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Research on the fusion imaging method of sign coherence and time reversal for Lamb wave sparse array λ波稀疏阵列符号相干与时间反转融合成像方法研究
IF 3.8 2区 物理与天体物理 Q1 ACOUSTICS Pub Date : 2024-10-11 DOI: 10.1016/j.ultras.2024.107489
Liu-Jia Sun, Qing-Bang Han, Cheng Yin, Qi-Lin Jin, Kao Ge
Time-reversal imaging struggles to detect plate-like structures due to interference from Lamb wave mode conversion and the processing demands, leading to less effective outcomes. This paper proposes a sign coherence factor and time reversal fusion (SCF-TR) imaging method based on amplitude and phase estimation. This method removes the coherence of array signals during signal reversal and refocusing. It reintroduces the sign coherence component to reduce interference from non-target scattered waves and partially overcome the constraints imposed by the Rayleigh criterion. The method allows imaging at a resolution smaller than the wavelength of Lamb and enhances the quality of the resulting images. In addition, a sparse array design utilizing the White Shark Optimisation Algorithm (WSO) is proposed to streamline the SCF-TR calculation process. This design utilizes sparse full matrix data to improve imaging efficiency. The experimental results show that for single blind hole defects, the SCF-TR method improves the array performance metrics and signal-to-noise ratio by 22.46% and 42.50%, respectively, compared to the TR method. For multiple asymmetric blind hole defects, when the defect size exceeds the resolution threshold, SCF-TR accurately reflects the position and morphology of defects smaller than the wavelength. When the defect size is below the resolution threshold, SCF-TR achieves super-resolution imaging. The sparse array designed using the White Shark Optimization algorithm demonstrates good sidelobe characteristics, effectively reducing sidelobe noise without reducing the array aperture. Moreover, the SCF-TR imaging time is reduced by approximately half while maintaining imaging accuracy.
由于 Lamb 波模式转换的干扰和处理要求,时间反转成像在检测板状结构方面很吃力,导致效果不佳。本文提出了一种基于振幅和相位估计的符号相干因子和时间反转融合(SCF-TR)成像方法。这种方法能消除信号反转和重新聚焦时阵列信号的相干性。它重新引入了符号相干分量,以减少非目标散射波的干扰,并部分克服了瑞利准则带来的限制。该方法允许在小于 Lamb 波长的分辨率下成像,并提高了所得图像的质量。此外,还提出了一种利用白鲨优化算法(WSO)的稀疏阵列设计,以简化 SCF-TR 计算过程。这种设计利用稀疏全矩阵数据来提高成像效率。实验结果表明,对于单个盲孔缺陷,SCF-TR 方法与 TR 方法相比,阵列性能指标和信噪比分别提高了 22.46% 和 42.50%。对于多个不对称盲孔缺陷,当缺陷尺寸超过分辨率阈值时,SCF-TR 能准确反映小于波长的缺陷的位置和形态。当缺陷尺寸低于分辨率阈值时,SCF-TR 可实现超分辨率成像。利用白鲨优化算法设计的稀疏阵列具有良好的侧叶特性,能在不减小阵列孔径的情况下有效降低侧叶噪声。此外,在保持成像精度的同时,SCF-TR 的成像时间缩短了约一半。
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引用次数: 0
Low-intensity pulsed ultrasound improves metabolic dysregulation in obese mice by suppressing inflammation and extracellular matrix remodeling 低强度脉冲超声通过抑制炎症和细胞外基质重塑改善肥胖小鼠的代谢失调
IF 3.8 2区 物理与天体物理 Q1 ACOUSTICS Pub Date : 2024-10-10 DOI: 10.1016/j.ultras.2024.107488
Min He , Hong Zhu , Jingsong Dong , Wenzhen Lin , Boyi Li , Ying Li , Dean Ta
Chronic inflammation in white adipose tissue is crucial in obesity and related metabolic disorders. Low-intensity pulsed ultrasound (LIPUS) is renowned for its anti-inflammatory effects as a non-invasive treatment, yet its precise role in obesity has been uncertain. Our study investigates the therapeutic effect of LIPUS and its underlying mechanism on obesity in mice, thereby offering a novel approach for non-invasive treatment of obesity and associated metabolic disorders for human. Male C57BL/6J mice aged 10 weeks were fed a high-fat diet (HFD) for 8 weeks to establish obesity model, then underwent 8 weeks of LIPUS (frequency: 1.0 MHz, duty cycle: 20 %, Isata: 58–61 mW/cm2, 20 min per day) stimulation of the epididymal white adipose tissue. Fat and lean mass were measured using nuclear magnetic resonance (NMR), while energy homeostasis was evaluated using metabolic cages. Insulin resistance was assessed using glucose tolerance tests (GTT) and insulin tolerance tests (ITT). Regulatory mechanisms were explored using RNA sequencing. Results showed that LIPUS significantly reduced obesity markers in obese mice, including body and adipose tissue weight, and improved insulin resistance, without affecting food intake. RNA sequencing showed 250 up-regulated and 351 down-regulated genes between HFD-LIPUS group and HFD-Sham group, suggesting anti-inflammatory action. Quantitative PCR confirmed reduced pro-inflammatory gene expression and macrophage infiltration in eWAT. Gene set enrichment analysis showed decreased NF-κB signaling and extracellular matrix-receptor interactions in LIPUS-treated mice. Thus, LIPUS effectively mitigates metabolic dysregulation in HFD-induced obesity through inflammation suppression and extracellular matrix remodeling, which provides a potential physical therapy for metabolic syndrome in clinic.
白色脂肪组织中的慢性炎症是肥胖和相关代谢紊乱的关键因素。低强度脉冲超声(LIPUS)作为一种非侵入性治疗方法,以其抗炎作用而闻名,但它在肥胖症中的确切作用还不确定。我们的研究调查了 LIPUS 对小鼠肥胖症的治疗效果及其内在机制,从而为人类提供了一种非侵入性治疗肥胖症及相关代谢紊乱的新方法。对年龄为 10 周的雄性 C57BL/6J 小鼠喂食高脂饮食(HFD)8 周以建立肥胖模型,然后对附睾白色脂肪组织进行为期 8 周的 LIPUS(频率:1.0 MHz,占空比:20%,等效功率:58-61 mW/cm2,每天 20 分钟)刺激。使用核磁共振(NMR)测量脂肪和瘦肉质量,使用代谢笼评估能量平衡。胰岛素抵抗通过葡萄糖耐量试验(GTT)和胰岛素耐量试验(ITT)进行评估。利用 RNA 测序探索了调控机制。结果表明,LIPUS能明显降低肥胖小鼠的肥胖指标,包括体重和脂肪组织重量,并改善胰岛素抵抗,而不影响食物摄入量。RNA测序显示,HFD-LIPUS组和HFD-Sham组分别有250个基因上调,351个基因下调,这表明LIPUS具有抗炎作用。定量 PCR 证实,eWAT 中的促炎基因表达和巨噬细胞浸润减少。基因组富集分析表明,LIPUS 治疗小鼠的 NF-κB 信号转导和细胞外基质-受体相互作用减少。因此,LIPUS 通过抑制炎症和细胞外基质重塑,有效缓解了高氟酸膳食诱导的肥胖症代谢失调,为临床治疗代谢综合征提供了一种潜在的物理疗法。
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引用次数: 0
Damage detection and localization in plate-like structures using sideband peak count (SPC) technique 利用边带峰值计数(SPC)技术检测和定位板状结构中的损伤。
IF 3.8 2区 物理与天体物理 Q1 ACOUSTICS Pub Date : 2024-10-05 DOI: 10.1016/j.ultras.2024.107485
Bo Hu , Tribikram Kundu
This paper addresses the critical issue of detecting and localizing damage in plate-like structures, which are commonly encountered in aerospace, marine and other engineering applications. To address this challenge, the current study introduces the sideband peak count (SPC) technique as the foundation for diagnostic imaging for damage detection in plate structures. The proposed damage detection algorithm requires only a limited number of sensor responses, streamlining the detection process. It does not rely on a reference baseline, thereby enhancing its efficiency and accuracy. This approach enables rapid and precise identification of damage and its location within the plate structure. To validate the effectiveness and applicability of the proposed method, finite element simulation results are utilized. These results demonstrate the capability of the proposed technique to accurately detect and localize damage, providing a promising solution for enhancing the structural health monitoring of plate-like structures in various engineering domains.
本文探讨了在航空航天、海洋和其他工程应用中常见的板状结构中检测和定位损伤的关键问题。为应对这一挑战,本研究引入了边带峰值计数(SPC)技术,作为板状结构损伤检测诊断成像的基础。所提出的损伤检测算法只需要数量有限的传感器响应,从而简化了检测过程。它不依赖参考基线,从而提高了效率和准确性。这种方法能够快速、精确地识别板结构中的损伤及其位置。为了验证所提方法的有效性和适用性,我们使用了有限元模拟结果。这些结果表明,所提出的技术具有准确检测和定位损伤的能力,为在各种工程领域中加强板状结构的结构健康监测提供了一个前景广阔的解决方案。
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引用次数: 0
A semi-analytical framework for predicting far-field responses of complex elastic waves emitters 预测复杂弹性波发射器远场响应的半分析框架。
IF 3.8 2区 物理与天体物理 Q1 ACOUSTICS Pub Date : 2024-10-03 DOI: 10.1016/j.ultras.2024.107483
Siddhesh Raorane, Tadeusz Stepinski, Pawel Packo
Applications of guided waves in various fields of engineering and science rely on elastic wave emitters for wave generation. Accurate prediction and understanding of the far-field responses of these wave emitters are crucial for the reliable and efficient application of guided waves-based technologies. In this paper, we propose a novel semi-analytical framework capable of predicting the far-field response of complex wave emitters of arbitrary shape and internal structure in any type of substrate. This framework is general, and is not confined to specific methods, enhancing its versatility. We applied the proposed semi-analytical framework to predict the directivity patterns of two different macro-fiber composite transducers, accurately modeled using their exact topologies. The framework’s validity was experimentally confirmed by comparing the predicted directivity patterns with the results obtained from experimental measurements.
导波在各个工程和科学领域的应用都依赖于弹性波发射器来产生波。准确预测和理解这些波发射器的远场响应,对于可靠、高效地应用基于导波的技术至关重要。在本文中,我们提出了一个新颖的半分析框架,能够预测任何类型基底中任意形状和内部结构的复杂波发射器的远场响应。该框架具有通用性,不局限于特定的方法,从而增强了其通用性。我们应用所提出的半分析框架预测了两种不同的宏纤维复合传感器的指向性模式,并使用它们的精确拓扑结构进行了精确建模。通过将预测的指向性模式与实验测量结果进行比较,实验证实了该框架的有效性。
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引用次数: 0
Beamforming-integrated neural networks for ultrasound imaging 用于超声波成像的波束成形集成神经网络。
IF 3.8 2区 物理与天体物理 Q1 ACOUSTICS Pub Date : 2024-10-03 DOI: 10.1016/j.ultras.2024.107474
Di Xiao, Alfred C.H. Yu
Sparse matrix beamforming (SMB) is a computationally efficient reformulation of delay-and-sum (DAS) beamforming as a single sparse matrix multiplication. This reformulation can potentially dovetail with machine learning platforms like TensorFlow and PyTorch that already support sparse matrix operations. In this work, using SMB principles, we present the development of beamforming-integrated neural networks (BINNs) that can rationally infer ultrasound images directly from pre-beamforming channel-domain radiofrequency (RF) datasets. To demonstrate feasibility, a toy BINN was first designed with two 2D-convolution layers that were respectively placed both before and after an SMB layer. This toy BINN correctly updated kernel weights in all convolution layers, demonstrating efficiency in both training (PyTorch – 133 ms, TensorFlow – 22 ms) and inference (PyTorch – 4 ms, TensorFlow – 5 ms). As an application demonstration, another BINN with two RF-domain convolution layers, an SMB layer, and three image-domain convolution layers was designed to infer high-quality B-mode images in vivo from single-shot plane-wave channel RF data. When trained using 31-angle compounded plane wave images (3000 frames from 22 human volunteers), this BINN showed mean-square logarithmic error improvements of 21.3 % and 431 % in the inferred B-mode image quality respectively comparing to an image-to-image convolutional neural network (CNN) and an RF-to-image CNN with the same number of layers and learnable parameters (3,777). Overall, by including an SMB layer to adopt prior knowledge of DAS beamforming, BINN shows potential as a new type of informed machine learning framework for ultrasound imaging.
稀疏矩阵波束成形(SMB)是对延迟与和(DAS)波束成形的一种计算高效的重构,是一种单一的稀疏矩阵乘法。这种重构有可能与 TensorFlow 和 PyTorch 等已经支持稀疏矩阵运算的机器学习平台对接。在这项工作中,我们利用 SMB 原理开发了波束成形集成神经网络(BINN),它可以直接从预波束成形信道域射频(RF)数据集合理推断超声图像。为了证明其可行性,我们首先设计了一个玩具 BINN,它有两个二维卷积层,分别位于 SMB 层之前和之后。这个玩具 BINN 正确更新了所有卷积层的内核权重,在训练(PyTorch - 133 毫秒,TensorFlow - 22 毫秒)和推理(PyTorch - 4 毫秒,TensorFlow - 5 毫秒)方面都表现出高效率。作为应用演示,我们设计了另一个具有两个射频域卷积层、一个 SMB 层和三个图像域卷积层的 BINN,用于从单发平面波通道射频数据推断高质量的活体 B 模式图像。在使用 31 角复合平面波图像(来自 22 名人体志愿者的 3000 帧图像)进行训练时,与具有相同层数和可学习参数(3,777)的图像到图像卷积神经网络(CNN)和射频到图像 CNN 相比,该 BINN 所推断的 B 型图像质量的均方对数误差分别提高了 21.3% 和 431%。总之,通过加入一个采用 DAS 波束成形先验知识的 SMB 层,BINN 显示出作为一种新型超声成像知情机器学习框架的潜力。
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引用次数: 0
A new theoretical model for high-order harmonics of SH0 mode ultrasonic guided waves based on magnetostrictive mechanism 基于磁致伸缩机制的 SH0 模式超声导波高阶谐波新理论模型。
IF 3.8 2区 物理与天体物理 Q1 ACOUSTICS Pub Date : 2024-09-30 DOI: 10.1016/j.ultras.2024.107480
Huan Wang , Xiucheng Liu , Bin Wu , Xiang Gao , Yao Liu , Cunfu He
In recent years, it was found that magnetostrictive ultrasonic guided wave transducers experimentally excited nonlinear harmonic components under a certain combination of dynamic and static magnetic fields. However, a satisfactory model for the relevant excitation mechanisms is not available. In this study, a new magnetostrictive guided wave excitation model was established and the causes for harmonics generation were analyzed. In addition, the calculation results of the model were obtained under different magnetic field parameters. We firstly changed the calculation conditions of magnetostrictive strain in the model and then theoretically calculated the odd and even harmonics of SH0 mode ultrasonic guided waves for the first time. Furthermore, the accuracy of the model was experimentally verified. By changing the strength ratio of the dynamic magnetic field to the static magnetic field (HD/HS), the excitation amplitudes of odd and even harmonics could be regulated with a magnetostrictive sensor. As the ratio of HD/HS increased, the normalized amplitude of the second harmonic firstly increased and then decreased, whereas the normalized amplitude of the third harmonic showed an exponential growth with different curvatures. This study enriched the theory of magnetostrictive guided wave excitation and provided a theoretical basis for the applications of magnetostrictive sensors.
近年来,人们发现磁致伸缩超声导波换能器在一定的动静态磁场组合下会激发非线性谐波成分。然而,目前还没有一个令人满意的相关激励机制模型。本研究建立了一个新的磁致伸缩导波激励模型,并分析了谐波产生的原因。此外,还获得了该模型在不同磁场参数下的计算结果。我们首先改变了模型中磁致伸缩应变的计算条件,然后首次从理论上计算了 SH0 模式超声导波的奇次谐波和偶次谐波。此外,还通过实验验证了模型的准确性。通过改变动态磁场与静态磁场的强度比(HD/HS),可以利用磁致伸缩传感器调节奇次谐波和偶次谐波的激励幅值。随着 HD/HS 比值的增大,二次谐波的归一化振幅先增大后减小,而三次谐波的归一化振幅则呈现出不同曲率的指数增长。这项研究丰富了磁致伸缩导波激励理论,为磁致伸缩传感器的应用提供了理论依据。
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引用次数: 0
Compensation of system nonlinearity in the measurement of acoustic nonlinearity parameters 测量声学非线性参数时的系统非线性补偿。
IF 3.8 2区 物理与天体物理 Q1 ACOUSTICS Pub Date : 2024-09-30 DOI: 10.1016/j.ultras.2024.107484
Jiung Yoo , Dong-Gi Song , Kyung-Young Jhang
The acoustic nonlinearity parameter is determined from the amplitudes of the fundamental and second harmonic component of the acoustic wave propagating through the material. However, the generally used through-transmission based measurements with PZT transducers contain high system nonlinearity, so that the received second harmonic component includes an extra component caused by the transducer, which significantly decrease the reliability of measurements. In this study, we proposed a novel method to reduce the system nonlinearity in the conventional through-transmission based measurements by adding a simple process in which the transmitting and receiving transducers are in direct contact without a specimen. The proposed method was experimentally validated for two materials, Al6061-T6 and Fused Silica. For both materials, several specimens with different thickness were prepared, and the measurement results showed that the magnitude of the second harmonic was proportional to the thickness, but there was an offset due to system nonlinearity. On the other hand, after applying the proposed technique, the offsets were greatly reduced, and furthermore, this performance was maintained even when the transducer setup was changed, and the ratio of nonlinearity parameters measured for the two materials was in good agreement with the known literature value.
声学非线性参数是根据声波在材料中传播时的基波和二次谐波分量的振幅确定的。然而,通常使用的基于 PZT 换能器的穿透式测量包含较高的系统非线性,因此接收到的二次谐波分量包含了由换能器引起的额外分量,这大大降低了测量的可靠性。在这项研究中,我们提出了一种新方法,通过添加一个简单的过程,使发射和接收传感器在没有试样的情况下直接接触,从而降低传统的穿透式测量中的系统非线性。所提出的方法在两种材料(Al6061-T6 和熔融石英)上进行了实验验证。测量结果表明,二次谐波的大小与厚度成正比,但由于系统的非线性,存在偏移。另一方面,在应用所提出的技术后,偏移量大大减少,而且即使改变传感器的设置也能保持这种性能,两种材料测得的非线性参数比率与已知文献值非常一致。
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引用次数: 0
Image quality improvement in single plane-wave imaging using deep learning 利用深度学习提高单平面波成像的图像质量。
IF 3.8 2区 物理与天体物理 Q1 ACOUSTICS Pub Date : 2024-09-30 DOI: 10.1016/j.ultras.2024.107479
Kanta Miura , Hiromi Shidara , Takuro Ishii , Koichi Ito , Takafumi Aoki , Yoshifumi Saijo , Jun Ohmiya
In ultrasound image diagnosis, single plane-wave imaging (SPWI), which can acquire ultrasound images at more than 1000 fps, has been used to observe detailed tissue and evaluate blood flow. SPWI achieves high temporal resolution by sacrificing the spatial resolution and contrast of ultrasound images. To improve spatial resolution and contrast in SPWI, coherent plane-wave compounding (CPWC) is used to obtain high-quality ultrasound images, i.e., compound images, by coherent addition of radio frequency (RF) signals acquired by transmitting plane waves in different directions. Although CPWC produces high-quality ultrasound images, their temporal resolution is lower than that of SPWI. To address this problem, some methods have been proposed to reconstruct a ultrasound image comparable to a compound image from RF signals obtained by transmitting a small number of plane waves in different directions. These methods do not fully consider the properties of RF signals, resulting in lower image quality compared to a compound image. In this paper, we propose methods to reconstruct high-quality ultrasound images in SPWI by considering the characteristics of RF signal of a single plane wave to obtain ultrasound images with image quality comparable to CPWC. The proposed methods employ encoder–decoder models of 1D U-Net, 2D U-Net, and their combination to generate the high-quality ultrasound images by minimizing the loss that considers the point spread effect of plane waves and frequency spectrum of RF signals in training. We also create a public large-scale SPWI/CPWC dataset for developing and evaluating deep-learning methods. Through a set of experiments using the public dataset and our dataset, we demonstrate that the proposed methods can reconstruct higher-quality ultrasound images from RF signals in SPWI than conventional method.
在超声图像诊断中,单平面波成像(SPWI)能以超过 1000 fps 的速度获取超声图像,已被用于观察组织细节和评估血流。SPWI 通过牺牲超声图像的空间分辨率和对比度来实现高时间分辨率。为了提高 SPWI 的空间分辨率和对比度,采用了相干平面波复合(CPWC)技术,通过将从不同方向发射平面波获得的射频(RF)信号相干相加,获得高质量的超声图像,即复合图像。虽然 CPWC 能生成高质量的超声图像,但其时间分辨率低于 SPWI。为了解决这个问题,有人提出了一些方法,利用从不同方向发射少量平面波获得的射频信号重建与复合图像相当的超声图像。这些方法没有充分考虑射频信号的特性,导致图像质量低于复合图像。在本文中,我们提出了通过考虑单个平面波的射频信号特性来重建 SPWI 中高质量超声波图像的方法,以获得与 CPWC 图像质量相当的超声波图像。所提出的方法采用一维 U-网络、二维 U-网络的编码器-解码器模型及其组合,通过最小化损耗生成高质量超声图像,其中考虑了训练中平面波的点扩散效应和射频信号的频谱。我们还创建了一个公开的大规模 SPWI/CPWC 数据集,用于开发和评估深度学习方法。通过使用公共数据集和我们的数据集进行一系列实验,我们证明了与传统方法相比,我们提出的方法可以从 SPWI 中的射频信号重建更高质量的超声图像。
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引用次数: 0
An environmentally sustainable ultrasonic-assisted exfoliation approach to graphene and its nanocompositing with polyaniline for supercapacitor applications 一种环境可持续的超声波辅助剥离石墨烯及其与聚苯胺的纳米复合方法,用于超级电容器。
IF 3.8 2区 物理与天体物理 Q1 ACOUSTICS Pub Date : 2024-09-29 DOI: 10.1016/j.ultras.2024.107482
Chandni A P, Suchitra Vattapparambil Chandran, Binitha N. Narayanan
In the present work, a green high-yielding method for the preparation of graphene is introduced via ultrasonic-assisted liquid phase exfoliation (LPE) of graphite in a green solvent medium, since the common preparation method of graphene via graphite oxide is hazardous. A high concentration of 3.2 mg/ml graphene is achieved here in a comparatively short duration of 3 h ultrasonication. By using a mixed solvents strategy (acetophenone and isopropyl alcohol, 1:19 V/V), surface energy requirements needed for the exfoliation of graphite are satisfied here with acetophenone, where isopropyl alcohol further facilitated the exfoliation via non-conventional CH-π and OH-π interactions. Turbostratic graphene in high-yield (16 %) in a simple means of ultrasonic assisted LPE is the added attraction of the present procedure. The less-defective structure of graphene, its few-layered turbostratic nature, and edge functionalization of the sheets are evident from the material characterization via Raman spectroscopy, XRD, TEM-SAED, and XPS analyses. Here, we report a combination of the attractive conducting polymer polyaniline (PANI) with the as-prepared graphene for supercapacitor applications, where the PANI/graphene nanocomposites with different aniline concentrations (PANI1.125/G, PANI4.5/G, and PANI9/G) have been prepared via in-situ polymerization of aniline in the graphene dispersion. The structure and morphology of the nanocomposites are investigated using different characterization techniques which revealed that the molecular structure of the PANI is retained in the nanocomposites even with a strong interaction with graphene. FESEM and TEM images revealed the good coverage of graphene sheets with PANI that limit the volume change of PANI during the repeated charge-discharge processes. Electrochemical studies showed that PANI4.5/G has the highest specific capacitance of 126.16 mF/cm2 at a current density of 1 mA/cm2, resulting from the perfect combination of the pseudocapacitance behavior of the PANI along with the electrical double layer capacitance of graphene. A symmetric supercapacitor device is also fabricated with PANI4.5/G, which showed the highest areal capacitance of 116.38 mF/cm2 similar to that with three-electrode studies and also good cycling stability with 87 % capacitance retention in the specific capacitance after 6000 cycles. It also exhibited an energy density of 16 µWh/cm2 (0.29 Wh/kg) and a power density of 3.99 mW/cm2 (72.72 W/kg).
由于通过氧化石墨制备石墨烯的普通方法具有危险性,本研究通过在绿色溶剂介质中对石墨进行超声波辅助液相剥离(LPE),引入了一种制备石墨烯的绿色高产方法。在相对较短的 3 小时超声时间内,就能获得 3.2 mg/ml 的高浓度石墨烯。通过使用混合溶剂(苯乙酮和异丙醇,1:19 V/V),苯乙酮满足了石墨剥离所需的表面能要求,而异丙醇则通过非常规的 CH-π 和 OH-π 相互作用进一步促进了石墨的剥离。通过超声波辅助 LPE 的简单方法就能获得高产率(16%)的透射石墨烯,是本制备过程的一大亮点。通过拉曼光谱、XRD、TEM-SAED 和 XPS 分析对材料进行表征,可以明显看出石墨烯的缺陷较少、具有少层湍流性质以及片层边缘功能化。在此,我们报告了一种将极具吸引力的导电聚合物聚苯胺(PANI)与制备的石墨烯结合用于超级电容器应用的方法,即通过苯胺在石墨烯分散体中的原位聚合,制备出不同苯胺浓度(PANI1.125/G、PANI4.5/G 和 PANI9/G)的 PANI/石墨烯纳米复合材料。使用不同的表征技术对纳米复合材料的结构和形态进行了研究,结果表明,即使与石墨烯发生了强烈的相互作用,PANI 的分子结构仍然保留在纳米复合材料中。FESEM 和 TEM 图像显示石墨烯片与 PANI 的良好覆盖,从而限制了 PANI 在反复充放电过程中的体积变化。电化学研究表明,在电流密度为 1 mA/cm2 时,PANI4.5/G 具有最高的比电容(126.16 mF/cm2),这是 PANI 的伪电容行为与石墨烯的双电层电容完美结合的结果。使用 PANI4.5/G 制备的对称超级电容器装置也显示出最高的面积电容(116.38 mF/cm2),与三电极研究结果相似,并且具有良好的循环稳定性,6000 次循环后比电容保持率为 87%。它的能量密度为 16 µWh/cm2(0.29 Wh/kg),功率密度为 3.99 mW/cm2(72.72 W/kg)。
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引用次数: 0
Quantum analogous spin states of ultrasonic guided waves 超声导波的量子类似自旋态
IF 3.8 2区 物理与天体物理 Q1 ACOUSTICS Pub Date : 2024-09-29 DOI: 10.1016/j.ultras.2024.107478
Sourav Banerjee
In quantum mechanics, spin is a physical property that dominates the topological behaviors. While manifesting the spin states they reveal complex interaction of physical parameters in a topological media. The guided waves’ inherent spin states are made of real physical spin angular momentum from the superposition of elastic waves. Thus, here the elastic spin state that naturally manifests by the ultrasonic guided waves in an elastic wave guide is explained through quantum analogous perspective. Guided wave modes are the superposition of two longitudinally polarized and two transverse polarized elastic wave potentials propagating in diverging and converging pattern. Spin nature of transverse waves is well known. Spin nature of longitudinal waves is also recently being explored. However, due to the unique modal superposition of guided Rayleigh-Lamb wave modes the physical understanding of spin state is incomplete for the guided waves in a bounded media. Unlike only one hybrid spin states described in earlier works, guided waves may manifest total six with four well defined hybrid spin states explicitly derived and explained in this article. These six spin states play crucial role in the physics of spin-momentum locking of guided waves. Two spin states originated from the interaction of similar potentials and four hybris spin states originated from the interaction of potentials with different directions of wave vector and polarization vector, as emerged in guided waves. Understanding from fundamentals and exploiting the phenomena of spin-momentum locking in guided waves may have several applications in nondestructive evaluation.
在量子力学中,自旋是一种主导拓扑行为的物理特性。在表现自旋态时,它们揭示了拓扑介质中物理参数的复杂相互作用。导波的固有自旋态是由弹性波叠加的真实物理自旋角动量构成的。因此,这里通过量子类比的视角来解释超声导波在弹性波导中自然表现出的弹性自旋态。导波模式是以发散和收敛模式传播的两个纵向极化和两个横向极化弹性波势的叠加。横波的自旋性质是众所周知的。纵波的自旋性质最近也得到了探索。然而,由于导波雷利-兰姆波模式的独特模态叠加,对于有界介质中的导波,人们对自旋态的物理理解并不完整。与早期著作中描述的只有一种混合自旋态不同,导波可以表现出总共六种混合自旋态,其中四种定义明确的混合自旋态在本文中得到了明确的推导和解释。这六种自旋态在导波的自旋动量锁定物理学中起着至关重要的作用。两种自旋态源于相似电势的相互作用,四种混合自旋态源于波矢量和极化矢量方向不同的电势的相互作用,正如导波中出现的那样。从根本上理解和利用导波中的自旋动量锁定现象可能会在无损评估中得到一些应用。
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