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Re-identifying farmland carbon neutrality gap under a new carbon counting and the framework of regional interactions in China. 在新的碳计数和中国区域互动框架下重新识别农田碳中和差距。
IF 8.2 1区 环境科学与生态学 Q1 ENVIRONMENTAL SCIENCES Pub Date : 2024-11-20 Epub Date: 2024-09-02 DOI: 10.1016/j.scitotenv.2024.175996
Jiqun Wen, Xiaowei Chuai, Ai Xiang, Yonghua Liu, Tong Wang, Yuting Luo, Lijuan Miao, Libao Zhang, Jianbao Li, Rongqin Zhao

The farmland ecosystem, with its numerous material cycles and energy flows, is an important part of the carbon cycle in terrestrial ecosystems. Focusing on the carbon neutrality of farmland is meaningful for mitigating global warming and serving national low-carbon strategies. This study enriches the carbon accounting items of farmland and establishes a new research framework to check the carbon neutrality of farmland from the aspect of regional interactions and, subsequently, the inequality among China's provinces. The results revealed that there is still a great gap in the capability of China's farmland to reach carbon neutrality, with a gap value of up to 10,503 × 104 t C. All of the provinces presented net carbon emissions, and the per unit area carbon neutrality gaps showed spatial regularity decreasing from the coastal regions to the inland areas. Anthropogenic carbon emissions on farmland played a dominant role compared with soil organic carbon. Five provinces had reduced interior-regional carbon emissions through grain trade, and the amounts were especially high for developed regions, such as Guangdong, Zhejiang, Beijing, Shanghai and Jiangsu. Sixteen provinces gained external carbon emissions through trade; these were the less developed regions located mainly in the north, such as Inner Mongolia, Hebei, Jilin, Heilongjiang and Xinjiang. Under regional inequality, 15 provinces added to the net amount of the carbon emissions generated in external regions, with China's megacities adding the highest percentage, especially Beijing, with 389.95 % compared with its original emissions. Inequality showed that most provinces had a moderate status. Sichuan and Hunan experienced weak advantages, and six provinces had disadvantages. Therefore, constructing compensation and trade-based rights and responsibilities traceability mechanisms is important.

农田生态系统具有众多的物质循环和能量流动,是陆地生态系统碳循环的重要组成部分。关注农田的碳中和问题,对于减缓全球变暖、服务国家低碳战略具有重要意义。本研究丰富了耕地碳核算项目,并建立了一个新的研究框架,从区域互动的角度来检验耕地碳中性,进而检验中国各省之间的不平等。结果表明,我国耕地碳中和能力仍存在较大差距,差距值高达 10,503×104 t C,所有省份均呈现碳净排放,单位面积碳中和差距呈现从沿海地区向内陆地区递减的空间规律性。与土壤有机碳相比,农田人为碳排放占主导地位。有 5 个省份通过粮食贸易减少了内陆地区的碳排放,尤其是广东、浙江、北京、上海和江苏等发达地区。有 16 个省份通过贸易增加了外部碳排放,这些省份主要位于北方欠发达地区,如内蒙古、河北、吉林、黑龙江和新疆。在地区不平等条件下,15 个省份增加了外部地区产生的净碳排放量,其中中国特大城市增加的比例最高,尤其是北京,与原始排放量相比增加了 389.95%。从不平等性来看,大多数省份处于中等水平。四川和湖南的优势较弱,6 个省份处于劣势。因此,构建基于补偿和贸易的权责追溯机制十分重要。
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引用次数: 0
A new perspective of sediment layering scour and migration under the coupled effects of particle distribution and bio-viscosity-cavitation erosion. 在颗粒分布和生物粘度-凹陷侵蚀的耦合效应下,沉积物分层冲刷和迁移的新视角。
IF 8.2 1区 环境科学与生态学 Q1 ENVIRONMENTAL SCIENCES Pub Date : 2024-11-20 Epub Date: 2024-09-01 DOI: 10.1016/j.scitotenv.2024.175929
Xuan Shi, Jin Zhang, Qize Wang, Kai Wang, Jianshuang Han, Yilian Hui, Xin Jin, Pengkang Jin

The scouring and migration of sediments in sewer systems are the key contributors to overflow pollution. Both physical and biological factors affect the erosion and migration of layered sediments. However, the functional characteristics of these factors and their quantification process still need to be further explored. In this study, the physical form and biological metabolism of the sediment are coupled, and the suspension mechanism under the dual action is proposed systematically and deeply. The influence coefficient of scour initiation was redefined as A^/prime, where the physical factors were particle size and mass, and the biological factors were bio-viscosity and internal cavitation. The bio-viscosity of layered sediment particles is provided by Extracellular Polymeric Substances (EPS). The slope value of |ΔD/-Δf| (ΔD: Dissipation; Δf: frequency) of surface EPS decreased from 0.489 to 0.315 when Quartz Crystal Microbalance with Dissipation (QCM-D) was used to analyse EPS viscosity, indicating that biological activities formed a dense biofilm on the sediment surface and enhanced the bond between particles. Meanwhile, by monitoring the accumulation density of sediments at different depths, it was found that the packing density of the bottom layer decreased from 1.50 to 1.45 g/cm3, which was mainly due to the internal cavitation caused by microorganism consuming organic matrix and releasing H2S and CH4. The delamination difference of EPS results in the uneven change of adhesion between different layers. This, combined with the internal erosion characteristics triggered by microbial stratified metabolism, collectively constitutes the biological effects on the sediment structure. Finally, the coupling mechanism of particle distribution and bio-viscous-cavitation erosion was formed, and the correctness of the formula was verified by repeated experiments, which proved the agreement between the theory and the practice and provided a scientific method for systematically analysing the erosion and migration law of sediment in the sewer system.

下水道系统中沉积物的冲刷和迁移是造成溢流污染的主要原因。物理和生物因素都会影响分层沉积物的冲刷和迁移。然而,这些因素的功能特征及其量化过程仍有待进一步探索。本研究将沉积物的物理形态与生物代谢耦合,系统深入地提出了双重作用下的悬浮机理。将冲刷起始的影响系数重新定义为 A^/prime,其中物理因子为粒径和质量,生物因子为生物粘度和内部空化。层状沉积物颗粒的生物粘度由细胞外高分子物质(EPS)提供。使用石英晶体微天平(QCM-D)分析 EPS 粘度时,表面 EPS 的斜率值 |ΔD/-Δf|(ΔD:耗散;Δf:频率)从 0.489 降至 0.315,表明生物活动在沉积物表面形成了致密的生物膜,增强了颗粒之间的粘结力。同时,通过监测不同深度沉积物的堆积密度,发现底层堆积密度从 1.50 g/cm3 降至 1.45 g/cm3,这主要是由于微生物消耗有机基质并释放出 H2S 和 CH4 而引起的内部空化。EPS 的分层差异导致不同层之间粘附力的不均匀变化。这与微生物分层代谢引发的内部侵蚀特征共同构成了对沉积物结构的生物效应。最后,形成了颗粒分布与生物-粘性-空穴侵蚀的耦合机理,并通过反复实验验证了公式的正确性,证明了理论与实践的一致性,为系统分析下水道系统中泥沙的侵蚀与迁移规律提供了科学方法。
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引用次数: 0
The heat-mortality association in Jordan: Effect modification by greenness, population density and urbanization level. 约旦高温与死亡率的关系:绿化、人口密度和城市化水平的影响。
IF 8.2 1区 环境科学与生态学 Q1 ENVIRONMENTAL SCIENCES Pub Date : 2024-11-20 Epub Date: 2024-09-02 DOI: 10.1016/j.scitotenv.2024.176010
L Luque-García, S Bataineh, J Al-Bakri, F A Abdulla, W K Al-Delaimy

Background: The Middle East is one of the most vulnerable regions to the impacts of climate change, yet evidence of the heat-related mortality remains limited in this area. Our present study investigated the heat-mortality association in Jordan and the potential modifying effect of greenness, population density and urbanization level on the association.

Methods: For each of the 42 included districts, daily meteorological and mortality data from 2000 to 2020 were obtained for the warmest months (May to September). First, a distributed lag non-linear model was applied to estimate the district level heat-mortality association, then the district specific estimates were pooled using multivariate meta-regression models to obtain an overall estimate. Last, the modifying effect of district level greenness, population density and urbanization level was examined through subgroup analysis.

Results: When compared to the minimum mortality temperature (MMT, percentile 0th, 22.20 °C), the 99th temperature percentile exhibited a relative risk (RR) of 1.34 (95 % CI 1.23, 1.45). Districts with low greenness had a higher heat-mortality risk (RR 1.39, 95 % CI 1.22, 1.58) when compared to the high greenness (RR 1.28, 95 % CI 1.13, 1.45). While heat-mortality risk did not significantly differ between population density subgroups, highly urbanized districts had a greater heat-mortality risk (RR 1.41, 95 % CI 1.23, 1.62) as compared to ones with low levels of urbanization (RR 1.32, 95 % CI 1.13, 1.55). Districts with high urbanization level had the highest heat-mortality risk if they were further categorized as having low greenness (RR 1.63, 95 % CI 1.30, 2.04).

Conclusion: Exposure to heat was associated with increased mortality risk in Jordan. This risk was higher in districts with low greenness and high urbanization level. As climate change-related heat mortality will be on the rise, early warning systems in highly vulnerable communities in Jordan are required and greening initiatives should be pursued.

背景:中东是最易受气候变化影响的地区之一,但该地区与高温相关的死亡率证据仍然有限。本研究调查了约旦高温与死亡率的关系,以及绿化、人口密度和城市化水平对这种关系的潜在调节作用:方法:我们获取了约旦 42 个地区从 2000 年至 2020 年最热月份(5 月至 9 月)的每日气象数据和死亡率数据。首先,应用分布式滞后非线性模型估算地区层面的高温与死亡率的关联,然后使用多元元回归模型将地区的具体估算值汇总,得出总体估算值。最后,通过分组分析研究了地区绿化程度、人口密度和城市化水平的调节作用:与最低死亡温度(MMT,百分位数第 0 位,22.20 °C)相比,温度百分位数第 99 位的相对风险(RR)为 1.34(95 % CI 1.23,1.45)。与高绿化率地区相比,低绿化率地区的高温致死风险更高(RR 1.39,95 % CI 1.22,1.58)(RR 1.28,95 % CI 1.13,1.45)。虽然不同人口密度分组的高温致死风险没有显著差异,但高度城市化地区的高温致死风险(RR 1.41,95 % CI 1.23,1.62)高于低度城市化地区(RR 1.32,95 % CI 1.13,1.55)。如果将城市化水平高的地区进一步归类为绿化程度低的地区,则这些地区的高温致死风险最高(RR 1.63,95 % CI 1.30,2.04):在约旦,暴露于高温与死亡风险增加有关。这一风险在绿化程度低和城市化水平高的地区更高。由于与气候变化相关的高温死亡率将呈上升趋势,因此需要在约旦高度脆弱的社区建立早期预警系统,并采取绿化措施。
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引用次数: 0
Discarded fishing net pollution in coastal areas of Bangladesh. 孟加拉国沿海地区的废弃渔网污染。
IF 8.2 1区 环境科学与生态学 Q1 ENVIRONMENTAL SCIENCES Pub Date : 2024-11-20 Epub Date: 2024-08-21 DOI: 10.1016/j.scitotenv.2024.175529
Gawsia Wahidunnessa Chowdhury, Heather J Koldewey, Md Nazmul Hasan Niloy, Mohammad Mizanur Rahman Khan, Nabanita Das, Surshti Patel, Bushra Nishat, Zoie T Diana, Nina Tsydenova, Subrata Sarker

Discarded fishing nets, a major source of marine litter, significantly threaten the marine environment and contribute to plastic pollution due to the synthetic polymers they contain. Though Bangladesh is a maritime country with 0.5 million of fishers dependent on coastal and marine fishing, there have been no studies to date on the plastic pollution impact of fishing nets. This study demonstrates the fishing nets associated with marine litter in two coastal locations of Bangladesh, Charfesson and Cox's Bazar. Fishing net samples were collected from local net shops and semi-structured interviews were taken of the shop owners to gather information about available fishing nets. This was complemented by photo-quadrat surveys to document waste fishing net materials on the shore in both locations. Among the 17 net samples, there were 12 types of gill nets, which showed a wide range of variation in price, material types, and longevity. Through the FTIR analysis, we identified the presence of Nylon 6, Polyethylene, Polyvinyl chloride, Polypropylene and Polyethylene terephthalate in the collected fishing net samples. Photoquadrat surveys found that fishing nets are related to plastic pollution in coastal areas. This study addressed the knowledge gap regarding the diversity and chemical characteristics of fishing nets and the resulting litter in Bangladesh.

废弃渔网是海洋垃圾的主要来源,由于含有合成聚合物,严重威胁海洋环境并造成塑料污染。虽然孟加拉国是一个海洋国家,有 50 万渔民依靠沿海和海洋捕鱼为生,但迄今为止还没有关于渔网对塑料污染影响的研究。本研究展示了孟加拉国两个沿海地区(查尔费松和考克斯巴扎尔)与海洋垃圾有关的渔网。研究人员从当地的渔网店收集了渔网样本,并对店主进行了半结构式访谈,以收集有关现有渔网的信息。此外,还进行了照相四分法调查,以记录两地海岸上的废弃渔网材料。在 17 个渔网样本中,有 12 种刺网,它们在价格、材料类型和使用寿命方面差异很大。通过傅立叶变换红外光谱分析,我们确定所采集的渔网样本中含有尼龙 6、聚乙烯、聚氯乙烯、聚丙烯和聚对苯二甲酸乙二醇酯。照相地形图调查发现**沿海地区存在与渔网有关的塑料污染。这项研究填补了孟加拉国在渔网的多样性和化学特性以及由此产生的垃圾方面的知识空白。
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引用次数: 0
Characterizing nitrogen deposited on urban road surfaces: Implication for stormwater runoff pollution control. 城市路面沉积氮的特征:对雨水径流污染控制的影响。
IF 8.2 1区 环境科学与生态学 Q1 ENVIRONMENTAL SCIENCES Pub Date : 2024-11-20 Epub Date: 2024-08-22 DOI: 10.1016/j.scitotenv.2024.175692
Zilin Yang, Yushan Chen, Jiawei Dong, Nian Hong, Qian Tan

Nitrogen (N) is one of the most important pollutants on urban road surfaces. Understanding the N deposition forms, load characteristics, and influential factors can help to provide management and control strategies for road stormwater runoff pollution. This study focuses on a highly urbanized area in Guangzhou, China, and presents the characteristics of both dissolved and particulate N deposition forms as well as their correlations with land-use types and traffic factors. In addition, an artificial neural network (ANN) based classification model is utilized to estimate N pollution hotspot area and total nitrogen (TN) flux from road to receiving water bodies. The results showed that N on urban road surfaces mainly existed in the form of particulate organic nitrogen. Land use types dominated by residential area (RA) and urban village (UV) have higher TN build-up loads. Geodetector analysis indicated that land use has a greater impact on nitrogen build-up loads than traffic factors. Through classification and estimation using the ANN model, RA, and UV were classified as hotspot areas, and the TN flux from roads in the study area was calculated to be 3.35 × 105 g. Furthermore, it was estimated that the annual TN flux from roads in Guangzhou accounts for 19 % of the city's total urban domestic discharge. These findings are expected to contribute to the pollution control of stormwater runoff from urban road surfaces and provide valuable guidance for enhancing the ecological health of urban water environments.

氮(N)是城市道路表面最重要的污染物之一。了解氮的沉积形式、负荷特征和影响因素,有助于为道路雨水径流污染提供管理和控制策略。本研究以中国广州的一个高度城市化地区为研究对象,介绍了溶解氮和颗粒氮沉积形式的特征及其与土地利用类型和交通因素的相关性。此外,还利用基于人工神经网络(ANN)的分类模型估算了氮污染热点区域以及从道路到受纳水体的总氮(TN)通量。结果表明,城市道路路面上的氮主要以颗粒有机氮的形式存在。以住宅区(RA)和城中村(UV)为主的土地利用类型具有较高的 TN 累积负荷。地质探测器分析表明,土地利用对氮累积负荷的影响大于交通因素。通过使用 ANN 模型进行分类和估算,将 RA 和 UV 划分为热点区域,并计算出研究区域内来自道路的 TN 通量为 3.35 × 105 g。此外,据估计,广州市每年来自道路的 TN 通量占全市城市生活污水排放总量的 19%。这些研究结果有望为城市道路路面雨水径流的污染控制作出贡献,并为提高城市水环境的生态健康水平提供有价值的指导。
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引用次数: 0
Combined effects of polyamide microplastic and sulfamethoxazole in modulating the growth and transcriptome profile of hydroponically grown rice (Oryza sativa L.). 聚酰胺微塑料和磺胺甲噁唑在调节水培水稻(Oryza sativa L.)的生长和转录组特征方面的联合效应。
IF 8.2 1区 环境科学与生态学 Q1 ENVIRONMENTAL SCIENCES Pub Date : 2024-11-20 Epub Date: 2024-09-02 DOI: 10.1016/j.scitotenv.2024.175909
Raza Ullah, Julia Farias, Biruk A Feyissa, Martin Tsz-Ki Tsui, Alex Chow, Clinton Williams, Tanju Karanfil, Ayalew Ligaba-Osena

The use of reclaimed water from wastewater treatment plants for irrigation has a risk of introducing micropollutants such as microplastics (MPs) and antimicrobials (AMs) into the agroecosystem. This study was conducted to investigate the effects of single and combined treatment of 0.1 % polyamide (PA ∼15 μm), and varying sulfamethoxazole (SMX) levels 0, 10, 50, and 150 mg/L on rice seedlings (Oryza sativa L.) for 12 days. The study aimed to assess the impact of these contaminants on the morphological, physiological, and biochemical parameters of the rice plants. The findings revealed that rice seedlings were not sensitive to PA alone. However, SMX alone or in combination with PA, significantly inhibited shoot and root growth, total biomass, and affected photosynthetic pigments. Higher concentrations of SMX increased antioxidant enzyme activity, indicating oxidative stress. The roots had a higher SMX content than the shoots, and the concentration of minerals such as iron, copper, and magnesium were reduced in roots treated with SMX. RNA-seq analysis showed changes in the expression of genes related to stress, metabolism, and transport in response to the micropollutants. Overall, this study provides valuable insights on the combined impacts of MPs and AMs on food crops, the environment, and human health in future risk assessments and management strategies in using reclaimed water.

使用污水处理厂的再生水进行灌溉有可能将微塑料 (MP) 和抗菌素 (AM) 等微污染物带入农业生态系统。本研究调查了 0.1 % 聚酰胺(PA ~15 μm)和不同浓度的磺胺甲噁唑(SMX)(0、10、50 和 150 mg/L)对水稻秧苗(Oryza sativa L.)的影响,处理时间为 12 天。研究旨在评估这些污染物对水稻植株形态、生理和生化参数的影响。研究结果表明,水稻秧苗对单独的 PA 并不敏感。然而,单独使用或与 PA 合用 SMX 会明显抑制芽和根的生长、总生物量,并影响光合色素。较高浓度的 SMX 会增加抗氧化酶的活性,表明存在氧化应激。根部的 SMX 含量高于芽部,用 SMX 处理的根部铁、铜和镁等矿物质浓度降低。RNA-seq 分析表明,与压力、新陈代谢和运输相关的基因表达在微污染物的作用下发生了变化。总之,这项研究为未来使用再生水的风险评估和管理策略提供了关于MPs和AMs对粮食作物、环境和人类健康的综合影响的宝贵见解。
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引用次数: 0
Assessing impact of elevated CO2 on heavy metal accumulation in crops: meta-analysis and implications for food security. 评估高浓度 CO2 对作物重金属积累的影响:荟萃分析及对粮食安全的影响。
IF 8.2 1区 环境科学与生态学 Q1 ENVIRONMENTAL SCIENCES Pub Date : 2024-11-20 Epub Date: 2024-09-01 DOI: 10.1016/j.scitotenv.2024.175949
Xunzhe Yang, Ping Yun, Xiaoxiang Zhao, Zhe Zhang, Chen Chen, Yonghong Zhou, Yinglong Chen, Haiqin Zhang, Sergey Shabala

Human activities led to elevation in carbon dioxide (CO2) concentrations in atmosphere. While such increase per se may be beneficial for the growth of some crops, it comes with a caveat of affecting crop nutritional status. Here, we present a comprehensive analysis of changes in concentration of essential (Cu, Fe, Mn, Zn, Mo, Ni) and non-essential (Ba, Cd, Cr, Hg, Pb, and Sr) heavy metals in response to elevated CO2, drawing on a meta-analysis of 1216 paired observations. The major findings are as follows: (1) Elevated CO2 leads to reduced concentrations of Cu, Fe, Mn, and Zn in crops; (2) the extent of above reduction varies among plants species and is most pronounced in cereals and then in legumes and vegetables; (3) reduction in accumulation of non-essential (toxic) metals is less pronounced, potentially leading to an unfavorable essential/non-essential metal ratio in plants; (4) the above effects will come with significant implication to human health, exacerbating effects of the "hidden hunger" caused by the lack of Fe and Zn in the human diets. The paper also analyses the mechanistic basis of nutrient acquisition (both at physiological and molecular levels) and calls for the changes in the governmental policies to increase efforts of plant breeders to create genotypes with improved nutrient use efficiency for essential micronutrients while uncoupling their transport from non-essential (toxic) heavy metals.

人类活动导致大气中二氧化碳(CO2)浓度升高。虽然这种增加本身可能有利于某些农作物的生长,但也有可能影响农作物的营养状况。在此,我们通过对 1216 项配对观测数据进行荟萃分析,全面分析了二氧化碳升高对必需重金属(铜、铁、锰、锌、钼、镍)和非必需重金属(钡、镉、铬、汞、铅和锶)浓度变化的影响。主要发现如下(1) 二氧化碳升高导致作物中铜、铁、锰和锌的浓度降低;(2) 上述降低的程度因植物种类而异,谷类最为明显,豆类和蔬菜次之;(3) 非必需(有毒)金属的积累减少不那么明显,可能导致植物中必需/非必需金属比例失衡;(4) 上述影响将对人类健康产生重大影响,加剧因人类饮食中缺乏铁和锌而造成的 "隐性饥饿"。本文还分析了养分获取的机理基础(生理和分子水平),并呼吁政府改变政策,加大植物育种者的工作力度,创造出能提高必需微量元素养分利用效率的基因型,同时将其与非必需(有毒)重金属的运输分离开来。
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引用次数: 0
Contamination of toxic elements in the sediments, water, and igneous rocks of the Sefid-rud River in Northern Iran using contamination indicators, with a specific focus on Ti-rich coastal sediments. 利用污染指标研究伊朗北部塞菲德鲁德河沉积物、水和火成岩中有毒元素的污染情况,特别关注富含钛的沿岸沉积物。
IF 8.2 1区 环境科学与生态学 Q1 ENVIRONMENTAL SCIENCES Pub Date : 2024-11-20 Epub Date: 2024-09-01 DOI: 10.1016/j.scitotenv.2024.175790
Shahram Nakhaei, Mojgan Salavati, Ali Moghimi Kandelus

The Sefid-rud River is a significant river on the southern coast of the Caspian Sea in Iran. In this study, we collected 28 samples of surface sediments and water to assess the level of metal contamination. Chemical analysis revealed that the average concentrations of heavy metals in both sediments and water increase from upstream to downstream. There is no clear significant relationship observed between changes in the values of investigated elements in sediments and water. The levels of these elements in the sediments, exceed toxic response thresholds. In the water samples, As, Ni and V concentrations exceed the WHO standard values. According to the Igeo, EF and PLI indices, the sediments at most stations are not contaminated by any of the elements. The CF and Dc indices suggest low contamination levels at all stations. The NIPI and ecological risk indices (Er and RI) indicate non-polluted conditions at all stations except SF22, SF20, SF11, and SF6. The MI and HEI indices indicate pollution in all water samples of the Sefid-rud, but critical values are only observed at SF5 and SF15. The other stations show no contamination. The Cf index indicates high pollution levels for all elements except Cu, Zn, and Pb. The upstream area poses a relatively high and considerable ecological risk according to the PERI index. In conclusion, the sediments of the Sefid-rud River have a higher potential for the exchange of toxic substances compared to the aquatic environment.

Sefid-rud 河是伊朗里海南岸的一条重要河流。在这项研究中,我们采集了 28 份表层沉积物和水样,以评估金属污染程度。化学分析显示,沉积物和水中重金属的平均浓度从上游到下游都在增加。在沉积物和水中的调查元素值的变化之间没有观察到明显的重要关系。这些元素在沉积物中的含量超过了毒性反应阈值。在水样中,砷、镍和钒的浓度超过了世界卫生组织的标准值。根据 Igeo、EF 和 PLI 指数,大多数站点的沉积物没有受到任何元素的污染。CF 和 Dc 指数表明,所有站点的污染程度都较低。NIPI 和生态风险指数(Er 和 RI)表明,除 SF22、SF20、SF11 和 SF6 站外,所有站点均未受到污染。MI和 HEI 指数显示,Sefid-rud 的所有水样都受到了污染,但只有 SF5 和 SF15 出现了临界值。其他站点未发现污染。Cf 指数表明,除铜、锌和铅外,所有元素的污染程度都很高。根据 PERI 指数,上游地区具有相对较高的生态风险。总之,与水生环境相比,Sefid-rud 河的沉积物具有更高的有毒物质交换潜力。
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引用次数: 0
Saturation of intracellular phosphorus uptake and prevalence of extracellular phosphorus entrapment in fluvial biofilms after long-term P pulses: Implications for river self-purification. 长期磷脉冲后河道生物膜细胞内磷吸收饱和及细胞外磷截留的普遍性:对河流自净的影响。
IF 8.2 1区 环境科学与生态学 Q1 ENVIRONMENTAL SCIENCES Pub Date : 2024-11-20 Epub Date: 2024-09-04 DOI: 10.1016/j.scitotenv.2024.175976
Nuria Perujo, Lola Neuert, Patrick Fink, Markus Weitere

Microbial consortia in riverbed substrates and their extracellular matrix (biofilms) play a key role in phosphorus (P) entrapment. When P entrapment saturates, the benthic compartment changes from a P sink to a P source thus increasing eutrophication risk. P entrapment saturation is expected to differ between intracellular and extracellular P entrapment and between different magnitudes and durations of P inputs. We studied biofilm P-entrapment following short (48 h) and long (14 days) P loading events in stream bypass flumes supplied with a gradient of dissolved P concentrations. This allowed us to link local biofilm processes in sediments to potential effects on river self-purification, via quantifying the P removal efficiency in the flumes. We found that in short-term events, biofilms develop intracellular mechanisms to cope with P inputs, while long-term events and high P inputs suppress the intracellular uptake mechanisms and increase the prevalence of extracellular entrapment. Specifically, long-term events lowered the threshold for intracellular P entrapment saturation, and decreased the ratio between intracellular and extracellular entrapment resulting in lower removal efficiency for dissolved phosphorus. Our results highlight the risk that aquatic ecosystems may face as the ratio of intracellular to extracellular P entrapment decreases, which may reduce their ability to deal with P inputs, thereby increasing risks of eutrophication.

河床基质中的微生物群落及其胞外基质(生物膜)在磷(P)吸附中起着关键作用。当磷(P)吸附饱和时,底栖区块就会从磷汇变成磷源,从而增加富营养化的风险。细胞内和细胞外磷(P)的截留饱和度预计会有所不同,输入磷(P)的量级和持续时间也会不同。我们在溶解 P 浓度梯度的溪流旁路水槽中研究了短时间(48 小时)和长时间(14 天)P 负荷事件后的生物膜 P 诱导饱和度。这使我们能够通过量化水槽中的磷去除效率,将沉积物中的局部生物膜过程与对河流自净的潜在影响联系起来。我们发现,在短期事件中,生物膜发展出细胞内机制来应对 P 输入,而长期事件和高 P 输入则抑制了细胞内吸收机制,增加了细胞外截留的普遍性。具体而言,长期事件降低了细胞内磷捕获饱和的阈值,降低了细胞内和细胞外捕获的比例,从而降低了对溶解磷的去除效率。我们的研究结果突显了水生生态系统可能面临的风险,即随着细胞内与细胞外磷捕集比的降低,水生生态系统处理磷输入的能力可能会降低,从而增加富营养化的风险。
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引用次数: 0
How plastic litter sunk by biofouling recovers buoyancy - The role of benthic predation. 被生物污损沉没的塑料垃圾如何恢复浮力--底栖生物捕食的作用。
IF 8.2 1区 环境科学与生态学 Q1 ENVIRONMENTAL SCIENCES Pub Date : 2024-11-20 Epub Date: 2024-09-01 DOI: 10.1016/j.scitotenv.2024.175910
Javier Pinochet, Martin Thiel, Mauricio Urbina

Estimates suggest that the amount of plastic litter discarded in the ocean is several times greater than what remains floating at the sea surface, raising questions about the fate of this marine debris. Fouling-induced sinking of plastic litter is one of the proposed mechanisms responsible for this mass difference. While some of this 'missing' plastic mass may be explained by the effects of fouling, it has also been hypothesized that sinking litter may return to the surface after benthic organisms consume the biofouling. However, this hypothesis has never been tested. The present study evaluated the structure and biomass of the fouling community in response to benthic predation in both summer and winter seasons. Floating PVC plates were installed during winter and summer in central Chile (36°S) until the growing biofouling community caused them to sink. Plates were then moved to the seabed, where they were exposed to benthic predation, while control plates were maintained in a mesh cage impeding predator access. In summer, all plates recovered their buoyancy, while in the winter only 60 % recovered buoyancy. All caged control samples remained on the bottom in both seasons. The community structure differed both in the treatments and across the seasons, with plates that recovered buoyancy initially being dominated by Ulva sp. and Ciona robusta. Conversely, plates that did not refloat were mainly covered by species resistant to predation such as Pyura chilensis, Austromegabalanus psittacus, and Balanus laevis. Thus, fouling community structure influences how predation facilitates buoyancy recovery, because not all epibionts can be consumed by predators. While previous studies had shown how fouling organisms cause sinking of floating litter, this is the first study to provide experimental evidence that predation can reverse this process and allow litter to resurface and become again available as dispersal vectors for native and invasive species.

据估计,丢弃在海洋中的塑料垃圾数量是漂浮在海面上的塑料垃圾数量的数倍,这引发了人们对这些海洋废弃物命运的疑问。由污垢引起的塑料垃圾下沉是造成这种质量差异的拟议机制之一。虽然部分 "失踪 "的塑料垃圾可以用污垢的影响来解释,但也有人假设,下沉的垃圾可能会在底栖生物吞噬生物污垢后返回海面。不过,这一假设从未得到验证。本研究评估了夏季和冬季底栖生物捕食时污损群落的结构和生物量。在智利中部(南纬 36°)的冬季和夏季安装了浮动聚氯乙烯板,直到不断增长的生物污损群落导致其下沉。然后将浮板移至海底,使其暴露于底栖生物的捕食,而对照浮板则放在一个网笼中,阻止捕食者进入。在夏季,所有平板都恢复了浮力,而在冬季,只有 60% 的平板恢复了浮力。在这两个季节里,所有笼子里的对照样本都保持在底部。不同处理和不同季节的群落结构各不相同,恢复浮力的平板最初以 Ulva sp.和 Ciona robusta 为主。相反,未恢复浮力的板块主要被抗捕食物种覆盖,如 Pyura chilensis、Austromegabalanus psittacus 和 Balanus laevis。因此,污损群落结构会影响捕食对浮力恢复的促进作用,因为并非所有附生生物都能被捕食者吃掉。以前的研究表明了污损生物是如何导致漂浮垃圾下沉的,而本研究则首次提供了实验证据,证明捕食可以逆转这一过程,使垃圾重新浮出水面,并再次成为本地物种和入侵物种的传播媒介。
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引用次数: 0
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