、3)纳米磷酸盐,并在 1100 °C 煅烧 3 h。研究了 Ga 含量对结构、光致发光 (PL) 和显著热致发光 (TL) 辉光曲线、剂量响应、重复性和衰减特性的影响。X 射线衍射 (XRD) 结果表明,所有合成样品均为纯石榴石相结晶。聚光发射光谱显示出一个宽发射带,对应于石榴石晶格中 Ce3+ 离子的 5 d → 4f (2F5/2, 2F7/2)转变。此外,随着镓含量的增加,发射强度也明显下降。用 β 射线辐照纳米粉体的 TL 特性表明,镓含量对 TL 辉光曲线的峰值位置、形状和强度有显著影响,这可以用能隙的减小和陷阱水平的分布来解释。对不同镓含量在 0.125-100 Gy 范围内的剂量响应线性进行了研究,结果表明 x = 0 和 1 Ga 具有良好的线性行为。此外,用 x = 0、1 和 2 Ga 制备的样品在一批 10 个样品中表现出较高的重复性。此外,还对 x = 0 和 1 Ga 合成的样品进行了长达 128 小时的衰减研究,结果表明这些样品具有很强的衰减性。这些结果表明了 Lu3Al5O12:Ce 和 Lu3Al4Ga1O12:Ce 在电离辐射剂量测定中的潜在应用。
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引用次数: 0
Significance and feasibility of air kerma length product and air kerma area product comparisons 空气气膜长度乘积和空气气膜面积乘积比较的意义和可行性
IF 1.6 3区 物理与天体物理 Q2 NUCLEAR SCIENCE & TECHNOLOGY Pub Date : 2024-09-10 DOI: 10.1016/j.radmeas.2024.107291
Miloš Živanović , Maja Vojnić Kortmiš , Nikola Kržanović , Miloš Đaletić , Ivana Komatina

Air kerma length product and air kerma area product are special quantities used in diagnostic radiology. They are measured using special measurement devices – CT-chambers and KAP-meters, in order to calculate quantities related to patient exposure. Appropriate calibration of all measurement devices is of vital importance, and comparisons between calibration laboratories are necessary to prove competence.

It is usually considered adequate to participate in air kerma comparisons to prove capabilities for special quantities, but the literature shows that some problems in calibration procedure can remain unknown. The comparisons directly in terms of special quantities provide additional burden to laboratories, and require special transfer instruments, but they allow checking the whole calibration procedures.

This paper describes a comparison between two calibration laboratories in terms of both air kerma length product and air kerma area product. Both laboratories achieved good results for all radiation qualities, considering the measurement uncertainty. Transfer instruments’ linearity, field size dependence and energy dependence were investigated. Even though the metrological properties of the transfer instruments are worse than the ionization chambers, they can be taken into account by introducing additional measurement uncertainty, performing appropriate corrections or choosing calibration points for the comparison for the values of influence quantities where the transfer instrument response is relatively flat. These comparisons provide additional value to calibration laboratories, but there are still several challenges related to their organization and execution.

空气介质长度积和空气介质面积积是放射诊断中使用的特殊数量。它们通过特殊的测量设备--CT-腔室和 KAP 计进行测量,以计算与患者照射有关的数量。对所有测量设备进行适当的校准至关重要,校准实验室之间的比较是证明能力的必要手段。本文介绍了两个校准实验室在空气热玛长度积和空气热玛面积积方面的比较。考虑到测量的不确定性,两个实验室在所有辐射质量方面都取得了良好的结果。对转移仪器的线性、场大小依赖性和能量依赖性进行了研究。尽管转移仪器的计量特性比电离室差,但可以通过引入额外的测量不确定性、进行适当的修正或为转移仪器响应相对平缓的影响量值的比较选择校准点来考虑这些特性。这些比对为校准实验室提供了额外的价值,但在其组织和执行方面仍存在一些挑战。
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引用次数: 0
International intercomparison and quality assessment of passive and active 222Rn measuring devices in the Asia-Pacific region 亚太地区无源和有源 222Rn 测量装置的国际互比和质量评估
IF 1.6 3区 物理与天体物理 Q2 NUCLEAR SCIENCE & TECHNOLOGY Pub Date : 2024-09-10 DOI: 10.1016/j.radmeas.2024.107295
N. Karunakara , A.P. Vijith , Rosaline Mishra , B.K. Sahoo , Miroslaw Janik , Sudeep Kumara , B.K. Sapra , Shinji Tokonami , Chutima Kranrod , S. Chandrasekaran , N. Chitra , Seon hong Kim , Juhee Yoo , Chao Zhao , Bo Chen , Hong-Gi Kim , Jin-il Kim , Josef Holecek , Le Dinh Cuong

Intercomparison exercise is an integral part of the quality assurance programmes in 222Rn measurements using active and passive devices. Ensuring the accuracy of data generated through measurements necessitates periodic performance checks. To achieve harmonization of methods, quantify biases and errors in measurements, and identify the reasons for discrepancies, there is a pressing need for periodic intercomparison exercises. To address this need of numerous laboratories, particularly in the Asia-Pacific region, a calibration facility for 222Rn measuring devices has been established at the Centre for Advanced Research in Environmental Radioactivity (CARER), Mangalore University, India. An international intercomparison exercise for the 222Rn measuring devices was conducted at this facility in the year 2022 with the participation of 10 laboratories from six countries. A total of 354 devices (comprising of both active and passive detectors) were subjected to intercomparison measurements by exposing them to three concentration levels: (5.97 ± 0.29) × 103 Bq m−3, (0.70 ± 0.09) × 103 Bq m−3 and (2.02 ± 0.20) × 103 Bq m−3 in separate experiments and the exposure durations were 7 days, 15 days, and 10 days respectively. The performance of each laboratory was evaluated following the criterion adopted by the International Atomic Energy Agency (IAEA) in its worldwide proficiency test programmes. This exercise brought out the fact that some of the laboratories need to improve their measurement practices to produce reliable data.

相互比较工作是使用有源和无源装置进行 222Rn 测量的质量保证计划的组成部分。要确保测量数据的准确性,就必须定期进行性能检查。为了实现方法的统一、量化测量中的偏差和误差并找出差异的原因,迫切需要进行定期的相互比对。为了满足众多实验室,特别是亚太地区实验室的这一需求,印度芒格洛尔大学环境放射性高级研究中心(CARER)建立了 222Rn 测量设备校准设施。2022 年,来自 6 个国家的 10 个实验室参加了在该设施举行的 222Rn 测量装置国际相互比对活动。共有 354 个装置(包括主动和被动探测器)接受了比对测量,分别暴露于三个浓度水平:(5.97 ± 0.29) × 103 Bq m-3、(0.70 ± 0.09) × 103 Bq m-3和(2.02 ± 0.20) × 103 Bq m-3,暴露时间分别为 7 天、15 天和 10 天。按照国际原子能机构(IAEA)在其全球能力测试计划中采用的标准,对每个实验室的性能进行了评估。这项工作表明,一些实验室需要改进其测量方法,以获得可靠的数据。
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引用次数: 0
Study on the effects of preparation processes on OSL and TL properties of NaMgF3:Dy,Eu 制备工艺对 NaMgF3:Dy,Eu 的光致发光(OSL)和热致发光(TL)特性的影响研究
IF 1.6 3区 物理与天体物理 Q2 NUCLEAR SCIENCE & TECHNOLOGY Pub Date : 2024-09-10 DOI: 10.1016/j.radmeas.2024.107297
Siyuan Zhang, Kaiyong Tang, Li Fu, Mo Zhou, Haijun Fan, Yan Zeng, Zhiyuan Li

OSL fading with storage time after irradiation remains a major obstacle in the development of ideal OSL materials. Dy and Eu co-doped NaMgF3 are attractive candidates for various rare earth doped matrix materials. In this study, NaMgF3:Dy,Eu was synthesized by a solid-state reaction, and the effects of heating temperature, duration, atmosphere, and cooling rate on XRD, TL and OSL properties were studied. A simple, safe, efficient, and time-saving solid-state reaction was identified as a potential method for the preparation of NaMgF3:Dy,Eu, which could be optimally prepared by heating at 750 °C for 2 h under nitrogen atmosphere (2 l/min) followed by rapid cooling. The results show that NaMgF3:Dy,Eu has a more stable OSL response and an excellent TL glow curve, with only a 0.4% decrease in the OSL signal read after 1 d of dose irradiation compared to that immediately after irradiation, and a high main TL peak at ∼320 °C. It has been indicated the OSL signal in this material seems to be strongly related to the main TL peak. The material has a considerable OSL sensitivity and decay rate than the Luxel Detector. NaMgF3:Dy,Eu will have a promising future in the field of OSL dosimetry due to its near tissue equivalence, low OSL fading without preheating, fast OSL decay rate, and predictable and easily reusable dose elimination.

辐照后,OSL 会随储存时间而衰减,这仍然是开发理想 OSL 材料的主要障碍。Dy和Eu共掺杂的NaMgF3是各种稀土掺杂基体材料的理想候选材料。本研究通过固态反应合成了 NaMgF3:Dy,Eu,并研究了加热温度、持续时间、气氛和冷却速率对 XRD、TL 和 OSL 性能的影响。结果表明,在氮气环境(2 升/分钟)下于 750 ℃加热 2 小时,然后快速冷却,可以制备出最佳的 NaMgF3:Dy,Eu。结果表明,NaMgF3:Dy,Eu 具有更稳定的 OSL 响应和出色的 TL 辉光曲线,在剂量辐照 1 d 后读取的 OSL 信号与辐照后立即读取的信号相比仅下降了 0.4%,并且在 ∼320 °C 处具有较高的 TL 主峰。这表明该材料中的 OSL 信号似乎与主 TL 峰密切相关。与 Luxel 探测器相比,该材料具有相当高的 OSL 灵敏度和衰减率。NaMgF3:Dy,Eu因其接近组织等效性、无需预热的低OSL衰减、快速的OSL衰减率以及可预测和易于重复使用的剂量消除,在OSL剂量测定领域前景广阔。
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Radiation Measurements
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