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Fragment-Imprinted Synergistic Copper Ion-Bridged Silver Nanocomposites Unlock Signal Activation for Picomolar-Level Sensing of l-Histidine 片段印迹协同铜离子桥接银纳米复合材料解锁信号激活的皮摩尔水平感应l-组氨酸
IF 9.5 2区 材料科学 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2026-02-11 DOI: 10.1021/acsami.6c00784
Ziwei Wang,Jiawei Li,Zhaoxuanxuan Chen,Zhanfang Ma,Hongliang Han
l-Histidine (l-His), as a semiessential amino acid in the human body, plays a crucial role in maintaining normal physiological functions, and abnormal levels of l-His may lead to the occurrence of various diseases. Therefore, achieving an ultrasensitive sensing interface for l-His is of critical importance for the clinical diagnosis and treatment of related diseases. Currently, the signal conduction mode of a molecularly imprinted electrochemical sensing interface for l-His mainly relies on the electrochemical activity of the target itself or changes in electrical signals caused by alterations in the impedance of the sensing interface. However, the two modes are limited by the weak electrochemical activity of the target itself and the susceptibility of the sensing interface to nonspecific adsorption interference, resulting in reduced sensitivity and selectivity of the sensing interface. Herein, a fragment-imprinted synergistic unlocking signal amplification activation strategy based on the probe labeling mode is proposed. Utilizing copper ion (Cu2+)-bridged silver nanoparticles ((AgNP-l-Cys-Cu2+)n), a (AgNP-l-Cys-Cu2+)n nanocomposite signal amplification probe is designed to label l-His fixed in fragment-molecularly imprinted polymers (F-MIP) through strong coordination, achieving ultrasensitive and specific electrochemical detection of l-His. The sensing interface can recognize l-His at the picomolar level, and the imprinting factor reached 6.74. This strategy provides a rational route to improve the performance of the MIP electrochemical sensing interfaces.
l-组氨酸(l- hisine, l- hisine)是人体半必需氨基酸,对维持正常生理功能起着至关重要的作用,其水平异常可导致多种疾病的发生。因此,实现l-His的超灵敏传感接口对于临床相关疾病的诊断和治疗具有至关重要的意义。目前,分子印迹l-His电化学传感接口的信号传导方式主要依赖于目标本身的电化学活性或传感接口阻抗改变引起的电信号变化。然而,这两种模式受到目标本身电化学活性较弱和感应界面对非特异性吸附干扰的敏感性的限制,导致感应界面的灵敏度和选择性降低。本文提出了一种基于探针标记模式的片段印迹协同解锁信号放大激活策略。利用铜离子(Cu2+)桥接银纳米粒子((AgNP-l-Cys-Cu2+)n),设计了一种(AgNP-l-Cys-Cu2+)n纳米复合信号放大探针,通过强配合对固定在片段分子印迹聚合物(F-MIP)中的l-His进行标记,实现了对l-His的超灵敏和特异的电化学检测。该传感接口可以识别皮摩尔水平的l-His,印迹因子达到6.74。该策略为提高MIP电化学传感接口的性能提供了一条合理的途径。
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引用次数: 0
In Situ Click Chemistry for Energy-Level-Tunable Mixed Self-Assembled Monolayers in Perovskite Solar Cells 钙钛矿太阳能电池中能量可调混合自组装单层的原位点击化学
IF 10.8 1区 材料科学 Q1 CHEMISTRY, MULTIDISCIPLINARY Pub Date : 2026-02-11 DOI: 10.1021/acs.nanolett.5c06186
Yu Feng,Jiefeng Luo,Xue Han,Yuqiang Wu,Kai Zhang,Yu Wang,Saisai Li,Saif M. H. Qaid,Yuanzhi Jiang,Mingjian Yuan
Buried interfacial energy alignment critically affects the performance of the inverted PSCs. Achieving an ideal alignment remains challenging as reliable strategies for precisely tuning the electronic structures of individual SAMs are still elusive. Here, we develop an in-situ click chemistry strategy under mild conditions and with high intrinsic reactivity to construct mixed SAMs with tunable energy levels. By modulation of precursor ratios, molecular coupling and energy-level modulation occur simultaneously. This strategy mitigates steric hindrance and competitive adsorption in conventional blending, enabling seamless energy alignment (ΔE = ∼0.01 eV) and improved interfacial properties. Calculations indicate that reduced electron localization in SAMs from this strategy facilitates enhanced charge transport. Optoelectronic characterizations confirm that mixed-SAMs/perovskite interfaces enhance hole extraction and suppress interfacial nonradiative recombination. Using this strategy, PSCs achieve a PCE of 26.83% (certified: 26.46%) and maintain 93% of initial efficiency after 2,000 h (ISOS-L-2), demonstrating universality across various perovskite compositions.
埋藏界面能排列对倒置聚氯乙烯的性能有重要影响。实现理想的对准仍然具有挑战性,因为精确调整单个sam电子结构的可靠策略仍然难以捉摸。在这里,我们开发了一种在温和条件下的原位点击化学策略,并具有高的内在反应性来构建具有可调能级的混合SAMs。通过调制前驱体比例,分子偶联和能级调制同时发生。该策略减轻了传统共混中的位阻和竞争性吸附,实现了无缝的能量排列(ΔE = ~ 0.01 eV)并改善了界面性能。计算表明,这种策略降低了SAMs中的电子局域化,促进了电荷输运。光电表征证实,混合的sams /钙钛矿界面增强了空穴提取,抑制了界面的非辐射复合。使用该策略,PSCs的PCE达到26.83%(认证为26.46%),并在2000 h后保持93%的初始效率(iso - l -2),证明了各种钙钛矿成分的普遍性。
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引用次数: 0
Recyclable Molten Salt-Assisted Synthesis of Fe@Fe3C Surface Anchored FeZnNC Hierarchical Composite for Oxygen Reduction Reaction 可回收熔盐辅助合成Fe@Fe3C表面锚定FeZnNC层状复合材料的氧还原反应
IF 6.2 2区 材料科学 Q2 CHEMISTRY, PHYSICAL Pub Date : 2026-02-11 DOI: 10.1016/j.jallcom.2026.186786
Sina Cheng, Hongyang Gao, Yichen Dai, Xueting Jiang, Li Li, Fan Zhang, Qiyong Zhu, Ping Yang, Shiliu Yang
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引用次数: 0
Dual-Defect Engineering Enables Enhanced Thermoelectric Performance in n-Type Mg3Bi1.5Sb0.5 Thin Films 双缺陷工程使n型Mg3Bi1.5Sb0.5薄膜的热电性能得到增强
IF 9.4 1区 材料科学 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2026-02-11 DOI: 10.1016/j.actamat.2026.122012
Yijun Ran, Wenxue Ma, Wenxia Li, Shengqian Li, Xiaoyang Wang, Xiong Ting, Dayi Zhou, Xiangshan Kong, Ning Gao, Zhi Yu, Kaiping Tai
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引用次数: 0
Fluctuating Peierls stress–governed plasticity and strengthening in high-entropy alloys: A discrete dislocation dynamics study 高熵合金的波动佩尔斯应力控制塑性和强化:一个离散位错动力学研究
IF 9.8 1区 材料科学 Q1 ENGINEERING, MECHANICAL Pub Date : 2026-02-11 DOI: 10.1016/j.ijplas.2026.104641
Xin Liu, Ang Li, Changwei Wang, Yinan Cui, Yaxin Zhu, Lv Zhao, Shuang Liang, Minsheng Huang, Zhenhuan Li
{"title":"Fluctuating Peierls stress–governed plasticity and strengthening in high-entropy alloys: A discrete dislocation dynamics study","authors":"Xin Liu, Ang Li, Changwei Wang, Yinan Cui, Yaxin Zhu, Lv Zhao, Shuang Liang, Minsheng Huang, Zhenhuan Li","doi":"10.1016/j.ijplas.2026.104641","DOIUrl":"https://doi.org/10.1016/j.ijplas.2026.104641","url":null,"abstract":"","PeriodicalId":340,"journal":{"name":"International Journal of Plasticity","volume":"4 1","pages":""},"PeriodicalIF":9.8,"publicationDate":"2026-02-11","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"146152796","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Narrowband green emission in CaF2: U6+ phosphors via dynamic F–O coordination and defect synergy CaF2: U6+荧光粉窄带绿色发射的动态F-O协调和缺陷协同
IF 9.4 1区 材料科学 Q1 CHEMISTRY, PHYSICAL Pub Date : 2026-02-11 DOI: 10.1016/j.jmat.2026.101185
Dilare Halmurat, Xinyu Zhang, Litipu Aihaiti, Rong-Jun Xie
{"title":"Narrowband green emission in CaF2: U6+ phosphors via dynamic F–O coordination and defect synergy","authors":"Dilare Halmurat, Xinyu Zhang, Litipu Aihaiti, Rong-Jun Xie","doi":"10.1016/j.jmat.2026.101185","DOIUrl":"https://doi.org/10.1016/j.jmat.2026.101185","url":null,"abstract":"","PeriodicalId":16173,"journal":{"name":"Journal of Materiomics","volume":"30 1","pages":""},"PeriodicalIF":9.4,"publicationDate":"2026-02-11","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"146152799","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Surface modification and microstructure regulation of SnS2 anodes for improved potassium-ion storage 改善钾离子储存的SnS2阳极表面改性及微观结构调控
IF 6.7 2区 材料科学 Q2 CHEMISTRY, PHYSICAL Pub Date : 2026-02-11 DOI: 10.1016/j.apsusc.2026.166262
Kangzhe Cao, Xiaoyue Su, Huimin Li, Yulian Dong, Yong Lei, Huiqiao Liu
{"title":"Surface modification and microstructure regulation of SnS2 anodes for improved potassium-ion storage","authors":"Kangzhe Cao, Xiaoyue Su, Huimin Li, Yulian Dong, Yong Lei, Huiqiao Liu","doi":"10.1016/j.apsusc.2026.166262","DOIUrl":"https://doi.org/10.1016/j.apsusc.2026.166262","url":null,"abstract":"","PeriodicalId":247,"journal":{"name":"Applied Surface Science","volume":"43 1","pages":""},"PeriodicalIF":6.7,"publicationDate":"2026-02-11","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"146152800","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Thermomechanical fatigue damage mechanisms and life prediction of thin-walled nickel-based superalloy tubes considering temperature gradients effect 考虑温度梯度效应的镍基高温合金薄壁管热疲劳损伤机理及寿命预测
IF 6 2区 材料科学 Q1 ENGINEERING, MECHANICAL Pub Date : 2026-02-11 DOI: 10.1016/j.ijfatigue.2026.109563
Hu xiaoan, Xiao Baolu, Sui Tianxiao, Yang Qinzheng
{"title":"Thermomechanical fatigue damage mechanisms and life prediction of thin-walled nickel-based superalloy tubes considering temperature gradients effect","authors":"Hu xiaoan, Xiao Baolu, Sui Tianxiao, Yang Qinzheng","doi":"10.1016/j.ijfatigue.2026.109563","DOIUrl":"https://doi.org/10.1016/j.ijfatigue.2026.109563","url":null,"abstract":"","PeriodicalId":14112,"journal":{"name":"International Journal of Fatigue","volume":"35 1","pages":""},"PeriodicalIF":6.0,"publicationDate":"2026-02-11","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"146152924","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Homogeneous Co2MoS4 on Carbon Nanotube Macrofilms as a Bifunctional Freestanding Electrode for Overall Water Splitting 碳纳米管宏观膜上均相Co2MoS4作为双功能独立电极的整体水分解
IF 6.6 3区 材料科学 Q1 ELECTROCHEMISTRY Pub Date : 2026-02-11 DOI: 10.1016/j.electacta.2026.148442
Yi Liu, Qinqi Zhan, Peng Deng, Yanhong Yin
{"title":"Homogeneous Co2MoS4 on Carbon Nanotube Macrofilms as a Bifunctional Freestanding Electrode for Overall Water Splitting","authors":"Yi Liu, Qinqi Zhan, Peng Deng, Yanhong Yin","doi":"10.1016/j.electacta.2026.148442","DOIUrl":"https://doi.org/10.1016/j.electacta.2026.148442","url":null,"abstract":"","PeriodicalId":305,"journal":{"name":"Electrochimica Acta","volume":"18 1","pages":""},"PeriodicalIF":6.6,"publicationDate":"2026-02-11","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"146153141","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Coacervate Microenvironments Modulate Fluorescent Dye Behaviour and Förster Energy Transfer Dynamics 凝聚微环境调节荧光染料行为和Förster能量转移动力学
IF 6.7 3区 材料科学 Q1 CHEMISTRY, MULTIDISCIPLINARY Pub Date : 2026-02-11 DOI: 10.1039/d5nr04690d
Mohit Kumar, Minea Kapzidic, Shikha Dhiman
Coacervates offer dynamic environments for molecular organization. Using complex coacervates of poly-L-lysine and anionic fluorophores, we show that coacervate microenvironment modulates dye photophysical properties through competing effects: fluorescence enhancement via local enrichment and aggregation-induced quenching at higher loading, while enabling energy transfer. These insights establish coacervates as versatile templates for designing adaptive nanoscale photonic and energy-transfer materials.
凝聚体为分子组织提供了动态环境。利用聚l -赖氨酸和阴离子荧光团的复杂凝聚体,我们发现凝聚体微环境通过竞争效应调节染料的光物理特性:通过局部富集和高负载下聚集诱导的猝灭来增强荧光,同时实现能量转移。这些见解确立了凝聚体作为设计自适应纳米级光子和能量转移材料的通用模板。
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引用次数: 0
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