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It is all about phases: ultrafast holographic photoelectron imaging 这一切都与相位有关:超快全息光电子成像
IF 18.1 1区 物理与天体物理 Q1 Physics and Astronomy Pub Date : 2019-06-27 DOI: 10.1088/1361-6633/ab5c91
C. Figueira de Morisson Faria, A. Maxwell
Photoelectron holography constitutes a powerful tool for the ultrafast imaging of matter, as it combines high electron currents with subfemtosecond resolution, and gives information about transition amplitudes and phase shifts. Similarly to light holography, it uses the phase difference between the probe and the reference waves associated with qualitatively different ionization events for the reconstruction of the target and for ascertaining any changes that may occur. These are major advantages over other attosecond imaging techniques, which require elaborate interferometric schemes in order to extract phase differences. For that reason, ultrafast photoelectron holography has experienced a huge growth in activity, which has led to a vast, but fragmented landscape. The present review is an organizational effort towards unifying this landscape. This includes a historic account in which a connection with laser-induced electron diffraction is established, a summary of the main holographic structures encountered and their underlying physical mechanisms, a broad discussion of the theoretical methods employed, and of the key challenges and future possibilities. We delve deeper in our own work, and place a strong emphasis on quantum interference, and on the residual Coulomb potential.
光电子全息术是物质超快成像的有力工具,因为它结合了高电流和亚飞秒分辨率,并提供了有关跃迁幅度和相移的信息。与光全息术类似,它利用探针和与定性不同电离事件相关的参考波之间的相位差来重建目标,并确定可能发生的任何变化。这是与其他阿秒成像技术相比的主要优势,后者需要复杂的干涉方案来提取相位差。因此,超快光电子全息术经历了活动的巨大增长,这导致了一个巨大的,但碎片化的景观。目前的审查是对统一这一景观的组织努力。这包括与激光诱导电子衍射建立联系的历史叙述,所遇到的主要全息结构及其潜在物理机制的总结,所采用的理论方法的广泛讨论,以及关键挑战和未来可能性。我们在自己的工作中进行了更深入的研究,并将重点放在量子干涉和剩余库仑势上。
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引用次数: 66
Tin titanate—the hunt for a new ferroelectric perovskite 钛锡——寻找一种新的铁电钙钛矿
IF 18.1 1区 物理与天体物理 Q1 Physics and Astronomy Pub Date : 2019-06-07 DOI: 10.1088/1361-6633/ab37d4
J. Gardner, Atul Thakre, Ashok Kumar, J. Scott
We review all the published literature and show that there is no experimental evidence for homogeneous tin titanate SnTiO3 in bulk or thin-film form. Instead a combination of unrelated artefacts are easily misinterpreted. The x-ray Bragg data are contaminated by double scattering from the Si substrate, giving a strong line at the 2θ angle exactly where perovskite SnTiO3 should appear. The strong dielectric divergence near 560 K is irreversible and arises from oxygen site detrapping, accompanied by Warburg/Randles interfacial anomalies. The small (4 µC cm−2) apparent ferroelectric hysteresis remains in samples shown to be pure (Sn,Ti)O2 rutile/cassiterite, in which ferroelectricity is forbidden. Only very recent work reveals real bulk SnTiO3, but it possesses an ilmenite-like structure with an elaborate array of stacking faults, not suitable for ferroelectric devices. Unpublished TEM data reveal an inhomogeneous SnO layered structured thin films, related to shell–core structures. The harsh conclusion is that there is a combination of unrelated artefacts masquerading as ferroelectricity in powders and ALD films; and only a trace of a second phase in PLD film data suggests any perovskite content at all. The fact that x-ray, dielectric, and hysteresis data all lead to the wrong conclusion is instructive and reminds us of earlier work on copper calcium titanate (a well-known boundary-layer capacitor).
我们回顾了所有已发表的文献,并表明没有实验证据表明钛酸锡SnTiO3是均匀的块状或薄膜形式。相反,不相关的工件的组合很容易被误解。x射线Bragg数据受到来自Si衬底的双重散射的污染,在钙钛矿SnTiO3应该出现的2θ角处给出了一条强线。560k附近的强介电散度是不可逆的,由氧位脱聚引起,伴有Warburg/Randles界面异常。在纯(Sn,Ti)O2金红石/锡石样品中,铁电性仍然很小(4µC cm−2)。直到最近的研究才揭示了真正的块状SnTiO3,但它具有钛铁矿样的结构,具有复杂的堆叠断层阵列,不适合用于铁电器件。未发表的透射电镜数据揭示了非均匀的SnO层状结构薄膜,与壳核结构有关。严酷的结论是,在粉末和ALD薄膜中有不相关的伪影伪装成铁电性;在PLD薄膜数据中,只有微量的第二相表明有钙钛矿含量。x射线、介电和迟滞数据都得出了错误的结论,这一事实具有指导意义,并使我们想起了早期关于钛酸铜钙(一种著名的边界层电容器)的工作。
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引用次数: 11
Programmable interactions with biomimetic DNA linkers at fluid membranes and interfaces 可编程的相互作用与仿生DNA连接在流体膜和界面
IF 18.1 1区 物理与天体物理 Q1 Physics and Astronomy Pub Date : 2019-03-31 DOI: 10.1088/1361-6633/ab37ca
B. Mognetti, P. Cicuta, L. Di Michele
At the heart of the structured architecture and complex dynamics of biological systems are specific and timely interactions operated by biomolecules. In many instances, biomolecular agents are spatially confined to flexible lipid membranes where, among other functions, they control cell adhesion, motility and tissue formation. Besides being central to several biological processes, multivalent interactions mediated by reactive linkers confined to deformable substrates underpin the design of synthetic-biological platforms and advanced biomimetic materials. Here we review recent advances on the experimental study and theoretical modelling of a heterogeneous class of biomimetic systems in which synthetic linkers mediate multivalent interactions between fluid and deformable colloidal units, including lipid vesicles and emulsion droplets. Linkers are often prepared from synthetic DNA nanostructures, enabling full programmability of the thermodynamic and kinetic properties of their mutual interactions. The coupling of the statistical effects of multivalent interactions with substrate fluidity and deformability gives rise to a rich emerging phenomenology that, in the context of self-assembled soft materials, has been shown to produce exotic phase behaviour, stimuli-responsiveness, and kinetic programmability of the self-assembly process. Applications to (synthetic) biology will also be reviewed.
生物系统的结构和复杂动力学的核心是由生物分子操作的特定和及时的相互作用。在许多情况下,生物分子制剂在空间上局限于柔性脂质膜,其中,除其他功能外,它们还控制细胞粘附、运动和组织形成。除了是几个生物过程的核心之外,受限于可变形基质的反应性连接物介导的多价相互作用是合成生物平台和先进仿生材料设计的基础。在这里,我们回顾了异质类仿生系统的实验研究和理论建模的最新进展,其中合成连接剂介导流体和可变形胶体单位(包括脂质囊泡和乳状液滴)之间的多价相互作用。连接体通常由合成的DNA纳米结构制备,使其相互作用的热力学和动力学性质完全可编程。多价相互作用的统计效应与基板流动性和可变形性的耦合产生了丰富的新兴现象学,在自组装软材料的背景下,已被证明会产生奇异的相行为、刺激响应性和自组装过程的动力学可编程性。应用(合成)生物学也将进行审查。
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引用次数: 27
One-dimensional mixtures of several ultracold atoms: a review 几种超冷原子的一维混合物:综述
IF 18.1 1区 物理与天体物理 Q1 Physics and Astronomy Pub Date : 2019-03-28 DOI: 10.1088/1361-6633/ab3a80
T. Sowiński, Miguel Ángel García-March
Recent theoretical and experimental progress on studying one-dimensional systems of bosonic, fermionic, and Bose–Fermi mixtures of a few ultracold atoms confined in traps is reviewed in the broad context of mesoscopic quantum physics. We pay special attention to limiting cases of very strong or very weak interactions and transitions between them. For bosonic mixtures, we describe the developments in systems of three and four atoms as well as different extensions to larger numbers of particles. We also briefly review progress in the case of spinor Bose gases of a few atoms. For fermionic mixtures, we discuss a special role of spin and present a detailed discussion of the two- and three-atom cases. We discuss the advantages and disadvantages of different computation methods applied to systems with intermediate interactions. In the case of very strong repulsion, close to the infinite limit, we discuss approaches based on effective spin chain descriptions. We also report on recent studies on higher-spin mixtures and inter-component attractive forces. For both statistics, we pay particular attention to impurity problems and mass imbalance cases. Finally, we describe the recent advances on trapped Bose–Fermi mixtures, which allow for a theoretical combination of previous concepts, well illustrating the importance of quantum statistics and inter-particle interactions. Lastly, we report on fundamental questions related to the subject which we believe will inspire further theoretical developments and experimental verification.
在介观量子物理的大背景下,综述了近年来在单维玻色子、费米子和玻色-费米混合系统研究中的理论和实验进展。我们特别注意非常强或非常弱的相互作用和它们之间的转换的极限情况。对于玻色子混合,我们描述了三原子和四原子系统的发展,以及不同的扩展到更大数量的粒子。我们还简要回顾了少数原子的旋量玻色气体的研究进展。对于费米子混合物,我们讨论了自旋的特殊作用,并详细讨论了两原子和三原子的情况。讨论了应用于具有中间相互作用的系统的不同计算方法的优缺点。在非常强的排斥力,接近无穷极限的情况下,我们讨论了基于有效自旋链描述的方法。我们还报告了最近关于高自旋混合物和组分间引力的研究。对于这两种统计,我们特别注意杂质问题和质量不平衡情况。最后,我们描述了捕获玻色-费米混合物的最新进展,它允许先前概念的理论组合,很好地说明了量子统计和粒子间相互作用的重要性。最后,我们报告与该主题有关的基本问题,我们认为这些问题将激发进一步的理论发展和实验验证。
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引用次数: 81
Geometric phases in 2D and 3D polarized fields: geometrical, dynamical, and topological aspects 二维和三维极化场的几何相位:几何、动态和拓扑方面
IF 18.1 1区 物理与天体物理 Q1 Physics and Astronomy Pub Date : 2019-03-04 DOI: 10.1088/1361-6633/ab4415
K. Bliokh, M. Alonso, Mark R. Dennis
Geometric phases are a universal concept that underpins numerous phenomena involving multi-component wave fields. These polarization-dependent phases are inherent in interference effects, spin–orbit interaction phenomena, and topological properties of vector wave fields. Geometric phases have been thoroughly studied in two-component fields, such as two-level quantum systems or paraxial optical waves. However, their description for fields with three or more components, such as generic nonparaxial optical fields routinely used in modern nano-optics, constitutes a nontrivial problem. Here we describe geometric, dynamical, and total phases calculated along a closed spatial contour in a multi-component complex field, with particular emphasis on 2D (paraxial) and 3D (nonparaxial) optical fields. We present several equivalent approaches: (i) an algebraic formalism, universal for any multi-component field; (ii) a dynamical approach using the Coriolis coupling between the spin angular momentum and reference-frame rotations; and (iii) a geometric representation, which unifies the Pancharatnam–Berry phase for the 2D polarization on the Poincaré sphere and the Majorana-sphere representation for the 3D polarized fields. Most importantly, we reveal close connections between geometric phases, angular-momentum properties of the field, and topological properties of polarization singularities in 2D and 3D fields, such as C-points and polarization Möbius strips.
几何相位是一个普遍的概念,支持许多涉及多分量波场的现象。这些与极化相关的相位是干涉效应、自旋轨道相互作用现象和矢量波场拓扑特性所固有的。几何相位在双分量领域,如双能级量子系统或近轴光波中得到了深入的研究。然而,它们对具有三个或更多分量的场的描述,例如现代纳米光学中常规使用的一般非傍轴光场,构成了一个非平凡的问题。在这里,我们描述了在多分量复杂场中沿封闭空间轮廓计算的几何相位、动态相位和总相位,特别强调了二维(近轴)和三维(非近轴)光场。我们提出了几个等价的方法:(i)一个代数形式,对任何多分量域都是通用的;(ii)利用自旋角动量和参照系旋转之间的科里奥利耦合的动力学方法;(iii)一个几何表示,它统一了庞加莱球上二维偏振的Pancharatnam-Berry相位和三维偏振场的Majorana-sphere表示。最重要的是,我们揭示了几何相位、场的角动量性质和二维和三维场中极化奇点(如c点和极化Möbius条)的拓扑性质之间的密切联系。
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引用次数: 78
Corrigendum: Composite laser-pulses spectroscopy for high-accuracy optical clocks: a review of recent progress and perspectives (2018 Rep. Prog. Phys. 81 094401) 更正:高精度光学钟的复合激光脉冲光谱学:最近进展和前景的回顾(2018年rep Prog.)。物理81 094401)
IF 18.1 1区 物理与天体物理 Q1 Physics and Astronomy Pub Date : 2018-10-29 DOI: 10.1088/1361-6633/AAE6B2
T. Zanon-Willette, R. Lefevre, R. Metzdorff, N. Sillitoe, S. Almonacil, M. Minissale, E. de Clercq, A. Taichenachev, V. Yudin, E. Arimondo
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引用次数: 1
Excimers 准分子
IF 18.1 1区 物理与天体物理 Q1 Physics and Astronomy Pub Date : 2018-10-08 DOI: 10.1088/0034-4885/38/8/001
J. B. Birks
Excimers are dimers with associated excited electronic states, dissociative ground states, and structureless emission spectra. Noble and other monatomic gases form atomic excimers. Aromatic molecules form excimers in fluid solutions, liquids, crystals and polymers, at crystal defects, and intramolecularly. Excimer interaction is attributed to configurational mixing of exciton and charge resonance states. The helium excimer and pyrene crystal dimer potential curves are compared. Aromatic excimers are discussed. Related photophysical studies on atomic excimers are considered. Saturated amines, which exhibit vapour and solution excimer fluorescence, provide a link between atomic and aromatic excimers. Aromatic molecules form complexes, exciplexes or mixed excimers with different molecules, and noble gas atoms form complexes or exciplexes with different atoms. Review completed in 1975.
准分子是具有相关激发态、离解基态和无结构发射光谱的二聚体。惰性气体和其他单原子气体形成原子准分子。芳香分子在流体溶液、液体、晶体和聚合物、晶体缺陷和分子内形成准分子。准分子相互作用归因于激子和电荷共振态的构型混合。比较了氦准分子和芘晶体二聚体的电位曲线。讨论了芳香准分子。考虑了原子准分子的相关光物理研究。饱和胺,其表现出蒸汽和溶液准分子荧光,提供原子和芳香准分子之间的联系。芳香分子与不同分子形成配合物、异构体或混合准分子,惰性气体原子与不同原子形成配合物或异构体。检讨于1975年完成。
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引用次数: 183
Holographic systems far from equilibrium: a review 远离平衡的全息系统:回顾
IF 18.1 1区 物理与天体物理 Q1 Physics and Astronomy Pub Date : 2018-10-04 DOI: 10.1088/1361-6633/ab4f91
Hong Liu, J. Sonner
In this paper we give an overview of some recent progress in using holography to study various far-from-equilibrium condensed matter systems. Non-equilibrium problems are notoriously difficult to deal with, not to mention at strong coupling and when including quantum effects. Remarkably, using holographic duality one can describe and follow the real-time evolution of far-from-equilibrium systems, including those which are spatially inhomogeneous and anisotropic, by solving partial differential gravity equations. We sample developments in two broad classes of question which have recently been of much interest to the condensed matter community: non-equilibrium steady states, and quantum systems undergoing a global quench. Our discussion focuses on the main physical insights obtained from the gravity approaches, rather than comprehensive treatment of each topic or detailed descriptions of gravity calculations. The paper also includes an overview of current numerical techniques, as well as the holographic Schwinger–Keldysh approach to real-time correlation functions.
本文综述了利用全息技术研究各种远平衡凝聚态体系的最新进展。众所周知,非平衡问题很难处理,更不用说强耦合和包括量子效应的情况了。值得注意的是,利用全息二象性,人们可以通过求解偏微分重力方程来描述和跟踪非平衡系统的实时演化,包括那些空间非均匀和各向异性的系统。我们以两大类问题的发展为例,这两大类问题最近引起了凝聚态界的极大兴趣:非平衡稳态和经历全局猝灭的量子系统。我们的讨论集中于从重力方法中获得的主要物理见解,而不是对每个主题的综合处理或重力计算的详细描述。本文还包括当前数值技术的概述,以及全息Schwinger-Keldysh方法实时相关函数。
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引用次数: 42
An introductory review of the resource theory approach to thermodynamics 热力学资源理论方法的介绍性回顾
IF 18.1 1区 物理与天体物理 Q1 Physics and Astronomy Pub Date : 2018-07-30 DOI: 10.1088/1361-6633/ab46e5
M. Lostaglio
I give a self-contained introduction to the resource theory approach to quantum thermodynamics. I will introduce in an elementary manner the technical machinery necessary to unpack and prove the core statements of the theory. The topics covered include the so-called ‘many second laws of thermodynamics’, thermo-majorisation and symmetry constraints on the evolution of quantum coherence. Among the elementary applications, I explicitly work out the bounds on deterministic work extraction and formation, discuss the complete solution of the theory for a single qubit and present the irreversibility of coherence transfers. The aim is to facilitate the task of those researchers interested in engaging and contributing to this topic, presenting scope and motivation of its core assumptions and discussing the relation between the resource theory and complementary approaches.
我对量子热力学的资源理论方法给出了一个完整的介绍。我将以一种基本的方式介绍必要的技术机制来解开和证明理论的核心陈述。涵盖的主题包括所谓的“热力学第二定律”,量子相干性演化中的热多数化和对称约束。在基本应用中,明确地给出了确定性功提取和形成的边界,讨论了单量子位理论的完全解,并给出了相干转移的不可逆性。其目的是促进那些有兴趣参与和贡献这一主题的研究人员的任务,提出其核心假设的范围和动机,并讨论资源理论和互补方法之间的关系。
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引用次数: 115
Multifractal analysis of financial markets: a review 金融市场的多重分形分析综述
IF 18.1 1区 物理与天体物理 Q1 Physics and Astronomy Pub Date : 2018-05-12 DOI: 10.1088/1361-6633/ab42fb
Zhi-Qiang Jiang, Wen-Jie Xie, Wei‐Xing Zhou, D. Sornette
Multifractality is ubiquitously observed in complex natural and socioeconomic systems. Multifractal analysis provides powerful tools to understand the complex nonlinear nature of time series in diverse fields. Inspired by its striking analogy with hydrodynamic turbulence, from which the idea of multifractality originated, multifractal analysis of financial markets has bloomed, forming one of the main directions of econophysics. We review the multifractal analysis methods and multifractal models adopted in or invented for financial time series and their subtle properties, which are applicable to time series in other disciplines. We survey the cumulating evidence for the presence of multifractality in financial time series in different markets and at different time periods and discuss the sources of multifractality. The usefulness of multifractal analysis in quantifying market inefficiency, in supporting risk management and in developing other applications is presented. We finally discuss open problems and further directions of multifractal analysis.
多重分形在复杂的自然和社会经济系统中无处不在。多重分形分析为理解时间序列在不同领域的复杂非线性性质提供了有力的工具。金融市场的多重分形分析与流体动力学湍流有着惊人的相似之处,多重分形的思想正是由此产生的。受此启发,金融市场的多重分形分析蓬勃发展,成为经济物理学的主要方向之一。本文综述了金融时间序列中采用或发明的多重分形分析方法和多重分形模型及其微妙性质,这些方法和模型适用于其他学科的时间序列。我们调查了在不同市场和不同时期的金融时间序列中多重分形存在的累积证据,并讨论了多重分形的来源。多重分形分析在量化市场无效率、支持风险管理和开发其他应用方面的有用性。最后讨论了多重分形分析有待解决的问题和进一步发展的方向。
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引用次数: 197
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