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Multi-Site Anchoring for Tilted Octahedral Structure Stability Toward Efficient Blue Perovskite LEDs 倾斜八面体结构对高效蓝钙钛矿led稳定性的多位点锚定
IF 11 1区 物理与天体物理 Q1 OPTICS Pub Date : 2026-01-15 DOI: 10.1002/lpor.202502898
Lyuchao Zhuang, Qi Wei, Ren Hui, Duanzijing Liu, Wei Gao, Yiming He
The [PbX6]4− octahedron, while serving as the fundamental building block in perovskites and endowing exceptional photoelectric properties, exhibits inherent molecular softness and structural distortion that led to dynamic instabilities. Notably, the collapse of lead-halide octahedra triggered by halide vacancies presents a critical challenge to stability and performance, particularly in mixed-halide perovskite systems. Herein, we demonstrate a molecular engineering strategy using alkali metal trifluoromethanesulfonate additives, which are proposed to stabilize the perovskite lattice via a multi-anchoring mechanism. The sulfonyl oxygen groups are believed to interact with under-coordinated Pb sites, while the alkali metal cations are suggested to associate with halide species at the crystal surface, collectively mitigating octahedral distortion. This cooperative stabilization is supported by enhanced phase purity, suppressed nonradiative recombination, and improved optical performance in quasi-2D perovskite films. Consequently, the optimized perovskite films exhibit superior blue emission characteristics with a high photoluminescence quantum yield (PLQY) of 65.32%. The resultant blue PeLEDs deliver an external quantum efficiency (EQE) of 15.60% at 487 nm with a device lifetime of 220 min, representing a competitive performance compared with state-of-the-art blue PeLEDs in this spectral range. This work establishes octahedral stabilization as a fundamental design principle for advancing high-performance perovskite optoelectronic devices.
[PbX6]4−八面体作为钙钛矿的基本组成部分,具有优异的光电性能,同时表现出固有的分子柔软性和结构畸变,导致其动态不稳定性。值得注意的是,卤化物空位引发的铅-卤化物八面体坍塌对稳定性和性能提出了重大挑战,特别是在混合卤化物钙钛矿体系中。在此,我们展示了一种使用碱金属三氟甲烷磺酸盐添加剂的分子工程策略,该添加剂通过多锚定机制来稳定钙钛矿晶格。磺酰氧基被认为与不配位的Pb位相互作用,而碱金属阳离子被认为与晶体表面的卤化物结合,共同减轻八面体畸变。在准二维钙钛矿薄膜中,增强的相纯度、抑制的非辐射复合和改善的光学性能支持了这种协同稳定。因此,优化后的钙钛矿薄膜具有优异的蓝色发射特性,光致发光量子产率(PLQY)高达65.32%。由此产生的蓝色ped在487 nm处提供15.60%的外部量子效率(EQE),器件寿命为220分钟,与该光谱范围内最先进的蓝色ped相比,具有竞争力的性能。这项工作确立了八面体稳定作为推进高性能钙钛矿光电器件的基本设计原则。
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引用次数: 0
Deep learning-assisted metalens imaging over a wide depth of field. 深度学习辅助超透镜成像的大视场深度。
IF 3.3 2区 物理与天体物理 Q2 OPTICS Pub Date : 2026-01-15 DOI: 10.1364/OL.580297
Ruixiang Song, Xiyao Song, Xutong Lu, Shuaihong Qi, Feng Wang, Jiaqi Cui, Zhangyuan Chen, Yanping Li

Miniaturized lenses with a large depth of field and high imaging quality are desirable for compact optical systems, as they eliminate the need for lens switching and repeated refocusing. Metalenses, composed of flat, subwavelength nanostructures, are well suited to this demand due to their ultra-thin profile and design flexibility. However, miniaturized metalenses typically require larger numerical apertures (NA), which lead to strong chromatic dispersion and resolution degradation. To address this limitation, we propose a Metalens Depth-of-Field Generative Adversarial Network tailored for restoring full-color images captured by a high-NA (0.447) millimeter-scale metalens. It achieves a 35% increase in peak signal-to-noise ratio and a 57.7% reduction in perceptual loss, while maintaining reconstruction quality across over 17.5 cm depth of field without additional training. This network provides a practical and scalable solution for enhancing image quality in miniaturized imaging systems.

具有大景深和高成像质量的小型化镜头对于紧凑型光学系统是理想的,因为它们消除了镜头切换和反复重新对焦的需要。超透镜由扁平的亚波长纳米结构组成,由于其超薄的外形和设计的灵活性,非常适合这种需求。然而,小型化的超透镜通常需要更大的数值孔径(NA),这会导致强烈的色散和分辨率下降。为了解决这一限制,我们提出了一个超透镜景深生成对抗网络,用于恢复由高na(0.447)毫米尺度超透镜捕获的全彩图像。它实现了峰值信噪比增加35%,感知损失减少57.7%,同时在没有额外训练的情况下保持超过17.5 cm景深的重建质量。该网络为提高小型化成像系统的图像质量提供了一种实用的、可扩展的解决方案。
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引用次数: 0
Hänsch-Couillaud locking of a large Sagnac interferometer: advancing below the flicker floor. Hänsch-Couillaud锁定一个大型Sagnac干涉仪:推进到闪烁地板以下。
IF 3.3 2区 物理与天体物理 Q2 OPTICS Pub Date : 2026-01-15 DOI: 10.1364/OL.581271
Jannik Zenner, Karl Ulrich Schreiber, Simon Stellmer

Large Sagnac interferometers in the form of active ring lasers have emerged as unique rotation sensors in the geosciences, where their sensitivity allows one to detect geodetic and seismological signals. The passive laser gyroscope variant, however, is still at a stage of development, and thus far, only the Pound-Drever-Hall frequency stabilization technique has been explored, a method limited by residual amplitude modulation. Here, as an alternative method, we present the first Hänsch-Couillaud locked passive laser gyroscope. We find that this method is limited by flicker noise, and we introduce a cost-effective lock-in scheme to overcome this limitation. We achieve a sensitivity of 3.1nrad/s, corresponding to a fraction of 7.7×10-5 in the Earth's rotation rate.

主动环形激光形式的大型Sagnac干涉仪已成为地球科学中独特的旋转传感器,其灵敏度允许人们检测大地测量和地震信号。然而,被动激光陀螺仪的变体仍处于发展阶段,迄今为止,仅探索了庞德-德雷弗-霍尔稳频技术,这是一种受剩余调幅限制的方法。在这里,作为一种替代方法,我们提出了第一个Hänsch-Couillaud锁定被动激光陀螺仪。我们发现这种方法受到闪烁噪声的限制,并引入了一种经济有效的锁相方案来克服这一限制。我们获得了3.1nrad/s的灵敏度,相当于地球自转速度7.7×10-5的一小部分。
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引用次数: 0
Optimization of iterative wavefront shaping algorithms for quantum light. 量子光迭代波前整形算法的优化。
IF 3.3 2区 物理与天体物理 Q2 OPTICS Pub Date : 2026-01-15 DOI: 10.1364/OL.580091
Kiran Bajar, Rounak Chatterjee, Vikas S Bhat, Sushil Mujumdar

Wavefront manipulation and correction using feedback-based optimization have long been employed in optical applications such as microscopy, optical sensing, astronomical imaging, and communication. With recent advances in quantum optics, wavefront correction has become a crucial tool in quantum imaging, quantum communication, and efficient photon coupling. Consequently, understanding the performance of optimization algorithms under low-photon conditions is essential for the effective deployment of quantum optical systems. This study investigates the performance of two algorithms in the photon-counting regime across varying mean photon rates through experiments and numerical simulations. Furthermore, we propose, simulate, and implement a novel, to the best of our knowledge, augmented algorithm that combines the strengths of both methods and is particularly well suited for quantum applications.

长期以来,基于反馈优化的波前操作和校正一直应用于光学应用,如显微镜、光学传感、天文成像和通信。随着量子光学的发展,波前校正已成为量子成像、量子通信和高效光子耦合的重要工具。因此,了解低光子条件下优化算法的性能对于量子光学系统的有效部署至关重要。本研究通过实验和数值模拟研究了两种算法在不同平均光子速率下的光子计数性能。此外,据我们所知,我们提出,模拟和实现了一种新颖的增强算法,该算法结合了两种方法的优势,特别适合量子应用。
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引用次数: 0
Optical crosstalk reduction of InGaN micro-LED array based on a reflective wall design for display applications. 显示应用中基于反射壁设计的InGaN微型led阵列光串扰减少。
IF 3.3 2区 物理与天体物理 Q2 OPTICS Pub Date : 2026-01-15 DOI: 10.1364/OL.582861
Junyuan Chen, Zhou Wang, Yijing Lin, Shiting Dou, Haoxiang Zhu, Yuhang Dai, Siqi Yang, Ting Zhi, Jin Wang, Lei Wang, Qiang Chen, Yan Gu, Xiaoyan Liu

Optical crosstalk plays a key role in degrading the color accuracy and contrast of GaN-based micro-light emitting diodes (micro-LEDs) in display applications, and a comprehensive solution to this issue remains elusive. In this Letter, we propose a micro-LED array structure featuring individual pixels surrounded by a circular wall deposited with silver (Ag) as a reflective medium, and the effect of crosstalk reduction is well demonstrated. Compared to the conventional micro-LED devices, the luminous intensity distribution mapping indicated that the proposed micro-LED structure achieves a significant light spot reduction under the injection current of about 0.5 mA, and a low-crosstalk display is achieved through a 16 × 16 array. Furthermore, the optical field distribution of the proposed micro-LED structure was studied based on finite-difference time-domain (FDTD) simulation. The results reveal that when the height and gap width of the reflective wall are 5 µm respectively, more than 55% of the light emission is effectively limited within the ±45 divergence angle. This work presents a promising solution for mitigating optical crosstalk in micro-LED displays, thereby enhancing their performance for high-quality display applications.

在显示应用中,光串扰是降低gan基微发光二极管(micro- led)色彩精度和对比度的关键因素,目前还没有一个全面的解决方案。在这篇论文中,我们提出了一种微型led阵列结构,其特征是单个像素被沉积银(Ag)作为反射介质的圆形壁包围,并且很好地证明了串扰减少的效果。与传统的微型led器件相比,发光强度分布图表明,在注入电流约0.5 mA的情况下,所提出的微型led结构实现了明显的光斑减少,并且通过16 × 16阵列实现了低串扰显示。此外,基于时域有限差分(FDTD)仿真研究了该微型led结构的光场分布。结果表明,当反射壁高度和缝隙宽度分别为5µm时,55%以上的光发射被有效地限制在±45°发散角范围内。这项工作提出了一种有前途的解决方案,可以减轻微型led显示器中的光串扰,从而提高其在高质量显示应用中的性能。
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引用次数: 0
Quasi-periodic vector optical field and its application in information encoding and transmission. 准周期矢量光场及其在信息编码和传输中的应用。
IF 3.3 2区 物理与天体物理 Q2 OPTICS Pub Date : 2026-01-15 DOI: 10.1364/OL.582891
Xu-Zhen Gao, Xue-Feng Sun, Yue Pan

Quasi-periodicity has numerous applications in various fields, such as the discovery and study of quasicrystals. In the region of manipulating vector optical fields (VOFs), the periodicity is very common, but the quasi-periodicity is rarely seen. Here, we propose a kind of two-dimensional quasi-periodic VOF, introducing the concept of quasi-periodicity into the region of manipulating VOFs. We then study the optical information encoding and transmission. It is demonstrated that the information can be accurately recovered even when up to 75% of the spectrum is obstructed by sector-shaped obstacle. The information remains highly robust under random interference affecting 90% of the wave front during propagation. This work demonstrates the convolution-based construction scheme of the quasi-periodic VOF, along with the explicit information-encoding protocol and experimental demonstration. The quasi-periodic VOF opens an avenue for robust optical information transmission over long-distances.

准周期性在许多领域都有广泛的应用,例如准晶体的发现和研究。在操纵矢量光场(VOFs)区域,周期性是很常见的,但准周期性很少见到。本文提出了一种二维准周期VOF,将准周期的概念引入到操纵VOF的领域。然后研究了光信息的编码和传输。结果表明,即使在高达75%的频谱被扇形障碍物阻挡的情况下,也能准确地恢复信息。在传播过程中,在影响90%波前的随机干扰下,该信息仍然具有很高的鲁棒性。本文提出了基于卷积的准周期VOF构造方案,并给出了明确的信息编码协议和实验演示。准周期VOF为鲁棒长距离光信息传输开辟了新的途径。
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引用次数: 0
Direct observation of the (de)lithiation process on the multi-particle LiFePO4 by in situ TEM 原位透射电镜直接观察多粒子LiFePO4的(脱)锂化过程
IF 4 2区 物理与天体物理 Q2 PHYSICS, APPLIED Pub Date : 2026-01-15 DOI: 10.1063/5.0308406
Weikang Dong, Ze Hua, Xiaoxue Chang, Lixia Bao, Ruiwen Shao, Jiafang Li
The development of nanostructured LiFePO4 (LFP) electrodes represents a prominent research direction in the Li-ion battery field, owing to its intrinsic advantages such as high theoretical capacity and excellent structural stability. Studying the electrochemical reaction mechanisms at the atomic scale by in situ TEM is essential; however, the mechanisms of ion migration on LFP have not yet been fully elucidated. We report atomic-scale in situ TEM studies of delithiation and lithiation in multi-particle LFP coupled to a Li-rich garnet (LLZNO) solid electrolyte. During delithiation, LFP converts to a metastable L0.5FP via a periodicity-doubling mechanism (every second layer) accompanied by the emergence of a solid-solution zone, and we directly observe interparticle Li+ transport that drives reversible LFP–L0.5FP–LFP cycles. Conversely, under reductive bias, lithiation proceeds by an interface-dominated crystalline–amorphous transformation, identifying amorphization as a primary particle-level failure pathway. Tracking the structural evolution of LiFePO4 at the atomic scale during (de)lithiation provides key insights into its kinetic limitations and phase stability, which is essential for optimizing its electrochemical performance.
纳米结构LiFePO4 (LFP)电极由于具有较高的理论容量和优异的结构稳定性等固有优势,是锂离子电池领域一个突出的研究方向。在原子尺度上用原位透射电镜研究电化学反应机理是必要的;然而,离子在LFP上的迁移机制尚未完全阐明。我们报道了与富锂石榴石(LLZNO)固体电解质耦合的多粒子LFP的原子尺度原位透射电镜研究。在衰减过程中,LFP通过周期性加倍机制(每隔第二层)转变为亚稳态L0.5FP,并伴有固溶区的出现,我们直接观察到粒子间Li+输运驱动可逆LFP - L0.5FP - LFP循环。相反,在还原性偏压下,锂化通过界面主导的结晶-非晶转变进行,将非晶化确定为主要的颗粒级失效途径。在原子尺度上跟踪LiFePO4在(去)锂化过程中的结构演变,可以深入了解其动力学限制和相稳定性,这对优化其电化学性能至关重要。
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引用次数: 0
Nuclear Data Sheets for A=69 A=69的核数据表
IF 2.7 1区 物理与天体物理 Q2 PHYSICS, NUCLEAR Pub Date : 2026-01-15 DOI: 10.1016/j.nds.2025.12.001
C.D. Nesaraja
Experimental data on ground- and excited-state properties for all known nuclei with mass number A=69 have been compiled and evaluated. States populated in radioactive decay, as well as in nuclear reactions, have been considered. For these nuclei, level and decay schemes, as well as tables of nuclear properties, are given in detail. This work supersedes the 2013 evaluation by C.D. Nesaraja (2014Ne01).
对所有已知质量数为A=69的原子核的基态和激发态性质的实验数据进行了汇编和评价。已经考虑了放射性衰变和核反应中人口稠密的国家。对于这些原子核,详细地给出了能级表和衰变表,以及核性质表。这项工作取代了2013年C.D. Nesaraja (2014Ne01)的评估。
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引用次数: 0
How Dark is Dark Energy? A Lightcones Comparison Approach 暗能量有多暗?lightcone比较方法
IF 2.8 4区 物理与天体物理 Q2 ASTRONOMY & ASTROPHYSICS Pub Date : 2026-01-15 DOI: 10.1007/s10714-025-03506-x
Mauro Carfora, Francesca Familiari

We present a detailed analysis that may significantly impact understanding the relationship between structure formation in the late-epoch Universe and dark energy as described by the Friedmann-Lemaître-Robertson-Walker (FLRW) cosmological constant density ({{widehat{Omega }}_Lambda }). Our geometrical approach provides a non-perturbative technique that allows the standard FLRW observer to evaluate a measurable, scale-dependent distance functional between her idealized FLRW past light cone and the actual physical past light cone. From the point of view of the FLRW observer, gathering data from sources at cosmological redshift ({widehat{z}}), this functional generates a geometry-structure-growth contribution ({Omega _Lambda ({widehat{z}})}) to ({{widehat{Omega }}_Lambda }). This redshift-dependent contribution erodes the interpretation of ({{widehat{Omega }}_Lambda }) as representing constant dark energy. In particular, ({Omega _Lambda ({widehat{z}})}) becomes significantly large at very low ({widehat{z}}), where structures dominate the cosmological landscape. At the pivotal galaxy cluster scale, where cosmological expansion decouples from the local gravitation dynamics, we get ({Omega _Lambda ({widehat{z}})/{widehat{Omega }}_Lambda },=,O(1)), showing that late-epoch structures provide an effective field contribution to the FLRW cosmological constant that is of the same order of magnitude of its assumed value. We prove that ({Omega _Lambda ({widehat{z}})}) is generated by a scale-dependent effective field governed by structures formation and related to the comparison between the idealized FLRW past light cone and the actual physical past light cone. These results are naturally framed in mainstream FLRW cosmology; they do not require the existence of exotic fields and provide a natural setting for analyzing the coincidence problem, leading to an interpretative shift in the current interpretation of constant dark energy.

我们提出了一个详细的分析,可能会显著影响理解晚期宇宙结构形成与暗能量之间的关系,由弗里德曼-莱马 (FLRW)宇宙常数密度({{widehat{Omega }}_Lambda })描述。我们的几何方法提供了一种非扰动技术,使标准FLRW观察者能够评估其理想FLRW过去光锥与实际物理过去光锥之间可测量的、依赖于尺度的距离函数。从FLRW观测者的角度来看,从宇宙学红移({widehat{z}})的来源收集数据,这个函数产生了一个几何结构增长贡献({Omega _Lambda ({widehat{z}})})到({{widehat{Omega }}_Lambda })。这种与红移相关的贡献削弱了({{widehat{Omega }}_Lambda })代表恒定暗能量的解释。特别是,({Omega _Lambda ({widehat{z}})})在非常低的({widehat{z}})处变得非常大,在那里结构主导着宇宙景观。在关键星系团尺度上,宇宙学膨胀与局部引力动力学解耦,我们得到({Omega _Lambda ({widehat{z}})/{widehat{Omega }}_Lambda },=,O(1)),表明晚期结构为FLRW宇宙学常数提供了有效的场贡献,其值与假设值相同数量级。我们证明({Omega _Lambda ({widehat{z}})})是由结构形成支配的尺度相关有效场产生的,并且与理想的FLRW过去光锥与实际物理过去光锥的比较有关。这些结果自然是主流FLRW宇宙学的框架;它们不需要奇异场的存在,并为分析巧合问题提供了一个自然的环境,导致了当前对恒定暗能量解释的解释转变。
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引用次数: 0
Study on a rapid measurement method for the deposition velocity of 220Rn progeny based on an imaging plate 基于成像板的220Rn子代沉积速度快速测量方法研究
IF 2.2 3区 物理与天体物理 Q2 NUCLEAR SCIENCE & TECHNOLOGY Pub Date : 2026-01-15 DOI: 10.1016/j.radmeas.2026.107620
Yufan Liu, Kexin Wang, Wenjie Xu, Jialu Feng, Tao Ao, Lidan Lv, Qingzhi Zhou, Zhengzhong He
The study of the deposition behavior of 220Rn progeny is crucial for the assessment of public and occupational radiation doses and for controlling progeny concentration in a thoron chamber. To address the difficulty of maintaining stable environmental conditions over long durations when studying deposition velocity variations, a rapid and accurate method for the deposition velocity measurement of 220Rn progeny is proposed in this study, based on a BAS-TR imaging plate (IP), which has advantages of high sensitivity, large detection area and portability. In this research, measurement procedures were optimized based on the analysis of uncertainty, whereby the total time for a single measurement can be limited within 8 h. A dedicated Python program was developed for the automatic processing of IP count data, and key parameters such as IP detection efficiency, IP scanner sensitivity, and IP fading correction were determined through experiments. Comparative experiment was conducted between IP and a calibrated alpha spectroscopy, with results showing good agreement between two method. This method was preliminarily applied on 220Rn progeny deposition velocity measurement using collection plates of different sizes. Compared to traditional techniques, multi-sample, large-area measurements of deposition velocity can be completed within 8 hours using the proposed method, thereby providing an new efficient approach for the study of the deposition of 220Rn progeny and other radionuclides.
研究220Rn子体的沉积行为对于评估公众和职业辐射剂量以及控制钍室子体浓度至关重要。针对研究沉积速度变化时难以长时间保持稳定环境条件的问题,本研究提出了一种基于BAS-TR成像板(IP)的220Rn子代沉积速度快速准确测量方法,该方法具有灵敏度高、检测面积大、便携性好等优点。本研究在不确定度分析的基础上对测量程序进行了优化,将单次测量的总时间控制在8 h以内。开发了专用Python程序对IP计数数据进行自动处理,并通过实验确定了IP检测效率、IP扫描器灵敏度、IP衰落校正等关键参数。将IP法与标定后的α光谱法进行了对比实验,结果表明两者吻合较好。该方法初步应用于不同尺寸采集板的220Rn子代沉积速度测量。与传统方法相比,该方法可在8小时内完成多样品、大面积的沉积速度测量,为研究220Rn子代及其他放射性核素的沉积提供了一种新的高效方法。
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引用次数: 0
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