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Recent developments in stimuli-responsive hydrogels for biomedical applications 生物医学应用刺激反应水凝胶的最新进展
Q3 Engineering Pub Date : 2022-10-13 DOI: 10.1049/bsb2.12050
Shuyun Liu, Xiaozhuang Li, Lu Han

Hydrogels exhibit a performance similar to that of the extracellular matrix and are compatible with human tissues and organs. Stimuli-responsive hydrogels that can respond smartly to a variety of stimuli have recently attracted extensive interest for biomedical applications. The response of these hydrogels to various single/multiple stimuli shows great potential for drug delivery, biosensors, wound dressing, cancer therapy, and tissue engineering. This review summarises the recent advances in the design of different stimuli-responsive hydrogels and their biomedical applications. We herein describe the mechanisms underlying the stimulus–response, and summarise the strategies for fabricating stimuli-responsive hydrogels that can respond to single or multiple stimuli from endogenous (i.e. pH, enzymes, glucose, and reactive oxygen species) or exogenous (i.e. magnetic and electric fields, temperature, and photo) sources. The current challenges faced by stimuli-responsive hydrogels are discussed and an outlook on future research directions is provided.

水凝胶表现出类似于细胞外基质的性能,并且与人体组织和器官相容。刺激反应水凝胶可以对各种刺激做出灵敏的反应,最近引起了生物医学应用的广泛兴趣。这些水凝胶对各种单一/多重刺激的反应在药物输送、生物传感器、伤口敷料、癌症治疗和组织工程方面显示出巨大的潜力。本文综述了不同刺激反应水凝胶的设计及其生物医学应用的最新进展。我们在此描述了刺激反应的机制,并总结了制造刺激反应水凝胶的策略,这种水凝胶可以对来自内源性(即pH、酶、葡萄糖和活性氧)或外源性(即磁场、电场、温度和光)的单一或多种刺激做出反应。讨论了当前刺激响应型水凝胶面临的挑战,并对未来的研究方向进行了展望。
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引用次数: 0
Recent progress of tree frog toe pads inspired wet adhesive materials 树蛙脚趾垫启发的湿粘合材料的最新进展
Q3 Engineering Pub Date : 2022-09-16 DOI: 10.1049/bsb2.12049
Yikai Zhang, Xizi Wan, Xuetao Xu, Peicheng Teng, Shutao Wang

Wet adhesion has widespread applications in the fields of wearable electronics, medical devices and intelligent robots. In nature, many organisms have evolved with unique wet adhesion properties to adapt to complex habitats and climb in wet environments without falling. Tree frogs, as crawling masters in tropical rain forests, are representative of wet adhesion and give novel inspirations to design artificial wet adhesive materials by mimicking their specialised hexagonal structures and/or mucus composition. In this review, we first overview the research progress of tree frog toe pads from the perspective of toe pad structure and adhesion mechanism. Then, wet adhesive materials inspired by tree frog toe pads are systematically summarised from (i) the typical polymers, (ii) the preparation approaches, (iii) the adhesion test methods and (iv) the typical artificial adhesion surfaces. Third, various applications of bioinspired wet adhesive surfaces are highlighted. Finally, we present future challenges and opportunities to develop tree frog-inspired wet adhesive materials.

湿式粘接技术在可穿戴电子、医疗器械、智能机器人等领域有着广泛的应用。在自然界中,许多生物进化出了独特的湿润粘附特性,以适应复杂的栖息地,在潮湿的环境中攀爬而不坠落。树蛙作为热带雨林的爬行高手,是湿黏附的代表,通过模仿其特殊的六边形结构和/或黏液成分,为设计人工湿黏附材料提供了新的灵感。本文首先从树蛙趾垫结构和粘附机理两方面综述了树蛙趾垫的研究进展。然后,从(i)典型聚合物,(ii)制备方法,(iii)粘附测试方法和(iv)典型人工粘附表面系统地总结了受树蛙脚趾垫启发的湿粘附材料。第三,重点介绍了仿生湿粘接表面的各种应用。最后,我们提出了未来的挑战和机遇,以发展树蛙启发湿粘接材料。
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引用次数: 8
Recent progress of bioinspired cartilage hydrogel lubrication materials 仿生软骨水凝胶润滑材料的研究进展
Q3 Engineering Pub Date : 2022-09-02 DOI: 10.1049/bsb2.12047
Xiaoduo Zhao, Weiyi Zhao, Yunlei Zhang, Xiaoqing Zhang, Zhengfeng Ma, Rui Wang, Qiangbing Wei, Shuanhong Ma, Feng Zhou

Hydrogels have been considered as potential candidates for cartilage replacement due to their high-water content, extreme network hydration, excellent biocompatibility and tunable mechanical properties. Currently, the development of high-performance cartilage-inspired hydrogel lubrication materials has become a hot topic in the field of biomedical materials. This review focusses on the recent development of cartilage-inspired high-strength hydrogels from the viewpoints of bionic surface/interface and biotribology. Specifically, the composition structure and extraordinary lubrication mechanism of the natural articular cartilage are overviewed first. Subsequently, some of the novel biomimetic design strategies for preparing high strength cartilage hydrogels with various network structures are summarised in detail, while systematic evaluation of lubrication properties and mechanisms are discussed. Furthermore, new surface modification means for improving the lubrication feature of high strength cartilage hydrogel materials are presented. In addition, in order to demonstrate the application potential of cartilage hydrogels in clinical, several bonding methods to decorate hydrogels onto surfaces of natural bone tissues or artificial joint materials are introduced. Finally, current challenges and future research directions are discussed for cartilage-inspired hydrogel lubrication materials.

水凝胶由于其高含水量、极端网络水化、优异的生物相容性和可调节的机械性能而被认为是软骨替代的潜在候选材料。目前,高性能软骨型水凝胶润滑材料的开发已成为生物医学材料领域的研究热点。本文从仿生表面/界面和生物摩擦学的角度综述了近年来软骨型高强度水凝胶的研究进展。具体来说,首先概述了天然关节软骨的组成结构和特殊的润滑机制。随后,详细总结了制备具有各种网状结构的高强度软骨水凝胶的一些新型仿生设计策略,并对其润滑性能和机理进行了系统评价。提出了提高高强度软骨水凝胶材料润滑性能的表面改性新方法。此外,为了展示软骨水凝胶在临床中的应用潜力,介绍了几种将水凝胶装饰在天然骨组织或人工关节材料表面的粘接方法。最后,对软骨型水凝胶润滑材料面临的挑战和未来的研究方向进行了讨论。
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引用次数: 2
Recent progress on smart hydrogels for biomedicine and bioelectronics 生物医学和生物电子学领域智能水凝胶研究进展
Q3 Engineering Pub Date : 2022-09-02 DOI: 10.1049/bsb2.12046
Fa Zou, Jiefang Xu, Le Yuan, Qinyong Zhang, Lili Jiang

The increasing development of biomedicine and bioelectronics has highlighted the requirement for smart materials that can respond to changes in physical and chemical properties under external environments, such as magnetic fields, electric fields, and temperature. Accordingly, hydrogels have been widely evaluated as promising candidates for smart materials owing to their intriguing structures comprising a cross-linked network of polymer chains with interstitial spaces filled with solvent water. This feature endows hydrogels with soft and wet characteristics, which not only induce high tissue affinity but also allow the introduction of environmentally responsive nanoparticles to release specific smart properties. Herein, we reviewed novel smart hydrogels that can be applied in biomedicine and bioelectronics, and highlighted and discussed existing challenges in current technologies and research.

随着生物医学和生物电子学的不断发展,对能够响应外部环境(如磁场、电场和温度)下物理和化学性质变化的智能材料的需求日益突出。因此,水凝胶被广泛评价为智能材料的有前途的候选者,因为它们的有趣结构包括一个交联的聚合物链网络,间隙充满了溶剂水。这一特性赋予了水凝胶柔软湿润的特性,这不仅可以诱导高组织亲和力,还可以引入对环境敏感的纳米颗粒来释放特定的智能特性。本文综述了可用于生物医学和生物电子学的新型智能水凝胶,并重点讨论了当前技术和研究中存在的挑战。
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引用次数: 1
Non-chromate conversion process for zinc coating with durable hydrophobicity and enhanced corrosion resistance 具有持久疏水性和增强耐腐蚀性的锌涂层的非铬酸盐转化工艺
Q3 Engineering Pub Date : 2022-08-29 DOI: 10.1049/bsb2.12048
J. Y. Chen, Z. Y. Hu, Z. X. Li, X. L. Wang, C. D. Gu, J. P. Tu

A Zn-based coating with durable hydrophobicity and good corrosion resistance was formed on a mild steel substrate, which involves electroplating Zn from a non-aqueous electrolyte, followed by passivation in an oleic acid (OA) solution. The electrodeposited Zn coatings were porous, which facilitated the formation of a chemical conversion layer of Zn oleate (ZO) during OA passivation. The Zn coating after passivation had a two-layer structure, which included an outer layer of ZO with a thickness of ∼26 μm and an inner layer of Zn with a thickness of ∼6 μm. The outer layer ZO is a type of metal soap with a smooth surface and durable hydrophobicity, such that water droplets can easily slip off its surface. Corrosion testing and electrochemical measurements in 3.5 wt.% NaCl aqueous solution indicate that the Zn coating after OA passivation exhibits outstanding anti-corrosion properties compared with those exhibited by pure Zn coating. The corrosion products and mechanism of the two-layer coating were explored. This study shows that smooth metal oleate coatings can provide hydrophobicity and corrosion resistance simultaneously to mild steel substrates.

在低碳钢基体上形成了具有持久疏水性和良好耐腐蚀性的锌基涂层,该涂层采用非水电解质电镀Zn,然后在油酸(OA)溶液中钝化。电沉积Zn涂层具有多孔性,有利于在OA钝化过程中形成油酸锌(ZO)的化学转化层。钝化后的Zn涂层呈两层结构,外层为ZO,厚度为~ 26 μm,内层为Zn,厚度为~ 6 μm。外层ZO是一种金属肥皂,表面光滑,具有持久的疏水性,水滴很容易从其表面滑落。在3.5 wt.% NaCl水溶液中的腐蚀测试和电化学测试表明,与纯锌涂层相比,OA钝化后的锌涂层具有更好的防腐性能。探讨了两层涂层的腐蚀产物和腐蚀机理。研究表明,光滑的金属油酸盐涂层可以同时提供对低碳钢基体的疏水性和耐腐蚀性。
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引用次数: 0
Construction and application of bionic antifouling coatings inspired by soft coral 以软珊瑚为灵感的仿生防污涂料的构建与应用
Q3 Engineering Pub Date : 2022-08-19 DOI: 10.1049/bsb2.12041
Wei Bing, E. Jin, Limei Tian, Huichao Jin, Zhuo Liu

Marine biofouling will bring a series of environmental and social problems, which restrict the development and utilisation of marine resources. Therefore, how to prevent biofouling has become a global issue. With the exploration of antifouling methods, bionic antifouling technology with environmentally friendly, broad-spectrum, and long-term advantages has gradually attracted people's attention. Inspired by the antifouling strategy of soft coral (Sarcophyton trocheliophorum), the silicone rubber (RTV-2) with similar elasticity to coral skin was selected as the substrate. The composite structure of the upper transparent layer and the lower porous layer was prepared by simulating the structure of soft coral as the structural factors of the bionic antifouling coatings. Meanwhile, several organic antifouling components with high content contained in soft coral were added to the transparent layer and porous layer, respectively, as the component factors of biomimetic coatings. The bionic antifouling coatings, which are highly consistent with the coral structure, obtained the best antifouling performance under static and dynamic conditions. The above results provide new ideas for the synthesis of environmentally friendly bionic antifouling coatings.

海洋生物污染将带来一系列的环境和社会问题,制约着海洋资源的开发利用。因此,如何防止生物污染已成为一个全球性的问题。随着防污方法的探索,具有环保、广谱、长效优势的仿生防污技术逐渐受到人们的重视。受软珊瑚(Sarcophyton trocheliophorum)防污策略的启发,选择与珊瑚皮肤弹性相似的硅橡胶(r电视-2)作为基材。通过模拟软珊瑚的结构,制备上透明层和下多孔层的复合结构,作为仿生防污涂料的结构因子。同时,在透明层和多孔层中分别加入软珊瑚中含量较高的几种有机防污成分,作为仿生涂层的组成因子。与珊瑚结构高度一致的仿生防污涂料在静态和动态条件下均获得了最佳的防污性能。上述结果为环境友好型仿生防污涂料的合成提供了新的思路。
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引用次数: 0
Bionic superhydrophobic surfaces based on topography of copper oxides 基于铜氧化物形貌的仿生超疏水表面
Q3 Engineering Pub Date : 2022-08-17 DOI: 10.1049/bsb2.12045
Chen Chen, Haiyang Zhan, Xiangge Bai, Zichao Yuan, Lei Zhao, Yahua Liu, Shile Feng

Superhydrophobic surfaces (SHSs) exist in many biological organisms endowed by spectacular surface topographies, which provide important insights to drive a paradigm shift in design of engineering surfaces. Based on this, extensive progresses have been developed on bionic superhydrophobic strategies. Among them, SHSs based on topography of copper oxides exhibit considerable application prospects because of the steerability and diversity of topography, as well as additional performances, such as antibiosis, anticorrosion and catalysis. We first present a brief overview of the discovery of natural SHSs as well as fundamental understanding of surface wetting performance. Then, the structural effects in superhydrophobic systems based on the topographies of biological organisms and copper oxides are described. Finally, we highlight the perspectives on the novel design strategies of copper oxide-based SHSs that adapt to various practical applications.

超疏水表面(SHSs)存在于许多生物有机体中,具有壮观的表面地形,为推动工程表面设计的范式转变提供了重要的见解。基于此,仿生超疏水策略的研究取得了广泛的进展。其中,基于氧化铜形貌的SHSs由于形貌的可操控性和多样性,以及抗菌、防腐、催化等附加性能,具有相当大的应用前景。我们首先简要概述了天然SHSs的发现以及对表面润湿性能的基本理解。然后,描述了基于生物有机体和铜氧化物的拓扑结构在超疏水体系中的结构效应。最后,我们强调了适应各种实际应用的基于氧化铜的SHSs的新设计策略的观点。
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引用次数: 0
Topographical biointerface regulating cellular functions for bone tissue engineering 骨组织工程中调节细胞功能的地形生物界面
Q3 Engineering Pub Date : 2022-08-17 DOI: 10.1049/bsb2.12043
Mingyu Zhu, Rui Zhang, Zhixiang Mao, Ju Fang, Fuzeng Ren

The physiochemical properties of the implant interface significantly influence cell growth, differentiation, cellular matrix deposition, and mineralisation, and eventually, determine the bone regeneration efficiency. Cells directly sense and respond to the physical, chemical, and mechanical cues of the implant surface, and it is increasingly recognized that surface topography can evoke specific cellular responses, conferring biological functions on substrate materials and regulating tissue regeneration. Current progress towards the fundamental understanding of the interplay between the cell and topographical surface has been made by combined advance in fabrication technologies and cell biology. Particularly, the precise fabrication and control of nano/microscale topographies can provide the fundamental knowledge of the mechanotransduction process that governs the cellular response as well as the knowledge of how the specific features drive cells towards a defined differentiation outcome. In this review, we first introduce common techniques and substrate materials for designing and fabricating micro/nano-topographical surfaces for bone regeneration. We then illustrate the intrinsic relationship of topological cues, cellular signal transduction, and cell functions and fates in osteogenic differentiation. Finally, we discuss the challenges and the future of using topological cues as a cell therapy to direct bone tissue regeneration.

种植体界面的理化性质显著影响细胞生长、分化、细胞基质沉积和矿化,并最终决定骨再生效率。细胞直接感知并响应植入物表面的物理、化学和机械信号,并且越来越多的人认识到,表面形貌可以引起特定的细胞反应,赋予基质材料生物学功能并调节组织再生。目前对细胞和地形表面之间相互作用的基本理解的进展是由制造技术和细胞生物学的综合进步取得的。特别是,纳米/微尺度地形的精确制造和控制可以提供控制细胞反应的机械转导过程的基本知识,以及特定特征如何驱动细胞走向确定的分化结果的知识。在这篇综述中,我们首先介绍了设计和制造用于骨再生的微/纳米形貌表面的常用技术和衬底材料。然后,我们说明了在成骨分化中拓扑线索、细胞信号转导和细胞功能和命运的内在关系。最后,我们讨论了使用拓扑线索作为细胞疗法来指导骨组织再生的挑战和未来。
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引用次数: 2
Biomimetic directional transport for sustainable liquid usage 可持续液体使用的仿生定向输送
Q3 Engineering Pub Date : 2022-08-16 DOI: 10.1049/bsb2.12044
Jie Ma, Zhichao Dong

Through hundreds of millions of evolution, animals and plants have possessed their unique structures to adapt to natural variations. As a familiar process, liquid transportation plays an important part in both production and life, and researchers focus on how to achieve this process in a convenient and efficient way without energy input. Inspired by nature, various bioinspired structures are reported and have won multiple achievements. This review starts from basic theory about surface wettability, and then summarises the creatures with special liquid transport functions as well as crucial structures that cause this phenomenon. Next, the recent articles about transporting liquid by bioinspired materials are introduced. Finally, we proposed a brief conclusion and the prospect of bionic materials in the future.

经过几亿次的进化,动物和植物已经拥有了它们独特的结构来适应自然变化。液体输送作为一种熟悉的过程,在生产和生活中都起着重要的作用,如何在不输入能量的情况下方便、高效地实现这一过程是研究的重点。受到大自然的启发,各种生物启发结构被报道并获得了多项成就。本文从表面润湿性的基本理论入手,综述了具有特殊液体输送功能的生物及其产生润湿性的关键结构。其次,介绍了近年来生物材料在液体输送方面的研究进展。最后,对仿生材料的研究进行了简要的总结和展望。
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引用次数: 0
Preparation of metal-organic frameworks and their derivatives for supercapacitors 超级电容器用金属有机骨架及其衍生物的制备
Q3 Engineering Pub Date : 2022-08-15 DOI: 10.1049/bsb2.12040
Youjian Li, Donglin Gan, Xu Deng, Lili Jiang, Chaoming Xie, Xiong Lu

To satisfy the requirements of social power development, it is urgently necessary to develop innovative and sustainable new energy storage devices. Supercapacitors have attracted considerable attention as a new type of energy storage device, owing to their high energy density, high power density, fast charging and discharging speeds, and long cycle life. The electrode material is an important factor in determining the electrochemical performance of supercapacitors. In recent years, researchers explored the application of metal-organic frameworks (MOFs) and their derivatives as electrode materials for supercapacitors. In this paper, the preparation of monometallic, bimetallic, and conductive MOFs, and their derivatives for application in supercapacitors are reviewed. In addition, challenges facing MOFs in the field of supercapacitors and their future development prospects are discussed.

为了满足社会电力发展的要求,迫切需要开发创新、可持续的新型储能装置。超级电容器作为一种新型的储能器件,以其高能量密度、高功率密度、充放电速度快、循环寿命长等优点而备受关注。电极材料是决定超级电容器电化学性能的重要因素。近年来,研究人员探索了金属有机骨架及其衍生物作为超级电容器电极材料的应用。本文综述了单金属、双金属和导电mof的制备及其衍生物在超级电容器中的应用。此外,还讨论了mof在超级电容器领域面临的挑战和未来的发展前景。
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引用次数: 0
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