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Atomic-scale imaging of laser-driven electron dynamics in solids 固体中激光驱动电子动力学的原子尺度成像
IF 5.4 1区 物理与天体物理 Q1 PHYSICS, MULTIDISCIPLINARY Pub Date : 2024-10-02 DOI: 10.1038/s42005-024-01810-7
Daria Popova-Gorelova, Robin Santra
Resolving laser-driven electron dynamics on their natural time and length scales is essential for understanding and controlling light-induced phenomena. Capabilities to reveal these dynamics are limited by challenges in interpreting wave mixing of a driving and a probe pulse, low energy resolution at ultrashort time scales and a lack of atomic-scale resolution by standard spectroscopic techniques. Here, we demonstrate how ultrafast x-ray diffraction can access fundamental information on laser-driven electronic motion in solids. We propose a method based on subcycle-resolved x-ray-optical wave mixing that allows for a straightforward reconstruction of key properties of strong-field-induced electron dynamics with atomic spatial resolution. Namely, this technique provides both phases and amplitudes of the spatial Fourier transform of optically-induced charge distributions, their temporal behavior, and the direction of the instantaneous microscopic optically-induced electron current flow. It captures the rich microscopic structures and symmetry features of laser-driven electronic charge and current density distributions. Manipulation of materials properties by laser driving can lead to future technological applications, but a complete picture of its mechanisms is missing. In their paper, authors propose a method based on ultrafast x-ray diffraction that allows for resolving laser-driven electron dynamics on their natural time and length scales.
在自然时间和长度尺度上解析激光驱动的电子动力学对于理解和控制光诱导现象至关重要。由于在解释驱动脉冲和探测脉冲的混合波方面存在挑战、超短时间尺度的能量分辨率低以及标准光谱技术缺乏原子尺度的分辨率,揭示这些动态的能力受到了限制。在这里,我们展示了超快 X 射线衍射如何获取固体中激光驱动电子运动的基本信息。我们提出了一种基于亚周期分辨 X 射线光波混合的方法,可以直接重建强场诱导电子动力学的关键特性,并具有原子空间分辨率。也就是说,这种技术可以提供光诱导电荷分布的空间傅立叶变换的相位和振幅、它们的时间行为以及瞬时微观光诱导电子流的方向。它能捕捉到激光驱动的电子电荷和电流密度分布的丰富微观结构和对称特征。通过激光驱动对材料特性的操纵可带来未来的技术应用,但对其机理的完整描述尚缺。在他们的论文中,作者提出了一种基于超快 X 射线衍射的方法,可以在自然时间和长度尺度上解析激光驱动的电子动力学。
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引用次数: 0
Spontaneous reversal of spin chirality and competing phases in the topological magnet EuAl4 拓扑磁体 EuAl4 中自旋手性的自发逆转和竞争相
IF 5.4 1区 物理与天体物理 Q1 PHYSICS, MULTIDISCIPLINARY Pub Date : 2024-09-30 DOI: 10.1038/s42005-024-01802-7
Anuradha M. Vibhakar, Dmitry D. Khalyavin, Fabio Orlandi, Jamie M. Moya, Shiming Lei, Emilia Morosan, Alessandro Bombardi
Materials exhibiting a spontaneous reversal of spin chirality have the potential to drive the widespread adoption of chiral magnets in spintronic devices. Unlike the majority of chiral magnets that require the application of an external field to reverse the spin chirality, we observe the spin chirality to spontaneously reverse in the topological magnet EuAl4. Using resonant elastic x-ray scattering we demonstrate that all four magnetic phases in EuAl4 are single-k, where the first two magnetic phases are characterized by spin density wave order and the last two by helical spin order. A single spin chirality was stabilised across the 1mm2 sample, and the reversal of spin chirality occurred whilst maintaining a helical magnetic structure. At the onset of the helical magnetism, the crystal symmetry lowers to a chiral monoclinic space group, explaining the asymmetry in the chiral spin order, and establishing a mechanism by which the spin chirality could reverse via magnetostructural coupling. The reversal of spin chirality in the absence of any externally applied field would substantially broaden the use of chiral magnets for applications in spintronic devices. In this manuscript the authors demonstrate the spontaneous reversal of spin chirality in the topological magnet EuAl4 using resonant elastic x-ray scattering.
表现出自旋手性自发反转的材料有望推动手性磁体在自旋电子设备中的广泛应用。大多数手性磁体都需要施加外部磁场才能逆转自旋手性,与之不同的是,我们观察到拓扑磁体 EuAl4 中的自旋手性自发逆转。通过共振弹性 X 射线散射,我们证明了 EuAl4 中的所有四个磁相都是单 K 磁相,其中前两个磁相以自旋密度波序为特征,后两个磁相以螺旋自旋序为特征。在 1 平方毫米的样品中,单一的自旋手性得到了稳定,而自旋手性的逆转是在保持螺旋磁性结构的同时发生的。在螺旋磁性开始时,晶体对称性降低到手性单斜空间群,这解释了手性自旋顺序的不对称性,并建立了通过磁结构耦合实现自旋手性逆转的机制。在没有任何外加磁场的情况下逆转自旋手性将大大拓宽手性磁体在自旋电子器件中的应用。在这篇手稿中,作者利用共振弹性 X 射线散射证明了拓扑磁体 EuAl4 中自旋手性的自发反转。
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引用次数: 0
Gate tunable edge magnetoplasmon resonators 栅极可调边缘磁致共振器
IF 5.4 1区 物理与天体物理 Q1 PHYSICS, MULTIDISCIPLINARY Pub Date : 2024-09-30 DOI: 10.1038/s42005-024-01803-6
Elric Frigerio, Giacomo Rebora, Mélanie Ruelle, Hubert Souquet-Basiège, Yong Jin, Ulf Gennser, Antonella Cavanna, Bernard Plaçais, Emmanuel Baudin, Jean-Marc Berroir, Inès Safi, Pascal Degiovanni, Gwendal Fève, Gerbold C. Ménard
Quantum Hall systems are platforms of choice to study topological properties of condensed matter systems and anyonic exchange statistics. In this work we have developed a tunable radiofrequency edge magnetoplasmonic resonator controlled by both the magnetic field and a set of electrostatic gates, meant to serve as a versatile platform for future interferometric devices designed to evidence non-abelian anyons. In our device, gates allow us to change both the size of the resonant cavity and the electronic density of the two-dimensional electron gas. We show that we can continuously control the frequency response of our resonator, making it possible to develop an edge magnetoplasmon interferometer. As we reach smaller sizes of our resonator, finite size effects caused by the measurement probes manifest. In the future, such device will be a valuable tool to investigate the properties of non-abelian anyons in the fractional quantum Hall regime. Edge-magnetoplasmon interferometers have been proposed as a tool to investigate anyonic properties of quasiparticles in the regime of the Fractional Quantum Hall effect. In this work, the authors demonstrate the possibility to control electrostatically the resonance frequency of EMP resonators of micrometric size and explain the role of gates, paving the way toward the realization of anyonic interferometers.
量子霍尔系统是研究凝聚态系统拓扑特性和任意子交换统计的首选平台。在这项工作中,我们开发了一种可调谐射频边缘磁共振器,由磁场和一组静电门控制,旨在作为未来干涉装置的多功能平台,用于证明非阿贝尔任子。在我们的装置中,栅极允许我们改变谐振腔的大小和二维电子气体的电子密度。我们的研究表明,我们可以连续控制谐振器的频率响应,从而开发出边缘磁谱干涉仪。当我们的谐振器尺寸变小时,测量探针引起的有限尺寸效应就会显现出来。未来,这种装置将成为研究分数量子霍尔机制中非阿贝尔任子特性的重要工具。边缘磁谱干涉仪已被提出作为研究分数量子霍尔效应体系中准粒子的任子特性的工具。在这项工作中,作者展示了静电控制微米级 EMP 谐振器共振频率的可能性,并解释了门的作用,为实现任意子干涉仪铺平了道路。
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引用次数: 0
Photonic counterdiabatic quantum optimization algorithm 光子逆绝热量子优化算法
IF 5.4 1区 物理与天体物理 Q1 PHYSICS, MULTIDISCIPLINARY Pub Date : 2024-09-30 DOI: 10.1038/s42005-024-01807-2
Pranav Chandarana, Koushik Paul, Mikel Garcia-de-Andoin, Yue Ban, Mikel Sanz, Xi Chen
One of the key applications of near-term quantum computers has been the development of quantum optimization algorithms. However, these algorithms have largely been focused on qubit-based technologies. Here, we propose a hybrid quantum-classical approximate optimization algorithm for photonic quantum computing, specifically tailored for addressing continuous-variable optimization problems. Inspired by counterdiabatic protocols, our algorithm reduces the required quantum operations for optimization compared to adiabatic protocols. This reduction enables us to tackle non-convex continuous optimization within the near-term era of quantum computing. Through illustrative benchmarking, we show that our approach can outperform existing state-of-the-art hybrid adiabatic quantum algorithms in terms of convergence and implementability. Our algorithm offers a practical and accessible experimental realization, bypassing the need for high-order operations and overcoming experimental constraints. We conduct a proof-of-principle demonstration on Xanadu’s eight-mode nanophotonic quantum chip, successfully showcasing the feasibility and potential impact of the algorithm. The authors introduce a hybrid quantum-classical algorithm for photonic quantum computing that focuses on tackling continuous-variable optimization problems using fewer quantum operations than existing methods. The approach shows better performance and practical implementation potential, demonstrated on Xanadu’s quantum chip.
近期量子计算机的关键应用之一是开发量子优化算法。然而,这些算法主要集中在基于量子比特的技术上。在这里,我们为光子量子计算提出了一种混合量子-经典近似优化算法,专门用于解决连续变量优化问题。受反绝热协议的启发,与绝热协议相比,我们的算法减少了优化所需的量子操作。这种减少使我们能够在量子计算的近期时代解决非凸连续优化问题。通过说明性基准测试,我们表明我们的方法在收敛性和可实施性方面优于现有的最先进的混合绝热量子算法。我们的算法绕过了对高阶运算的需求,克服了实验限制,提供了一种切实可行、易于实现的实验方法。我们在 Xanadu 的八模纳米光子量子芯片上进行了原理验证演示,成功展示了该算法的可行性和潜在影响。作者介绍了一种用于光子量子计算的量子-经典混合算法,该算法侧重于使用比现有方法更少的量子操作来解决连续变量优化问题。该方法在 Xanadu 量子芯片上展示了更好的性能和实际应用潜力。
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引用次数: 0
Constraints on fifth forces and ultralight dark matter from OSIRIS-REx target asteroid Bennu OSIRIS-REx目标小行星贝努对第五力和超轻暗物质的制约
IF 5.4 1区 物理与天体物理 Q1 PHYSICS, MULTIDISCIPLINARY Pub Date : 2024-09-20 DOI: 10.1038/s42005-024-01779-3
Yu-Dai Tsai, Davide Farnocchia, Marco Micheli, Sunny Vagnozzi, Luca Visinelli
It is important to test the possible existence of fifth forces, as ultralight bosons that would mediate these are predicted to exist in several well-motivated extensions of the Standard Model. Recent work indicated asteroids as promising probes, but applications to real data are lacking so far. Here we use the OSIRIS-REx mission and ground-based tracking data for the asteroid Bennu to derive constraints on fifth forces. Our limits are strongest for mediator masses m ~ (10−18-10−17) eV, where we currently achieve the tightest bounds. These can be translated to a wide class of models leading to Yukawa-type fifth forces, and we demonstrate how they apply to U(1)B dark photons and baryon-coupled scalars. Our results demonstrate the potential of asteroid tracking in probing well-motivated extensions of the Standard Model and ultralight bosons near the fuzzy dark matter range. Asteroid tracking has been demonstrated as a promising and prominent probe of fifth forces arising in several well-motivated models beyond the Standard Model of particle physics. The authors use the state-of-art tracking data for the asteroid Bennu from the OSIRIS-REx mission to derive the tightest limits on fifth forces and ultralight dark matter at the lengths of solar-system objects.
对可能存在的第五种力进行测试非常重要,因为在标准模型的几个动机良好的扩展中,预测会存在介导第五种力的超轻玻色子。最近的工作表明小行星是很有希望的探测器,但迄今为止还缺乏对真实数据的应用。在这里,我们利用 OSIRIS-REx 任务和小行星贝努的地面跟踪数据,推导出对第五力的限制。我们对介质质量 m ~ (10-18-10-17) eV 的限制是最强的,目前我们在这方面达到了最严格的界限。这些限制可以转化为导致育川型第五力的多种模型,我们还演示了它们如何适用于 U(1)B 暗光子和重子耦合标量。我们的结果证明了小行星追踪在探测标准模型的动机良好的扩展和模糊暗物质范围附近的超轻玻色子方面的潜力。小行星追踪已被证明是对粒子物理标准模型之外的几个动机良好的模型中产生的第五力的一种有前途的突出探测。作者利用 OSIRIS-REx 任务对小行星贝努(Bennu)的最新跟踪数据,推导出太阳系天体长度上第五力和超轻暗物质的最严格限制。
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引用次数: 0
Droplets can enhance microcapsule deformation in channel flow 液滴可增强通道流中的微囊变形
IF 5.4 1区 物理与天体物理 Q1 PHYSICS, MULTIDISCIPLINARY Pub Date : 2024-09-20 DOI: 10.1038/s42005-024-01805-4
Dalei Jing, Ruixin Lu, Alexander Farutin, Ziyu Guo, Fan Wang, Wen Wang, Chaouqi Misbah, Yi Sui
The dynamics of soft microparticles enclosed in a droplet flowing in a channel is an unexplored fundamental problem that lies at the heart of numerous applications, including droplet-based microfluidics, tissue engineering and smart material synthesis. Here we show that enclosing a flexible capsule into a droplet can amplify the capsule’s deformation parameters in channel flow by up to two orders of magnitude. Previously unreported capsule equilibrium shapes in channel flow, including an oblate spheroid and a reversed bullet, have also been discovered. We propose two theoretical models to predict the equilibrium position of the capsule inside the droplet, and estimate the capsule deformation, respectively. The present study provides an effective but simple approach to enhance and control the deformation of soft particles in a flowing suspension, which may inspire widespread applications, from high-throughput single-cell mechanical phenotyping, enhanced cross-membrane drug delivery, to manufacturing shape-controlled non-spherical particles and artificial cells. Enhancing deformation of soft microparticles such as cells, capsules and vesicles has widespread applications in cell phenotyping, drug/gene delivery and smart material synthesis. Here, the authors demonstrate that enclosing a capsule into a droplet can amplify the capsule deformation parameter by up to two orders of magnitude, compared with an isolated capsule experiencing identical channel flow conditions.
液滴中的软微粒在通道中流动时的动力学是一个尚未探索的基本问题,它是众多应用的核心,包括基于液滴的微流体、组织工程和智能材料合成。在这里,我们展示了将柔性胶囊包围在液滴中可以将胶囊在通道流动中的变形参数放大两个数量级。我们还发现了以前未报道过的胶囊在通道流中的平衡形状,包括扁球形和反向子弹形。我们提出了两个理论模型,分别用于预测液滴内胶囊的平衡位置和估计胶囊的变形。本研究提供了一种有效而简单的方法来增强和控制流动悬浮液中软颗粒的形变,它可能会激发从高通量单细胞机械表型、增强跨膜给药到制造形状可控的非球形颗粒和人造细胞等方面的广泛应用。增强细胞、胶囊和囊泡等软性微颗粒的变形在细胞表型、药物/基因递送和智能材料合成方面有着广泛的应用。作者在本文中证明,与经历相同通道流动条件的孤立胶囊相比,将胶囊包围在液滴中可将胶囊变形参数放大两个数量级。
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引用次数: 0
Addendum: Testing structural balance theories in heterogeneous signed networks 增编:在异质签名网络中检验结构平衡理论
IF 5.4 1区 物理与天体物理 Q1 PHYSICS, MULTIDISCIPLINARY Pub Date : 2024-09-20 DOI: 10.1038/s42005-024-01793-5
Anna Gallo, Diego Garlaschelli, Renaud Lambiotte, Fabio Saracco, Tiziano Squartini
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引用次数: 0
Emergence of group size disparity in growing networks with adoption 在不断扩大的网络中,群体规模的差异随着采用而出现
IF 5.4 1区 物理与天体物理 Q1 PHYSICS, MULTIDISCIPLINARY Pub Date : 2024-09-19 DOI: 10.1038/s42005-024-01799-z
Jun Sun, Fariba Karimi
Social and technical networks undergo constant evolution driven by both existing entities and newcomers. In academia, research papers are continually cited by new papers, while senior researchers integrate newly arrived junior researchers into their academic networks. Moreover, social systems can be influenced by external factors that could indirectly impact their growth patterns. For instance, systematic discrimination against certain groups in academia or managerial positions can impede their long-term growth, especially when combined with group-level preferences in hiring or adoption, as observed in our study. To address this, we introduce a network growth and adoption model where generalised preferential attachment and asymmetric mixing act as the two fundamental mechanisms of growth and adoption. We show analytically and numerically that these mechanisms can recover the empirical properties of citation and collaboration growth, as well as the inequalities observed in the growth dynamics of groups. This model can be used to investigate the effect of intervention in group mixing preferences to overcome the cumulative disparities in the group-level dynamics. The authors introduce a network growth and adoption model with preferential attachment and asymmetric mixing that can explain the inequalities observed in the group growth dynamics in scientific citation and collaboration. This model can be used to investigate the effect of intervention in group mixing preferences to overcome cumulative disparities.
社会和技术网络在现有实体和新来者的推动下不断演变。在学术界,研究论文不断被新论文引用,而资深研究人员则将新来的初级研究人员纳入其学术网络。此外,社会系统也会受到外部因素的影响,从而间接影响其发展模式。例如,在学术界或管理岗位上对某些群体的系统性歧视可能会阻碍他们的长期发展,尤其是在招聘或采用方面与群体层面的偏好相结合时,正如我们的研究中所观察到的那样。为了解决这个问题,我们引入了一个网络增长和采用模型,其中广义优先依附和非对称混合是增长和采用的两个基本机制。我们通过分析和计算表明,这些机制可以恢复引用和协作增长的经验属性,以及在群体增长动态中观察到的不平等现象。该模型可用于研究干预群体混合偏好的效果,以克服群体层面动态中的累积差异。
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引用次数: 0
Designer spin-orbit superlattices: symmetry-protected Dirac cones and spin Berry curvature in two-dimensional van der Waals metamaterials 设计师自旋轨道超晶格:二维范德华超材料中受对称保护的狄拉克锥和自旋贝里曲率
IF 5.4 1区 物理与天体物理 Q1 PHYSICS, MULTIDISCIPLINARY Pub Date : 2024-09-19 DOI: 10.1038/s42005-024-01801-8
L. M. Martelo, Aires Ferreira
The emergence of strong relativistic spin-orbit effects in low-dimensional systems provides a rich opportunity for exploring unconventional states of matter. Here, we present a route to realise tunable relativistic band structures based on the lateral patterning of proximity-induced spin-orbit coupling. The concept is illustrated on a patterned graphene–transition metal dichalcogenide heterostructure, where the spatially periodic spin-orbit coupling induces a rich mini-band structure featuring massless and massive Dirac bands carrying large spin Berry curvature. The envisaged systems support robust and gate-tunable spin Hall responses driven by the quantum geometry of mini-bands, which can be tailored through metasurface fabrication methods and twisting effects. These findings open pathways to two-dimensional quantum material design and low-power spintronic applications. Engineering sizeable spin-orbit coupling (SOC) in graphene generates effects unmatched in traditional low-dimensional systems. Here, the authors show that the periodic modulation of SOC in 1D patterned graphene heterostructures leads to unusual mini-band structures with symmetry-protected Dirac cones featuring enhanced spin Berry curvature, which paves the way to tunable spin Hall responses.
低维系统中出现的强相对论自旋轨道效应为探索非传统的物质状态提供了丰富的机会。在此,我们提出了一条基于近距离自旋轨道耦合的横向图案化来实现可调相对论能带结构的途径。这一概念在图案化的石墨烯-过渡金属二掺杂异质结构上得到了诠释,其中空间周期性自旋轨道耦合诱导了丰富的迷你带状结构,具有无质量和大质量的狄拉克带,并携带大自旋贝里曲率。设想中的系统支持由迷你带量子几何驱动的稳健且可门控调谐的自旋霍尔响应,可通过元表面制造方法和扭曲效应对其进行定制。这些发现为二维量子材料设计和低功耗自旋电子应用开辟了道路。
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引用次数: 0
Purification scheduling control for throughput maximization in quantum networks 实现量子网络吞吐量最大化的净化调度控制
IF 5.4 1区 物理与天体物理 Q1 PHYSICS, MULTIDISCIPLINARY Pub Date : 2024-09-18 DOI: 10.1038/s42005-024-01796-2
Zirui Xiao, Jian Li, Kaiping Xue, Nenghai Yu, Ruidong Li, Qibin Sun, Jun Lu
Quantum networks can establish End-to-End (E2E) entanglement connections between two arbitrary nodes with desired entanglement fidelity by performing entanglement purification to support quantum applications reliably. The existing works mainly focus on link-level purification scheduling and lack consideration of purifications at network-level, which fails to offer an effective solution for concurrent requests, resulting in low throughput. However, efficiently allocating scarce resources to purify entanglement for concurrent requests remains a critical but unsolved problem. To address this problem, we explore the purification resource scheduling problem from a network-level perspective. We analyze the cost of purification, design the E2E fidelity calculation method in detail, and propose an approach called Purification Scheduling Control (PSC). The basic idea of PSC is to determine the appropriate purification through jointly optimizing purification and resource allocation processes based on conflict avoidance. We conduct extensive experiments that show that PSC can maximize throughput under the fidelity requirement. In quantum networks, entanglement purification is required to ensure that the E2E fidelity of the entanglement connections can support quantum applications reliably. Here, the authors explore the purification resource scheduling problem from a network-level perspective by jointly optimizing purification and resource allocation processes to maximize the throughput under the fidelity requirement.
量子网络可以通过执行纠缠净化,在两个任意节点之间建立端到端(E2E)纠缠连接,并达到所需的纠缠保真度,从而可靠地支持量子应用。现有研究主要关注链路级净化调度,缺乏对网络级净化的考虑,无法为并发请求提供有效的解决方案,导致吞吐量较低。然而,有效分配稀缺资源以净化并发请求的纠缠仍是一个关键但尚未解决的问题。为了解决这个问题,我们从网络层面的角度探讨了净化资源调度问题。我们分析了净化的成本,详细设计了 E2E 保真度计算方法,并提出了一种称为净化调度控制(PSC)的方法。PSC 的基本思想是在避免冲突的基础上,通过联合优化净化和资源分配过程来确定适当的净化。我们进行了大量实验,结果表明 PSC 可以在保真度要求下最大限度地提高吞吐量。
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引用次数: 0
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Communications Physics
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