首页 > 最新文献

Resources Environment and Sustainability最新文献

英文 中文
Seasonal climate drives soil salinity dynamics through vegetation and water regulation 季节性气候通过植被和水分调节驱动土壤盐分动态
IF 7.8 Q1 ENVIRONMENTAL SCIENCES Pub Date : 2025-12-01 Epub Date: 2025-09-09 DOI: 10.1016/j.resenv.2025.100266
Danyang Wang , Jiaying Zheng , Yayi Tan , Zeqi Wei , Jingda Xin , Yihan Lu , Weijie Huang , Yunqi Wang , Huan Zhang , Changbo Zhong , Haiyan Zhao , Jianjun Pan , Zhaofu Li
Soil salinization threatens global agriculture and ecosystems, posing a critical challenge for sustainable development. Understanding how seasonal variations and environmental factors influence salinity dynamics is essential. However, current research relies heavily on single-time-point remote sensing, which offers limited temporal insights and fails to uncover the mechanisms driving seasonal changes. This study proposed the dynamic time warping-based model transfer-structural equation model (DBS) framework, which integrates dynamic time warping (DTW), base model transfer, and structural equation modeling (SEM), to explore the regulatory mechanisms of environmental factors on soil salinity dynamics. The framework includes building a stacking-electrical conductivity (EC) base model, aligning multi-month data with DTW, and analyzing environmental factors through SEM. Key predictors identified were normalized difference vegetation index (NDVI), normalized difference water index (NDWI), air temperature (AT), and precipitation. NDVI reduced salt accumulation by lowering evaporation and stabilizing soil moisture, while NDWI reflected precipitation-driven dilution and leaching. Temperature influenced salinity indirectly by regulating NDVI and NDWI. SEM confirmed NDVI and NDWI had direct effects on EC, while AT and precipitation acted indirectly. Model validation showed high accuracy and adaptability, with R-squared (R2), Nash–Sutcliffe efficiency coefficient (NSE), and Kling–Gupta Efficiency (KGE) values of 0.93, 0.94, and 0.89 for training and 0.86, 0.85, and 0.79 for validation, respectively. After DTW optimization, R2 improved by 0.12–0.22, NSE by 0.07–0.18, and KGE by 0.02–0.12, demonstrating significant performance gains. The framework demonstrated strong migration capability across different soil types and vegetation covers, achieving R2 of 0.73–0.96, The root mean squared error (RMSE) of 1–20, and residual prediction deviation (RPD) of 1.22–1.95. This study highlights the dominant role of climate-ecological interactions in salinity regulation and offers a robust, transferable method for multi-temporal salinity prediction. The findings provide critical insights for precision soil salinity management, sustainable agriculture, and climate resilience strategies, particularly in regions vulnerable to salinization.
土壤盐碱化威胁着全球农业和生态系统,对可持续发展构成重大挑战。了解季节变化和环境因素如何影响盐度动态是必要的。然而,目前的研究严重依赖于单时间点遥感,这提供了有限的时间见解,未能揭示驱动季节变化的机制。本研究提出了基于动态时间翘曲的模型转移-结构方程模型(DBS)框架,将动态时间翘曲(DTW)、基本模型转移和结构方程模型(SEM)相结合,探讨环境因子对土壤盐分动态的调控机制。该框架包括建立堆叠电导率(EC)基础模型,将多个月的数据与DTW对齐,并通过SEM分析环境因素。主要预测因子为归一化植被指数(NDVI)、归一化水指数(NDWI)、气温(AT)和降水量。NDVI通过降低蒸发和稳定土壤水分来减少盐的积累,而NDWI则反映降水驱动的稀释和淋滤。温度通过调节NDVI和NDWI间接影响盐度。SEM证实NDVI和NDWI对EC有直接影响,而AT和降水对EC有间接影响。模型验证具有较高的准确性和适应性,训练模型的R-squared (R2)、Nash-Sutcliffe效率系数(NSE)和Kling-Gupta效率(KGE)值分别为0.93、0.94和0.89,验证模型的R-squared、Nash-Sutcliffe效率系数(NSE)和KGE值分别为0.86、0.85和0.79。DTW优化后,R2提高0.12-0.22,NSE提高0.07-0.18,KGE提高0.02-0.12,性能提升显著。该框架在不同土壤类型和植被覆盖下具有较强的迁移能力,R2为0.73 ~ 0.96,均方根误差(RMSE)为1 ~ 20,残差预测偏差(RPD)为1.22 ~ 1.95。该研究强调了气候-生态相互作用在盐度调节中的主导作用,并为多时间盐度预测提供了一个可靠的、可转移的方法。这些发现为精确的土壤盐渍化管理、可持续农业和气候适应战略提供了重要见解,特别是在易受盐渍化影响的地区。
{"title":"Seasonal climate drives soil salinity dynamics through vegetation and water regulation","authors":"Danyang Wang ,&nbsp;Jiaying Zheng ,&nbsp;Yayi Tan ,&nbsp;Zeqi Wei ,&nbsp;Jingda Xin ,&nbsp;Yihan Lu ,&nbsp;Weijie Huang ,&nbsp;Yunqi Wang ,&nbsp;Huan Zhang ,&nbsp;Changbo Zhong ,&nbsp;Haiyan Zhao ,&nbsp;Jianjun Pan ,&nbsp;Zhaofu Li","doi":"10.1016/j.resenv.2025.100266","DOIUrl":"10.1016/j.resenv.2025.100266","url":null,"abstract":"<div><div>Soil salinization threatens global agriculture and ecosystems, posing a critical challenge for sustainable development. Understanding how seasonal variations and environmental factors influence salinity dynamics is essential. However, current research relies heavily on single-time-point remote sensing, which offers limited temporal insights and fails to uncover the mechanisms driving seasonal changes. This study proposed the dynamic time warping-based model transfer-structural equation model (DBS) framework, which integrates dynamic time warping (DTW), base model transfer, and structural equation modeling (SEM), to explore the regulatory mechanisms of environmental factors on soil salinity dynamics. The framework includes building a stacking-electrical conductivity (EC) base model, aligning multi-month data with DTW, and analyzing environmental factors through SEM. Key predictors identified were normalized difference vegetation index (NDVI), normalized difference water index (NDWI), air temperature (AT), and precipitation. NDVI reduced salt accumulation by lowering evaporation and stabilizing soil moisture, while NDWI reflected precipitation-driven dilution and leaching. Temperature influenced salinity indirectly by regulating NDVI and NDWI. SEM confirmed NDVI and NDWI had direct effects on EC, while AT and precipitation acted indirectly. Model validation showed high accuracy and adaptability, with R-squared (R<sup>2</sup>), Nash–Sutcliffe efficiency coefficient (NSE), and Kling–Gupta Efficiency (KGE) values of 0.93, 0.94, and 0.89 for training and 0.86, 0.85, and 0.79 for validation, respectively. After DTW optimization, R<sup>2</sup> improved by 0.12–0.22, NSE by 0.07–0.18, and KGE by 0.02–0.12, demonstrating significant performance gains. The framework demonstrated strong migration capability across different soil types and vegetation covers, achieving R<sup>2</sup> of 0.73–0.96, The root mean squared error (RMSE) of 1–20, and residual prediction deviation (RPD) of 1.22–1.95. This study highlights the dominant role of climate-ecological interactions in salinity regulation and offers a robust, transferable method for multi-temporal salinity prediction. The findings provide critical insights for precision soil salinity management, sustainable agriculture, and climate resilience strategies, particularly in regions vulnerable to salinization.</div></div>","PeriodicalId":34479,"journal":{"name":"Resources Environment and Sustainability","volume":"22 ","pages":"Article 100266"},"PeriodicalIF":7.8,"publicationDate":"2025-12-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145105303","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
A meta-analysis of feeding strategies for dairy cattle performance and greenhouse gas mitigation across the world 全球奶牛生产性能和温室气体减排的饲养策略荟萃分析
IF 7.8 Q1 ENVIRONMENTAL SCIENCES Pub Date : 2025-12-01 Epub Date: 2025-09-21 DOI: 10.1016/j.resenv.2025.100271
Aurele Gnetegha Ayemele , Josy Karel Ngueuyim Nono , Herbert Gnetegha Fotsidie , Mbezele Junior Yannick Ngaba , Mekonnen Tilahun , Lu Ma , Dengpan Bu , Jianchu Xu
Studies on the effects of cattle feeding strategies on greenhouse gas emissions are fragmented and cannot provide a global comparison of the feeding management practices that lead to optimal production while substantially reducing methane (CH4) and ammonia (NH3) emissions. The present study explains variability in enteric CH4, NH3 mitigations and cattle milk performance due to several diet composition and structure, feed management, breeding, animal experimental designs and CH4 measurement tools. Effects from 80 treatments were meta-analyzed from an initial 4394 screened papers and we retained 31 articles distributed across 15 countries on four continents. Minerals in feed additive types increased milk yield the most (90 ​%) and, concomitantly, reduced CH4 production by 33 ​%. Feed additive dosage ranging between 1 and 4 ​% also contributed to increasing milk yield by 47 ​% while reducing CH4 by 58 ​%. Meanwhile the impact of 3-nitrooxypropanol (3-NOP) feed additive on health safety is still controversial. Although a partial mixed ration system highly contributed to milk yield (102 ​%), it did not contribute to CH4 reduction as much as a total mixed ration system (39 ​%). The highest CH4 reduction levels were recorded with GreenFeed (80 ​%) and a rotating experimental design (37 ​%). The Holstein cattle breed was more productive with an increase of 46 ​% of milk production while reducing CH4 by 34 ​%. Grass forage increased NH3 by 5 ​% while crop forage reduced it by 21 ​%. Agriculture can effectively reduce its emissions and contribute to climate-neutral goals as part of a coordinated, global effort involving multiple sectors.
关于牛饲养策略对温室气体排放影响的研究是零散的,无法提供全球比较的饲养管理做法,这些做法可以在大幅减少甲烷(CH4)和氨(NH3)排放的同时实现最佳生产。本研究解释了饲粮组成和结构、饲料管理、育种、动物实验设计和CH4测量工具对肠道CH4、NH3缓解和奶牛产奶性能的影响。我们从最初筛选的4394篇论文中对80种治疗方法的效果进行了荟萃分析,并保留了分布在四大洲15个国家的31篇文章。饲料添加剂类型中的矿物质提高产奶量最多(90%),同时减少甲烷产量33%。饲料添加剂添加量在1 ~ 4%之间也有助于提高产奶量47%,减少甲烷58%。同时,3-硝基氧丙醇(3-NOP)饲料添加剂对健康安全的影响仍存在争议。虽然部分混合日粮系统对产奶量贡献很大(102%),但它对减少CH4的贡献不如完全混合日粮系统(39%)。采用GreenFeed(80%)和旋转实验设计(37%)记录的CH4减少水平最高。荷斯坦牛品种产量更高,产奶量增加46%,CH4减少34%。草料使NH3增加5%,而作物饲料使NH3减少21%。农业可以通过涉及多个部门的协调一致的全球努力,有效地减少排放,为实现气候中和目标作出贡献。
{"title":"A meta-analysis of feeding strategies for dairy cattle performance and greenhouse gas mitigation across the world","authors":"Aurele Gnetegha Ayemele ,&nbsp;Josy Karel Ngueuyim Nono ,&nbsp;Herbert Gnetegha Fotsidie ,&nbsp;Mbezele Junior Yannick Ngaba ,&nbsp;Mekonnen Tilahun ,&nbsp;Lu Ma ,&nbsp;Dengpan Bu ,&nbsp;Jianchu Xu","doi":"10.1016/j.resenv.2025.100271","DOIUrl":"10.1016/j.resenv.2025.100271","url":null,"abstract":"<div><div>Studies on the effects of cattle feeding strategies on greenhouse gas emissions are fragmented and cannot provide a global comparison of the feeding management practices that lead to optimal production while substantially reducing methane (CH<sub>4</sub>) and ammonia (NH<sub>3</sub>) emissions. The present study explains variability in enteric CH<sub>4</sub>, NH<sub>3</sub> mitigations and cattle milk performance due to several diet composition and structure, feed management, breeding, animal experimental designs and CH<sub>4</sub> measurement tools. Effects from 80 treatments were meta-analyzed from an initial 4394 screened papers and we retained 31 articles distributed across 15 countries on four continents. Minerals in feed additive types increased milk yield the most (90 ​%) and, concomitantly, reduced CH<sub>4</sub> production by 33 ​%. Feed additive dosage ranging between 1 and 4 ​% also contributed to increasing milk yield by 47 ​% while reducing CH<sub>4</sub> by 58 ​%. Meanwhile the impact of 3-nitrooxypropanol (3-NOP) feed additive on health safety is still controversial. Although a partial mixed ration system highly contributed to milk yield (102 ​%), it did not contribute to CH<sub>4</sub> reduction as much as a total mixed ration system (39 ​%). The highest CH<sub>4</sub> reduction levels were recorded with GreenFeed (80 ​%) and a rotating experimental design (37 ​%). The Holstein cattle breed was more productive with an increase of 46 ​% of milk production while reducing CH<sub>4</sub> by 34 ​%. Grass forage increased NH<sub>3</sub> by 5 ​% while crop forage reduced it by 21 ​%. Agriculture can effectively reduce its emissions and contribute to climate-neutral goals as part of a coordinated, global effort involving multiple sectors.</div></div>","PeriodicalId":34479,"journal":{"name":"Resources Environment and Sustainability","volume":"22 ","pages":"Article 100271"},"PeriodicalIF":7.8,"publicationDate":"2025-12-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145226849","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Nitrogen recovery from digestate via stripping–scrubbing using citric acid: Potential effects of recirculation and postdigestion on additional biogas recovery, and assessment of the fertilizer potential of end-products 利用柠檬酸通过剥脱洗涤从消化物中回收氮:再循环和消化后对额外沼气回收的潜在影响,以及最终产品肥料潜力的评估
IF 7.8 Q1 ENVIRONMENTAL SCIENCES Pub Date : 2025-12-01 Epub Date: 2025-08-06 DOI: 10.1016/j.resenv.2025.100258
Thaís Guedes Silveira , Rahim Molaey , Çağrı Akyol , Nick Sweygers , Nimisha Edayilam , Sofie Houtmeyers , Erik Meers , Lise Appels
This study investigated nitrogen (N) recovery from digestate via the N-stripping–scrubbing process and the effects of digestate recirculation and postdigestion on biogas yield during digestate posttreatment. Citric acid was tested as an alternative scrubbing agent to conventional sulfuric acid, forming ammonium citrate (AC) instead of ammonium sulfate (AS). In a cascade approach, the N release dynamics of the resulting by-products and end-products (scrubbing waters (AC, AS) and manure digestate-derived products) in amended soils were assessed via soil incubation tests to obtain a reliable estimation of the N value of these potential biobased fertilizers in comparison to that of commercial synthetic fertilizer (calcium ammonium nitrate (CAN)). The recirculation of the digestate resulted in a limited effect on additional biogas yield; however, up to a 47.2% increase in biogas yield was achieved during postdigestion at a stripping temperature of 70 °C, where 86% of the ammonia was removed from the digestate at pH 9.5. The use of citric acid as a scrubbing agent resulted in 80.6% ammonia recovery, which was slightly lower than when sulfuric acid was used (87.5%). Soil incubation tests showed N-net release values in the following order: AS (91%) > CAN (85%) > the liquid fraction (LF) of raw digestate (RD) (73%) > AC (70%) > RD (64%) > LF of N-stripped digestate (SD) (23%) > SD (12%). These results indicate the high N-fertilizing potential of AS, RD and its LF, and AC, highlighting the benefit of using citric acid as a novel and more sustainable scrubbing agent.
本研究探讨了溶氮-洗涤工艺对沼液中氮的回收,以及沼液后处理过程中沼液循环和消化后对沼气产量的影响。用柠檬酸代替常规硫酸,制备柠檬酸铵(AC)代替硫酸铵(as)。在级联方法中,通过土壤培养试验评估了改良土壤中产生的副产品和最终产物(洗涤水(AC, AS)和粪便消化产物衍生产品)的N释放动态,以获得这些潜在生物基肥料与商业合成肥料(硝酸铵钙(CAN))的N值的可靠估计。消化液的再循环对额外的沼气产量影响有限;然而,在溶出温度为70°C的消化后,沼气产量增加了47.2%,其中86%的氨在pH为9.5的消化池中被去除。使用柠檬酸作为洗涤剂,氨回收率为80.6%,略低于使用硫酸的87.5%。土壤培养试验结果显示,氮净释放值依次为:AS (91%) > CAN (85%) >;生消化液液体部分(LF) (RD) (73%) > AC (70%) > RD (64%) >;脱氮消化液LF (SD) (23%) >; SD(12%)。这些结果表明,AS、RD及其LF和AC具有较高的施氮潜力,突出了使用柠檬酸作为一种新型且更可持续的洗涤剂的好处。
{"title":"Nitrogen recovery from digestate via stripping–scrubbing using citric acid: Potential effects of recirculation and postdigestion on additional biogas recovery, and assessment of the fertilizer potential of end-products","authors":"Thaís Guedes Silveira ,&nbsp;Rahim Molaey ,&nbsp;Çağrı Akyol ,&nbsp;Nick Sweygers ,&nbsp;Nimisha Edayilam ,&nbsp;Sofie Houtmeyers ,&nbsp;Erik Meers ,&nbsp;Lise Appels","doi":"10.1016/j.resenv.2025.100258","DOIUrl":"10.1016/j.resenv.2025.100258","url":null,"abstract":"<div><div>This study investigated nitrogen (N) recovery from digestate via the N-stripping–scrubbing process and the effects of digestate recirculation and postdigestion on biogas yield during digestate posttreatment. Citric acid was tested as an alternative scrubbing agent to conventional sulfuric acid, forming ammonium citrate (AC) instead of ammonium sulfate (AS). In a cascade approach, the N release dynamics of the resulting by-products and end-products (scrubbing waters (AC, AS) and manure digestate-derived products) in amended soils were assessed via soil incubation tests to obtain a reliable estimation of the N value of these potential biobased fertilizers in comparison to that of commercial synthetic fertilizer (calcium ammonium nitrate (CAN)). The recirculation of the digestate resulted in a limited effect on additional biogas yield; however, up to a 47.2% increase in biogas yield was achieved during postdigestion at a stripping temperature of 70 °C, where 86% of the ammonia was removed from the digestate at pH 9.5. The use of citric acid as a scrubbing agent resulted in 80.6% ammonia recovery, which was slightly lower than when sulfuric acid was used (87.5%). Soil incubation tests showed N-net release values in the following order: AS (91%) &gt; CAN (85%) &gt; the liquid fraction (LF) of raw digestate (RD) (73%) &gt; AC (70%) &gt; RD (64%) &gt; LF of N-stripped digestate (SD) (23%) &gt; SD (12%). These results indicate the high N-fertilizing potential of AS, RD and its LF, and AC, highlighting the benefit of using citric acid as a novel and more sustainable scrubbing agent.</div></div>","PeriodicalId":34479,"journal":{"name":"Resources Environment and Sustainability","volume":"22 ","pages":"Article 100258"},"PeriodicalIF":7.8,"publicationDate":"2025-12-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144895435","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
A sustainable strategy for upcycling spent NCM into Li1.2Ni0.13Co0.13Mn0.54O2 cathode material for advanced lithium-ion batteries 废NCM升级为先进锂离子电池正极材料Li1.2Ni0.13Co0.13Mn0.54O2的可持续策略
IF 7.8 Q1 ENVIRONMENTAL SCIENCES Pub Date : 2025-12-01 Epub Date: 2025-08-06 DOI: 10.1016/j.resenv.2025.100257
Jing Sun, Wenxin Chen, Shuo Lu, Zhanlong Song, Wenlong Wang, Xiqiang Zhao, Yanpeng Mao
The recycling paradigm for spent lithium-ion batteries is undergoing fundamental transformation, as traditional recycling approaches that prioritize the extraction of valuable metals increasingly confront process complexity and marginal economic viability. Herein, we propose a sustainable upcycling strategy that directly converts spent LiNixCoyMn1xyO2 (SNCM) into high-performance lithium-rich manganese-based cathode material (i.e., Li1.2Ni0.13Co0.13Mn0.54O2, LNCM) through an innovative integrated approach. Crucially, microwave-assisted acetic acid leaching facilitates the effective and eco-friendly conversion of SNCM into soluble Ni/Co/Mn acetate, which can be then directly co-precipitated with oxalic acid to produce an oxalate precursor, simultaneously generating acetic acid that can be reused in the microwave-assisted leaching process, enabling a closed-loop for the leaching reagent. The pH of the leach solution emerges as a critical parameter, significantly influencing the co-precipitation process as well as the structural and morphological properties of the precursor. Through systematic optimization of precursor via pH adjustment and a two-stage calcination with a 5% excess of Li2CO3, the regenerated LNCM-7.5 (pH = 7.5) exhibits a well-ordered layered structure (c/a = 5.0016) with minimal cation mixing (I003/I104 = 1.46), uniform particle morphology, enhanced Li+ diffusion and thereby exceptional cycling stability-delivering 165.7 mAh g1 at 1 C after 100 cycles with 89.01% capacity retention, performance parity with virgin materials synthesized from commercial acetates. This work not only demonstrates the feasibility of upcycling SNCM into high-performance LNCM cathodes, but also establishes a sustainable and economically viable solution for advancing circular economy practices in the energy storage industry, mitigating resource scarcity and pollution.
废旧锂离子电池的回收模式正在发生根本性的转变,因为传统的回收方法优先考虑提取有价值的金属,越来越多地面临工艺复杂性和边际经济可行性的问题。在此,我们提出了一种可持续的升级回收策略,通过创新的集成方法直接将废LiNixCoyMn1−x−yO2 (SNCM)转化为高性能富锂锰基正极材料(即Li1.2Ni0.13Co0.13Mn0.54O2, LNCM)。重要的是,微波辅助乙酸浸出有助于SNCM有效且环保地转化为可溶的Ni/Co/Mn醋酸盐,然后可以直接与草酸共沉淀生成草酸前体,同时生成可在微波辅助浸出过程中重复使用的乙酸,从而实现浸出试剂的闭环。浸出液的pH值是一个关键参数,它对共沉淀过程以及前驱体的结构和形态特性有重要影响。通过调整pH值对前驱体进行系统优化,并在过量5% Li2CO3的条件下进行两段煅烧,再生的LNCM-7.5 (pH = 7.5)呈现出有序的层状结构(c/a = 5.0016),阳离子混合最少(I003/I104 = 1.46),颗粒形态均匀,Li+扩散增强,因此具有优异的循环稳定性——在1℃下循环100次后,容量保持率为89.01%,可输送165.7 mAh g - 1。性能与商业醋酸酯合成的原始材料相当。这项工作不仅证明了将SNCM升级为高性能LNCM阴极的可行性,而且还为推进储能行业的循环经济实践,缓解资源短缺和污染建立了可持续和经济可行的解决方案。
{"title":"A sustainable strategy for upcycling spent NCM into Li1.2Ni0.13Co0.13Mn0.54O2 cathode material for advanced lithium-ion batteries","authors":"Jing Sun,&nbsp;Wenxin Chen,&nbsp;Shuo Lu,&nbsp;Zhanlong Song,&nbsp;Wenlong Wang,&nbsp;Xiqiang Zhao,&nbsp;Yanpeng Mao","doi":"10.1016/j.resenv.2025.100257","DOIUrl":"10.1016/j.resenv.2025.100257","url":null,"abstract":"<div><div>The recycling paradigm for spent lithium-ion batteries is undergoing fundamental transformation, as traditional recycling approaches that prioritize the extraction of valuable metals increasingly confront process complexity and marginal economic viability. Herein, we propose a sustainable upcycling strategy that directly converts spent LiNi<span><math><msub><mrow></mrow><mrow><mi>x</mi></mrow></msub></math></span>Co<span><math><msub><mrow></mrow><mrow><mi>y</mi></mrow></msub></math></span>Mn<span><math><msub><mrow></mrow><mrow><mn>1</mn><mo>−</mo><mi>x</mi><mo>−</mo><mi>y</mi></mrow></msub></math></span>O<sub>2</sub> (SNCM) into high-performance lithium-rich manganese-based cathode material (i.e., Li<span><math><msub><mrow></mrow><mrow><mn>1</mn><mo>.</mo><mn>2</mn></mrow></msub></math></span>Ni<span><math><msub><mrow></mrow><mrow><mn>0</mn><mo>.</mo><mn>13</mn></mrow></msub></math></span>Co<span><math><msub><mrow></mrow><mrow><mn>0</mn><mo>.</mo><mn>13</mn></mrow></msub></math></span>Mn<span><math><msub><mrow></mrow><mrow><mn>0</mn><mo>.</mo><mn>54</mn></mrow></msub></math></span>O<sub>2</sub>, LNCM) through an innovative integrated approach. Crucially, microwave-assisted acetic acid leaching facilitates the effective and eco-friendly conversion of SNCM into soluble Ni/Co/Mn acetate, which can be then directly co-precipitated with oxalic acid to produce an oxalate precursor, simultaneously generating acetic acid that can be reused in the microwave-assisted leaching process, enabling a closed-loop for the leaching reagent. The pH of the leach solution emerges as a critical parameter, significantly influencing the co-precipitation process as well as the structural and morphological properties of the precursor. Through systematic optimization of precursor via pH adjustment and a two-stage calcination with a 5% excess of Li<sub>2</sub>CO<sub>3</sub>, the regenerated LNCM-7.5 (pH <span><math><mo>=</mo></math></span> 7.5) exhibits a well-ordered layered structure (<em>c</em>/<em>a</em> <span><math><mo>=</mo></math></span> 5.0016) with minimal cation mixing (I<sub>003</sub>/I<sub>104</sub>\u0000 <span><math><mo>=</mo></math></span> 1.46), uniform particle morphology, enhanced Li<span><math><msup><mrow></mrow><mrow><mo>+</mo></mrow></msup></math></span> diffusion and thereby exceptional cycling stability-delivering 165.7 mAh g<span><math><msup><mrow></mrow><mrow><mo>−</mo><mn>1</mn></mrow></msup></math></span> at 1 C after 100 cycles with 89.01% capacity retention, performance parity with virgin materials synthesized from commercial acetates. This work not only demonstrates the feasibility of upcycling SNCM into high-performance LNCM cathodes, but also establishes a sustainable and economically viable solution for advancing circular economy practices in the energy storage industry, mitigating resource scarcity and pollution.</div></div>","PeriodicalId":34479,"journal":{"name":"Resources Environment and Sustainability","volume":"22 ","pages":"Article 100257"},"PeriodicalIF":7.8,"publicationDate":"2025-12-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144885520","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Calcium-rich bone biochar boosts fat, oil, and grease (FOG) biodegradability: Methane maximization and microbial community pattern 富钙骨生物炭提高脂肪、油和油脂(FOG)的可生物降解性:甲烷最大化和微生物群落模式
IF 7.8 Q1 ENVIRONMENTAL SCIENCES Pub Date : 2025-12-01 Epub Date: 2025-09-26 DOI: 10.1016/j.resenv.2025.100274
Ting Li , Shah Faisal , Jialing Tang , Mahdy Elsayed , Nousheen Iqbal , Ye Pu , Joachim Henjes , Stephan Ende , Abdelfatah Abomohra
The present study evaluated calcium-rich bone biochar, derived from pig and chicken bones, for enhanced anaerobic digestion of FOG (fat, oil, grease). The study aimed to maximise energy recovery by reducing the negative impact of long-chain fatty acids (LCFAs) and to evaluate the subsequent effect on the microbial community structure. A series of 2.0 ​% FOG batch trials was prepared, adding pig bone biochar (PB) and chicken bone biochar (CB) based on their calcium (Ca) content to maintain (0.1, 0.5, and 1.0 ​% Ca concentrations). Parallelly, Ca was used at the same concentrations without biochar. Supplementation of 0.5 ​% PB, CB, and Ca individually enhanced LCFAs degradation up to 81.6 ​%, 81.0 ​%, and 84.8 ​%, respectively. Therefore, the accumulative methane yield increased by 4-, 3.9-, and 5.2-fold over the control FOG2.0 ​%. Reduction in methane production was observed at 1.0 ​% PB, CB, and Ca compared with 0.5 ​% but, interestingly, 1.0 ​% PB and CB showed higher accumulative methane yield of 135.6 ​mL ​g−1 VS and 125.3 ​mL ​g−1 VS, respectively, in comparison to Ca (60.7 ​mL ​g−1 VS). There was enhancement in Firmicutes and Campylobacteriotes, accompanied by a simultaneous rise in Methanosarcina at 0.5 ​% PB (from 23.7 ​% to 78.1 ​%) and Methanoculleus at 0.5 ​% Ca (from 41.3 ​% to 50.0 ​%). Ca-rich PB and CB biochar significantly enhanced FOG anaerobic digestion through synergistic mechanisms, including reducing inhibition, stimulating microbes, facilitating electron transfer, and improving nutrient supply. Using animal bone residues for FOG anaerobic digestion provides both a sustainable waste management route and an efficient calcium-rich material to boost energy recovery.
本研究评估了从猪和鸡骨头中提取的富钙骨生物炭,以增强对FOG(脂肪、油、油脂)的厌氧消化。该研究旨在通过减少长链脂肪酸(LCFAs)的负面影响来最大化能量回收,并评估其对微生物群落结构的后续影响。制备了一系列2.0% FOG批量试验,根据猪骨生物炭(PB)和鸡骨生物炭(CB)的钙含量分别添加,以维持(0.1、0.5和1.0%的钙浓度)。同时,在不使用生物炭的情况下,在相同浓度下使用Ca。添加0.5%的PB、CB和Ca分别提高了LCFAs的降解率,分别达到81.6%、81.0%和84.8%。因此,累积甲烷产量比对照FOG2.0 %分别提高了4倍、3.9倍和5.2倍。1.0%的PB、CB和Ca与0.5%相比,甲烷产量减少,但有趣的是,1.0%的PB和CB的累积甲烷产量分别为135.6 mL g−1 VS和125.3 mL g−1 VS,高于Ca (60.7 mL g−1 VS)。厚壁菌门(Firmicutes)和弯曲菌门(campylobacteria)的数量增加,同时在0.5% PB条件下Methanosarcina(从23.7%增加到78.1%)和0.5% Ca条件下Methanoculleus(从41.3%增加到50.0%)的数量也增加。富钙PB和CB生物炭通过减少抑制、刺激微生物、促进电子转移和改善养分供应等协同机制显著促进FOG厌氧消化。使用动物骨骼残留物进行FOG厌氧消化既提供了可持续的废物管理途径,又提供了有效的富钙材料,以促进能量回收。
{"title":"Calcium-rich bone biochar boosts fat, oil, and grease (FOG) biodegradability: Methane maximization and microbial community pattern","authors":"Ting Li ,&nbsp;Shah Faisal ,&nbsp;Jialing Tang ,&nbsp;Mahdy Elsayed ,&nbsp;Nousheen Iqbal ,&nbsp;Ye Pu ,&nbsp;Joachim Henjes ,&nbsp;Stephan Ende ,&nbsp;Abdelfatah Abomohra","doi":"10.1016/j.resenv.2025.100274","DOIUrl":"10.1016/j.resenv.2025.100274","url":null,"abstract":"<div><div>The present study evaluated calcium-rich bone biochar, derived from pig and chicken bones, for enhanced anaerobic digestion of FOG (fat, oil, grease). The study aimed to maximise energy recovery by reducing the negative impact of long-chain fatty acids (LCFAs) and to evaluate the subsequent effect on the microbial community structure. A series of 2.0 ​% FOG batch trials was prepared, adding pig bone biochar (PB) and chicken bone biochar (CB) based on their calcium (Ca) content to maintain (0.1, 0.5, and 1.0 ​% Ca concentrations). Parallelly, Ca was used at the same concentrations without biochar. Supplementation of 0.5 ​% PB, CB, and Ca individually enhanced LCFAs degradation up to 81.6 ​%, 81.0 ​%, and 84.8 ​%, respectively. Therefore, the accumulative methane yield increased by 4-, 3.9-, and 5.2-fold over the control FOG2.0 ​%. Reduction in methane production was observed at 1.0 ​% PB, CB, and Ca compared with 0.5 ​% but, interestingly, 1.0 ​% PB and CB showed higher accumulative methane yield of 135.6 ​mL ​g<sup>−1</sup> VS and 125.3 ​mL ​g<sup>−1</sup> VS, respectively, in comparison to Ca (60.7 ​mL ​g<sup>−1</sup> VS). There was enhancement in <em>Firmicutes</em> and <em>Campylobacteriotes</em>, accompanied by a simultaneous rise in <em>Methanosarcina</em> at 0.5 ​% PB (from 23.7 ​% to 78.1 ​%) and <em>Methanoculleus</em> at 0.5 ​% Ca (from 41.3 ​% to 50.0 ​%). Ca-rich PB and CB biochar significantly enhanced FOG anaerobic digestion through synergistic mechanisms, including reducing inhibition, stimulating microbes, facilitating electron transfer, and improving nutrient supply. Using animal bone residues for FOG anaerobic digestion provides both a sustainable waste management route and an efficient calcium-rich material to boost energy recovery.</div></div>","PeriodicalId":34479,"journal":{"name":"Resources Environment and Sustainability","volume":"22 ","pages":"Article 100274"},"PeriodicalIF":7.8,"publicationDate":"2025-12-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145266218","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Bio-based flame retardants derived from forest industry — An approach towards circular economy 来自森林工业的生物基阻燃剂——走向循环经济的途径
IF 12.4 Q1 ENVIRONMENTAL SCIENCES Pub Date : 2025-09-01 Epub Date: 2025-04-21 DOI: 10.1016/j.resenv.2025.100229
Sritama Mukherjee , Khan Mohammad Ahsan Uddin , Irina Turku , Anti Rohumaa , Juha Lipponen
Several environmental studies on conventional flame retardants (FR) have shown them as presistent chemicals that may end up being environmental and health hazards. The advancement of eco-friendly FRs is accelerating due to the needs of improved safety and environmental sustainability. Developing bio-based FR composite materials is crucial due to their regenerable resources, low toxicity, controllable biodegradability, and versatility in application. This review examines recent advancements in utilizing forest industry products, including cellulose and nanocellulose, along with byproducts like lignin and hemicellulose. It also addresses valorized organic waste streams of pulp industries, such as tannins and biopolyols, in the creation of materials that exhibit flame retardancy in polymers and textiles. The review demonstrates functionalization methodologies, qualitative and quantitative characterization carried out on their flame retardant properties following an overview of the FR mechanisms. Finally, the opportunities and challenges for the future development of bio-based FRs are briefly identified, emphasizing on the need of utilizing waste materials as chemical precursors that can alleviate prevailing ecological concerns and open a new set of possibilities in material development in a circular economy.
几项关于传统阻燃剂(FR)的环境研究表明,它们是持久性化学品,最终可能对环境和健康造成危害。由于提高安全性和环境可持续性的需要,生态友好型反应堆的发展正在加速。生物基FR复合材料具有资源可再生、毒性低、可生物降解性可控、应用广泛等特点,因此开发生物基FR复合材料至关重要。本文综述了利用森林工业产品的最新进展,包括纤维素和纳米纤维素,以及木质素和半纤维素等副产品。它还解决了纸浆工业的有机废物流,如单宁和生物多元醇,在聚合物和纺织品中表现出阻燃性的材料的创造。概述了阻燃机理后,综述了功能化方法,对阻燃性能进行了定性和定量表征。最后,简要地确定了生物基燃料燃料未来发展的机遇和挑战,强调需要利用废物作为化学前体,这可以缓解普遍的生态问题,并在循环经济中开辟材料开发的一系列新的可能性。
{"title":"Bio-based flame retardants derived from forest industry — An approach towards circular economy","authors":"Sritama Mukherjee ,&nbsp;Khan Mohammad Ahsan Uddin ,&nbsp;Irina Turku ,&nbsp;Anti Rohumaa ,&nbsp;Juha Lipponen","doi":"10.1016/j.resenv.2025.100229","DOIUrl":"10.1016/j.resenv.2025.100229","url":null,"abstract":"<div><div>Several environmental studies on conventional flame retardants (FR) have shown them as presistent chemicals that may end up being environmental and health hazards. The advancement of eco-friendly FRs is accelerating due to the needs of improved safety and environmental sustainability. Developing bio-based FR composite materials is crucial due to their regenerable resources, low toxicity, controllable biodegradability, and versatility in application. This review examines recent advancements in utilizing forest industry products, including cellulose and nanocellulose, along with byproducts like lignin and hemicellulose. It also addresses valorized organic waste streams of pulp industries, such as tannins and biopolyols, in the creation of materials that exhibit flame retardancy in polymers and textiles. The review demonstrates functionalization methodologies, qualitative and quantitative characterization carried out on their flame retardant properties following an overview of the FR mechanisms. Finally, the opportunities and challenges for the future development of bio-based FRs are briefly identified, emphasizing on the need of utilizing waste materials as chemical precursors that can alleviate prevailing ecological concerns and open a new set of possibilities in material development in a circular economy.</div></div>","PeriodicalId":34479,"journal":{"name":"Resources Environment and Sustainability","volume":"21 ","pages":"Article 100229"},"PeriodicalIF":12.4,"publicationDate":"2025-09-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143921720","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
How does the long-term return of mix-sowing green manures increase nitrogen utilization and decrease ecological costs of wheatland under reduced chemical nitrogen input? 在化学氮投入减少的情况下,混播绿肥的长期回报是如何提高小麦地氮素利用率和降低生态成本的?
IF 12.4 Q1 ENVIRONMENTAL SCIENCES Pub Date : 2025-09-01 Epub Date: 2025-03-30 DOI: 10.1016/j.resenv.2025.100220
Jingui Wei, Wen Yin, Qiang Chai, Zhilong Fan, Falong Hu, Lianhao Zhao
Increasing nitrogen (N) utilization and reducing ecological costs of farmland are key objectives for mitigating environmental pollution and advancing sustainable agricultural development. Green manure is widely used to increase crop N efficiency while replacing partial chemical N input. However, it remains uncertain whether reducing chemical N supply, combined with mix-sowing green manures, could increase N utilization and reduce ecological costs of wheatland, revealing its mechanisms of soil N regulation and bacteria diversity. A 6-year field experiment was conducted in an arid irrigation area of northwestern China, implementing wheat multi-cropping different green manures and mix-sowing green manures (F, fallow; CV, common vetch; R, rapeseed; HCV, hairy vetch and common vetch) under reduced chemical N (N3, conventional N application rate; N2, reduced N by 20%; N1, reduced N by 40%). Our results showed that reducing chemical N decreased wheat yield and N efficiency, while green manure return increased wheat yield and N efficiency. Under N2, HCV had a higher wheat yield and N efficiency than CV, R, and F. Wheat N uptake and active N loss were decreased with chemical N reduction but enhanced with green manure return. HCVN2 improved wheat N uptake by 8.3% while reducing ammonia volatilization, nitrous oxide emissions, and nitrate leaching by 12.5%, 17.2%, and 22.1%, respectively, compared to FN3. The mechanisms of HCVN2 enhanced N utilization and reduced ecological costs of wheatland, mainly including increased N contents in the 0–40 cm soil layer, improved soil enzyme activities of N metabolism, and enriched soil bacterial diversity. Therefore, mix-sowing green manures return enhanced N utilization and decreased ecological costs of wheatland under a 20% reduction in chemical N input.
提高农田氮素利用率,降低农田生态成本,是缓解环境污染、促进农业可持续发展的关键目标。绿肥被广泛用于提高作物氮效率,同时替代部分化学氮输入。然而,减少化学施氮与混播绿肥是否能提高小麦地氮素利用率,降低生态成本,揭示其对土壤氮素调控和细菌多样性的机制尚不明确。在西北干旱灌区进行了为期6年的大田试验,采用小麦复种不同绿肥和混播绿肥(F、休耕;CV,普通紫薇;R,油菜籽;还原性化学N (N3,常规施氮量)条件下HCV、毛叶黄鼠和普通叶黄鼠;N2,使N降低20%;N1, N降低40%)。结果表明,化学施氮降低了小麦产量和氮素效率,而绿肥还田提高了小麦产量和氮素效率。氮肥处理下,HCV比CV、R和f具有更高的小麦产量和氮素效率,化学降氮降低了小麦氮素吸收和活性氮素损失,绿肥还田提高了氮素吸收和活性氮素损失。与FN3相比,HCVN2使小麦氮素吸收提高了8.3%,同时使氨挥发、一氧化二氮排放和硝酸盐淋溶分别降低了12.5%、17.2%和22.1%。HCVN2提高小麦地氮素利用和降低生态成本的机制主要包括提高0 ~ 40 cm土层氮素含量、提高土壤氮素代谢酶活性和丰富土壤细菌多样性。因此,在化学施氮量减少20%的情况下,混播绿肥能提高小麦地氮素利用率,降低生态成本。
{"title":"How does the long-term return of mix-sowing green manures increase nitrogen utilization and decrease ecological costs of wheatland under reduced chemical nitrogen input?","authors":"Jingui Wei,&nbsp;Wen Yin,&nbsp;Qiang Chai,&nbsp;Zhilong Fan,&nbsp;Falong Hu,&nbsp;Lianhao Zhao","doi":"10.1016/j.resenv.2025.100220","DOIUrl":"10.1016/j.resenv.2025.100220","url":null,"abstract":"<div><div>Increasing nitrogen (N) utilization and reducing ecological costs of farmland are key objectives for mitigating environmental pollution and advancing sustainable agricultural development. Green manure is widely used to increase crop N efficiency while replacing partial chemical N input. However, it remains uncertain whether reducing chemical N supply, combined with mix-sowing green manures, could increase N utilization and reduce ecological costs of wheatland, revealing its mechanisms of soil N regulation and bacteria diversity. A 6-year field experiment was conducted in an arid irrigation area of northwestern China, implementing wheat multi-cropping different green manures and mix-sowing green manures (F, fallow; CV, common vetch; R, rapeseed; HCV, hairy vetch and common vetch) under reduced chemical N (N3, conventional N application rate; N2, reduced N by 20%; N1, reduced N by 40%). Our results showed that reducing chemical N decreased wheat yield and N efficiency, while green manure return increased wheat yield and N efficiency. Under N2, HCV had a higher wheat yield and N efficiency than CV, R, and F. Wheat N uptake and active N loss were decreased with chemical N reduction but enhanced with green manure return. HCVN2 improved wheat N uptake by 8.3% while reducing ammonia volatilization, nitrous oxide emissions, and nitrate leaching by 12.5%, 17.2%, and 22.1%, respectively, compared to FN3. The mechanisms of HCVN2 enhanced N utilization and reduced ecological costs of wheatland, mainly including increased N contents in the 0–40 cm soil layer, improved soil enzyme activities of N metabolism, and enriched soil bacterial diversity. Therefore, mix-sowing green manures return enhanced N utilization and decreased ecological costs of wheatland under a 20% reduction in chemical N input.</div></div>","PeriodicalId":34479,"journal":{"name":"Resources Environment and Sustainability","volume":"21 ","pages":"Article 100220"},"PeriodicalIF":12.4,"publicationDate":"2025-09-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143790923","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Trajectory, drivers, and reduction of greenhouse gas emissions from urban water system in China during 1980–2030 1980-2030年中国城市水系温室气体排放轨迹、驱动因素及减排
IF 12.4 Q1 ENVIRONMENTAL SCIENCES Pub Date : 2025-09-01 Epub Date: 2025-06-25 DOI: 10.1016/j.resenv.2025.100244
Shiyu Pei, Zonghan Li, Yi Liu, Chunyan Wang, Hao Wu, Shuming Liu, Yujun Huang
Urban water systems (UWSs) continuously evolve in response to changes in urban populations, technological advancements, and lifestyle shifts, resulting in significant changes in greenhouse gas (GHG) emissions. Understanding how GHG emissions vary across the different developmental stages of a UWS is crucial for charting pathways toward carbon neutrality under varying levels of urbanization and infrastructure maturity. To explore the long-term patterns of GHG emissions from the UWS, we developed a systematic accounting framework encompassing four energy-related subsystems: water extraction, water supply, residential water use, and wastewater treatment. We applied this framework to China’s UWS across its transitional trajectory—from early development to system-wide maturity (1980–2020) at the provincial level. Results show that over the 40 years, GHG emissions from China’s UWS increased approximately 14-fold, surpassing the overall rate of population growth by 143.9%. From the early 1990s till now, residential water use emerged as the dominant source of UWS-related emissions, accounting for approximately 77.6% of total emissions. Our scenario analysis estimates a potential 34.0% reduction in China’s carbon emissions (128.3 Mt CO2-eq) by 2030 through water-saving strategies. This study offers critical insights into promoting low-carbon operations and sustainable management of UWS, and serves as an important reference for global efforts net-zero water infrastructure.
城市水系统(UWSs)随着城市人口、技术进步和生活方式的变化而不断发展,导致温室气体(GHG)排放发生重大变化。了解温室气体排放在UWS不同发展阶段的变化,对于绘制不同城市化水平和基础设施成熟度下的碳中和路径至关重要。为了探索UWS温室气体排放的长期模式,我们开发了一个系统的核算框架,包括四个与能源相关的子系统:取水、供水、住宅用水和废水处理。我们将这一框架应用于中国大学在省级层面的过渡轨迹——从早期发展到全系统成熟(1980-2020)。结果表明,在过去的40年中,中国UWS的温室气体排放量增长了约14倍,超过整体人口增长率143.9%。从20世纪90年代初至今,居民用水成为uws相关排放的主要来源,约占总排放量的77.6%。我们的情景分析估计,通过节水战略,到2030年中国的碳排放量可能减少34.0%(1.283亿吨二氧化碳当量)。本研究为促进水系统的低碳运营和可持续管理提供了重要见解,并为全球实现水基础设施净零提供了重要参考。
{"title":"Trajectory, drivers, and reduction of greenhouse gas emissions from urban water system in China during 1980–2030","authors":"Shiyu Pei,&nbsp;Zonghan Li,&nbsp;Yi Liu,&nbsp;Chunyan Wang,&nbsp;Hao Wu,&nbsp;Shuming Liu,&nbsp;Yujun Huang","doi":"10.1016/j.resenv.2025.100244","DOIUrl":"10.1016/j.resenv.2025.100244","url":null,"abstract":"<div><div>Urban water systems (UWSs) continuously evolve in response to changes in urban populations, technological advancements, and lifestyle shifts, resulting in significant changes in greenhouse gas (GHG) emissions. Understanding how GHG emissions vary across the different developmental stages of a UWS is crucial for charting pathways toward carbon neutrality under varying levels of urbanization and infrastructure maturity. To explore the long-term patterns of GHG emissions from the UWS, we developed a systematic accounting framework encompassing four energy-related subsystems: water extraction, water supply, residential water use, and wastewater treatment. We applied this framework to China’s UWS across its transitional trajectory—from early development to system-wide maturity (1980–2020) at the provincial level. Results show that over the 40 years, GHG emissions from China’s UWS increased approximately 14-fold, surpassing the overall rate of population growth by 143.9%. From the early 1990s till now, residential water use emerged as the dominant source of UWS-related emissions, accounting for approximately 77.6% of total emissions. Our scenario analysis estimates a potential 34.0% reduction in China’s carbon emissions (128.3 Mt CO<sub>2</sub>-eq) by 2030 through water-saving strategies. This study offers critical insights into promoting low-carbon operations and sustainable management of UWS, and serves as an important reference for global efforts net-zero water infrastructure.</div></div>","PeriodicalId":34479,"journal":{"name":"Resources Environment and Sustainability","volume":"21 ","pages":"Article 100244"},"PeriodicalIF":12.4,"publicationDate":"2025-09-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144596932","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Spatio-temporal evolution of sloping farmland and identification of its erosion risk management and control zones in the Three Gorges Reservoir Area, China 三峡库区坡耕地时空演变及侵蚀风险管控区划
IF 7.8 Q1 ENVIRONMENTAL SCIENCES Pub Date : 2025-09-01 Epub Date: 2025-08-06 DOI: 10.1016/j.resenv.2025.100255
Lidong Pan, Yun Chen, Dongmei Shi, Jiayong Gao, Yufu Jiang, Fangyuan Liu
Sloping farmland in the Three Gorges Reservoir Area (TGRA) is crucial for national food and ecological security. In this study, methods such as terrain gradient classification, kernel density estimation, and erosion risk identification model were used to analyze the spatio-temporal evolution and influencing factors of sloping farmland in the TGRA during 1990–2020, and its erosion risk control areas were identified. The sloping farmland in the TGRA exhibited spatial distribution characteristics of more in the central and western regions, less in the eastern region, with a high degree of fragmentation. It was concentrated in areas with slopes of 8–25° and altitudes of 200–1000 m, accounting for approximately 63% and 80% of sloping farmland, respectively. In the last 30 years, the distribution of sloping farmland with slopes >15° and altitudes >1000 m has gradually decreased and shifted to areas of 8–15° and 400–800 m, respectively. The sloping farmland has decreased by 343.93 km2, mainly converted into forest land, grassland, paddy field, and construction land. Slope and altitude were the main natural factors affecting the spatio-temporal evolution of sloping farmland, while the urbanization rate and disposable income of rural residents were the key human influence factors. Sloping farmland above the high-risk level of erosion was mainly distributed in counties such as Wuxi, Kaizhou, Wushan, Fengjie, Yunyang, and Wanzhou, concentrated in the terrain gradient area with slopes of 10–35° and altitudes of 200–1000 m, with the most distribution at 15–25° and 200–400 m. For these high erosion risk areas, prioritized regulation should be carried out for sloping farmland. These findings can optimize the use of sloping farmland resources, strengthening the prevention and control of erosion risks, and promoting the sustainable agricultural development.
三峡库区坡耕地是关系到国家粮食安全与生态安全的重要区域。采用地形梯度分类、核密度估算、侵蚀风险识别模型等方法,对1990-2020年青藏高原坡耕地时空演变特征及影响因素进行了分析,并对其侵蚀风险控制区进行了划分。TGRA坡耕地呈现中西部多、东部少、破碎化程度高的空间分布特征。主要分布在坡度为8 ~ 25°、海拔为200 ~ 1000 m的地区,分别约占坡耕地面积的63%和80%。近30年来,坡度为15°和海拔为1000 m的坡耕地分布逐渐减少,分别向8-15°和400-800 m地区转移。坡耕地减少343.93 km2,主要转化为林地、草地、水田和建设用地。坡度和海拔是影响坡耕地时空演变的主要自然因素,城市化率和农村居民可支配收入是影响坡耕地时空演变的主要人为因素。侵蚀高风险等级以上坡耕地主要分布在无锡、开州、巫山、奉节、云阳、万州等县,集中在坡度10 ~ 35°、海拔200 ~ 1000 m的地形梯度区,15 ~ 25°、200 ~ 400 m分布最多。对于这些高侵蚀风险地区,应优先对坡耕地进行治理。研究结果对优化坡耕地资源利用,加强水土流失风险防控,促进农业可持续发展具有重要意义。
{"title":"Spatio-temporal evolution of sloping farmland and identification of its erosion risk management and control zones in the Three Gorges Reservoir Area, China","authors":"Lidong Pan,&nbsp;Yun Chen,&nbsp;Dongmei Shi,&nbsp;Jiayong Gao,&nbsp;Yufu Jiang,&nbsp;Fangyuan Liu","doi":"10.1016/j.resenv.2025.100255","DOIUrl":"10.1016/j.resenv.2025.100255","url":null,"abstract":"<div><div>Sloping farmland in the Three Gorges Reservoir Area (TGRA) is crucial for national food and ecological security. In this study, methods such as terrain gradient classification, kernel density estimation, and erosion risk identification model were used to analyze the spatio-temporal evolution and influencing factors of sloping farmland in the TGRA during 1990–2020, and its erosion risk control areas were identified. The sloping farmland in the TGRA exhibited spatial distribution characteristics of more in the central and western regions, less in the eastern region, with a high degree of fragmentation. It was concentrated in areas with slopes of 8–25° and altitudes of 200–1000 m, accounting for approximately 63% and 80% of sloping farmland, respectively. In the last 30 years, the distribution of sloping farmland with slopes <span><math><mo>&gt;</mo></math></span>15° and altitudes <span><math><mo>&gt;</mo></math></span>1000 m has gradually decreased and shifted to areas of 8–15° and 400–800 m, respectively. The sloping farmland has decreased by 343.93 km<sup>2</sup>, mainly converted into forest land, grassland, paddy field, and construction land. Slope and altitude were the main natural factors affecting the spatio-temporal evolution of sloping farmland, while the urbanization rate and disposable income of rural residents were the key human influence factors. Sloping farmland above the high-risk level of erosion was mainly distributed in counties such as Wuxi, Kaizhou, Wushan, Fengjie, Yunyang, and Wanzhou, concentrated in the terrain gradient area with slopes of 10–35° and altitudes of 200–1000 m, with the most distribution at 15–25° and 200–400 m. For these high erosion risk areas, prioritized regulation should be carried out for sloping farmland. These findings can optimize the use of sloping farmland resources, strengthening the prevention and control of erosion risks, and promoting the sustainable agricultural development.</div></div>","PeriodicalId":34479,"journal":{"name":"Resources Environment and Sustainability","volume":"21 ","pages":"Article 100255"},"PeriodicalIF":7.8,"publicationDate":"2025-09-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144842606","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Livestock rearing as a key component of mitigation efforts for non-CO2 greenhouse gas emissions in global crop-livestock system 牲畜饲养是减缓全球作物-牲畜系统非二氧化碳温室气体排放努力的关键组成部分
IF 12.4 Q1 ENVIRONMENTAL SCIENCES Pub Date : 2025-09-01 Epub Date: 2025-07-10 DOI: 10.1016/j.resenv.2025.100248
Li Zheng , Qingwen Zhang , Ji Chen , Baojing Gu , Xiaoying Zhan , Bowei Yu , Yulong Shi , Hafiz Athar Hussain , Xuekai Jing
Non-carbon dioxide greenhouse gas (non-CO2 GHG) emissions from global crop-livestock systems, primarily driven by enteric fermentation and manure-related emissions, pose significant challenges to climate mitigation. Identifying emission hotspots and simulating future mitigation potential are crucial for achieving agricultural carbon neutrality. Constructed a comprehensive dataset spanning 138 countries (1961–2020), integrating FAO statistics, literature-derived emission factors, and socioeconomic data, this study quantified spatiotemporal emission trends and identified decoupling patterns between emissions and economic development. The Logarithmic Mean Divisia Index (LMDI) was used to decompose drivers and six scenarios (BAU (Baseline), RSA (Rearing Structure Adjustment), LMO (Livestock Management Optimization), BMPs-30% and BMPs-50% (best management practices with a manure substitution ratio of 30% or 50%), and NMA (No Manure Application)) were developed to assess mitigation potential. Results revealed that global non-CO2 GHG emissions from crop-livestock systems increased by 61.9% from 2696.5 to 4365.0 Mt CO2-eq. yr−1 from 1961 to 2020, with India, Brazil, China, and the United States accounting for about 40% of total emissions in 2020. Significant decoupling occurred in developed countries, such as the United States, around in 1985 at approximately $10,000 per-capita GDP. In developing countries like China, significant decoupling was evident around in 1990 at approximately $3000 per-capita GDP. Ambitious scenarios (BMPs-50%) could reduce global emissions by 3.2–6.7 Gt CO2-eq. yr−1 by 2060, with major contributions from India (671.3 Mt CO2-eq. yr−1), Brazil (494.2 Mt CO2-eq. yr−1), China (486.1 Mt CO2-eq. yr−1), and the USA (238.8 Mt CO2-eq. yr−1). The findings confirmed the decoupling of non-CO2GHG emissions within crop-livestock systems from economic growth in developed countries but highlight persistent challenges in developing regions. Strategic shifts toward monogastric livestock, manure recycling, and dietary transitions emerge as critical pathways for aligning food security with carbon neutrality goals.
全球作物-牲畜系统的非二氧化碳温室气体(非co2 GHG)排放主要由肠道发酵和粪便相关排放驱动,对减缓气候变化构成重大挑战。确定排放热点和模拟未来的缓解潜力对于实现农业碳中和至关重要。本研究构建了涵盖138个国家(1961-2020年)的综合数据集,整合了粮农组织统计数据、文献导出的排放因子和社会经济数据,量化了排放的时空趋势,并确定了排放与经济发展之间的脱钩模式。采用对数平均划分指数(LMDI)对驱动因素进行分解,并制定了6个情景(BAU(基线)、RSA(饲养结构调整)、LMO(牲畜管理优化)、bmp -30%和bmp -50%(粪肥替代率为30%或50%的最佳管理实践)和NMA(不施用粪肥))来评估缓解潜力。结果显示,全球作物-牲畜系统的非二氧化碳温室气体排放量从2696.5亿吨二氧化碳当量增加到4365.0亿吨二氧化碳当量,增加了61.9%。到2020年,印度、巴西、中国和美国约占总排放量的40%。显著的脱钩发生在发达国家,比如美国,1985年左右人均GDP约为1万美元。在像中国这样的发展中国家,显著的脱钩在1990年左右的人均GDP约为3000美元时是明显的。雄心勃勃的方案(bmp -50%)可以使全球排放量减少3.2-6.7亿吨二氧化碳当量。到2060年,印度将做出主要贡献(6.713亿吨二氧化碳当量)。年−1),巴西(4.942亿吨二氧化碳当量)。年−1),中国(4.861亿吨二氧化碳当量)。年−1),美国(2.388亿吨二氧化碳当量)。年−1)。研究结果证实了发达国家作物-牲畜系统内的非二氧化碳温室气体排放与经济增长的脱钩,但强调了发展中地区持续存在的挑战。向单胃制牲畜、粪便循环利用和饮食转变的战略转变成为使粮食安全与碳中和目标保持一致的关键途径。
{"title":"Livestock rearing as a key component of mitigation efforts for non-CO2 greenhouse gas emissions in global crop-livestock system","authors":"Li Zheng ,&nbsp;Qingwen Zhang ,&nbsp;Ji Chen ,&nbsp;Baojing Gu ,&nbsp;Xiaoying Zhan ,&nbsp;Bowei Yu ,&nbsp;Yulong Shi ,&nbsp;Hafiz Athar Hussain ,&nbsp;Xuekai Jing","doi":"10.1016/j.resenv.2025.100248","DOIUrl":"10.1016/j.resenv.2025.100248","url":null,"abstract":"<div><div>Non-carbon dioxide greenhouse gas (non-CO<sub>2</sub> GHG) emissions from global crop-livestock systems, primarily driven by enteric fermentation and manure-related emissions, pose significant challenges to climate mitigation. Identifying emission hotspots and simulating future mitigation potential are crucial for achieving agricultural carbon neutrality. Constructed a comprehensive dataset spanning 138 countries (1961–2020), integrating FAO statistics, literature-derived emission factors, and socioeconomic data, this study quantified spatiotemporal emission trends and identified decoupling patterns between emissions and economic development. The Logarithmic Mean Divisia Index (LMDI) was used to decompose drivers and six scenarios (BAU (Baseline), RSA (Rearing Structure Adjustment), LMO (Livestock Management Optimization), BMPs-30% and BMPs-50% (best management practices with a manure substitution ratio of 30% or 50%), and NMA (No Manure Application)) were developed to assess mitigation potential. Results revealed that global non-CO<sub>2</sub> GHG emissions from crop-livestock systems increased by 61.9% from 2696.5 to 4365.0 Mt CO<sub>2</sub>-eq. yr<sup>−1</sup> from 1961 to 2020, with India, Brazil, China, and the United States accounting for about 40% of total emissions in 2020. Significant decoupling occurred in developed countries, such as the United States, around in 1985 at approximately $10,000 per-capita GDP. In developing countries like China, significant decoupling was evident around in 1990 at approximately $3000 per-capita GDP. Ambitious scenarios (BMPs-50%) could reduce global emissions by 3.2–6.7 Gt CO<sub>2</sub>-eq. yr<sup>−1</sup> by 2060, with major contributions from India (671.3 Mt CO<sub>2</sub>-eq. yr<sup>−1</sup>), Brazil (494.2 Mt CO<sub>2</sub>-eq. yr<sup>−1</sup>), China (486.1 Mt CO<sub>2</sub>-eq. yr<sup>−1</sup>), and the USA (238.8 Mt CO<sub>2</sub>-eq. yr<sup>−1</sup>). The findings confirmed the decoupling of non-CO<sub>2</sub>GHG emissions within crop-livestock systems from economic growth in developed countries but highlight persistent challenges in developing regions. Strategic shifts toward monogastric livestock, manure recycling, and dietary transitions emerge as critical pathways for aligning food security with carbon neutrality goals.</div></div>","PeriodicalId":34479,"journal":{"name":"Resources Environment and Sustainability","volume":"21 ","pages":"Article 100248"},"PeriodicalIF":12.4,"publicationDate":"2025-09-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144631364","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
期刊
Resources Environment and Sustainability
全部 IZV-PHYS SOLID EART+ Contrib. Mineral. Petrol. Conserv. Genet. Resour. Communications Earth & Environment Geol. J. Geobiology ASTROBIOLOGY 液晶与显示 Ann. Glaciol. J. Opt. Gondwana Res. PERIOD MINERAL J PHYS A-MATH THEOR J. Hydrol. 2013 Abstracts IEEE International Conference on Plasma Science (ICOPS) APL Photonics High Pressure Res. Paleontol. J. Clean-Soil Air Water ACTA DIABETOL Geosci. J. Environmental Progress ASTRON ASTROPHYS J APPL METEOROL CLIM J. Mol. Spectrosc. Geosci. Front. Geochim. Cosmochim. Acta Environmental Epigenetics J NONLINEAR OPT PHYS Ocean and Coastal Research ENVIRONMENT Ocean Sci. OPTICA ERN: Other Microeconomics: General Equilibrium & Disequilibrium Models of Financial Markets (Topic) Chem. Ecol. Environmental Control in Biology LIGHT-SCI APPL FRONT EARTH SCI-PRC 国际生物医学工程杂志 Ann. Phys. Basin Res. Annu. Rev. Earth Planet. Sci. ACTA REUMATOL PORT J. Appl. Phys. OPT LASER TECHNOL Nucl. Fusion EUR PHYS J-SPEC TOP Geochem. Trans. ARCHAEOMETRY Biomed Eng (NY) Aquat. Geochem. Am. Mineral. Atmos. Res. Atmos. Meas. Tech. Acta Geophys. GEOTECH LETT Carbon Balance Manage. Administration and Policy in Mental Health and Mental Health Services Research Asia-Pac. J. Atmos. Sci. Acta Antiqua Academiae Scientiarum Hungaricae Am. J. Phys. Anthropol. 2010 International Conference on Mechanic Automation and Control Engineering ARCH ACOUST Clim. Change J. Nanophotonics Org. Geochem. Appl. Geochem. Acta Geochimica INFRARED PHYS TECHN ATMOSPHERE-BASEL [Rinsho ketsueki] The Japanese journal of clinical hematology Acta Oceanolog. Sin. Ecol. Eng. ACTA GEOL POL Energy Environ. GEOLOGY AAPG Bull. IEEE Trans. Appl. Supercond. Archaeol. Anthropol. Sci. Am. J. Sci. Opt. Commun. Int. J. Biometeorol. BIOGEOSCIENCES J. Electron. Spectrosc. Relat. Phenom. ACTA GEOL SIN-ENGL Astrophys. Space Sci. Adv. Atmos. Sci. ICARUS Appl. Clay Sci. Acta Geod. Geophys. ARCT ANTARCT ALP RES EUR PHYS J-APPL PHYS B SOC GEOL MEX ECOSYSTEMS J. Math. Phys. ACTA PETROL SIN J. Atmos. Chem. ECOL RESTOR Geostand. Geoanal. Res. Isl. Arc
×
引用
GB/T 7714-2015
复制
MLA
复制
APA
复制
导出至
BibTeX EndNote RefMan NoteFirst NoteExpress
×
0
微信
客服QQ
Book学术公众号 扫码关注我们
反馈
×
意见反馈
请填写您的意见或建议
请填写您的手机或邮箱
×
提示
您的信息不完整,为了账户安全,请先补充。
现在去补充
×
提示
您因"违规操作"
具体请查看互助需知
我知道了
×
提示
现在去查看 取消
×
提示
确定
Book学术官方微信
Book学术文献互助
Book学术文献互助群
群 号:604180095
Book学术
文献互助 智能选刊 最新文献 互助须知 联系我们:info@booksci.cn
Book学术提供免费学术资源搜索服务,方便国内外学者检索中英文文献。致力于提供最便捷和优质的服务体验。
Copyright © 2023 Book学术 All rights reserved.
ghs 京公网安备 11010802042870号 京ICP备2023020795号-1